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| 1 | PROTAC-induced BTK degradation as a novel therapy for mutated BTK C481S induced ibrutinib-resistant B-cell malignancies显示文摘 | Yonghui Sun Xingwang Zhao Ning Ding Hongying Gao Yue Wu Yiqing Yang Meng Zhao Jinseok Hwang Yuqin Song Wanli Liu Yu Rao | 2018 | Cell Research2018，28，7： | 29 |
| 2 | Cenozoic uplift of the Tibetan Plateau:Evidence from the tectonic-sedimentary evolution of the western Qaidam Basin显示文摘Geologists agree that the collision of the Indian and Asian plates caused uplift of the Tibet Plateau.However,controversy still exists regarding the modes and mechanisms of the Tibetan Plateau uplift.Geology has recorded this uplift well in the Qaidam Basin.This paper analyzes the tectonic and sedimentary evolution of the western Qaidam Basin using sub-surface seismic and drill data. The Cenozoic intensity and history of deformation in the Qaidam Basin have been reconstructed based on the tectonic developments,faults growth index,sedimentary facies variations,and the migration of the depositional depressions.The changes in the sedimentary facies show that lakes in the western Qaidam Basin had gone from inflow to still water deposition to withdrawal.Tectonic movements controlled deposition in various depressions,and the depressions gradually shifted southeastward.In addition,the morphology of the surface structures in the western Qaidam Basin shows that the Cenozoic tectonic movements controlled the evolution of the Basin and divided it into(a) the southern fault terrace zone, (b) a central Yingxiongling orogenic belt,and(c) the northern fold-thrust belt;divided by the XI fault (Youshi fault) and Youbei fault,respectively.The field data indicate that the western Qaidam Basin formed in a Cenozoic compressive tectonic environment caused by the India—Asia plate collision. Further,the Basin experienced two phases of intensive tectonic deformation.The first phase occurred during the Middle Eocene—Early Miocene(Xia Ganchaigou Fm.and Shang Ganchaigou Fm.,43.8—22 Ma),and peaked in the Early Oligocene(Upper Xia Ganchaigou Fm.,31.5 Ma).The second phase occurred between the Middle Miocene and the Present(Shang Youshashan Fm.and Qigequan Fm., 14.9—0 Ma),and was stronger than the first phase.The tectonic—sedimentary evolution and the orientation of surface structures in the western Qaidam Basin resulted from the Tibetan Plateau uplift,and recorded the periodic northward growth of the Plateau.Recognizing this early tectonic—sedimentary evolution supports the previous conclusion that northern Tibet responded to the collision between India and Asia shortly after its initiation.However,the current results reveal that northern Tibet also experienced another phase of uplift during the late Neogene.The effects of these two stages of tectonic activity combined to produce the current Tibetan Plateau. | Yadong Wang Jianjing Zheng Weilin Zhang Shiyuan Li Xingwang Liu Xin Yang Yuhu Liu | 2012 | Geoscience Frontiers2012，3，2： | 23 |
| 3 | Gas Hydrates in the Qilian Mountain Permafrost, Qinghai, Northwest China显示文摘Qilian Mountain permafrost, with area about 10×104 km2, locates in the north of Qinghai-Tibet plateau. It equips with perfect conditions and has great prospecting potential for gas hydrate. The Scientific Drilling Project of Gas Hydrate in Qilian Mountain permafrost, which locates in Juhugeng of Muri Coalfield, Tianjun County, Qinghai Province, has been implemented by China Geological Survey in 2008–2009. Four scientific drilling wells have been completed with a total footage of 2059.13 m. Samples of gas hydrate are collected separately from holes DK-1, DK-2 and DK-3. Gas hydrate is hosted under permafrost zone in the 133–396 m interval. The sample is white crystal and easily burning. Anomaly low temperature has been identified by the infrared camera. The gas hydrate-bearing cores strongly bubble in the water. Gas-bubble and water-drop are emitted from the hydrate-bearing cores and then characteristic of honeycombed structure is left. The typical spectrum curve of gas hydrate is detected using Raman spectrometry. Furthermore, the logging profile also indicates high electrical resistivity and sonic velocity. Gas hydrate in Qilian Mountain is characterized by a thinner permafrost zone, shallower buried depth, more complex gas component and coal-bed methane origin etc. | ZHU Youhai ZHANG Yongqin WEN Huaijun LU Zhenquan JIA Zhiyao LI Yonghong LI Qinghai LIU Changling WANG Pingkang GUO Xingwang | 2010 | Acta Geologica Sinica(English Edition)2010，84，1： | 19 |
| 4 | Relationship between genetic polymorphisms of metabolizing enzymes CYP2E1, GSTM1 and Kazakh's esophageal squamous cell cancer in Xinjiang, China显示文摘AIM: To analyze the relationship between genetic polymorphisms of metabolizing enzymes CYP2E1, GSTM1 andKazakh's esophageal squamous cell cancer in China.METHODS: The genotypes of cytochromes P450 (CYP) 2E1 and glutathione S-transferase (GST) M1 were investigated by polymerase chain reaction (PCR) and restriction fragment length polymorphism (RFLP) following PCR in 104 Kazakh's patients with esophageal cancer (EC) and 104 non-cancer controls.RESULTS: The frequency of CYP2E1 c1/c1 genotype was significantly higher in patients with cancer (77.9%) thanin control subjects (24.0%) (P<0.05; OR, 11.13; 95%CI,5.84-21.22). The difference of GSTM1 null was significantly more frequent in the cancer (34.6%) vsthe control group (3.8%) (P<0.05; OR, 13.24; 95%CI, 4.50-38.89). On the other hand, the combination of GSTM1 presence and CYP2E1 c1/c1 genotypes increased the risk for cancer (P<0.05;OR, 13.42; 95%CI, 6.29-28.3).CONCLUSION: The CYP2E1 c1/c1, GSTM1 deletion genotypes are genetically susceptible biomarkers for ESCC in Kazakh population. Individuals with allele c1 of RsaI polymorphic locus for CYP2E1 may increase the risk of ESCC. Moreover, CYP2E1 wild type (c1/c1) increased thesusceptibility to ESCC risk in Kazakh individuals with GSTM1 presence genotype. | Xiao-MeiLu Yue-MingZhang Ren-YongLin ArziGul XingWang Ya-LouZhang YanZhang YanWang HaoWen | 2005 | World Journal of Gastroenterology2005，11，24： | 15 |
| 5 | p53 polymorphism in human papillomavirus-associated Kazakh's esophageal cancer in Xinjiang,China显示文摘AIM: To investigate the relationship between p53 codon 72 polymorphism and human papillomavirus (HPV) type 16 infection in Kazakh's esophageal cancer (EC) in Xinjiang, China.METHODS: Encoding regions of p53codon 72 and HPV-16 E6 were amplified by polymerase chain reaction-restriction fragment length polymorphism (PCR-RFLP) and polymerase chain reaction (PCR) methods using pairs of primary esophageal squamous cell carcinoma (SCC) tissue and corresponding normal mucosa, which were collected from 104 patients of Kazakh in Xinjiang, China. RESULTS: Only arginine allele was detected in 70.1% (39/55) of HPV-16-E6-positive cases but only in 40.8% (20/49) of HPV-16-E6-negative cases (P<0.05; OR, 3.53; 95% CI, 1.57-7.98). In contrast, such a significant correlation between p53 polymorphism and HPV infection was not evident in corresponding normal mucosae. The allele frequency of Arg allele in cancer cases (0.68) was higher than that in normal mucosa samples (0.54) (P<0.05; OR, 1.80; 95% CI, 1.21-2.69).CONCLUSION: p53 codon 72 Arg homozygous genotype is one of the high-risk genetic factors for HPV-associated SCC of Kazakh. Individuals carrying Arg allele compared to those with Pro allele have an increased risk for esophageal SCC. | Xiao-MeiLu Yue-MingZhang Ren-YonaLin Xiao-HuiLiang Ya-LouZhang XingWang YanZhang YanWang HaoWen | 2004 | World Journal of Gastroenterology2004，10，19： | 14 |
| 6 | PKS5,a SNF1-related kinase,interacts with and phosphorylates NPR1,and modulates expression of WRKY38 and WRKY62显示文摘NPR1 (Nonexpressor of Pathogenesis-Related gene 1) is a major co-activator of plant defense. Phosphorylations of NPR1 play impor-tant roles in fine-tuning its activity, however a kinase corresponding to such modification remains uncharacterized. Here, we report that NPR1 interacts with PKS5 (SOS2-like Protein Kinase 5). The AKR (AnKyrin Repeats) motif of NPR1 is required for this interaction. PKS5 phosphorylates NPR1 at the C-terminal region. Expression of PKS5 is induced quickly by Pseudomonas syringae pv. tomato DC3000. Expression level of two NPR1 target genes, WRKY38 and WRKY62, is reduced and/or delayed in pks5 mutants. Moreover, the expression of WRKY38 and WRKY62 displays a similar pattern in npr1-1pks5-1 double mutant comparing to that in npr1-1. Our results suggest that PKS5 functions at the upstream of NPR1 and might mediate expression of WRKY38 and WRKY62 possibly by interacting with and phosphorylating NPR1. | Changgen Xie Xiaona Zhou Xingwang Deng Yan Guo | 2010 | Journal of Genetics and Genomics2010，37，6： | 14 |
| 7 | A novel advanced oxidation process——wet electrocatalytic oxidation for high concentrated organic wastewater treatment显示文摘A novel advanced oxidation process——wet electrocatalytic oxidation (WEO) was studied with p-nitrophenol as model pollutant and β-PbO2 electrode as the anode. Compared with the effect of the individual wet air oxidation (WAO) and electrochemical oxidation (EO), the effect of WEO showed syn- ergistic effect on COD removal under the conditions of temperature 160℃, C=1000 mg·L-1, PN2=0.50 MPa, PO2=0.9 MPa, current density = 3 mA·cm-2, Na2SO4 3 g·L-1. And the synergistic factor got the best value of 0.98 within 120 min after 180 min treatment. The synergistic factor was studied after 120 min treatment at 100℃, 120℃, 140℃ and 160℃, and the effect of 120℃ was the best with the value of 1.26. Possible mechanism for the synergistic effect was discussed based on the analysis of free-radical generation and intermediates detected by HPLC and GC/MS. | DAI QiZhou ZHOU MingHua LEI LeCheng ZHANG XingWang | 2007 | Chinese Science Bulletin2007，52，12： | 11 |
| 8 | Comprehensive analysis of NAC transcription factors and their expression during fruit spine development in cucumber (Cucumis sativus L.)显示文摘The cucumber(Cucumis sativus L.)is an important vegetable crop worldwide,and fruit trichomes or spines are an important trait for external fruit quality.The mechanisms underlying spine formation are not well understood,but the plant-specific NAC family of transcription factors may play important roles in fruit spine initiation and development.In this study,we conducted a genome-wide survey and identified 91 NAC gene homologs in the cucumber genome.Clustering analysis classified these genes into six subfamilies;each contained a varying number of NAC family members with a similar intron–exon structure and conserved motifs.Quantitative real-time PCR analysis revealed tissue-specific expression patterns of these genes,including 10 and 12 that exhibited preferential expression in the stem and fruit,respectively.Thirteen of the 91 NAC genes showed higher expression in the wild-type plant than in its near-isogenic trichome mutant,suggesting their important roles in fruit spine development.Exogenous application of four plant hormones promoted spine formation and increased spine density on the cucumber fruits;several NAC genes showed differential expression over time in response to phytohormone treatments on cucumber fruit,implying their essential roles in fruit-trichome development.Among the NAC genes identified,12 were found to be targets of 13 known cucumber micro-RNAs.Collectively,these findings provide a useful resource for further analysis of the interactions between NAC genes and genes underlying trichome organogenesis and development during fruit spine development in cucumber. | Xingwang Liu Ting wang Ezra Bartholomew Kezia Black Mingming Dong Yaqi Zhang Sen Yang Yanling Cai Shudan Xue Yiqun Weng Huazhong Ren | 2018 | Horticulture Research2018，5，1： | 10 |
| 9 | Gas chromatography-mass spectrometry analysis of essential oils from five parts of Chaihu(Radix Bupleuri Chinensis)显示文摘OBJECTIVE: To analyze the essential oils from flowers, leaves, stems, roots, and fruits of Chaihu(Radix Bupleuri Chinensis).METHODS: We extracted essential oils from different parts of Chaihu(Radix Bupleuri Chinensis) using a steam distillation method. The essential oils were analyzed by gas chromatography-mass spectrometry(GC-MS). Data were collected in full scan mode(m/z 60-600). Volatile components were identified based on their retention indices and by comparing their mass spectra with those in the National Institute of Standards and Technology 2005 database assisted by tandem mass spectrometry information. The relative content of each constituent wasdetermined by area normalization.RESULTS: We identified 111 components, of which12 were common to all 5 parts, 30 were found only in roots, 14 were found only in flowers, 6 were found only in leaves, 4 were found only in stems,and 17 were found only in fruits.CONCLUSION: Our results show that the stems,flowers, leaves, and fruits of Chaihu(Radix Bupleuri Chinensis)contain a high concentration of essential oils, and that the exact composition of the essential oils differs among the plant parts. To develop new medicines and make full use of the Chaihu(Radix Bupleuri Chinensis)resource, it is important to characterize the essential oils from different parts of the plant. In future research, it will be important to determine the pharmacological effects of the various components and the essential oil mixtures. | Jie Meng Xingfu Chen Wenyu Yang Jiuhua Song Yu Zhang Zhifei Li Xingwang Yang Zhanguo Yang | 2014 | Journal of Traditional Chinese Medicine2014，34，6： | 9 |
| 10 | Synthesis and fluorescent properties in complexes of Eu( Ⅲ), Tb( Ⅲ), and Sm( Ⅲ) with β-diketone and 2,2′-bipyridine显示文摘Three new rare earth ternary complexes, RE(PB)_3bpy (RE=Sm^(3+) , Eu^(3+) , and Tb^(3+) ), were synthesized by the reaction of 1-(p-phenylethynyl- phenyl)-1,3-butanedione (HPB) and 2,2′-bipyridine (bpy) with rare earth chloride RECl_3 , respectively, in alcohol solution. The compositions were characterized by means of infrared (IR) spectra, chemical analysis, elemental analysis, and thermodynamic analysis. Luminescent properties of the three complexes were studied. At room temperature, under UV light excitation, the Sm^(3+) , Eu^(3+) , and Tb^(3+) complexes exhibit characteristic emission of the central ions. The fluorescence spectra show that the fluorescence emission intensity of Eu^(3+) complex is the strongest. The narrow strongest emission band of Eu^(3+) complex is considered to be a valuable material with bright red fluorescence. | LIU Xingwang JIANG Jiadong GUO Yuwei YONG Shengli YANG Kun NIE Lu | 2012 | Rare Metals2012，31，5： | 9 |
| 11 | Cullin-RING Ubiquitin Ligase Family in Plant Abiotic Stress Pathways显示文摘The ubiquitin-proteasome system is a key mechanism that plants use to generate adaptive responses in coping with various en- vironmental stresses. Cullin-RING (CRL) complexes represent a predominant group of ubiquitin E3 ligases in this system. In this review, we focus on the CRL E3s that have been implicated in abiotic stress signaling pathways in Arabidopsis. By comparing and analyzing these cases, we hope to gain a better understanding on how CRL complexes work under various settings in an attempt to decipher the clues about the regulatory mechanism of CRL E3s. | Liquan Guo Cynthia D.Nezames Lianxi Sheng Xingwang Deng Ning Wei | 2013 | Journal of Integrative Plant Biology2013，55，1： | 9 |
| 12 | Synthesis and luminescence properties of rare earth ternary complexes consisting of Tb(Ⅲ), β-diketones and 1,10-phenanthroline (phen)显示文摘In order to study the luminescent properties of ternary rare earth complexes with β-diketone ligand, three new β-diketone ligands, 1-phenyl-3-(p-phenylethynylphenyl)-1,3-propanedione(HPPP), 1-(2-thienyl)-3-(p-phenylethynylphenyl)-1,3-propanedione (HTPP) and 1-(2-furyl)-3-(p-phenylethynylphenyl)-1,3-propanedione (HFPP), were synthesized by Sonogashira coupling reaction and Claisen condensa- tion. Three new ternary rare earth complexes, TbL3phen (L = PPP, TPP, or FPP), were synthesized by the reaction of rare earth chloride TbCl3,1,10-phenanthroline (phen) with HPPP, HTPP, or HFPP respectively, in alcohol solution. The compositions were characterized by means of elemental analysis, chemical analysis, and IR spectra. Luminescent properties of the three new complexes have been studied. The results show that the ternary Tb(III) complexes only emit the weak fluorescence of the Tb(III) ion, which reveals the triplet state energy of the ligands does not match well with the excited state vibrating energy of Tb3+ ion. | LIU Xingwang WANG Na SUO Quanling | 2008 | Rare Metals2008，27，6： | 8 |
| 13 | Fabrication of visible-light responsive S-F-codoped TiO_2 nanotubes显示文摘Fabrication and S-F-codoping of TiO2 nanotubes were carried out by a one-step electrochemical ano-dization process to extend the photoresponse of TiO2 to the visible-light region. The prepared samples were annealed in air and detected by SEM,XRD,XPS and UV-vis DRS spectrophotometer. The results showed that the average tube diameter of the nanotubes was 150 nm and the average tube length was 400 nm. The doped TiO2 nanotubes exhibited strong absorption in visible-light region. Photoelectro-catalytic degradation efficiency of 4-CP over S-F-codoped TiO2 nanotubes was 39.7% higher than that of only-F-doped sample. Moreover,sulfur and fluorine codoped into substitutional sites of TiO2 had been proven to be indispensable for strong response and high photocatalytic activity under visible light,as assessed by XPS. | CHEN XiuQin SU YaLing ZHANG XingWang LEI LeCheng | 2008 | Chinese Science Bulletin2008，53，13： | 7 |
| 14 | Synthesis,luminescent properties,and theoretical study of novel Sm^(3+) and Dy^(3+) complexes containing β-diketone and 1,10-phenanthroline显示文摘Two new ternary complexes of 1-(2-thienyl)-3-(p-phenylethynylphenyl)-1,3-propanedione(HTPP) and 1,10-phenanthroline(phen) with Sm3+ and Dy3+ were synthesized.The composition of the ternary complexes was characterized as Sm(TPP)3phen and Dy(TPP)3phen,respectively,by infrared(IR) spectra,chemical analysis,elemental analysis,and thermodynamic analysis.At room temperature,under UV light excitation,the Sm3+ and Dy3+ complexes exhibit characteristic emissions of the central ions.It is found that the fluorescence intensity of Sm(TPP)3phen is stronger than that of Dy(TPP)3phen.In order to explain this phenomenon,an accurate quantum chemistry calculation was carried out,and the result is in good agreement with the experiment data. | LIU Xingwang GAO Saishengtai WANG Li SHEN Leijun JIANG Jiadong GAO Junfang | 2011 | Rare Metals2011，30，1： | 7 |
| 15 | Two energy balance closure approaches: applications and comparisons over an oasis-desert ecotone显示文摘Studies of energy balance that rely on eddy covariance(EC) are always challenged by energy balance closure, which is mainly caused by the underestimations of latent heat flux(LE) and sensible heat flux(Hs). The Bowen ratio(BR) and energy balance residual(ER) approaches are two widely-used methods to correct the LE. A comprehensive comparison of those two approaches in different land-use types is essential to accurately correcting the LE and thus improving the EC experiments. In this study, two energy balance approaches(i.e., BR and ER) were compared to correct the LE measured at six EC sites(i.e., three vegetated, one mixed and two non-vegetated sites) in an oasis-desert ecotone of the Heihe River Basin, China. The influences of meteorological factors on those two approaches were also quantitatively assessed. Our results demonstrated that the average energy closure ratio((LE+Hs)/(Rn–Gs); where Rn is the surface net radiation and Gs is the surface soil heat flux) was approximately close to 1.0 at wetland, maize and village sites, but far from 1.0 at orchard, Gobi and desert sites, indicating a significant energy imbalance at those three latter sites. After the corrections of BR and ER approaches that took into account of soil heat storage, the corrected LE was considerably larger than the EC-measured LE at five of six EC sites with an exception at Gobi site. The BR and ER approaches yielded approximately similar corrected LE at vegetated and mixed sites, but they generated dissimilar results at non-vegetated sites, especially at non-vegetated sites with low relative humidity, strong wind, and large surface-air temperature difference. Our findings provide insight into the applicability of BR and ER approaches to correcting EC-based LE measurements in different land-use types. We recommend that the BR-corrected and ER-corrected LE could be seriously reconsidered as validation references in dry and windy areas. | PAN Xin LIU Yuanbo FAN Xingwang GAN Guojing | 2017 | Journal of Arid Land2017，9，1： | 7 |
| 16 | Enhanced Vitamin C Production Mediated by an ABA-Induced PTP-like Nucleotidase Improves Plant Drought Tolerance in Arabidopsis and Maize显示文摘Abscisic acid(ABA)is a key phytohormone that mediates environmental stress responses.Vitamin C,or L-ascorbic acid(AsA),is the most abundant antioxidant protecting against stress damage in plants.How the ABA and AsA signaling pathways interact in stress responses remains elusive.In this study,we characterized the role of a previously unidentified gene,PTPN(PTP-like Nucleotidase)in plant drought tolerance.In Arabidopsis,(AtPTPN was expressed in multiple tissues and upregulated by ABA and drought treatments.Loss-of-function mutants oiAtPTPN were hyposensitive to ABA but hypersensitive to drought stresses,whereas plants with enhanced expression AtPTPN showed opposite phenotypes to.Overexpression of maize PTPN(ZmPTPN)promoted,while knockdown oiZmPTPN inhibited plant drought tolerance,indicating conserved and positive roles of PTPN in plant drought tolerance.We found that both AtPTPN and ZmPTPN release Pi by hydrolyzing GDP/GMP/dGMP/IMP/dIMP,and that AtPTPN positively regulated AsA production via endogenous Pi content control.Consistently,overexpression of VTC2,the rate-limiting synthetic enzyme in AsA biosynthesis,promoted AsA production and plant drought tolerance,and these effects were largely dependent on AtPTPN activity.Furthermore,we demonstrated that the heat shock transcription factor HSFA6a directly binds the AtPTPN promoter and activates AtPTPN expression.Genetic analyses showed that AtPTPN is required for HSFA6a to regulate ABA and drought responses.Taken together,our data indicate that PTPN-mediated crosstalk between the ABA signaling and AsA biosynthesis pathways positively controls plant drought tolerance. | Hui Zhang Yanli Xiang Neng He Xiangguo Liu Hongbo Liu Liping Fang Fei Zhang Xiaopeng Sun Delin Zhang Xingwang Li William Terzaghi Jianbing Yan Mingqiu Dai | 2020 | Molecular Plant2020，13，5： | 7 |
| 17 | Protectin D1 promotes resolution of inflammation in a murine model of lipopolysaccharide-induced acute lung injury via enhancing neutrophil apoptosis显示文摘 | Li Xingwang Li Chunlai Liang Wandong Bi Yuntian Chen Maohua Dong Sheng | 2014 | Chinese Medical Journal2014，，5： | 6 |
| 18 | Synergistic improvement of perovskite film quality for efficient solar cells via multiple chloride salt additives显示文摘Perovskite crystal film quality is critical for obtaining efficient perovskite solar cells. Anti-solvent processing was used for fast crystallization of perovskite precursor film, which can form dense perovskite film.However, the crystals from this method are usually small due to the fast crystal growth process, which could lead to grain boundary recombination. Here, element chloride is introduced to enhance the perovskite layer crystallinity via slowing down the perovskite crystallization process by simultaneous introduction of methylammounium chloride(MACl) and cesium chloride(CsCl) into precursor solution.As a result, we achieve high quality of pin-hole free perovskite film with large crystal size. A power conversion efficiency of 21.55% with free of hysteresis of the device is obtained, which is among the highest efficiency of planar structure perovskite solar cells. | Pengyang Wang Qi Jiang Yang Zhao Yong Chen Zema Chu Xingwang Zhang Yuqin Zhou Jingbi You | 2018 | Science Bulletin2018，63，11： | 6 |
| 19 | Non-noble metal single-atom catalysts prepared by wet chemical method and their applications in electrochemical water splitting显示文摘Water splitting by electrolysis is an appealing pathway for sustainable hydrogen production. The practical performance of water splitting is highly dependent on the efficiency of electrocatalysts, which can promote the anodic oxygen evolution reaction(OER) or cathodic hydrogen evolution reaction(HER). Downsizing the metal nanostructures to atomic level to construct single-atom catalysts(SACs) has attracted enormous attention due to its distinct advantages in maximizing the efficiency of metal atom utilization and enhancing activity over corresponding metal nanoparticles. Research on SACs towards electrochemical water splitting application is an emerging field and intensive investigations have been focused on their rational syntheses and applications in HER/OER. In this review, we focus on the wet chemical method developed to prepare non-noble metal based SACs with an emphasis on the synthetic strategies and structure-activity relationship between single metal atoms and catalytic activity. Finally, the challenges and future opportunities for application of single-atom catalysts in water splitting are briefly addressed. | Wei Liu Hongxiu Zhang Chuanming Li Xin Wang Jingquan Liu Xingwang Zhang | 2020 | Journal of Energy Chemistry2020，29，8： | 6 |
| 20 | Application of in-plasma catalysis and post-plasma catalysis for methane partial oxidation to methanol over a Fe_2O_3-CuO/γ-Al_2O_3 catalyst显示文摘Methane partial oxidation to methanol (MPOM) using dielectric barrier discharge over a Fe2O3-CuO/γ-Al2O3 catalyst was performed.The multicomponent catalyst was combined with plasma in two different configurations,i.e.,in-plasma catalysis (IPC) and post-plasma catalysis (PPC).It was found that the catalytic performance of the catalysts for MPOM was strongly dependent on the hybrid configuration.A better synergistic performance of plasma and catalysis was achieved in the IPC configuration,but the catalysts packed in the discharge zone showed lower stability than those connected to the discharge zone in sequence.Active species,such as ozone,atomic oxygen and methyl radicals,were produced from the plasma-catalysis process,and made a major contribution to methanol synthesis.These active species were identified by the means of in situ optical emission spectra,ozone measurement and FT-IR spectra.It was confirmed that the amount of active species in the IPC system was greater than that in the PPC system.The results of TG,XRD,and N2 adsorption-desorption revealed that carbon deposition on the spent catalyst surface was responsible for the catalyst deactivation in the IPC configuration. | Lin Chen Xingwang Zhang Liang Huang Lecheng Lei | 2010 | Journal of Natural Gas Chemistry2010，19，6： | 5 |
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