|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Deposition of FeCoNiCrMn high entropy alloy(HEA) coating via cold spraying显示文摘High entropy alloys(HEAs) are of great interest in the community of materials science and engineering due to their unique phase structure. They are constructed with five or more principal alloying elements in equimolar or near-equimolar ratio. Therefore, HEAs can derive their performance from multiple principal elements rather than a single element. In this work, solid-state cold spraying(CS) was applied for the first time to produce FeCoNiCrMn HEA coating. The experimental results confirm that CS can be used to produce a thick HEA coating with low porosity. As a low-temperature deposition process, CS completely retained the HEA phase structure in the coating without any phase transformation. The characterization also reveals that the grains in the CSed HEA coating had experienced significant refinement as compared to those in the as-received HEA powder due the occurrence of dynamic recrystallization at the highly deformed interparticle region. Due to the increased dislocation density and grain boundaries,CSed HEA coating was much harder than the as-received powder. The tribological study shows that the CSed FeCoNiCrMn HEA coating resulted in lower wear rate than laser cladded HEA coatings. | Shuo Yin Wenya Li Bo Song Xingchen Yan Min Kuang Yaxin Xu Kui Wen Rocco Lupoi | 2019 | Journal of Materials Science & Technology2019，35，6： | 13 |
| 2 | Effects of metabolizable energy and crude protein levels on laying performance,egg quality and serum biochemical indices of Fengda-1 layers显示文摘This study was conducted to investigate the effects of dietary ME and CP levels on laying performance, egg quality and serum biochemical indices of Fengda-1 layers. In a 2 × 3 factorial arrangement, 2,400 Fengda-1 layers(32 wk of age) were randomly assigned to 6 experimental diets with 2,650 and 2,750 kcal of ME/kg of diet, each containing 14.50%, 15.00% and 15.50% CP, respectively. Each dietary treatment was replicated 5 times, and feed and water were provided ad libitum. The trial lasted for 10 wk, including a2-week acclimation period and an 8-week experimental period. Our results showed that ADFI decreased as the ME level of diet increased from 2,650 to 2,750 kcal/kg(P< 0.05). Layers fed diets with 2,750 kcal/kg ME exhibited higher mortality than those fed with 2,650 kcal/kg ME(P < 0.05). Birds fed with 14.50% and15.00% CP had higher egg production(EP) and egg mass(EM) than those fed with 15.50% CP(P < 0.05).Yolk color increased as the ME level of the diet increased from 2,650 to 2,750 kcal/kg, however, the eggshell thickness decreased(P < 0.05). Serum concentrations of uric acid and triglyceride in layers fed diets with 2,750 kcal/kg ME were higher than those fed diets with 2,650 kcal/kg ME(P < 0.05). There was no significant interaction between ME and CP on laying performance, egg quality, or serum biochemical indices(P > 0.05). Based on the data under the experimental conditions, the optimal dietary ME and CP levels of Fengda-1 layers are 2,650 kcal/kg and 15.00%(33 to 41 wk of age). | Yang Ding Xingchen Bu Nannan Zhang Lanlan Li Xiaoting Zou | 2016 | Animal Nutrition2016，，2： | 11 |
| 3 | Wheat breeding history reveals synergistic selection of pleiotropic genomic sites for plant architecture and grain yield显示文摘Diversity surveys of crop germplasm are important for gaining insights into the genomic basis for plant architecture and grain yield improvement,which is still poorly understood in wheat.In this study,we exome sequenced 287 wheat accessions that were collected in the past 100 years.Population genetics analysis identified that 6.7%of the wheat genome falls within the selective sweeps between landraces and cultivars,which harbors the genes known for yield improvement.These regions were asymmetrically distributed on the A and B subgenomes with regulatory genes being favorably selected.Genome-wide association study(GWAS)identified genomic loci associated with traits for yield potential,and two underlying genes,TaARF12 encoding an auxin response factor and TaDEP1 encoding the G-proteinγ-subunit,were located and characterized to pleiotropically regulate both plant height and grain weight.Elite single-nucleotide haplotypes with increased allele frequency in cultivars relative to the landraces were identified and found to have accumulated over the course of breeding.Interestingly,we found that TaARF12 and TaDEP1 function in epistasis with the classical plant height Rht-1 locus,leading to propose a“Green Revolution”-based working model for historical wheat breeding.Collectively,our study identifies selection signatures that fine-tune the gibberellin pathway during modern wheat breeding and provides a wealth of genomic diversity resources for the wheat research community. | Aili Li Chenyang Hao Zhenyu Wang Shuaifeng Geng Meiling Jia Fang Wang Xiang Han Xingchen Kong Lingjie Yin Shu Tao Zhongyin Deng Ruyi Liao Guoliang Sun Ke Wang Xingguo Ye Chengzhi Jiao Hongfeng Lu Yun Zhou Dengcai Liu Xiangdong Fu Xueyong Zhang Long Mao | 2022 | Molecular Plant2022，15，3： | 4 |
| 4 | CRISPR/Cas9:A powerful tool for crop genome editing显示文摘The CRISPR/Cas9 technology is evolved from a type II bacterial immune system and represents a new generation of targeted genome editing technology that can be applied to nearly all organisms. Site-specific modification is achieved by a single guide RNA(usually about 20nucleotides) that is complementary to a target gene or locus and is anchored by a protospaceradjacent motif. Cas9 nuclease then cleaves the targeted DNA to generate double-strand breaks(DSBs), which are subsequently repaired by non-homologous end joining(NHEJ) or homology-directed repair(HDR) mechanisms. NHEJ may introduce indels that cause frame shift mutations and hence the disruption of gene functions. When combined with double or multiplex guide RNA design, NHEJ may also introduce targeted chromosome deletions,whereas HDR can be engineered for target gene correction, gene replacement, and gene knock-in. In this review, we briefly survey the history of the CRISPR/Cas9 system invention and its genome-editing mechanism. We also describe the most recent innovation of the CRISPR/Cas9 technology, particularly the broad applications of modified Cas9 variants, and discuss the potential of this system for targeted genome editing and modification for crop improvement. | Gaoyuan Song Meiling Jia Kai Chen Xingchen Kong Bushra Khattak Chuanxiao Xie Aili Li Long Mao | 2016 | The Crop Journal2016，4，2： | 4 |
| 5 | Ni-doped ZnCo2O4 atomic layers to boost the selectivity in solar-driven reduction of CO2显示文摘 | Katong Liu Xiaodong Li Liang Liang Ju Wu Xingchen Jiao Jiaqi Xu Yongfu Sun Yi Xie | 2018 | Nano Research2018，11，6： | 3 |
| 6 | An elevated preoperative serum calcium level is a significant predictor for positive peritoneal cytology in endometrial carcinoma显示文摘Objective:To evaluate preoperative serum calcium concentration and investigate the association between calcium level and positive peritoneal cytology in endometrial carcinoma(EC).Methods:A total of 510 patients who were diagnosed with EC and had surgery were initially enrolled in this study at Peking University People's Hospital between January 2012 and December 2016.Clinical characteristics and preoperative serum calcium,albumin,carbohydrate antigen(CA)125,CA19-9,carcinoembryonic antigen(CEA)were extracted from patient records and evaluated according to postoperative peritoneal cytology.Predictive factors were assessed with Cox univariate and multivariate analyses.Factors selected from multivariate analysis results were used to build a predictive model.Results:A total of 510 patients are identified in our database and 444 patients who fulfilled inclusion and exclusion criteria are included in this study.Univariate analysis revealed that ionized calcium concentration was closely related to positive peritoneal cytology,tumor grade and lymph-vascular space invasion(LVSI).Moreover,peritoneal cytology was significantly associated with hypertension,tubal ligation,serum CA125,CA19-9,CEA and ionized calcium level.Multivariate analysis revealed that albumin-adjusted calcium level,CA125 and tubal ligation were independent predictive factors of positive peritoneal cytology(P<0.05).A combination of ionized calcium level with the other two indexes yielded significantly great area under the curve(AUC=0.824).Conclusions:This study enhanced the value of preoperative ionized calcium level.We also identified several potential biomarkers to predict positive peritoneal cytology in EC patients before surgery. | Xingchen Li Yuan Cheng Yangyang Dong Boqiang Shen Xiao Yang Jiaqi Wang Jingyi Zhou Jianliu Wang | 2019 | Chinese Journal of Cancer Research2019，31，6： | 3 |
| 7 | Storage capacity allocation strategy for distribution network with distributed photovoltaic generators显示文摘Distributed photovoltaic generators(DPGs) have been integrated into the medium/low voltage distribution network widely. Due to the randomness and fluctuation of DPG, however, the distribution and direction of power flow changed frequently some days. Therefore, more attention is needed to ensure the safe operation of the distribution network. The installation of energy storage systems(ESSs) can help the network withstand thefluctuations caused by DPG. Based on the discrete Fourier transform method, this paper presents an ESS capacity allocation strategy for the medium/low voltage distribution network with DPG. The reliability scenario models are created via Latin hypercube sampling with Cholesky decomposition and scenario reduction. Numerical results show that the proposed strategy can reduce the power flow fluctuation with less ESS capacity, and increase the penetration capacity of DPG in the distribution network while maintaining the quality of the power supply. | Bin LI Xingchen LI Xiaoqing BAI Zhineng LI | 2018 | Journal of Modern Power Systems and Clean Energy2018，6，6： | 2 |
| 8 | Effect of hole arrangement patterns on the leakage and rotordynamic characteristics of the honeycomb seal显示文摘The honeycomb seal is a vital component to reduce the leakage flow and improvethe system stability for the turbomachines. In this work, a three-dimensional model is established for the interlaced hole honeycomb seal (IHHCS) and the non-interlaced hole honeycombseal (NIHHCS) to investigate its leakage and rotordynamic characteristics by adopting computational fluid dynamics (CFD). Results show that the hole arrangement patterns have littleimpact on the pressure drop and turbulence kinetic energy distribution for the seals, and theIHHCS possesses a slightly lower leakage flow rate than the NIHHCS. Moreover, the numericalresults also show that the NIHHCS possesses a better rotordynamic performance than theIHHCS at all investigated conditions. Both seals show a larger k and a lower Ceff with the increase of the positive preswirl ratios and rotational speeds, while the negative preswirl ratioswould reduce the k and improve the Ceff. The NIHHCS possesses a higher absolute value ofFt for all operating conditions, this could explain the distinction of Ceff for both seals atdifferent working conditions. | Wanfu Zhang Chengjing Gu Xingchen Yang Kexin Wu Chun Li | 2022 | Propulsion and Power Research2022，11，2： | 2 |
| 9 | iRGD decorated liposomes:A novel actively penetrating topical ocular drug delivery strategy显示文摘Ocular drug delivery remains a significant challenge that is limited by poor corneal retention and permeation,resulting in low ocular bioavailability(<5%).Worse still,the most convenient and safe route of ocular drug administration,topical administration results in a drug bioavailability of less than 1%.iRGD modified drug delivery strategies have been developed for cancer therapy,however active targeting iRGD platforms for ocular drug delivery have yet to be explored.Herein,an iRGD modified liposomes was developed for ocular drug delivery via topical administration.The results indicated that iRGD modified liposomes could prolong the corneal retention time and enhance corneal permeability in an iRGD receptor mediated manner.These findings provided a novel strategy for topical ocular drug delivery for the treatment of posterior ocular diseases. | Hai Huang Xiaorong Yang Huili Li Hansi Lu James Oswald Yongmei Liu Jun Zeng Chaohui Jin Xingchen Peng Jiyan Liu Xiangrong Song | 2020 | Nano Research2020，13，11： | 2 |
| 10 | Large-size niobium disulfide nanoflakes down to bilayers grown by sulfurization显示文摘Atomically thin layers of group VB transition metal dichalcogenides (TMDs)provide a unique platform for studying two-dimensional (2D) superconductivityand charge density waves. Thus far, the bottom-up synthesis of these 2D TMDshas often involved precursors that are corrosive or toxic, and their lateral sizesare typically only a few micrometers. In this paper, we report the growth ofNbS2 nanoflakes with a thickness down to bilayers and a lateral dimension upto tens of micrometers without using harsh chemical species. NbS2 nanoflakeseither standing or lying with respect to the sapphire substrate were obtained bysulfurization of niobium oxide films that were prepared via pulsed laser deposition.Standing nanoflakes are considered to grow epitaxiaUy on the sapphire substrateaccording to their ordered orientation, while lying nanoflakes with randomorientations were grown directly on top of the niobium oxide films. The Ramanspectra of the 3R-phase exhibit strong dependence on the layer thickness, wherethe A1 mode softens as the layer number decreases. In contrast to the stable bulkNbS2, the ultra-thin nanoflakes were oxidized on their top surfaces after prolongedexposure to air, as revealed by X-ray photoelectron spectroscopy. Our workexplores an important route to synthesize large-size NbS2 nanoflakes and studiesthe oxidation process, which is a critical factor to consider if practical applicationsshould be realized in the future. | Zhen Li Wencao Yang Yaroslav Losovyj Jun Chen Enzhi Xu Haoming Liu Madilynn Werbianskyj Herbert A. Fertig Xingchen Ye Shixiong Zhang | 2018 | Nano Research2018，11，11： | 2 |
| 11 | The Scorpion Venom Peptide Smp76 Inhibits Viral Infection by Regulating Type-Ⅰ Interferon Response显示文摘Dengue virus(DENV) and Zika virus(ZIKV) have spread throughout many countries in the developing world and infect millions of people every year, causing severe harm to human health and the economy. Unfortunately, there are few effective vaccines and therapies available against these viruses. Therefore, the discovery of new antiviral agents is critical.Herein, a scorpion venom peptide(Smp76) characterized from Scorpio maurus palmatus was successfully expressed and purified in Escherichia coli BL21(DE3). The recombinant Smp76(rSmp76) was found to effectively inhibit DENV and ZIKV infections in a dose-dependent manner in both cultured cell lines and primary mouse macrophages. Interestingly,rSmp76 did not inactivate the viral particles directly but suppressed the established viral infection, similar to the effect of interferon(IFN)-b. Mechanistically, rSmp76 was revealed to upregulate the expression of IFN-b by activating interferon regulatory transcription factor 3(IRF3) phosphorylation, enhancing the type-Ⅰ IFN response and inhibiting viral infection.This mechanism is significantly different from traditional virucidal antimicrobial peptides(AMPs). Overall, the scorpion venom peptide Smp76 is a potential new antiviral agent with a unique mechanism involving type-Ⅰ IFN responses,demonstrating that natural AMPs can enhance immunity by functioning as immunomodulators. | Zhenglin Ji Fangfang Li Zhiqiang Xia Xingchen Guo Minjun Gao Fang Sun Yuting Cheng Yingliang Wu Wenxin Li Syed Abid Ali Zhijian Cao | 2018 | Virologica Sinica2018，33，6： | 2 |
| 12 | Trajectory planning and motion control of full-row seedling pick-up arm显示文摘Frequent start-stops of automatic seedling transplanters would lengthen the seedling picking time due to alternating movement of the motor,and cause positioning errors and frequent motor vibrations when starting the machine.To solve these problems and ensure the pick-up continuity of automatic transplanters,in this study the smooth circular arc interpolation algorithm and the least square method for multinomial curve fitting were used to conduct the trajectory planning of automatic transplanter based on the movement of the pick-up arm of the transplanter.Velocity and time curves were fitted in segments to acquire motion control parameters and further tracking control was conducted.The mathematical model of the control system was established using Simulink,and simulation analysis and system debugging test were performed.Experiments show that the trajectory curves obtained by MATLAB’s data processing can realize the continual and smooth motion trajectory of the pick-up arm;stepper motor velocity control can effectively track the planning curve and improve the seedling pick-up efficiency.The pick-up and pushing time of each motion of the planned plug seedling transplanter reduced by 1.0678 s and the start-stop times reduced from 6 to 1,which solved the frequent motor vibrations when starting the machine and improved the stability of the system.In addition,overstep and out-of-step of the motor at the start-stop moment were avoided and displacement error was reduced. | Ling Ren Ning Wang Weibin Cao Jiangquan Li Xingchen Ye | 2020 | International Journal of Agricultural and Biological Engineering2020，13，3： | 1 |
| 13 | In-plane heterostructured Ag_(2)S-In_(2)S_(3) atomic layers enabling boosted CO_(2) photoreduction into CH_(4)显示文摘Sluggish separation and migration kinetics of the photogenerated carriers account for the low-efficiency of CO_(2) photoreduction into CH_(4). Design and construction two-dimensional (2D) in-plane heterostructures demonstrate to be an appealing approach to address above obstacles. Herein, we fabricate 2D in-plane heterostructured Ag_(2)S-In_(2)S_(3) atomic layers via an ion-exchange strategy. Photoluminescence spectra, time-resolved photoluminescence spectra, and photoelectrochemical measurements firmly affirm the optimized carrier dynamics of the In_(2)S_(3) atomic layers after the introduction of in-plane heterostructure. In-situ Fourier transform infrared spectroscopy spectra and density functional theory (DFT) calculations disclose the in-plane heterostructure contributes to CO_(2) activation and modulates the adsorption strength of CO* intermediates to facilitate the formation of CHO* intermediates, which are further protonated to CH4. In consequence, the in-plane heterostructure achieves the CH_(4) evolution rate of 20 µmol·g^(−1)·h^(−1), about 16.7 times higher than that of the In2S3 atomic layers. In short, this work proves construction of in-plane heterostructures as a promising method for obtaining high-efficiency CO_(2)-to-CH_(4) photoconversion properties. | Weiwei Shao Shumin Wang Juncheng Zhu Xiaodong Li Xingchen Jiao Yang Pan Yongfu Sun Yi Xie | 2021 | Nano Research2021，14，12： | 1 |
| 14 | Correlations between the North China Craton and the Indian Shield:Constraints from regional metallogeny显示文摘The correlation between the North China Craton(NCC) and the Indian Shield(IND) has been a hot topic in recent years,On the basis of ore deposit databases,the NCC and IND have shown broad similarity in metallogenesis from the middle Archaean to the Mesoproterozoic,The two blocks both have three major metallogenic systems:(1) the Archaean BIF metallogenic system;(2) the Paleoproterozoic Cu-Pb-Zn metallogenic system;and(3) the Mesoproterozoic Fe-Pb-Zn system,In the north margin of the NCC and the west margin of the IND,the Archaean BIF-Au-Cu-Pb-Zn deposits had the same petrogenesis and host rocks,the Paleoproterozoic Cu-Pb-Zn deposits were controlled by active belts,and the Mesoproterozoic Fe-Pb-Zn deposits were mainly related to multi-stage rifting,Matching regional mineralization patterns and geological features has established the continental assembly referred to as 'NCWI',an acronym for the north margin of the NCC(NC) and the west margin of the IND(WI) during the middle Archaean to the Mesoproterozoic,In this assembly,the available geological and metallogenic data from the Eastern Block and active belts of NC fit those from the Dharwar craton and the Aravalli-DelhiVindhyan belt of WI,respectively,Moreover,the depositional model and environment of Paleoproterozoic metasedimentary manganese deposits in NCWI implied that the assembly may be located at low latitudes,where the conditions were favorable for dissolving ice and precipitating manganese deposits, | Caifeng Li Dongyue Chen Jianping Chen Xizhen Chen Xingchen Yang M.A.Aboelnour | 2015 | Geoscience Frontiers2015，6，6： | 1 |
| 15 | Analysis on Pigment and Photosynthetic Characteristics of Leaves of New Strain of Rehmannia glutinosa显示文摘Through the analysis on the leaf color and photosynthetic characteristics of new strains and main cultivars of Rehmannia glutinosa,it is expected to provide theoretical basis for breeding of new varieties. Chlorophyll,anthocyanin,and net photosynthetic rate(Pn),stomatal conductance(Cond),transpiration rate(Tr),and intercellular CO2concentration(Ci) in 8 varieties of Rehmannia glutinosa were measured by spectrophotometer and LI-6400 XT Portable Photosynthesis System. The results showed that the chlorophyll content of Huaidijin 8(2. 84 mg/g),Huaidi 81(2. 71 mg/g),Huaidi 85-5(2. 69 mg/g),Jinjiu(2. 66 mg/g) and Huaidi 83(2. 63 mg/g) was higher; the anthocyanin content of Jinjiu(0. 169) and Huaidijin 8(0. 165) was higher,while the anthocyanin content Huaidi 83(0. 060) was the lowest; Pn of Huaidi81[2. 41 μmol/(m2·s) ],Huaidi 83[2. 37 μmol/(m2·s) ]and Huaidijin 8[2. 25 μmol/(m2·s) ]was higher,and the anthocyanin content was positively correlated with Pn,while the anthocyanin content was negatively correlated with Pn; Huaidijin 8 and Huaidi 83 showed dominant advantages in single plant fresh weight,indicator component,and resistance over the main cultivars. This indicates that the new variety Huaidijin 8 and Huaidi 83 have excellent comprehensive traits and can be properly popularized. | Xing FAN Xiaoting ZHOU Jun WANG Xingchen SHANG Jianjun LI | 2017 | Asian Agricultural Research2017，9，6： | 1 |
| 16 | The soft glumes of common wheat are sterile-lemmas as determined by the domestication gene Q显示文摘The Q gene in common wheat encodes an APETALA2(AP2) transcription factor that causes the free threshing attribute. Wheat spikelets bearing several florets are subtended by a pair of soft glumes that allow free liberation of seeds. In wild species, the glumes are tough and rigid,making threshing difficult. However, the nature of these 'soft glumes', caused by the domestication allele Q is not clear. Here, we found that over expression of Q in common wheat leads to homeotic florets at glume positions. We provide phenotypic, microscopy, and marker genes evidence to demonstrate that the soft glumes of common wheat are in fact lemma-like organs, or so-called sterile-lemmas. By comparing the structures subtending spikelets in wheat and other crops such as rice and maize, we found that AP2 genes may play conserved functions in grasses by manipulating vestigial structures, such as floret-derived soft glumes in wheat and empty glumes in rice. Conversion of these seemingly vegetative organs to reproductive organs may be useful in yield improvement of crop species. | Gaoyuan Song Guoliang Sun Xingchen Kong Meiling Jia Ke Wang Xingguo Ye Yun Zhou Shuaifeng Geng Long Mao Aili Li | 2019 | The Crop Journal2019，7，1： | 1 |
| 17 | NAS4RRAM: neural network architecture search for inference on RRAM-based accelerators显示文摘The RRAM-based accelerators enable fast and energy-efficient inference for neural networks.However, there are some requirements to deploy neural networks on RRAM-based accelerators, which are not considered in existing neural networks.(1) Because the noise problem and analog-digital converters/digitalanalog converters(ADC/DAC) affect the prediction accuracy, they should be modeled in networks.(2) Because the weights are mapped to the RRAM cells, they should be quantized, and the number of weights is limited by the number of RRAM cells in the accelerator. These requirements motivate us to customize the hardware-friendly network for the RRAM-based accelerator. We take the idea of network architecture search(NAS) to design networks with high prediction accuracy that meet the requirements. We propose a framework called NAS4RRAM to search for the optimal network on the given RRAM-based accelerator. The experiments demonstrate that NAS4RRAM can apply to different RRAM-based accelerators with different scales. The performance of searched networks outperforms the manually designed ResNet. | Zhihang YUAN Jingze LIU Xingchen LI Longhao YAN Haoxiang CHEN Bingzhe WU Yuchao YANG Guangyu SUN | 2021 | Science China(Information Sciences)2021，64，6： | 0 |
| 18 | Sustainability performance analysis of environment innovation systems using a two-stage network DEA model with shared resources显示文摘The term environmental innovation system refers to an innovation network composed of enterprises,universities,and research institutions involved in the development and diffusion of environmental technology,with the participation of a government.An environmental innovation system not only exerts important impact on the achievement of carbon neutrality but also affects social and economic activities.Investigations on environmental innovation system performance constantly assume a singlestage independent system while ignoring its internal structure.However,such systems are composed of environmental innovation research and development(R&D)and environmental innovation conversion subsystems.A two-stage data envelopment analysis(DEA)model is developed in this study to analyze the efficiency of Chinese regional environmental innovation system by opening the'black box'and considering shared resources.Empirical results indicated that China presents high overall environmental innovation efficiency although some regions need to improve.Regions with low efficiencies in both environmental innovation R&D(EIR)and environmental innovation conversion(EIC)subsystems should expand their investment in and strengthen the management of environmental innovation resources.Regions with low EIR efficiency should improve the absorption and transformation of environmental innovation achievements.Regions with low EIC efficiency should increase investment in the commercialization of environmental innovation achievements and encourage green economy industries,such as new energy,art,tourism,and environmental protection. | Jiangjiang YANG Jie WU Xingchen LI Qingyuan ZHU | 2022 | Frontiers of Engineering Management2022，9，3： | 0 |
| 19 | Enhanced room-temperature Naþionic conductivity in Na_(4.92)Y_(0.92)Zr_(0.08)Si_(4)O_(12)显示文摘Developing cost-effective and reliable solid-state sodium batteries with superior performance is crucial for stationary energy storage.A key component in facilitating their application is a solid-state electrolyte with high conductivity and stability.Herein,we employed aliovalent cation substitution to enhance ionic conductivity while preserving the crystal structure.Optimized substitution of Y^(3+)with Zr^(4+)in Na_(5)YSi_(4)O_(12) introduced Naþion vacancies,resulting in high bulk and total conductivities of up to 6.5 and 3.3 mS cm^(-1),respectively,at room temperature with the composition Na_(4.92)Y_(0.92)Zr_(0.08)Si_(4)O_(12)(NYZS).NYZS shows exceptional electrochemical stability(up to 10 V vs.Naþ/Na),favorable interfacial compatibility with Na,and an excellent critical current density of 2.4 mA cm^(-2).The enhanced conductivity of Naþions in NYZS was elucidated using solid-state nuclear magnetic resonance techniques and theoretical simulations,revealing two migration routes facilitated by the synergistic effect of increased Naþion vacancies and improved chemical environment due to Zr^(4+)substitution.NYZS extends the list of suitable solid-state electrolytes and enables the facile synthesis of stable,low-cost Naþion silicate electrolytes. | Aikai Yang Kai Yao Mareen Schaller Enkhtsetseg Dashjav Hang Li Shuo Zhao Qiu Zhang Martin Etter Xingchen Shen Huimin Song Qiongqiong Lu Ruijie Ye Igor Moudrakovski Quanquan Pang Sylvio Indris Xingchao Wang Qianli Ma Frank Tietz Jun Chen Olivier Guillon | 2023 | eScience2023，3，6： | 0 |
| 20 | A Federated Domain Adaptation Algorithm Based on Knowledge Distillation and Contrastive Learning显示文摘Smart manufacturing suffers from the heterogeneity of local data distribution across parties,mutual information silos and lack of privacy protection in the process of industry chain collaboration.To address these problems,we propose a federated domain adaptation algorithm based on knowledge distillation and contrastive learning.Knowledge distillation is used to extract transferable integration knowledge from the different source domains and the quality of the extracted integration knowledge is used to assign reasonable weights to each source domain.A more rational weighted average aggregation is used in the aggregation phase of the center server to optimize the global model,while the local model of the source domain is trained with the help of contrastive learning to constrain the local model optimum towards the global model optimum,mitigating the inherent heterogeneity between local data.Our experiments are conducted on the largest domain adaptation dataset,and the results show that compared with other traditional federated domain adaptation algorithms,the algorithm we proposed trains a more accurate model,requires fewer communication rounds,makes more effective use of imbalanced data in the industrial area,and protects data privacy. | HUANG Fang FANG Zhijun SHI Zhicai ZHUANG Lehui LI Xingchen HUANG Bo | 2022 | Wuhan University Journal of Natural Sciences2022，27，6： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员