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| 1 | Vacancy manipulating of molybdenum carbide MXenes to enhance Faraday reaction for high performance lithium-ion batteries显示文摘“Intrinsic”strategies for manipulating the local electronic structure and coordination environment of defect-regulated materials can optimize electrochemical storage performance.Nevertheless,the structure–activity relationship between defects and charge storage is ambiguous,which may be revealed by constructing highly ordered vacancy structures.Herein,we demonstrate molybdenum carbide MXene nanosheets with customized in-plane chemical ordered vacancies(Mo_(1.33)CT_(x)),by utilizing selective etching strategies.Synchrotron-based X-ray characterizations reveal that Mo atoms in Mo1.33CTx show increased average valence of+4.44 compared with the control Mo_(2)CT_(x).Benefited from the introduced atomic active sites and high valence of Mo,Mo_(1.33)CT_(x)achieves an outstanding capacity of 603 mAh·g^(−1)at 0.2 A·g^(−1),superior to most original MXenes.Li+storage kinetics analysis and density functional theory(DFT)simulations show that this optimized performance ensues from the more charge compensation during charge–discharge process,which enhances Faraday reaction compared with pure Mo_(2)CT_(x).This vacancy manipulation provides an efficient way to realize MXene’s potential as promising electrodes. | Xin Guo Changda Wang Wenjie Wang Quan Zhou Wenjie Xu Pengjun Zhang Shiqiang Wei Yuyang Cao Kefu Zhu Zhanfeng Liu Xiya Yang Yixiu Wang Xiaojun Wu Li Song Shuangming Chen Xiaosong Liu | 2022 | Nano Research Energy2022,1,3: | 2 |
| 2 | Multiplexed cytokine profiling of serum for detection of colorectal cancer显示文摘 | Zhang Pengjun Wen Xinyu Gu Feng Deng Xinxin Liu Yulan Li Juan Jia Xingwang Dong Zhennan Tian Yaping | 2013 | Future Oncol2013,,7: | 2 |
| 3 | Motivating Ru-bri site of RuO_(2)by boron doping toward high performance acidic and neutral oxygen evolution显示文摘The electrocatalysis of oxygen evolution reaction(OER)plays a key role in clean energy storage and transfer.Nonetheless,the sluggish kinetics and poor durability under acidic and neutral conditions severely hinder practical applications such as electrolyzer compatible with the powerful proton exchange membrane and biohybrid fuel production.Here,we report a borondoped ruthenium dioxide electrocatalyst(B-RuO_(2))fabricated by a facile boric acid assisted strategy which demonstrates excellent acidic and neutral OER performances.Density functional theory calculations and advanced characterizations reveal that the boron species form an anomalous B–O covalent bonding with the oxygen atoms of RuO_(2)and expose the fully coordinately bridge ruthenium site(Ru-bri site),which seems like a switch that turns on the inactive Ru-bri site into OER-active,resulting in more exposed active sites,modified electronic structure,and optimized binding energy of intermediates.Thus,the B-RuO_(2)exhibits an ultralow overpotential of 200 mV at 10 mA/cm^(2)and maintains excellent stability compared to commercial RuO_(2)in 0.5 M sulfuric acid.Moreover,the superior performance is as well displayed in neutral electrolyte,surpassing most previously reported catalysts. | Chongjing Liu Beibei Sheng Quan Zhou Dengfeng Cao Honghe Ding Shuangming Chen Pengjun Zhang Yujian Xia Xiaojun Wu Li Song | 2022 | Nano Research2022,15,8: | 1 |
| 4 | Biomass-derived hard carbon microtubes with tunable apertures for high-performance sodium-ion batteries显示文摘Sodium-ion batteries(SIBs)are considered the most up-and-coming complements for large-scale energy storage devices due to the abundance and cheap sodium.However,due to the bigger radius,it is still a great challenge to develop anode materials with suitable space for the intercalation of sodium ions.Herein,we present hard carbon microtubes(HCTs)with tunable apertures derived from low-cost natural kapok fibers via a carbonization process for SIBs.The resulted HCTs feature with smaller surface area and shorter Na+diffusion path benefitting from their unique micro-nano structure.Most importantly,the wall thickness of HCTs could be regulated and controlled by the carbonization temperature.At a high temperature of 1,600℃,the carbonized HCTs possess the smallest wall thickness,which reduces the diffusion barrier of Na+and enhances the reversibility Na+storage.As a result,the 1600HCTs deliver a high initial Coulombic efficiency of 90%,good cycling stability(89.4%of capacity retention over 100 cycles at 100 mA·g^(−1)),and excellent rate capacity.This work not only charts a new path for preparing hard carbon materials with adequate ion channels and novel tubular micro-nano structures but also unravels the mechanism of hard carbon materials for sodium storage. | Pin Song Shiqiang Wei Jun Di Jun Du Wenjie Xu Daobin Liu Changda Wang Sicong Qiao Yuyang Cao Qilong Cui Pengjun Zhang Liaobo Ma Jiewu Cui Yan Wang Yujie Xiong | 2023 | Nano Research2023,16,4: | 1 |
| 5 | Densovirus is a mutualistic symbiont of a global crop pest (Helicoverpa ar- migera) and protects against a Baculovirus and Bt biopesticide 显示文摘 | Xu Pengjun Liu Yongqiang Graham R I | 2014 | PLoS Pathogens2014,10,10: | 1 |
| 6 | In-Situ Synthesis of CQDs/BiOBr Material via Mechanical Ball Milling with Enhanced Photocatalytic Performances显示文摘Designing simple, efficient, and environmentally friendly methods to construct high-efficient photocatalysts is an important strategy to promote the further development of the field of photocatalysis. Herein, flower-like carbon quantum dots(CQDs)/Bi OBr composite photocatalysts have been prepared via in-situ synthesis by mechanical ball milling in the existence of ionic liquid. The CQDs/Bi OBr composites exhibit higher photo-degradation performance for tetracycline(TC) than Bi OBr monomer and the commercial Bi_(2)O_(3) under visible light irradiation. For comparison, the different Br sources and synthetic methods are chosen to prepare Bi OBr and CQDs/Bi OBr composites. Photocatalysts prepared by ball milling and ionic liquid present significantly enhanced photocatalytic performance for removing TC. In addition, the introduction of CQDs could distinctly enhance the photocatalytic performances of pure Bi OBr. The reason is that CQDs as electron acceptor effectively separate electrons and holes and inhibit their recombination. The intermediates during photocatalytic degradation were tested using liquid chromatography-mass spectrometry(LC-MS) and possible degradation pathways were given. During degradation, ·OH, O_(2)^(·-)and h^(+) were identified to be the main active species based on electron spin resonance(ESR) spectra and free radical trapping experiments. A possible mechanism of CQDs/Bi OBr with enhanced photocatalytic performances was further proposed. | Xingwang Yan Bin Wang Mengxia Ji Qi Jiang Gaopeng Liu Pengjun Liu Sheng Yin Huaming Li Jiexiang Xia | 2022 | Chinese Journal of Structural Chemistry2022,41,8: | 1 |
| 7 | Investigation on the toxic interaction of toluidine blue with calf thymus DNA显示文摘 | Zhenxing Chi Rutao Liu Yajing Sun Meijie Wang Pengjun Zhang Canzhu Gao | 2009 | Journal of Hazardous Materials2009,,1: | 1 |
| 8 | Synchronous activation of Ag nanoparticles and BiOBr for boosting solar-driven CO_(2)reduction显示文摘Artificial photosynthesis of valuable chemicals from CO_(2)is a potential way to achieve sustainable carbon cycle.The CO_(2)conversion activity is still inhibited by the sluggish charge kinetics and poor CO_(2)activation.Herein,Ag nanoparticles coupled Bi OBr have been constructed by in-situ photoreduction strategy.The crafting of interface between Ag nanoparticles and Bi OBr nanosheets,achieving an ultra-fast charge transfer.The Bi OBr semiconductor excited electrons and plasmonic Ag nanoparticles generated high-energy hot electrons synchronous accelerates the C=O double bond activation.Thus,the optimized Ag/BiOBr-2 heterostructure shows excellent CO_(2)photoreduction activity with CO production of 133.75 and 6.83μmol/g under 5 h of 300 W Xe lamp and visible light(λ>400 nm)irradiation,which is 1.51 and 2.81 folds versus the pristine Bi OBr,respectively.The mechanism of CO_(2)photoreduction was in-depth understood through in-situ FT-IR spectrum and density functional theory calculations.This study provides some new perspectives into efficient photocatalytic CO_(2)reduction. | Gaopeng Liu Lin Wang Bin Wang Xingwang Zhu Jinman Yang Pengjun Liu Wenshuai Zhu Ziran Chen Jiexiang Xia | 2023 | Chinese Chemical Letters2023,34,6: | 1 |
| 9 | Molecular cloning and characterization of four heat shock protein genes from Macrocentrus cingulum (Hymenoptera: Braconidae)显示文摘 | Pengjun Xu Jinhua Xiao Li Liu Tong Li Dawei Huang | 2010 | Molecular Biology Reports2010,,5: | 1 |
| 10 | Gene cloning, expression and characterization of an α-galactosidase from Pedobacter nyackensis MJ11 CGMCC 2503 with potential as an aquatic feed additive显示文摘 | Xiaodan Liu Kun Meng Yaru Wang Pengjun Shi Tiezheng Yuan Peilong Yang Huiying Luo Yingguo Bai Bin Yao | 2009 | World Journal of Microbiology and Biotechnology2009,,9: | 1 |
| 11 | A Distributed and Efficient Flooding Scheme Using 1-hop Information in Mobile Ad Hoc Networks显示文摘 | Liu Hai Jia Xiaohua Wan Pengjun | 2007 | IEEE Transactions on Parallel and Distributed Systems2007,18,5: | 1 |
| 12 | Charge density wave phase suppression in 1T-TiSe_(2) through Sn intercalation显示文摘Taking advantage of the unique layered structure of TiSe2,the intrinsic electronic properties of two-dimensional materials can easily be tuned via heteroatomic engineering.Herein,we show that the charge density wave(CDW)phase in 1T-TiSe_(2) single-crystals can be gradually suppressed through Sn atoms intercalation.Using angle-resolved photoemission spectroscopy(ARPES)and temperature-dependent resistivity measurements,this work reveals that Sn atoms can induce charge doping and modulate the intrinsic electronic properties in the host 1T-TiSe_(2).Notably,our temperature-dependent ARPES results highlight the role exciton-phonon interaction and the Jahn-Teller mechanism through the formation of backfolded bands and exhibition of a downward Se shift of 4p valence band in the formation of CDW in this material. | Mukhtar Lawan Adam Hongen Zhu Zhanfeng Liu Shengtao Cui Pengjun Zhang Yi Liu Guobin Zhang Xiaojun Wu Zhe Sun Li Song | 2022 | Nano Research2022,15,3: | 1 |
| 13 | Maximizing lifetime of sensor surveillance systems显示文摘 | LIU HAI JIA XIAOHUA WAN PENGJUN | 2007 | IEEE/ACM Transactions on Networking2007,15,2: | 1 |
| 14 | Classification of bio-potential surface electrode based on FKCM and SVM显示文摘 | Liu Hao Tao Xiaoming Xu Pengjun | 2011 | Journal of Software2011,6,5: | 1 |
| 15 | Grooming of Arbitrary Traf- fic in SONET/WDM BLSRS 显示文摘 | WAN Pengjun LIU Liwu FRIEDER O | 2000 | Journal on Selected Areas in Com- munications2000,18,10: | 1 |
| 16 | Maximizing Lifetime of Sensor Surveillance Systems显示文摘 | Liu Hai Jia Xiaohua Wan Pengjun | 2007 | IEEE/ACM Transactions on Networking2007,15,2: | 1 |
| 17 | Circulation of Development Factors Promoted by Innovation of Land Management Under Background of Rural Vitalization:A Case Study of Tengtou Village in Zhejiang Province,China显示文摘Land is the space carrier for the existence and flow of other development factors.Activating rural land and promoting the circulation of other development factors through land management innovation is necessary to realize rural vitalization.This paper identifies the connotation of factor flow in the rural vitalization context,the action mechanism of land management innovation to boost the flow of development factors,the issues and obstacles restricting factor circulation,and the realization mechanism of the flow of development factors in rural vitalization.Based on the analytic paradigm constructed in the paper,the successful practice of promoting the flow of development factors through innovative land management in a model village is examined.The results show that:1)the unreasonable systems characterized by the land use system in rural areas are the main obstacles causing circulation issues in development factors.It is essential to engage in comprehensive reform to break down these long-lasting obstacles to the smooth flow of development factors.2)The land should play a leading role in the circulation of development factors in the background of rural vitalization;the main purpose of land management innovation is to activate the land factor,thereby promoting the circulation of other factors.3)The activated land factor will act as a‘trigger’to promote capital and technology in rural settings and use capital and technology to attract the inflow of talents and the return of migrant workers,whereby the population factor will act as a‘catalyst’for the cultivation of rural culture,bringing about the integration of various development factors.4)The innovation of land use and management,increased funding,and new technologies have brought multiple talents to Tengtou Village.The high-frequency mutual feedback between the village’s own and the external development factors resulted in its successful integration of industrial development. | WEI Pengjun LIU Yongqiang YAN Jinlong LI Meiting ZHANG Yingnan | 2023 | Chinese Geographical Science2023,33,5: | 0 |
| 18 | Improved algorithm of cluster-based routing protocols for agricultural wireless multimedia sensor networks显示文摘Low Energy Adaptive Clustering Hierarchy(LEACH)is a routing algorithm in agricultural wireless multimedia sensor networks(WMSNs)that includes two kinds of improved protocol,LEACH_D and LEACH_E.In this study,obstacles were overcome in widely used protocols.An improved algorithm was proposed to solve existing problems,such as energy source restriction,communication distance,and energy of the nodes.The optimal number of clusters was calculated by the first-order radio model of the improved algorithm to determine the percentage of the cluster heads in the network.High energy and the near sink nodes were chosen as cluster heads based on the residual energy of the nodes and the distance between the nodes to the sink node.At the same time,the K-means clustering analysis method was used for equally assigning the nodes to several clusters in the network.Both simulation and the verification results showed that the survival number of the proposed algorithm LEACH-ED increased by 66%.Moreover,the network load was high and network lifetime was longer.The mathematical model between the average voltage of nodes(y)and the running time(x)was concluded in the equation y=−0.0643x+4.3694,and the correlation coefficient was R2=0.9977.The research results can provide a foundation and method for the design and simulation of the routing algorithm in agricultural WMSNs. | Zhang Fu Liu Hongmei Wang Jun Qiu Zhaomei Mao Pengjun Zhang Yakun | 2016 | International Journal of Agricultural and Biological Engineering2016,9,4: | 0 |
| 19 | Survey and Prospect for Applying Knowledge Graph in Enterprise Risk Management显示文摘Enterprise risk management holds significant importance in fostering sustainable growth of businesses and in serving as a critical element for regulatory bodies to uphold market order.Amidst the challenges posed by intricate and unpredictable risk factors,knowledge graph technology is effectively driving risk management,leveraging its ability to associate and infer knowledge from diverse sources.This review aims to comprehensively summarize the construction techniques of enterprise risk knowledge graphs and their prominent applications across various business scenarios.Firstly,employing bibliometric methods,the aim is to uncover the developmental trends and current research hotspots within the domain of enterprise risk knowledge graphs.In the succeeding section,systematically delineate the technical methods for knowledge extraction and fusion in the standardized construction process of enterprise risk knowledge graphs.Objectively comparing and summarizing the strengths and weaknesses of each method,we provide recommendations for addressing the existing challenges in the construction process.Subsequently,categorizing the applied research of enterprise risk knowledge graphs based on research hotspots and risk category standards,and furnishing a detailed exposition on the applicability of technical routes and methods.Finally,the future research directions that still need to be explored in enterprise risk knowledge graphs were discussed,and relevant improvement suggestions were proposed.Practitioners and researchers can gain insights into the construction of technical theories and practical guidance of enterprise risk knowledge graphs based on this foundation. | Pengjun Li Qixin Zhao Yingmin Liu Chao Zhong Jinlong Wang Zhihan Lyu | 2024 | Computers, Materials & Continua2024,78,3: | 0 |
| 20 | M1 macrophage-related gene model for NSCLC immunotherapy response prediction显示文摘Patients diagnosed with non-small cell lung cancer(NSCLC)have a limited lifespan and exhibit poor immunotherapy outcomes.M1 macrophages have been found to be essential for antitumor immunity.This study aims to develop an immunotherapy response evaluation model for NSCLC patients based on transcription.RNA sequencing profiles of 254 advanced-stage NSCLC patients treated with immunotherapy are downloaded from the POPLAR and OAK projects.Immune cell infiltration in NSCLC patients is examined,and thereafter,different coexpressed genes are identified.Next,the impact of M1 macrophage-related genes on the prognosis of NSCLC patients is investigated.Six M1 macrophage coexpressed genes,namely,NKX2-1,CD8A,SFTA3,IL2RB,IDO1,and CXCL9,exhibit a strong association with the prognosis of NSCLC and serve as effective predictors for immunotherapy response.A response model is constructed using a Cox regression model and Lasso Cox regression analysis.The M1 genes are validated in our TD-FOREKNOW NSCLC clinical trial by RT-qPCR.The response model shows excellent immunotherapy response prediction and prognosis evaluation value in advanced-stage NSCLC.This model can effectively predict advanced NSCLC prognosis and aid in identifying patients who could benefit from customized immunotherapy as well as sensitive drugs. | Sifan Wu Qiqi Sheng Pengjun Liu Zhe Jiao Jinru Lv Rong Qiao Dongkun Xie Zanhan Wang Jiamei Ge Penghui Li Tiaoxia Wei Jie Lei Jieyi Fan Liang Wang | 2024 | Acta Biochimica et Biophysica Sinica2024,56,3: | 0 |