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| 1 | Donor-Acceptor Typed AIE Luminogens with Near-infrared Emission for Super-resolution Imaging显示文摘Aggregation-induced emission(AIE)luminogens(AIEgens)with high brightness in aggregates exhibit great potentials in biological imaging,but these AIEgens are seldom applied in super-resolution biological imaging,especially in the imaging by using the structural illumination microscope(SIM).Based on this consideration,we synthesized the donor-acceptor typed AIEgen of DTPA-BTN,which not only owns high brightness in the near-infrared(NIR)emission region from 600 nm to 1000 nm(photoluminescence quantum yield,PLQYs=11.35%),but also displays excellent photo-stability.In addition,AIE nanoparticles based on 4,7-ditriphenylamine-[1,2,5]-thiadiazolo[3,4-c]pyridine(DTPA-BTN)were also prepared with highly emissive features and excellent biocompatibility.Finally,the developed DTPA-BTN-based AIE nanoparticles were applied in the super-resolution cellular imaging via SIM,where much smaller full width at half-maximum values and high signal to noise ratios were obtained,indicating the superior imaging resolution.The results here imply that highly emissive AIEgens or AIE nanoparticles can be promising imaging agents for super-resolution imaging via SIM. | SHEN Qifei XU Ruohan WANG Zhi ZHAO Tianyu ZHOU Yu XU Yanzi YANG Zhiwei LEI Ming MENG Lingjie DANG Dongfeng | 2021 | Chemical Research in Chinese Universities2021，37，1： | 0 |
| 2 | Chemical cross-linking and mechanically reinforced carbon network constructed by graphene boosts potassium ion storage显示文摘Carbon-based electrodes of potassium-ion batteries are of great research interest ascribed to their low cost and environmentally friendly distinctions.However,traditional carbon materials usually exhibit weak mechanical properties and incomplete crosslinking,resulting in poor stability and electrochemical performance.Herein,we report a new strategy for modifying reduced graphene oxide into a uniform few-layer structure through a sol–gel method combined with acid etching treatment.The obtained chemical cross-linking and mechanically reinforced carbon network constructed by graphene(CNCG)demonstrates excellent electrochemical and mechanical properties.Adopted as a free-standing anode(~7 mg·cm^(−2))for potassium ion battery,the asachieved CNCG delivers a high reversible specific capacity of 317.7 mAh·g^(−1) at a current density of 50 mA·g^(−1) and admirable cycle stability(208.4 mAh·g^(−1) at 50 mA·g^(−1) after 500 cycles).The highly reversible structural stability and fully cross-linked properties during potassiation are revealed by ex-situ characterization.This work provides new ideas for the synthesis of new carbon materials and the development of high-performance electrodes. | Chenxu Wang Ruohan Yu Wen Luo Wencong Feng Yuanhao Shen Nuo Xu Liqiang Mai | 2022 | Nano Research2022，15，10： | 0 |
| 3 | Dynamic Routing of Multiple QoS-Required Flows in Cloud-Edge Autonomous Multi-Domain Data Center Networks显示文摘The 6th generation mobile networks(6G)network is a kind of multi-network interconnection and multi-scenario coexistence network,where multiple network domains break the original fixed boundaries to form connections and convergence.In this paper,with the optimization objective of maximizing network utility while ensuring flows performance-centric weighted fairness,this paper designs a reinforcement learning-based cloud-edge autonomous multi-domain data center network architecture that achieves single-domain autonomy and multi-domain collaboration.Due to the conflict between the utility of different flows,the bandwidth fairness allocation problem for various types of flows is formulated by considering different defined reward functions.Regarding the tradeoff between fairness and utility,this paper deals with the corresponding reward functions for the cases where the flows undergo abrupt changes and smooth changes in the flows.In addition,to accommodate the Quality of Service(QoS)requirements for multiple types of flows,this paper proposes a multi-domain autonomous routing algorithm called LSTM+MADDPG.Introducing a Long Short-Term Memory(LSTM)layer in the actor and critic networks,more information about temporal continuity is added,further enhancing the adaptive ability changes in the dynamic network environment.The LSTM+MADDPG algorithm is compared with the latest reinforcement learning algorithm by conducting experiments on real network topology and traffic traces,and the experimental results show that LSTM+MADDPG improves the delay convergence speed by 14.6%and delays the start moment of packet loss by 18.2%compared with other algorithms. | Shiyan Zhang Ruohan Xu Zhangbo Xu Cenhua Yu Yuyang Jiang Yuting Zhao | 2024 | Computers, Materials & Continua2024，78，2： | 0 |
| 4 | Synthesis of D-A typed AIE luminogens in isomeric architecture and their application in latent fingerprints imaging显示文摘Among the emitters in powder dusting to visualize the latent fingerprints(LFPs),aggregation-induced emission luminogens(AIEgens)are well employed for their high brightness and resistance to photobleaching.However,the serious background interference and low resolution still limit their fast development.Therefore,to further enhance the signal-to-noise ratio in LFPs imaging,especially to improve the analysis for level 3 details,donor-acceptor(D-A)typed AIEgens of DTPA-2,3-P,DTPA-2,5-P and DTPA-2,6-P are designed here.It is observed that strong emission covering from 450nm to 650nm can be obtained for all these molecules,especially that a high PLQY value of 10.06%in solids is achieved in DTPA-2,3-P.This is much higher than that of the other two cases(0.80%and 0.51%).By utilizing the DTPA-2,3-P in powder dusting,fluorescence imaging of LFPs can be clearly captured on both smooth and rough substrates.Moreover,confocal laser scanning microscope(CLSM)enables us to achieve high-resolution LFPs imaging in both 2D and 3D views,providing more detailed information of fingerprints pores in width,distance,distribution,and shapes.The results here demonstrate that highly emissive AIEgen of DTPA-2,3-P could be an excellent candidate for the visualization of fingerprints,thus providing the potential application in criminal investigation in the future. | Peijuan Zhang Qifei Shen Yu Zhou Fengyi He Bo Zhao Zhi Wang Ruohan Xu Yanzi Xu Zhiwei Yang Lingjie Meng Dongfeng Dang | 2023 | Chinese Chemical Letters2023，34，8： | 0 |
| 5 | ZIF-Mediated Anchoring of Co species on N-doped Carbon Nanorods as an Efficient Cathode Catalyst for Zn-Air Batteries显示文摘Developing efficient oxygen reduction reaction(ORR)catalyst is essential for the practical application of Zn-air batteries(ZABs).In this contribution,we develop a novel zeolitic imidazolate framework(ZIF)-mediated strategy to anchor Co species on N-doped carbon nanorods for efficient ORR.Featuring ultrahigh N-doping(10.29 at.%),monodisperse Co nanocrystal decoration,and well-dispersed Co-N_(x)functionalization,the obtained Co-decorated N-doped carbon nanorods(Co@NCNR)exhibit a decent ORR performance comparable to commercial Pt/C in alkaline media.Aqueous ZABs have been assembled using Co@NCNR as the cathode catalyst.The assembled ZABs manifest high initial open-circuit voltage as well as high energy density.In addition,the Co@NCNR also demonstrates ideal ORR performance in quasi-solid-state ZABs. | Qiang Yu Jianshuai Lv Jiantao Li Ruohan Yu Jinsong Wu Shibo Xi Xinyuan Li Nuo Xu Liang Zhou Liqiang Ma | 2023 | Energy & Environmental Materials2023，6，3： | 0 |
| 6 | Realizing Plain Optimization of the Thermoelectric Properties in BiCuSeO Oxide via Self-Substitution-Induced Lattice Dislocations显示文摘Seeking new strategies to tune the intrinsic defect and optimize the thermoelectric performance via no or less use of external doped elements(i.e.,plain optimization)is an important method to realize the sustainable development of thermoelectric materials.Meanwhile,creating dislocation defects in oxide systems is quite challenging because the rigid and stiff ionic/covalent bonds can hardly tolerate the large strain energy associated with dislocations.Herein,taking BiCuSe_(O) oxide as an example,the present work reports a successful construction of dense lattice dislocations in BiCuSe_(O) by self-doping of Se at the O site(i.e.,Se_(O) self-substitution),and achieves plain optimization of the thermoelectric properties with only external Pb doping.Owing to the self-substitution-induced large lattice distortion and the potential reinforcement effect by Pb doping,high-density(about 3.0×10^(14 )m^(−2))dislocations form in the grains,which enhances the scattering strength of mid-frequency phonon and results in a substantial low lattice thermal conductivity of 0.38 W m^(−1) K^(−1) at 823 K in Pb-doped BiCuSe_(O).Meanwhile,PbBi doping and Cu vacancy markedly improve the electrical conductivity while maintaining a competitively high Seebeck coefficient,thereby contributing to a highest power factor of 942μW m^(−1) K^(−2).Finally,a remarkably enhanced zT value of 1.32 is obtained at 823 K in Bi_(0.94)Pb_(0.06)Cu_(0.97)Se_(1.05)O_(0.95) with almost compositional plainification.The high-density dislocation structure reported in this work will also provide a good inspiration for the design and construction of dislocations in other oxide systems. | Rui Xu Zhiwei Chen Qizhu Li Xiaoyu Yang Han Wan Mengruizhe Kong Wei Bai Nengyuan Zhu Ruohan Wang Jiming Song Zhou Li Chong Xiao Binghui Ge | 2023 | Research2023，，4： | 0 |
| 7 | Metabolic signatures and potential biomarkers for the diagnosis and treaeatment of colon cancer cachexia显示文摘Cancer cachexia(CAC)is a debilitating condition that often arises from noncachexia cancer(NCAC),with distinct metabolic characteristics and medical treatments.However,the metabolic changes and underlying molecular mechanisms during cachexia progression remain poorly understood.Understanding the progression of CAC is crucial for developing diagnostic approaches to distinguish between CAC and NCAC stages,facilitating appropriate treatment for cancer patients.In this study,we establish a mouse model of colon CAC and categorize the mice into three groups:CAC,NCAC and normal control(NOR).By performing nuclear magnetic resonance(NMR)-based metabolomic profiling on mouse sera,we elucidate the metabolic properties of these groups.Our findings unveil significant differences in the metabolic profiles among the CAC,NCAC and NOR groups,highlighting significant impairments in energy metabolism and amino acid metabolism during cachexia progression.Additionally,we observe the elevated serum levels of lysine and acetate during the transition from the NCAC to CAC stages.Using multivariate ROC analysis,we identify lysine and acetate as potential biomarkers for distinguishing between CAC and NCAC stages.These biomarkers hold promise for the diagnosis of CAC from noncachexia cancer.Our study provides novel insights into the metabolic mechanisms underlying cachexia progression and offers valuable avenues for the diagnosis and treatment of CAC in clinical settings. | Xu Qiu Ruohan Lu Qiqing He Shu Chen Caihua Huang Donghai Lin | 2023 | Acta Biochimica et Biophysica Sinica2023，55，12： | 0 |
| 8 | Inhibition of aryl hydrocarbon receptor signaling promotes the terminal differentiation of human erythroblasts显示文摘The aryl hydrocarbon receptor(AHR)plays an important role during mammalian embryo development.Inhibition of AHR signaling promotes the development of hematopoietic stem/progenitor cells.AHR also regulates the functional maturation of blood cells,such as T cells and megakaryocytes.However,little is known about the role of AHR modulation during the development of erythroid cells.In this study,we used the AHR antagonist StemRegenin 1(SR1)and the AHR agonist 2,3,7,8-tetrachlorodibenzo-p-dioxin during different stages of human erythropoiesis to elucidate the function of AHR.We found that antagonizing AHR signaling improved the production of human embryonic stem cell derived erythrocytes and enhanced erythroid terminal differentiation.RNA sequencing showed that SR1 treatment of proerythroblasts upregulated the expression of erythrocyte differentiation-related genes and downregulated actin organization-associated genes.We found that SR1 accelerated F-actin remodeling in terminally differentiated erythrocytes,favoring their maturation of the cytoskeleton and enucleation.We demonstrated that the effects of AHR inhibition on erythroid maturation were associated with F-actin remodeling.Our findings help uncover the mechanism for AHRmediated human erythroid cell differentiation.We also provide a new approach toward the large-scale production of functionally mature human pluripotent stem cell-derived erythrocytes for use in translational applications. | Yijin Chen Yong Dong Xulin Lu Wanjing Li Yimeng Zhang Bin Mao Xu Pan Xiaohong Li Ya Zhou Quanming An Fangxin Xie Shihui Wang Yuan Xue Xinping Cai Mowen Lai Qiongxiu Zhou Yan Yan Ruohan Fu Hong Wang Tatsutoshi Nakahata Xiuli An Lihong Shi Yonggang Zhang Feng Ma | 2022 | Journal of Molecular Cell Biology2022，14，2： | 0 |
| 9 | Controlling Factors and Accumulation Model of Hydrocarbon Reservoirs in the Upper Cretaceous Yogou Formation, Koulele Area, Termit Basin, Niger显示文摘Based on the sedimentary and tectonic background of the Termit Basin, this paper focuses on the Upper Cretaceous Yogou Formation and uses organic geochemistry, logging, oil testing and seismic data to analyze the primary control factors of the hydrocarbon accumulation and establish corresponding model in order to predict favorable exploration target zones of hydrocarbon reservoirs. This study demonstrates that the Upper Cretaceous Yogou Formation is a self-generation and self-accumulation type reservoir. The Yogou Formation hydrocarbon reservoirs in the Koulele area are controlled by four factors:(1) the source rock is controlled by a wide range of YS1-YS2 marine shale,(2) the sandstone reservoir is controlled by the YS3 underwater distributary channel and storm dunes,(3) migration of hydrocarbons is controlled by faults and the regional monocline structure, and(4) the accumulation of hydrocarbons is controlled by lateral seal. The structures in the western Koulele area are primarily reverse fault-blocks with large throws, and the structures in the east are dominantly fault-blocks with small throws(co-rotating and reverse) and a fault-nose. In the western Koulele area, where the facies are dominated by storm dunes on a larger scale, it is easier to form lithologic reservoirs of sandstone lens. In the eastern Koulele area, high-quality channel sandstone reservoirs, fault-blocks with small throws, and the monocline structure benefit for the formation of updip pinch out lithologic traps, fault lithologic reservoirs and fault-nose structural reservoirs. Future exploration targets should be focused in the western storm dunes zone and eastern distributary channel sand zone with small fault-blocks. | Xuying Wang Lunkun Wan Zaixing Jiang Ruohan Liu Xiabin Wang Wangxin Tang Yi Gao Shengqian Liu Wenmao Xu | 2017 | Journal of Earth Science2017，28，6： | 0 |
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