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| 1 | Strategies of Removing Residual Lithium Compounds on the Surface of Ni-Rich Cathode Materials显示文摘Ni-rich cathode materials have become one of the most promising cathode materials for advanced high-energy Li-ion batteries(LIBs)owing to their high specific capacity.However,Ni-rich cathode materials are sensitive to the trace H2O and CO2 in the air,and tend to react with them to generate LiOH and Li2COg at the particle surface region(named residual lithium compounds,labeled as RLCs).The RLCs will deteriorate the comprehensive performances of Ni-rich cathode materials and make trouble in the subsequent manufacturing process of electrode,including causing low initial coulombic efficiency and poor storage property,bringing about potential safety hazards,and gelatinizing the electrode slurry.Therefore,it is of considerable significance to remove the RLCs.Researchers have done a lot of work on the corresponding field,such as exploring the formation mechanism and elimination methods.This paper investigates the origin of the surface residual lithium compounds on Ni-rich cathode materials,analyzes their adverse effects on the per-formance and the subsequent electrode production process,and summarizes various kinds of feasible methods for removing the RLCS.Finally,we propose a new research direction of eliminating the lithium residuals after comparing and summing up the above.We hope this work can provide a reference for alleviating the adverse effects of residual lithium compounds for Ni-rich cathode materials'industrial production. | Yuefeng Su Linwei Li Gang Chen Lai Chen Ning Li Yun Lu Liying Bao Shi Chen Feng Wu | 2021 | Chinese Journal of Chemistry2021，39，1： | 4 |
| 2 | Centrifugal model test on a riverine landslide in the Three Gorges Reservoir induced by rainfall and water level fluctuation显示文摘Frequent soil landslide events are recorded in the Three Gorges Reservoir area,China,making it necessary to investigate the failure mode of such riverside landslides.Geotechnical centrifugal test is considered to be the most realistic laboratory model,which can reconstruct the required geo-stress.In this study,the Liangshuijing landslide in the Three Gorgers Reservoir area is selected for a scaled centrifugal model experiment,and a water pump system is employed to retain the rainfall condition.Using the techniques of digital photography and pore water pressure transducers,water level fluctuation is controlled,and multi-physical data are thus obtained,including the pore water pressure,earth pressure,surface displacement and deep displacement.The analysis results indicate that:Three stages were set in the test(waterflooding stage,rainfall stage and drainage stage).Seven transverse cracks with wide of 1–5 mm appeared during the model test,of which 3 cracks at the toe landslide were caused by reservoir water fluctuation,and the cracks at the middle and rear part were caused by rainfall.During rainfall process,the maximum displacement of landslide model reaches 3 cm.And the maximum deformation of the model exceeds 12 cm at the drainage stage.The failure process of the slope model can be divided into four stages:microcracks appearance and propagation stage,thrust-type failure stage,retrogressive failure stage,and holistic failure stage.When the thrust-type zone caused by rainfall was connected or even overlapped with the retrogressive failure zone caused by the drainage,the landslide would start,which displayed a typical composite failure pattern.The failure mode and deformation mechanism under the coupling actions of water level fluctuation and rainfall are revealed in the model test,which could appropriately guide for the analysis and evaluation of riverside landslides. | Fasheng Miao Yiping Wu Ákos Török Linwei Li Yang Xue | 2022 | Geoscience Frontiers2022，13，3： | 3 |
| 3 | Responses of the functional structure of soil microbial community to livestock grazing in the T ibetan alpine grassland显示文摘 | Yunfeng Yang Linwei Wu Qiaoyan Lin Mengting Yuan Depeng Xu Hao Yu Yigang Hu Jichuang Duan Xiangzhen Li Zhili He Kai Xue Joy van Nostrand Shiping Wang Jizhong Zhou | 2012 | Glob Change Biol2012，，2： | 1 |
| 4 | Model for end-stage liver disease versus the Child-Pugh score in predicting the post-transplant 3-month and 1-year mortality in a cohort of Chinese recipients显示文摘 | Zhiyong Guo Xiaoshun He Linwei Wu Weiqiang Ju Anbin Hu Qiang Tai Dongping Wang Yi Ma Guodong Wang Xiaofeng Zhu Jiefu Huang | 2010 | Surgery Today2010，，1： | 1 |
| 5 | Study of the Sensitive Properties of Marine Gas Hydrate Based on the Prestack Elastic Inversion显示文摘Using a bottom simulating reflector(BSR)on a seismic profile to identify marine gas hydrate is a traditional seismic exploration method.However,owing to the abundance differences between the gas hydrate and free gas in different regions,the BSR may be unremarkable on the seismic profile and invisible in certain cases.With the improvement of exploration precision,difficulty arises in meeting the requirements of distinguishing the abundance differences in the gas hydrate based on BSR.Hence,we studied other sensitive attributes to ascertain the existence of gas hydrate and its abundance variations,eventually improving the success rate of drilling and productivity.In this paper,we analyzed the contradiction between the seismic profile data and drilling sampling data from the Blake Ridge.We extracted different attributes and performed multi-parameter constraint analysis based on the prestack elastic wave impedance inversion.Then,we compared the analysis results with the drilling sampling data.Eventually,we determined five sensitive attributes that can better indicate the existence of gas hydrate and its abundance variations.This method overcomes the limitations of recognizing the gas hydrate methods based on BSR or single inversion attribute.Moreover,the conclusions can notably improve the identification accuracy of marine gas hydrate and provide excellent reference significance for the recognition of marine gas hydrate.Notably,the different geological features of reservoirs feature different sensitivities to the prestacking attributes when using the prestack elastic inversion in different areas. | TONG Siyou WANG Jialin LI Linwei ZHANG Haiqi WU Zhiqiang SHAO Yulan | 2019 | Journal of Ocean University of China2019，18，5： | 1 |
| 6 | Reverse-Time Migration of Converted S-Waves of Varying Densities显示文摘Ocean-Bottom Node(OBN)acquisitions provide both non-converted and converted reflection energy.There is a clear advantage to independently imaging both P-and S-waves,as they provide more information collectively than either does alone.In many conventional converted-wave pre-stack migration algorithms,density is treated as a constant,which is not the real-life case on earth.S-wave velocity and density information is crucial for hydrocarbon detection because it helps in the identification of porefilling fluids.In this paper,we focused on the effect of density on imaging,and developed a method of reverse-time migration(RTM)on converted s-waves of varying densities(VD-RTMCS).Phase correction was required prior to pre-stack migration to avoid constructive interference between data from adjacent sources.Synthetic data examples showed that when density variations were included,image profiles showed advantages in signal-to-noise ratio,vertical resolution and imaging of complex structures. | TONG Siyou CHEN Ming ZHOU Huawei LI Linwei XU Xiugang WU Zhiqiang | 2019 | Journal of Ocean University of China2019，18，5： | 1 |
| 7 | Can Immune Cell Function Assay Identify Patients at Risk of Infection or Rejection? A Meta-Analysis显示文摘 | Xiaoting Ling Jun Xiong Wenhua Liang Paul M. Schroder Linwei Wu Weiqiang Ju Yuan Kong Yushu Shang Zhiyong Guo Xiaoshun He | 2012 | Transplantation2012，，7： | 1 |
| 8 | Model for end-stage liver disease versus the Child-Pugh score in predicting the post-transplant 3-month and 1-year mortality in a cohort of Chinese recipients显示文摘 | Zhiyong Guo Xiaoshun He Linwei Wu Weiqiang Ju Anbin Hu Qiang Tai Dongping Wang Yi Ma Guodong Wang Xiaofeng Zhu Jiefu Huang | 2010 | Surgery Today2010，，1： | 1 |
| 9 | Living donor liver transplantation versus deceased donor liver transplantation for hepatocellular carcinoma: A meta‐analysis显示文摘 | Wenhua Liang Linwei Wu Xiaoting Ling Paul M. Schroder Weiqiang Ju Dongping Wang Yushu Shang Yuan Kong Zhiyong Guo Xiaoshun He | 2012 | Liver Transpl2012，，10： | 1 |
| 10 | Radiation-induced one-pot synthesis of grafted covalent organic frameworks显示文摘Post-synthetic functionalization of covalent organic frameworks(COFs)is an alternative way to enhance and broaden their properties and potential applications.However,the chemical functionalization of COFs is a great challenge because traditional procedures are often time-and energy-consuming,while the crystallinity of COFs can be damaged under harsh conditions.Here we report the in-situ introduction of functional graft chains onto the skeleton of COFs during the synthesis process through the combination of radiation-induced synthesis and graft polymerization techniques under ^(60)Co gamma-ray radiation.The synthesis and functionalization of COFs are simultaneously accomplished in a chemical system under ambient conditions yielding a large number of different functionalized COFs.The obtained carboxyl-functionalized COFs exhibit excellent radioactive uranium removal capabilities from aqueous solution with fast uptake dynamics,high adsorption capacity,and excellent selectivity over other competing metal ions. | Mingxing Zhang Mengjia Yuan Xiaofang Zhao Junchang Chen Linwei He Qianhong Gao Jiangtao Hu Guozhong Wu Zhifang Chai Shuao Wang | 2023 | Science China Chemistry2023，66，6： | 0 |
| 11 | Assessing mechanisms for microbial taxa and community dynamics using process models显示文摘Disentangling the assembly mechanisms controlling community composition,structure,distribution,functions,and dynamics is a central issue in ecology.Although various approaches have been proposed to examine community assembly mechanisms,quanti-tative characterization is challenging,particularly in microbial ecology.Here,we present a novel approach for quantitatively delineating community assembly mechanisms by combining the consumer–resource model with a neutral model in stochastic differential equations.Using time-series data from anaerobic bioreactors that target microbial 16S rRNA genes,we tested the applicability of three ecological models:the consumer–resource model,the neutral model,and the combined model.Our results revealed that model performances varied substantially as a function of population abundance and/or process conditions.The combined model performed best for abundant taxa in the treatment bioreactors where process conditions were manipulated.In contrast,the neutral model showed the best performance for rare taxa.Our analysis further indicated that immigration rates decreased with taxa abundance and com-petitions between taxa were strongly correlated with phylogeny,but within a certain phylogenetic distance only.The determinism underlying taxa and community dynamics were quantitatively assessed,showing greater determinism in the treatment bioreactors that aligned with the subsequent abnormal system functioning.Given its mechanistic basis,the framework developed here is expected to be potentially applicable beyond microbial ecology. | Linwei Wu Yunfeng Yang Daliang Ning Qun Gao Huaqun Yin Naija Xiao Benjamin YZhou Si Chen Qiang He Jizhong Zhou | 2023 | mLife2023，2，3： | 0 |
| 12 | Synergy of first-and second-sphere interactions in a covalent organic framework boosts highly selective platinum uptake显示文摘Platinum recovery from waste electrical and electronic equipment(WEEE) in highly acidic solutions is significant to the electronics industry and environmental remediation. However, the lack of ingenious design and synergetic coordination gives rise to unsatisfied PtCl_(4)^(2-)extraction capacities and selectivities in most previously reported adsorbents(e.g., polymeric and inorganic materials). Herein, we proposed a synergistic strategy that realizes highly selective PtCl_(4)^(2-)uptake through first-and second-sphere coordinations. The proof-of-concept imine-linked covalent organic framework(SCU-COF-3) was found to chelate Pt Cl42-via the direct N…Pt coordination and the synergistically interlaminar N–H…Cl hydrogen bonds, which was disclosed by the comprehensive analysis of extended X-ray adsorption fine structure(EXAFS) characterizations and density functional theory(DFT) calculations. The unique adsorption mechanism imparts a superior adsorption capacity(168.4 mg g-1)and extraordinary Pt(II) selectivity to SCU-COF-3 under static conditions. In addition, SCU-COF-3 exhibits an upgraded distribution coefficient of 1.62 × 10^(5)mL· g^(-1), one order of magnitude higher than those of reported natural adsorbents. Specifically, SCU-COF-3 can extract PtCl_(4)^(2- )quantitatively from a simulated acidic waste solution coexisting with other 12 competitive ions, suggesting its promising application in practical scenarios. | Linwei He Baoyu Li Zhonglin Ma Lixi Chen Shicheng Gong Mingxing Zhang Yaoyao Bai Qi Guo Fuqi Wu Fuqiang Zhao Jie Li Duo Zhang Daopeng Sheng Xing Dai Long Chen Jie Shu Zhifang Chai Shuao Wang | 2023 | Science China Chemistry2023，66，3： | 0 |
| 13 | Superior Iodine Uptake Capacity Enabled by an Open Metal-Sulfide Framework Composed of Three Types of Active Sites显示文摘Efficient adsorption of gaseous radioiodine is pivotal for the sustainable development of nuclear energy and the long-termradiation safety of the ecological system.However,state-of-the-art adsorbents(e.g.metal-organic frameworks and covalent-organic frameworks)currently under exploration suffer severely from limited adsorption capacity,especially under a real-world scenariowith extremely lowradioiodine concentration and elevated temperature.This mostly originates from the relatively weak sorption driving forces mainly determinedby the iodine-adsorbent interaction consistingof noncovalent interactionswith a small fraction of strong chemical bonding.Here,we document the discovery of an open metal-sulfide framework((NH_(4))_(2)(Sn_(3)S_(7)),donated as SCU-SnS)constructed by three different types of active sites as a superior iodine adsorbent.Benefiting from the ability of iodine for pre-enrichment into the framework by charge-balancing NH_(4)^(+)through N-H···I interaction,the efficient reduction of I^(2)affording I^(-)by S^(2-),and extremely high binding affinity between Sn_(4)^(+)and I^(-),SCU-SnS exhibit a record-breaking iodine adsorption capacity(2.12 g/g)under dynamic breakthrough conditions and the highest static capacity(6.12 g/g)among all reported inorganic adsorbents,both at 348 K.Its facile synthesis and low cost endow SCU-SnS with powerful application potential for the nuclear industry. | Yugang Zhang Linwei He Tingting Pan Jian Xie Fuqi Wu Xinglong Dong Xia Wang Lixi Chen Shicheng Gong Wei Liu Litao Kang Junchang Chen Lanhua Chen Long Chen Yu Han Shuao Wang | 2023 | CCS Chemistry2023，5，7： | 0 |
| 14 | Effects of acid mine drainage on photochemical and biological degradation of dissolved organic matter in karst river water显示文摘Dissolved organic matter(DOM)can be removed or transformed by photochemical and biological processes,producing the negative effect of transforming organic carbon into inorganic carbon,which plays a vital role in the karst carbon cycle.However,acid mine drainage(AMD)will affect this process,so the degradation of DOM in karst river water(KRW)needs to be studied in this context.In this study,to reveal the evolution processes of DOM under photochemical and biological conditions in AMD-impacted KRW,AMD and KRW were mixed in different ratios under conditions of visible light irradiation(VL),biodegradation(BD),ultraviolet irradiation(UV)and ultraviolet irradiation+biodegradation(UV+BD).The average DOC concentrations in samples after mixing AMD and KRW in different proportions decreased significantly(by 23%)in UV+BD,which was 1.2–1.4 times higher than under the other conditions and would lead to a significant release of inorganic carbon.Further analysis of the fluorescence parameters via parallel factor analysis(PARAFAC)revealed that the DOM fluorescence components in AMD comprised mainly protein-like substances derived from autochthonous components,while the DOM fluorescence components in KRW were mainly humic-like substances with both autochthonous and allochthonous sources.Therefore,AMD could promote both the photochemical and biological degradation of DOM in karst receiving streams,resulting in the conversion of DOC to inorganic carbon.The results showed that the synergistic effects of UV+BD and AMD accelerated the degradation of DOM and the release of inorganic carbon in KRW,thus affecting the stability of the karst carbon cycle. | Linwei Li Xingxing Cao Chujie Bu Pan Wu Biao Tian Yongheng Dai Yeye Ren | 2024 | Journal of Environmental Sciences2024，，1： | 0 |
| 15 | Structural effects of sulfonamides on the proliferation dynamics of sulfonamide resistance genes in the sequencing batch reactors and the mechanism显示文摘Antibiotic resistance genes(ARGs)can be easily promoted by antibiotics,however,the structural effects of antibiotics on the proliferation of ARGs dynamic and the associated mechanisms remain obscure in,especially,activated sludge sequencing batch reactors.In the present study,the effects of 9 sulfonamides(SAs)with different structures on the proliferation dynamic of sulfonamide resistance genes(Suls)in the activated sludge sequencing batch reactors and the corresponding mechanisms were determined(30 days),and the results showed that the largest proliferation value(ΔA^(R))of Suls dynamic for SAs(sulfachloropyridazine)was approximately 2.9 times than that of the smallest one(sulfadiazine).The proliferation of Suls was significantly related to the structural features(minHBint6,SssNH,SHBd and SpMax2_Bhm)that represent the biological activity of SAs.To interpret the phenomenon,a mechanistic model was developed and the results indicated that the biodegradation of SAs(T_(1/2))rather than conjugative transfer frequency or mutation frequency tends to be the key process for affecting Suls proliferation.T_(1/2)was proved to be dependent on the interactions between SAs and receptors(E_(binding)),the cleavage mode(bond dissociation energy),and the site of nucleophilic assault.Besides,the metagenomic analysis showed that SAs posed significant effect on antibiotic resistome and Tnp31 played a vital role in the proliferation of Suls.Overall,our findings provide important insight into a theoretical basis for understanding the structural effects of SAs on the proliferation of ARGs in SBR systems. | Ligui Wu Mingyu Wang Lingling Rong Wenbiao Wang Linwei Chen Qiaofeng Wu Haoyu Sun Xiangfeng Huang Xiaoming Zou | 2024 | Journal of Environmental Sciences2024，，1： | 0 |
| 16 | Slope Instability Analysis of the Qiongdongnan Basin in the Northern Part of the South China Sea:Implications for the Risk Evaluation of Deepwater Drilling显示文摘The instability of continental slopes damages marine engineering equipment,such as submarine pipelines,resulting in the generation of tsunamis,which endangers the safety of nearshore personnel.Therefore,research on the instability of continental slopes where submarine landslides usually occur is crucial to the risk evaluation of deepwater drilling.Previous studies were mainly based on simplified 2D and 3D models,which extend the 2D model applied on submarine slopes with complex topography.In this study,a numerical model with bathymetric data from the Qiongdongnan Basin was established.Furthermore,3D slope stability analysis and static and dynamic analyses were conducted.The static analysis found two discussions where slopes are most likely to occur.Through the analysis of different seismic forces,the dynamic result showed that an instability area is added to the two positions where the static analysis is unstable.Topography scatters and transmits seismic waves and controls the accumulation and diffusion of seismic energy.3D calculations and analysis revealed that the direction of slope instability is closely related to terrain inclination,slope,terrain effect,and terrain curvature.Data showed that instability situations could not be derived from a single direction or profile data.Such situations are an important factor in slope stability analysis and are critical to the prediction and evaluation of marine geological disasters. | MA Linwei WU Shiguo LIU Yanrui SUN Jin OUYANG Min LI Qingping QIN Yongpeng WANG Dawei | 2023 | Journal of Ocean University of China2023，22，2： | 0 |
| 17 | Band alignment and interlayer hybridization in monolayer organic/WSe_(2) heterojunction显示文摘Semiconducting heterojunctions(HJs),comprised of atomically thin transition metal dichalcogenides(TMDs),have shown great potentials in electronic and optoelectronic applications.Organic/TMD hybrid bilayers hold enhanced pumping efficiency of interfacial excitons,tunable electronic structures and optical properties,and other superior advantages to these inorganic HJs.Here,we report a direct probe of the interfacial electronic structures of a crystalline monolayer(ML)perylene-3,4,9,10-tetracarboxylic-dianhydride(PTCDA)/ML-WSe_(2) HJ using scanning tunneling microscopy,photoluminescence,and first-principle calculations.Strong PTCDAAA/Se_(2) interfacial interactions lead to appreciable hybridization of the WSe_(2) conduction band with PTCDA unoccupied states,accompanying with a significant amount of PTCDA-to-WSe_(2) charge transfer(by 0.06 e/PTCDA).A type-ll band alignment was directly determined with a valence band offset of-1.69 eV,and an apparent conduction band offset of-1.57 eV.Moreover,we found that the local stacking geometry at the HJ interface differentiates the hybridized interfacial states. | Yanping Guo Linlu Wu Jinghao Deng Linwei Zhou Wei Jiang Shuangzan Lu Da Huo Jiamin Ji Yusong Bai Xiaoyu Lin Shunping Zhang Hongxing Xu Wei Ji Chendong Zhang | 2022 | Nano Research2022，15，2： | 0 |
| 18 | All-stage targeted therapy for the brain metastasis from triple-negative breast cancer显示文摘Brain metastasis is a common and serious complication of breast cancer,which is commonly associated with poor survival and prognosis.In particular,the treatment of brain metastasis from triplenegative breast cancer(BM-TNBC)has to face the distinct therapeutic challenges from tumor heterogeneity,circulating tumor cells(CTCs),blood-brain barrier(BBB)and blood-tumor barrier(BTB),which is in unmet clinical needs.Herein,combining with the advantages of synthetic and natural targeting moieties,we develop a“Y-shaped”peptide pVAP-decorated platelet-hybrid liposome drug delivery system to address the all-stage targeted drug delivery for the whole progression of BM-TNBC.Inherited from the activated platelet,the hybrid liposomes still retain the native affinity toward CTCs.Further,the peptide-mediated targeting to breast cancer cells and transport across BBB/BTB are demonstrated in vitro and in vivo.The resultant delivery platform significantly improves the drug accumulation both in orthotopic breast tumors and brain metastatic lesions,and eventually exhibits an outperformance in the inhibition of BM-TNBC compared with the free drug.Overall,this work provides a promising prospect for the comprehensive treatment of BMTNBC,which could be generalized to other cell types or used in imaging platforms in the future. | Zimiao Luo Sunyi Wu Jianfen Zhou Weixia Xu Qianzhu Xu Linwei Lu Cao Xie Yu Liu Weiyue Lu | 2023 | Acta Pharmaceutica Sinica B2023，13，1： | 0 |
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