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| 1 | Polymorphisms in PPARD,PPARG and APM1 associated with four types of Traditional Chinese Medicine constitutions显示文摘Based on the theory of constitution of Traditional Chinese Medicine (TCM), the human population is divided into nine constitutions including one balanced constitution (Normality) and eight unbalanced constitutions (Yang-deficiency, Yin-deficiency, Phlegm-wetness, Qi-deficiency, Wetness-heat, Blood stasis, Depressed constitution, and Inherited special constitution). Different constitutions have specific metabolic features and different susceptibility to certain diseases. However, whether a genetic basis accounts for such constitution classifica-tion is yet to be determined. Here we performed a genetic study to assess the association between genetic variations of metabolic genes in-cluding PPARD, PPARG and APM1 and the constitutions. A total of 233 individuals of the Han population in China were classified into four groups, Normality, Yang-deficiency, Yin-deficiency and Phlegm-wetness with whom 23 single nucleotide polymorphisms (SNPs) in the three genes were genotyped using polymerase chain reaction-restriction fragment length polymorphism (PCR-RFLP) method. Biased distri-bution of PPARD rs2267669 and rs2076167, APM1 rs7627128 and rs1063539 in Yang-deficiency, PPARG Pro12Ala in Yin-deficiency and PPARD rs2076167, APM1 rs266729 and rs7627128 in Phlegm-wetness were observed. The frequencies of Haplotype13 (Hap13) of PPARG in Yin-deficiency, Hap25 of APM1 in Yang-deficiency and Hap2 of PPARD and Hap14 of PPARG in Phlegm-wetness, were significantly different from those in Normality, suggesting those might be group-associated haplotypes. These results suggested that single SNP and hap-lotypes of PPARD, PPARG and APM1 may underlie the genetic basis of the constitutions classified in TCM. | Yanrui Wu Yina Cun Jing Dong Jingru Shao Shengjun Luo Shengjie Nie Haijing Yu Bingrong Zheng Qi Wang Chunjie Xiao | 2010 | Journal of Genetics and Genomics2010，37，6： | 36 |
| 2 | Benzoate anions-intercalated NiFe-layered double hydroxide nanosheet array with enhanced stability for electrochemical seawater oxidation显示文摘Seawater electrolysis is an extremely attractive approach for harvesting clean hydrogen energy,but detrimental chlorine species(i.e.,chloride and hypochlorite)cause severe corrosion at the anode.Here,we report our recent finding that benzoate anions-intercalated NiFe-layered double hydroxide nanosheet on carbon cloth(BZ-NiFe-LDH/CC)behaves as a highly efficient and durable monolithic catalyst for alkaline seawater oxidation,affords enlarged interlayer spacing of LDH,inhibits chlorine(electro)chemistry,and alleviates local pH drop of the electrode.It only needs an overpotential of 320 mV to reach a current density of 500 mA·cm^(−2)in 1 M KOH.In contrast to the fast activity decay of NiFe-LDH/CC counterpart during long-term electrolysis,BZ-NiFe-LDH/CC achieves stable 100-h electrolysis at an industrial-level current density of 500 mA·cm^(−2)in alkaline seawater.Operando Raman spectroscopy studies further identify structural changes of disorderedδ(NiIII-O)during the seawater oxidation process. | Longcheng Zhang Jie Liang Luchao Yue Kai Dong Jun Li Donglin Zhao Zerong Li Shengjun Sun Yongsong Luo Qian Liu Guanwei Cui Abdulmohsen Ali Alshehri Xiaodong Guo Xuping Sun | 2022 | Nano Research Energy2022，1，3： | 6 |
| 3 | The Tibetan Plateau Surface–Atmosphere Coupling System and Its Weather and Climate Effects: The Third Tibetan Plateau Atmospheric Science Experiment显示文摘The Tibetan Plateau(TP) is a key area affecting forecasts of weather and climate in China and occurrences of extreme weather and climate events over the world. The China Meteorological Administration, the National Natural Science Foundation of China, and the Chinese Academy of Sciences jointly initiated the Third Tibetan Plateau Atmospheric Science Experiment(TIPEX-Ⅲ) in 2013, with an 8–10-yr implementation plan. Since its preliminary field measurements conducted in 2013, routine automatic sounding systems have been deployed at Shiquanhe, Gaize, and Shenzha stations in western TP, where no routine sounding observations were available previously. The observational networks for soil temperature and soil moisture in the central and western TP have also been established. Meanwhile, the plateau-scale and regional-scale boundary layer observations, cloud–precipitation microphysical observations with multiple radars and aircraft campaigns, and tropospheric–stratospheric air composition observations at multiple sites, were performed. The results so far show that the turbulent heat exchange coefficient and sensible heat flux are remarkably lower than the earlier estimations at grassland, meadow, and bare soil surfaces of the central and western TP. Climatologically, cumulus clouds over the main body of the TP might develop locally instead of originating from the cumulus clouds that propagate northward from South Asia. The TIPEX-Ⅲ observations up to now also reveal diurnal variations, macro-and microphysical characteristics, and water-phase transition mechanisms, of cumulus clouds at Naqu station. Moreover, TIPEX-Ⅲ related studies have proposed a maintenance mechanism responsible for the Asian 'atmospheric water tower' and demonstrated the effects of the TP heating anomalies on African, Asian, and North American climates. Additionally, numerical modeling studies show that the Γ distribution of raindrop size is more suitable for depicting the TP raindrop characteristics compared to the M–P distribution, the overestimation of sensible heat flux can be reduced via modifying the heat transfer parameterization over the TP, and considering climatic signals in some key areas of the TP can improve the skill for rainfall forecast in the central and eastern parts of China. Furthermore, the TIPEX-Ⅲ has been promoting the technology in processing surface observations, soundings, and radar observations, improving the quality of satellite retrieved soil moisture and atmospheric water vapor content products as well as high-resolution gauge–radar–satellite merged rainfall products, and facilitating the meteorological monitoring, forecasting, and data sharing operations. | Ping ZHAO Yueqing LI Xueliang GUO Xiangde XU Yimin LIU Shihao TANG Wenming XIAO Chunxiang SHI Yaoming MA Xing YU Huizhi LIU La JIA Yun CHEN Yanju LIU Jian LI Dabiao LUO Yunchang CAO Xiangdong ZHENG Junming CHEN An XIAO Fang YUAN Donghui CHEN Yang PANG Zhiqun HU Shengjun ZHANG Lixin DONG Juyang HU Shuai HAN Xiuji ZHOU | 2019 | Journal of Meteorological Research2019，33，3： | 4 |
| 4 | N, O-doped carbon foam as metal-free electrocatalyst for efficient hydrogen production from seawater显示文摘Seawater electrolysis is the most promising technology for large scale hydrogen production due to the abundance and low cost of seawater in nature.However,compared with the traditional freshwater electrolysis,the issues of electrode poisoning and corrosion will occur during the seawater electrolysis process,and active and stable electrocatalysts for the hydrogen evolution reaction(HER)are thus highly desired.In this work,N,O-doped carbon foam in-situ derived from commercial melamine foam is proposed as a high-active metal-free HER electrocatalyst for seawater splitting.In acidic seawater,our catalyst shows high hydrogen generation performance with small overpotential of 161 mV at 10 mA·cm^(−2),a low Tafel slop of 97.5 mV·dec^(−1),and outstanding stability. | Qian Liu Shengjun Sun Longcheng Zhang Yongsong Luo Qin Yang Kai Dong Xiaodong Fang Dongdong Zheng Abdulmohsen Ali Alshehri Xuping Sun | 2022 | Nano Research2022，15，10： | 2 |
| 5 | A Novel Route to Prepare Nanocomposites in Larger Scale显示文摘准备 nanocomposites 的一条新奇线路通过润滑油的 preparingoverbased 钙石油 sulfonate 被说明净化在旋转 packedbed ( RPB )代替常规反应 vessel.The 被用作反应堆的地方,结果证明 thecarbonation 效率被改进,原料消费被减少,并且 thedispersibilities ,在 overbased 的 缩放nano 的 CaCO3 粒子的尺寸和形态学净化的 areenhanced.It 相当被推出这条线路能是广泛地 | Wei WU Lailong LUO Guangwen CHU Shengjun BAI Haikui ZOU Jianfeng CHEN | 2007 | Journal of Materials Science & Technology2007，23，3： | 2 |
| 6 | Enhanced N_(2)-to-NH_(3)conversion efficiency on Cu3P nanoribbon electrocatalyst显示文摘Ambient electroreduction of nitrogen(N_(2))is considered as a green and feasible approach for ammonia(NH_(3))synthesis,which urgently demands for efficient electrocatalyst.Morphology has close relationship with catalytic activity of heterogeneous catalysts.Nanoribbon is attractive nanostructure,which possesses the flexibility of one-dimensional nanomaterials,the large surface area of two-dimensional nanomaterials,and lateral size confinement effects.In this work,Cu_(3)P nanoribbon is proposed as a highly efficient electrocatalyst for N_(2)-to-NH_(3)conversion under benign conditions.When measured in N_(2)-saturated 0.1 M HCl,such Cu_(3)P nanoribbon achieves high performance with an excellent Faradaic efficiency as high as 37.8%and a large yield of 18.9μg·h^(−1)·mgcat.−1 at−0.2 V.It also demonstrates outstanding stability in long-term electrolysis test at least for 45 h. | Qian Liu Yiting Lin Shuang Gu Ziqiang Cheng Lisi Xie Shengjun Sun Longcheng Zhang Yongsong Luo Abdulmohsen Ali Alshehri Mohamed SHamdy Qingquan Kong Jiahong Wang Xuping Sun | 2022 | Nano Research2022，15，8： | 1 |
| 7 | Controllable synthesis of PbO nano/microstructures using a porous alumina template显示文摘 | Wang Qiang Sun Xun Luo Shengjun | 2007 | Crystal Growth & Design2007，7，12： | 1 |
| 8 | Controllable Synthesis of PbO Nano/Microstructures Using a Porous Alumina Template显示文摘 | Qaing Wang Xun Sun Shengjun Luo | 2007 | Crystal Growth and design2007，7，12： | 1 |
| 9 | Efficiency of CO2fixation by microalgae in a closed raceway pond显示文摘 | Shuwen Li Shengjun Luo Rongbo Guo | 2013 | Bioresource Technology2013，136，： | 1 |
| 10 | Biomass and lipid production of marine microalgae using municipal wastewater and high concentration of CO2 显示文摘 | JIANG Liling LUO Shengjun FAN Xiaolei | 2011 | Applied Energy2011，88，10： | 1 |
| 11 | Surface modification of magnesium hydroxide and its application in flame retardant polypropylene composites显示文摘 | Xiaolang Chen Jie Yu Shaoyun Guo Shengjun Lu Zhu Luo Min He | 2009 | Journal of Materials Science2009，，5： | 1 |
| 12 | Urban water system theory and its model development and application显示文摘The urban water system theory is an extension of the basin water system science on an urban scale, providing a new systematic solution for the unbalanced human-water relationship and severe water challenges, such as waterlogging, black and odorous water, and ecological degradation caused by urbanization. Most existing studies on urban water systems have focused on individual water cycle processes linked with water supply and sewage treatment plants, but mutual feedback between the water cycle and its associated material circulation and water ecology, as well as human processes, still needs further exploration. In this paper, the concept, theory, and technical methodology of the urban water system were developed based on the water cycle and basin water system science. The Urban Water System 5.0(UWS 5.0) model was developed by integrating the Time Variant Gain rainfall-runoff Model with Urban water system(TVGM_Urban) in different underlying surface conditions for analyzing the natural-social water cycle processes and their associated water environmental and ecological processes and the influence of multiscale sponge measures. Herein, five major simulation functions were realized: rainfall-runoff-nonpoint source pollutant load,water and pollutant transportations through the drainage network system, terminal regulation and purification, socioeconomic water cycle, and water system assessment and regulation. The location for the case study used in this paper was Wuhan City. The findings showed that the entire urban water system should consider the built-up area and its associated rivers and lakes as the research object and explore the integrations among the urban natural-social water cycle and river regulations inside and outside of the city as well as the effects of socioeconomic development and sponge measures on the water quantity-quality-ecology processes. The UWS 5.0 model efficiently simulated the urban rainfall-runoff process, total nitrogen(TN) and total phosphorus(TP) concentrations in water bodies, and characteristic indicators of socioeconomic development. For the rainfall-runoff simulations, the correlation coefficient and Nash-Sutcliffe efficiency(NSE) fall under the excellent and good classes, respectively. For the TN and TP concentration simulations, results exhibited good bias and the correlation coefficients exceeded 0.90 for 78.1% of the sampled sites. The simulation of 18 socioeconomic indicators provided excellent bias, correlation coefficient, and NSE values of 100%, 83.3%, and 69.4% to total indicators, respectively. Based on the well-calibrated UWS 5.0 model, the source sponge,artificial enhancement, and source reduction-path interception-terminal treatment measures were optimized, which considerably mitigated waterlogging, black and odorous water, and lake eutrophication, respectively. The mitigation performance revealed that the maximum inundated area for a once-in-10-year rainfall event was reduced by 32.6%, the removal ratio of the black and odorous water area was 65%, the comprehensive trophic state index of water bodies was reduced by 37%, and the green development level of Wuhan City in 2020 increased from 0.56 to 0.67. This study is expected to advance the intersection and development of multidisciplinary fields(e.g., urban hydrology, environmental science, and ecology) and offer an important theoretical and technical basis for solving urban complex water issues and promoting green development of cities. | Jun XIA Yongyong ZHANG Dunxian SHE Shiyan ZHANG Jun YANG Mingquan LV Xiang ZHANG Anqi LUO Shengjun WU Yang LIU | 2024 | Science China Earth Sciences2024，67，3： | 0 |
| 13 | CeO_(2) nanoparticles with oxygen vacancies decorated N-doped carbon nanorods:A highly efficient catalyst for nitrate electroreduction to ammonia显示文摘Electrocatalytic nitrate reduction reaction(NO_(3)−RR)emerges as a highly efficient approach toward ammonia synthesis and degrading NO_(3)−contaminant.In our study,CeO_(2) nanoparticles with oxygen vacancies(VO)decorated N-doped carbon nanorods on graphite paper(CeO_(2)−x@NC/GP)were demonstrated as a highly efficient NO_(3)−RR electrocatalyst.The CeO_(2)−x@NC/GP catalyst manifests a significant NH_(3 )yield up to 712.75μmol·h^(−1)·cm^(−2) at−0.8 V vs.reversible hydrogen electrode(RHE)and remarkable Faradaic efficiency of 92.93%at−0.5 V vs.RHE under alkaline conditions,with excellent durability.Additionally,an assembled Zn-NO_(3)−battery with CeO_(2)−x@NC/GP as cathode accomplishes a high-power density of 3.44 mW·cm^(−2) and a large NH3 yield of 145.08μmol·h^(−1)·cm^(−2).Density functional theory results further expose the NO_(3)−reduction mechanism on CeO_(2)(111)surface with VO. | Zerong Li Zhiqin Deng Ling Ouyang Xiaoya Fan Longcheng Zhang Shengjun Sun Qian Liu Abdulmohsen Ali Alshehri Yonglan Luo Qingquan Kong Xuping Sun | 2022 | Nano Research2022，15，10： | 0 |
| 14 | An amorphous FeMoO_(4) nanorod array enabled high-efficiency oxygen evolution electrocatalysis in alkaline seawater显示文摘The development of highly efficient and durable oxygen evolution reaction(OER)catalysts for seawater electrolysis is of great importance for applications.Here,an amorphous FeMoO_(4) nanorod array on Ni foam is reported as a highly active OER electrocatalyst in alkaline seawater,requiring only overpotentials of 303 and 332 mV to achieve 100 and 300 mA·cm^(-2),respectively.Moreover,it shows strong long-term electrochemical durability for at least 50 h. | Jie Tang Shengjun Sun Xun He Hui Zhang Chaoxin Yang Min Zhang Meng Yue Hefeng Wang Yuntong Sun Yonglan Luo Sulaiman Alfaifi Asmaa Farouk Mohamed S.Hamdy Xuping Sun Huiqing Wang Binwu Ying | 2024 | Nano Research2024，17，4： | 0 |
| 15 | Fe-doped Co_(3)O_(4) nanowire strutted 3D pinewood-derived carbon: A highly selective electrocatalyst for ammonia production via nitrate reduction显示文摘Nitrate(NO_(3)^(-)),a nitrogen-containing pollutant,is prevalent in aqueous solutions,contributing to a range of environmental and health-related issues.The electrocatalytic reduction of NO_(3)^(-)holds promise as a sustainable approach to both eliminating NO_(3)^(-)and generating valuable ammonia(NH_(3)).Nevertheless,the reduction reaction of NO_(3)^(-)(NO_(3)^(-)RR),involving 8-electron transfer process,is intricate,necessitating highly efficient electrocatalysts to facilitate the conversion of NO_(3)^(-)to NH_(3).In this study,Fe-doped Co_(3)O_(4) nanowire strutted three-dimensional(3D)pinewood-derived carbon(Fe-Co_(3)O_(4)/PC)is proposed as a high-efficiency NO_(3)^(-)RR electrocatalyst for NH_(3) production.Operating within 0.1 M NaOH containing NO_(3)^(-),Fe-Co_(3)O_(4)/PC demonstrates exceptional performance,obtain an impressively large NH_(3) yield of 0.55 mmol·h^(-1)·cm^(-2) and an exceptionally high Faradaic efficiency of 96.5%at-0.5 V,superior to its Co_(3)O_(4)/PC counterpart(0.2 mmol·h^(-1)·cm^(-2),73.3%).Furthermore,the study delves into the reaction mechanism of Fe-Co_(3)O_(4) for NO_(3)^(-)RR through theoretical calculations. | Xuwei Liu Chaozhen Liu Xun He Zhengwei Cai Kai Dong Jun Li Xiaoya Fan Ting Xie Xiya Yang Yonglan Luo Dongdong Zheng Shengjun Sun Sulaiman Alfaifi Feng Gong Xuping Sun | 2024 | Nano Research2024，17，4： | 0 |
| 16 | Enhancing the stability of Ni Fe-layered double hydroxide nanosheet array for alkaline seawater oxidation by Ce doping显示文摘Electrocatalytic hydrogen production from seawater holds enormous promise for clean energy generation.Nevertheless,the direct electrolysis of seawater encounters significant challenges due to poor anodic stability caused by detrimental chlorine chemistry.Herein,we present our recent discovery that the incorporation of Ce into Ni Fe layered double hydroxide nanosheet array on Ni foam(Ce-Ni Fe LDH/NF)emerges as a robust electrocatalyst for seawater oxidation.During the seawater oxidation process,CeO_(2)is generated,effectively repelling Cl^(-)and inhibiting the formation of Cl O-,resulting in a notable enhancement in the oxidation activity and stability of alkaline seawater.The prepared Ce-Ni Fe LDH/NF requires only overpotential of 390 m V to achieve the current density of 1 A cm^(-2),while maintaining long-term stability for 500 h,outperforming the performance of Ni Fe LDH/NF(430 m V,150 h)by a significant margin.This study highlights the effectiveness of a Ce-doping strategy in augmenting the activity and stability of materials based on Ni Fe LDH in seawater electrolysis for oxygen evolution. | Yongchao Yao Shengjun Sun Hui Zhang Zixiao Li Chaoxin Yang Zhengwei Cai Xun He Kai Dong Yonglan Luo Yan Wang Yuchun Ren Qian Liu Dongdong Zheng Weihua Zhuang Bo Tang Xuping Sun Wenchuang(Walter)Hu | 2024 | Journal of Energy Chemistry2024，91，4： | 0 |
| 17 | Efficient promotion of methane hydrate formation and elimination of foam generation using fluorinated surfactants显示文摘Methane hydrate preparation is an effective method to store and transport methane.In promoters to facilitate methane hydrate formation,homogeneous surfactant solutions,sodium dodecyl sulfate(SDS)in particular,are more favorable than heterogeneous particles,thanks to their faster reaction rate,more storage capacity,and higher stability.Foaming,however,could not be avoided during hydrate dissociation with the presence of SDS.This paper investigated the ability of five fluorinated surfactants:potassium perfluorobutane sulfonate(PBS),potassium perfluorohexyl sulfonate(PHS),potassium perfluorooctane sulfonate(POS),ammonium perfluorooctane sulfonate(AOS),and tetraethylammonium perfluorooctyl sulfonate(TOS)to promote methane hydrate formation.It was found that both PBS and PHS achieve a storage capacity of 150(V/V,the volume of methane that can be stored by one volume of water)within 30 min,more than that of SDS.Cationic ions and the carbon chain length were then discussed on their effects during the formation.It was concluded that PBS,PHS,and POS produced no foam during hydrate dissociation,making them promising promoters in large-scale application. | Quan CAO Dongyan XU Huanfei XU Shengjun LUO Rongbo GUO | 2020 | Frontiers in Energy2020，14，3： | 0 |
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