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| 1 | Rare earths (Ce, Y, Pr) modified Pd/La2O3-ZrO2-Al2O3 catalysts usedin lean-burn natural gas fueled vehicles显示文摘14%REO_x-2.5%La_2 O_3-33.5%ZrO_2-50%Al_2 O_3(RE = Ce, Y, Pr) composites were prepared by a coprecipitation method. The Pd catalysts were obtained by an aqueous solution of Pd(NO_3)_2 loaded on the rare earths modified composites with an initial wet impregnated method. The experiment results show that catalytic activity of the rare earths modified Pd/La_2 O_3-ZrO_2-Al_2 O_3 catalysts is better than bare sample for methane oxidation. The structural characterization results reveal that the rare earths modified Pd catalysts increase amounts of surface active oxygen species by X-ray photoelectron spectroscopy(XPS) analysis and improve the dispersion of active component from H2-temperature programmed reduction(H2-TPR) measurement compared with bare sample. Especially,Pd/14%Y_2 O_3-2.5%La_2 O_3-33.5%ZrO_2-50%Al_2 O_3 sample exhibits highly active stability, it is related to the Pd particles highly dispersion,which was observed by transmission electron microscope(TEM) images. | Haoxin Liu Baiwen Zhao Yusheng Chen Chengdun Ren Yaoqiang Chen | 2017 | Journal of Rare Earths2017，35，11： | 6 |
| 2 | Upconversion nanoparticles regulated drug&gas dual-effective nanoplatform for the targeting cooperated therapy of thrombus and anticoagulation显示文摘Thromboembolism is the leading cause of cardiovascular mortality.Currently,for the lack of targeting,short half-life,low bioavailability and high bleeding risk of the classical thrombolytic drugs,pharmacological thrombolysis is usually a slow process based on micro-pumping.In addition,frequently monitoring and regulating coagulation functions are also required during(and after)the process of thrombolysis.To address these issues,a targeted thrombolytic and anticoagulation nanoplatform(UCATS-UK)is developed based on upconversion nanoparticles(UCNPs)that can convert 808 or 980 nm near-infrared(NIR)light into UV/blue light.This nanoplatform can target and enrich in the thrombus site.Synergistic thrombolysis and anticoagulation therapy thus could be realized through the controlled release of urokinase(UK)and nitric oxide(NO).Both in vitro and in vivo experiments have confirmed the excellent thrombolytic and anticoagulative capabilities of this multifunctional nanoplatform.Combined with the unique fluorescent imaging capability of UCNPs,this work is expected to contribute to the development of clinical thrombolysis therapy towards an integrated system of imaging,diagnosis and treatment. | Shichen Liu Yao Sun Teng Zhang Longtao Cao Zhiwei Zhong Haoxin Cheng Qingqing Wang Zhuang Qiu Weimin Zhou Xiaolei Wang | 2022 | Bioactive Materials2022，7，12： | 1 |
| 3 | Inhibition of hydrogen sulfide synthesis provides protection for severe acute pancreatitis rats via apoptosis pathway显示文摘 | Gang Wang Bing Han Haoxin Zhou Linfeng Wu Yongwei Wang Guang Jia Jiachen Lv Zhuoxin Cheng Shangha Pan Ji Liu Yinan Zhou Bei Sun | 2013 | Apoptosis2013，，1： | 1 |
| 4 | Climate change and water security in the northern slope of the Tianshan Mountains显示文摘Water security is under threat worldwide from climate change. A warming climate would accelerate evaporationand cryosphere melting, leading to reduced water availability and unpredictable water supply. However, thewater crisis in the Northern Slope of Tianshan Mountains(NSTM) faces dual challenges because water demandsforfast-growing urban areas have put heavy pressure on water resources. The mountain-oasis-desert system featuresglacier-fed rivers that sustain intensive water use in the oasis and end in the desert as fragile terminal lakes.The complex balance between water conservation and economic development is subtle. This paper investigateschanges in hydroclimatic variables and water security-related issues on the NSTM. The spatiotemporal variationsin glaciers, climatic variables, rivers, lakes and reservoirs, groundwater, surface water, human water use, andstreamflow were analyzed for the past four decades. The results show that temperature in the NSTM exhibitedan apparent upward trend with a more significant warming rate in the higher altitude regions. Glacier massloss and shrinkage was strong. The average annual streamflow increased from 1980-1989 to 2006–2011 at mosthydrological stations. The monthly dynamics of surface water area showed notable variability at both inter-annual and seasonal scales, revealing the impacts of both natural and anthropogenic drivers on surface wateravailability in the region. The terrestrial water storage anomaly showed a decreasing trend, which might berelated to groundwater pumping for irrigation. Human water use for agriculture and industry grew with theincrease in cultivated land area and gross domestic product (GDP). The increased agricultural water use wasstrongly associated with the expansion of oases. It is unclear whether water availability would remain high underfuture climatic and hydrological uncertainties, posing challenges to water management. In the context of rapidurban growth and climate change, balancing water for humans and nature is vital in achieving the SustainableDevelopment Goals (SDGs) in NSTM. This study provides a baseline understanding of the interplay among water,climate change, and socio-economic development in NSTM. It would also shed light on wise water managementunder environmental changes for other rapidly developing mountain-oasis-desert systems worldwide. | Qiuhong Tang Xingcai Liu Yuanyuan Zhou Puyu Wang Zhongqin Li Zhixin Hao Suxia Liu Gang Zhao Bingqi Zhu Xinlin He Fadong Li Guang Yang Li He Haoxin Deng Zongxia Wang Xiang Ao Zhi Wang Paul P.J.Gaffney Lifeng Luo | 2022 | Geography and Sustainability2022，3，3： | 1 |
| 5 | Yellow responsive material based modification to reduce earphone induced Infection and hearing loss显示文摘Today,earphones have almost been owned by everyone.However,wearing earphones for a long time can cause two serious problems:(1)irreversible damage to hearing;(2)rapid proliferation of bacteria in the ear canal.Herein,an earphone modification strategy is developed for the first time,to reduce hearing loss and inhibit bacteria simultaneously.This earphone is equipped with a high purity yellow light(YL)light-emitting diode chip developed by our university.Then,the surface of the earphone is loaded with porous zinc oxide and silver nanoparticle composite material(ZnO-Ag)that can respond to the YL.Under the excitation of YL,the porous ZnO-Ag can release reactive oxygen species with strong antibacterial activity.More importantly,we discover that YL can reduce the expression of matrix metalloproteinase-3,the secretion of inflammatory factors,and apoptosis in the cochlea,thereby effectively reduce hearing loss. | Haoxin Cheng Hongmei Liu Zhiqiang Liu Ziying Xu Xiaorong Liu Shuang Jia Chaonan He Shichen Liu Jiao Zhang Xiaolei Wang | 2022 | Nano Research2022，15，7： | 0 |
| 6 | The Warm Arctic-Cold Eurasia Pattern and Its Key Region in Winter in CMIP6 Model Simulations显示文摘An enhanced Warm Arctic-Cold Eurasia(WACE)pattern has been a notable feature in recent winters of the Northern Hemisphere.However,divergent results between model and observational studies of the WACE still remain.This study evaluates the performance of 39 climate models participating in the Coupled Model Intercomparison Project Phase 6(CMIP6)in simulating the WACE pattern in winter of 1980-2014 and explores the key factors causing the differences in the simulation capability among the models.The results show that the multimodel ensemble(MME)can better simulate the spatial distribution of the WACE pattern than most single models.Models that can/cannot simulate both the climatology and the standard deviation of the Eurasian winter surface air temperature well,especially the latter,usually can/cannot simulate the WACE pattern well.This mainly results from the different abilities of the models to simulate the range and intensity of the warm anomaly in the Barents Sea-Kara seas(BKS)region.Further analysis shows that a good performance of the models in the BKS area is usually related to their ability to simulate location and persistence of Ural blocking(UB),which can transport heat to the BKS region,causing the warm Arctic,and strengthen the westerly trough downstream,cooling central Eurasia.Therefore,simulation of UB is key and significantly affects the model’s performance in simulating the WACE. | Liang ZHAO Yunwen LIU Yihui DING Qingquan LI Wei DONG Xinyong SHEN Wei CHENG Haoxin YAO Ziniu XIAO | 2023 | Advances in Atmospheric Sciences2023，40，12： | 0 |
| 7 | Influences of fluorination on homoleptic iridium complexes with C^N=N type ligand to material properties, ligand orientation and OLED performances显示文摘Two new iridium complexes with C^N=N type ligand(i.e., Ir(BFPPya)3{tris[3,6-bis(4-fluorophenyl)pyridazine]iridium(III)} and Ir(BDFPPya)3{tris[3,6-bis(2,4-di-fluorophenyl)pyridazine]iridium(III)}) attaching with fluorine atoms, were synthesized and the effects of fluorination on the material properties and device performance were investigated. Compared with our previously reported fluorine-free analogue material, that is Ir(BPPya)3{tris[3,6-bis(phenyl)pyridazine]iridium(III)}, blue shifts in the emission spectra as well as in the long wavelength region of the absorptions were observed. The photoluminescence quantum yield(PLQY)(0.44 and 0.84 vs. 0.29), phosphoresces lifetime(0.88 and 1.31 vs. 0.66 μs), and oxidation potential(1.10 and 1.37 vs. 0.95 V) increased obviously after fluorinating the ligand. In contrast, the thermal stability of the iridium complexes decreased slightly(Td: 435 and 402 vs. 440 °C). In the density functional theory(DFT) calculations, by comparing the steric shape of the three ligands within one optimized molecule, orientational differences among the complexes were observed. In OLED device studies, bluish green electroluminescence with peak emission of 500 nm, using the electron-transporting host of TPBI [2,2',2''-(1,3,5-benzenetriyl)tris(1-phenyl-1H-benzimidazole)] and the most fluorinated dopant of Ir(BDFPPya)3, was achieved with maximum efficiency of 20.3 cd/A. On one hand this efficiency is not satisfactory considering a high PLQY of 0.84. On the other hand with the similar device structure, that the(HOMO-LUMO)s of all the dopants are wrapped within that of the host TPBI, and all the triplet energies of the dopants are smaller than that of the host TPBI, it is abnormal that the ordering of device efficiencies is contradictory to that of PLQY. Assisting with the phosphorescent spectrum of TPBI and the absorption spectra of the dopant, the contradiction was interpreted reasonably. | Chen Liu Le Mao Haoxin Jia Zhangjin Liao Hongjiao Wang Baoxiu Mi Zhiqiang Gao | 2015 | Science China Chemistry2015，58，4： | 0 |
| 8 | Simulation of Ultrasonic Propagation in Transformers within Thermal Fields and Intelligent Methodology for Hot-spot Temperature Recognition显示文摘Hot-spot temperature of transformer windings is a crucial indicator of internal defects.However,current methods for measuring the hot-spot temperature of transformers do not apply to those already in operation and suffer from data lag.This study introduces a novel inversion method that combines ultrasonic sensing technology,multiphysics simulation,and the K-nearest neighbors algorithm.Leveraging the penetrative ability and temperature sensitivity of ultrasonic sensing,a detailed physical field simulation model was established.This study extensively investigates the characteristics of ultrasonic wave signals inside transformers.The investigation includes different temperature fields,ranging from 40℃ to 110℃ at 10℃ intervals,and various ultrasonic wave emitter conditions.By extracting the key features of the acoustic signals,such as the peak time,propagation time,and peak amplitude,an accurate inversion of the winding hot-spot temperature is successfully achieved.The results demonstrate that this method achieves a high accuracy rate(98.57%)in inverting the internal winding hot-spot temperatures of transformers,offering an efficient and reliable new approach for measuring winding hot-spot temperatures. | Dongxin He Dechao Yang Xinhua Guo Jiefeng Liu Haoxin Guo Qingquan Li Gilbert Teyssedre | 2024 | Chinese Journal of Electrical Engineering2024，10，1： | 0 |
| 9 | Discovery of novel exceptionally potent and orally active c-MET PROTACs for the treatment of tumors with MET alterations显示文摘Various c-mesenchymal-to-epithelial transition(c-MET) inhibitors are effective in the treatment of non-small cell lung cancer;however, the inevitable drug resistance remains a challenge, limiting their clinical efficacy. Therefore, novel strategies targeting c-MET are urgently required. Herein, through rational structure optimization, we obtained novel exceptionally potent and orally active c-MET proteolysis targeting chimeras(PROTACs) namely D10 and D15 based on thalidomide and tepotinib. D10 and D15 inhibited cell growth with low nanomolar IC_(50) values and achieved picomolar DC_(50) values and>99% of maximum degradation(D_(max)) in EBC-1 and Hs746T cells. Mechanistically, D10 and D15dramatically induced cell apoptosis, G1 cell cycle arrest and inhibited cell migration and invasion.Notably, intraperitoneal administration of D10 and D15 significantly inhibited tumor growth in the EBC-1 xenograft model and oral administration of D15 induced approximately complete tumor suppression in the Hs746T xenograft model with well-tolerated dose-schedules. Furthermore, D10 and D15 exerted significant anti-tumor effect in cells with c-MET^(Y1230H) and c-MET^(D1228N) mutations, which are resistant to tepotinib in clinic. These findings demonstrated that D10 and D15 could serve as candidates for the treatment of tumors with MET alterations. | Pengyun Li Changkai Jia Zhiya Fan Xiaotong Hu Wenjuan Zhang Ke Liu Shiyang Sun Haoxin Guo Ning Yang Maoxiang Zhu Xiaomei Zhuang Junhai Xiao Zhibing Zheng Song Li | 2023 | Acta Pharmaceutica Sinica B2023，13，6： | 0 |
| 10 | Wafer-scale fabrication of carbon-nanotube-based CMOS transistors and circuits with high thermal stability显示文摘Thanks to its single-atomic-layer structure,high carrier transport,and low power dissipation,carbon nanotube electronics is a leading candidate towards beyond-silicon technologies.Its low temperature fabrication processes enable three-dimensional(3D)integration with logic and memory(static random access memory(SRAM),magnetic random access memory(MRAM),resistive random access memory(RRAM),etc.)to realize efficient near-memory computing.Importantly,carbon nanotube transistors require good thermal stability up to 400℃ processing temperature to be compatible with back-end-of-line(BEOL)process,which has not been previously addressed.In this work,we developed a robust wafer-scale process to build complementary carbon nanotube transistors with high thermal stability and good uniformity,where AlN was employed as electrostatic doping layer.The gate stack and passivation layer were optimized to realize high-quality interfaces.Specifically,we demonstrate 1-bit carbon nanotube full adders working under 250℃ with rail-to-rail outputs. | Nan Wei Ningfei Gao Haitao Xu Zhen Liu Lei Gao Haoxin Jiang Yu Tian Yufeng Chen Xiaodong Du Lian-Mao Peng | 2022 | Nano Research2022，15，11： | 0 |
| 11 | CeO_(2-x) modified Ru/γ-Al_(2)O_(3) catalysts for ammonia decomposition reaction显示文摘Developing high-performance ammonia decomposition catalysts for preparing COx-free hydrogen shows great practical significance.Herein,CeO_(2) is used as a promoter to modulate the metal-support interaction to enhance the catalytic performance of Ru/Al_(2)O_(3) catalysts.A series of 1Ru/xCe-10AI(x=0.5,1,or 3)catalysts was prepared by a facile colloidal deposition method.We find that the optimized 1 Ru/1Ce-10Al catalyst exhibits excellent activity for the decomposition of ammonia with a very high hydrogen yield of7097 mmolH2/(gRu·min)at 450℃.It is confirmed that Ru species are highly dispersed on the support surface as stable small clusters(~1.3 nm).More importantly,due to the interaction between Ru species and partially reduced CeO_(2-x),the electron density of Ru species is increased,which is beneficial to the high activity of the 1 Ru/xCe-10Al catalysts.This work paves a way to construct high-efficiency ammonia decomposition catalysts modified by CeO_(2). | Qinglu Meng Haoxin Liu Kai Xu Weiwei Wang Chunjiang Jia | 2023 | Journal of Rare Earths2023，41，6： | 0 |
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