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| 1 | One ion to catch them all: Targeted high-precision Boltzmann thermometry over a wide temperature range with Gd^(3+)显示文摘Ratiometric luminescence thermometry with trivalent lanthanide ions and their 4f^(n) energy levels is an emerging technique for non-invasive remote temperature sensing with high spatial and temporal resolution.Conventional ratiometric luminescence thermometry often relies on thermal coupling between two closely lying energy levels governed by Boltzmann’s law.Despite its simplicity,Boltzmann thermometry with two excited levels allows precise temperature sensing,but only within a limited temperature range.While low temperatures slow down the nonradiative transitions required to generate a measurable population in the higher excitation level,temperatures that are too high favour equalized populations of the two excited levels,at the expense of low relative thermal sensitivity.In this work,we extend the concept of Boltzmann thermometry to more than two excited levels and provide quantitative guidelines that link the choice of energy gaps between multiple excited states to the performance in different temperature windows.By this approach,it is possible to retain the high relative sensitivity and precision of the temperature measurement over a wide temperature range within the same system.We demonstrate this concept using YAl_(3)(BO_(3))_(4)(YAB):Pr^(3+),Gd^(3+)with an excited 6 PJ crystal field and spin-orbit split levels of Gd^(3+)in the UV range to avoid a thermal black body background even at the highest temperatures.This phosphor is easily excitable with inexpensive and powerful blue LEDs at 450 nm.Zero-background luminescence thermometry is realized by using blue-to-UV energy transfer upconversion with the Pr^(3+)−Gd^(3+)couple upon excitation in the visible range.This method allows us to cover a temperature window between 30 and 800 K. | Dechao Yu Huaiyong Li Dawei Zhang Qinyuan Zhang Andries Meijerink Markus Suta | 2021 | Light(Science & Applications)2021，10，12： | 4 |
| 2 | Leucocyte apheresis in the treatment of paediatric ulcerative colitis显示文摘 | Tarja Ruuska Marja-Leena L? hdeaho Yelda Sutas Merja Ashorn Juhani Gr? nlund | 2007 | Scandinavian Journal of Gastroenterology2007，，11： | 1 |
| 3 | Probiotics:effects on immunity显示文摘 | Yelda Sutas Pasi Kankaanp (aa) Heikki Arvilommi and Seppo Salminen | 2001 | Am J Clin Nutr2001，73，： | 1 |
| 4 | Probiotics:effects on immunity显示文摘 | Isolauri E Sutas Y Kankaanpaa P | 2001 | Am J Clin Nutr2001，73，： | 1 |
| 5 | Probiotics : effects on immunity 显示文摘 | Isolauri E Sutas Y Kankaanpaa P | 2001 | The American Journal of Clinical Nutrition2001，73，2： | 1 |
| 6 | Detection of human papillomavirus DNA by PCR/microfluorometry for sceening of cervical cancer显示文摘 | Yamaguchi A Hashimoto N T sutae W | 2002 | Clin Chim Acta2002，318，12： | 1 |
| 7 | MRI of malignant melanom of liver显示文摘 | 2,Furuta M Suta H Nakamoto S | 1995 | RadiatMed1995，13，： | 1 |
| 8 | Probiotics: effects on immunity显示文摘 | Isolauri E Sutas Y Kankaanpaa P | 2001 | Am J Clin Nutr2001，，： | 1 |
| 9 | Probiotics:effects on immunity显示文摘 | Isolauri E Sutas Y Kankaanpaa P | 2001 | Am J Clin Nutr2001，73，2： | 1 |
| 10 | Interleukin-10 generation in atopic children following oral lactobacillus rhamnosus GG显示文摘 | sutas Y Hurme M | 2000 | Clin Exp Allergy2000，30，12： | 1 |
| 11 | Probiotics in the management of atopic eczema显示文摘 | Arvola T Sutas Y | 2000 | Clin Exp Allergy2000，30，11： | 1 |
| 12 | Probiotics in the management of atopic eczema显示文摘 | ISOLAURI E ARVOLA T SUTAS Y | 2000 | Clinical and Experimental Allergy2000，，30： | 1 |
| 13 | Cortical representation of species- specific vocalizations in Guinea pig 显示文摘 | Suta D Popelar J Burianova J | 2013 | PLoS One2013，8，65： | 1 |
| 14 | Oral cow milk challenge abolishes antigen - speciilc interferon - gamma production in the peripheral blood of children with atopic dermatitis and cow milk allergy显示文摘 | Sutas Y Hurme M Isolauri E | 1997 | Clin Exper Allergy1997，27，3： | 1 |
| 15 | Probiotics in the manage-ment of atopic eczema显示文摘 | Isolauri E Arvola T Sutas Y | 2000 | Clin Exp Allergy2000，30，11： | 1 |
| 16 | Probiotics:effects on immunity显示文摘 | ISOLAURI E SUTAS Y KANKAA P | 2001 | Am J Clin Nutr2001，73，： | 1 |
| 17 | Probiotics in the management of atopic eczema显示文摘 | Isolauri E Arvola T Sutas Y | | 0，，11： | 1 |
| 18 | Mandibular third molar surgery with primary closure and tube drain显示文摘 | Sutas Rakprasitkul Verasak Pairuchvej | 1997 | International Journal of Oral & Maxillofacial Surgery1997，，3： | 1 |
| 19 | Suppression of lymphocyte proliferation in vitro by bovine caseins hydrolyzed with Lactobacillus casei GG-derived enzymes显示文摘 | SUTAS Y SOPPI E KORHONEN H | 1996 | Journal of Allergy and Cliuical Immunology1996，98，1： | 1 |
| 20 | Regulation of osteoblast differentiation mediated by bone morphogenetic proteins,hedgehogs,and cbfa1显示文摘 | Yamaguchi A Komori T Suta T | 2000 | Endocr Rev2000，21，4： | 1 |
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