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| 1 | A Review of Technical Advances,Barriers,and Solutions in the Power to Hydrogen(P2H)Roadmap显示文摘Power to hydrogen(P2H)provides a promising solution to the geographic mismatch between sources of renewable energy and the market,due to its technological maturity,flexibility,and the availability of technical and economic data from a range of active demonstration projects.In this review,we aim to provide an overview of the status of P2H,analyze its technical barriers and solutions,and propose potential opportunities for future research and industrial demonstrations.We specifically focus on the transport of hydrogen via natural gas pipeline networks and end-user purification.Strong evidence shows that an addition of about 10%hydrogen into natural gas pipelines has negligible effects on the pipelines and utilization appliances,and may therefore extend the asset value of the pipelines after natural gas is depleted.To obtain pure hydrogen from hydrogen-enriched natural gas(HENG)mixtures,end-user separation is inevitable,and can be achieved through membranes,adsorption,and other promising separation technologies.However,novel materials with high selectivity and capacity will be the key to the development of industrial processes,and an integrated membrane-adsorption process may be considered in order to produce high-purity hydrogen from HENG.It is also worth investigating the feasibility of electrochemical separation(hydrogen pumping)at a large scale and its energy analysis.Cryogenics may only be feasible when liquefied natural gas(LNG)is one of the major products.A range of other technological and operational barriers and opportunities,such as water availability,byproduct(oxygen)utilization,and environmental impacts,are also discussed.This review will advance readers’understanding of P2H and foster the development of the hydrogen economy. | Guoping Hu Chao Chen Hiep Thuan Lu Yue Wu Congmin Liu Lefu Tao Yuhan Men Guangli He Kevin Gang Li | 2020 | Engineering2020，6，12： | 7 |
| 2 | Pseudomonas aeruginosa:pathogenesis,virulence factors,antibiotic resistance,interaction with host,technology advances and emerging therapeutics显示文摘Pseudomonas aeruginosa(P.aeruginosa)is a Gram-negative opportunistic pathogen that infects patients with cystic fibrosis,burn wounds,immunodeficiency,chronic obstructive pulmonary disorder(COPD),cancer,and severe infection requiring ventilation,such as COVID-19.P.aeruginosa is also a widely-used model bacterium for all biological areas.In addition to continued,intense efforts in understanding bacterial pathogenesis of P.aeruginosa including virulence factors(LPS,quorum sensing,two-component systems,6 type secretion systems,outer membrane vesicles(OMVs),CRISPR-Cas and their regulation),rapid progress has been made in further studying host-pathogen interaction,particularly host immune networks involving autophagy,inflammasome,noncoding RNAs,cGAS,etc.Furthermore,numerous technologic advances,such as bioinformatics,metabolomics,scRNA-seq,nanoparticles,drug screening,and phage therapy,have been used to improve our understanding of P.aeruginosa pathogenesis and host defense.Nevertheless,much remains to be uncovered about interactions between P.aeruginosa and host immune responses,including mechanisms of drug resistance by known or unannotated bacterial virulence factors as well as mammalian cell signaling pathways.The widespread use of antibiotics and the slow development of effective antimicrobials present daunting challenges and necessitate new theoretical and practical platforms to screen and develop mechanism-tested novel drugs to treat intractable infections,especially those caused by multi-drug resistance strains.Benefited from has advancing in research tools and technology,dissecting this pathogen’s feature has entered into molecular and mechanistic details as well as dynamic and holistic views.Herein,we comprehensively review the progress and discuss the current status of P.aeruginosa biophysical traits,behaviors,virulence factors,invasive regulators,and host defense patterns against its infection,which point out new directions for future investigation and add to the design of novel and/or alternative therapeutics to combat this clinically significant pathogen. | Shugang Qin Wen Xiao Chuanmin Zhou Qinqin Pu Xin Deng Lefu Lan Haihua Liang Xiangrong Song Min Wu | 2022 | Signal Transduction and Targeted Therapy2022，7，7： | 5 |
| 3 | Habitat influences on diversity of bacteria found on German cockroach in Beijing显示文摘Cockroaches are worldwide indoor pests carrying microorganisms of medical importance.German cockroaches(Blattella germanica) were sampled in five habitats(hospital,restaurant,offce home,and market) in Beijing,and the bacteria were isolated from their external surface and alimentary tract and identified using a Biolog identification system.Cockroach densities significantly differed among habitats(market > home > offce > restaurant > hospital).However,no significant differences in bacterial abundance carried by individual German cockroaches(of either sex) were found among habitats.The bacterial abundance in the gut was significantly higher than that on the surface.There were no significant differences in bacterial species richness observed among habitats,sex,carrying position or their interaction.Cluster analysis showed that cockroach densities and bacterial abundance found in the market differed significantly from the other four habitats.The bacterial diversity was not significantly reduced in sensitive facilities such as hospital and restaurant,even though pesticide and bactericide were more frequently applied there.The implications of these findings were discussed in this article. | FU Xue YE Lefu GE Feng | 2009 | Journal of Environmental Sciences2009，21，2： | 5 |
| 4 | Synthesis and luminescence properties of apatite-type red-emitting Ba_(2)La_(8)(GeO_(4))_(6)O_(2):Eu^(3+)phosphors显示文摘A new kind of apatite-type red-emitting Ba_(2)La_(8)(GeO_(4))_(6)O_(2):Eu^(3+)phosphor was prepared by high temperature solid-state method.The Rietveld analysis based on the powder diffraction data shows that Ba_(2)La_(8)(GeO_(4))_(6)O_(2):Eu^(3+)phosphors possess a pure apatite phase without any impurity.The emission spectrum of Ba_(2)La_(8)(GeO_(4))_(6)O_(2):Eu^(3+)phosphor consists of two bands,an orange emission band from 500 to 600 nm and a red emission band from 600 to 680 nm.By varying the amount of the doped europium ions from 0.02 to 0.14 mol,it is found that the luminescent properties of this rare earth phosphor are the best when the concentration of europium ion is 0.08 mol.The optimum concentration is eventually proved to be 0.08 mol.The Eu^(3+)doping dependent luminescence quenching can be further ascribed to dipole-quadrupole interactions.The quantum yield of Ba_(2)La_(7.92)(GeO_(4))_(6)O_(2):0.08 Eu^(3+)is 37.23%.The CIE analysis confirms a reddish emission in the near ultraviolet(n-UV)excitation.All these above properties of the phosphor can help in contribution of promoting white light-emitting diode. | Kun Nie Xiaoxue Ma Panlong Lin Navnita Kumar Luoxin Wang Lefu Mei | 2021 | Journal of Rare Earths2021，39，11： | 5 |
| 5 | Cumene Liquid Oxidation to Cumene Hydroperoxide over CuO Nanoparticle with Molecular Oxygen under Mild Condition显示文摘CuO nanoparticle 经由湿化学方法被综合并且被 X 光检查描绘衍射(XRD ) ,氮吸附解吸附作用,和扫描电子显微镜学(SEM ) 。有分子的氧的 cumene 的催化氧化在 CuO nanoparticle 上被学习。催化剂作为与常规方法, CuO/Al2O3,或同类的铜催化剂在可比较的反应条件下面准备的 CuO 相比显示出显著地更高的活动。用在为 7 h 的 358 K 的 0.25 g CuO nanoparticle 催化剂和 0.1 摩尔 cumene 的 cumene 变换, cumene 水疗院过氧化物(CHP ) 收益,和选择分别地是 44.2% , 41.2% 和 93.2% 。催化剂能被再循环。在 6 个再循环的实验以后,催化活动的损失都没被观察。 | Meiying Zhang Lefu Wang Hongbing Ji Bing Wu Xiaoping Zeng | 2007 | Journal of Natural Gas Chemistry2007，16，4： | 4 |
| 6 | Ionic liquids: Efficient solvent and medium for the transformation of renewable lignocellulose显示文摘Carbon-enriched lignocelluloses are regarded as the perfect alternative for nonrenewable fossil fuel, and have a great potential to alleviate the increasing energy crisis and climate change. However, the tightly covalent structure and strong intra and in- ter-molecular hydrogen bonding in lignocellulose make it high recalcitrance to transformation due to the poor solubility in wa- ter or common organic solvents. Dissolution and transformation of lignocellulose and its constituents in ionic liquids have therefore attracted much attention recently due to the tunable physical-chemical properties. Here, ionic liquids with excellent dissolving capability for biomass and its ingredients were examined. The technologies for lignocellulose biorefining in the presence of ionic liquid solvents or catalysts were also summarized. Some pertinent suggestions for the future catalytic conver- sion and unitization of this sustained carbon-rich resource are proposed. | LONG JinXing LI XueHui WANG LeFu ZHANG Ning | 2012 | Science China Chemistry2012，55，8： | 3 |
| 7 | Recent progress on lanthanide complexes/clay minerals hybrid luminescent materials显示文摘The unique luminescent performance of lanthanide complexes/clay minerals hybrid materials has been fascinating many researchers for recent decades.It not only retains the excellent luminescent characteristics of lanthanide complexes but also improves the poor stability of the complexes.In this article,we introduce the luminescence mechanism of lanthanide complexes and point out the necessity of their combination with clay minerals.After the analysis of the structure and interlayer environment differences of 1:1-type and 2:1-type clay minerals,the intercalation methods(covalent grafting and ion exchange)appropriate for different clay minerals are summarized with examples.Based on the luminescence characteristics of the hybrid materials,the applications of these materials as luminescent probes in recognition of specific metal cations and molecules,detection of pH value,and temperature are reviewed.Finally,the current problems in the preparation of lanthanide complexes/clay minerals hybrid luminescent materials and shortcomings that need improvement in their performance are analyzed,and the application prospect is forecast. | Ga Zhang Lefu Mei Junjie Ding Ke Su Qingfeng Guo Guocheng Lv Libing Liao | 2022 | Journal of Rare Earths2022，40，9： | 2 |
| 8 | Which is the determinant for cellulose degradation in cooperative ionic liquid pairs: dissolution or catalysis?显示文摘Catalytic conversion of sustainable cellulose to the value-added chemicals and high quality biofuel has been recognized as a perfect approach for the alleviation of the dependence on the non-renewable fossil resources. Previously, we successfully designed and explored novel and efficient cooperative ionic liquid pairs for this renewable material, which has advantages of high reactor efficiency than current technologies because of the dissolution and in situ catalytic decomposition mechanism. Here, the determinant of this process is further studied by the intensive investigation on the relationship between the cellulose conversion and the properties of ionic liquid catalyst and solvent. Scanning electron microscope(SEM), thermogravimetric analysis(TG) and elemental analysis were used for the comparative characterization of raw cellulose and the residues. The results demonstrate that this consecutive dissolution and in situ catalysis process is much more dependent on the dissolution capability of ionic liquid solvent, while comparatively, the effect of in situ acid catalysis is relatively insignificant. | Jinxing Long Yangyu Zhang Lefu Wang Xuehui Li | 2016 | Science China Chemistry2016，59，5： | 2 |
| 9 | Corrosion behavior of Hastelloy C-276 in supercritical water显示文摘 | Qiang Zhang Rui Tang Kaiju Yin Xin Luo Lefu Zhang | 2009 | Corrosion Science2009，，9： | 2 |
| 10 | Load TiO2 or TiO2-N on the porous carbon显示文摘 | CHEN Jie MEI Lefu LIAO Libing | 2012 | Key Engineering Materials2012，5125，： | 1 |
| 11 | Microarray Analysis of Gene Expression Involved in Anther Development in rice (Oryza sativa L.)显示文摘 | Zhen Wang Yu Liang Chijun Li Yunyuan Xu Lefu Lan Dazhong Zhao Changbin Chen Zhihong Xu Yongbiao Xue Kang Chong | 2005 | Plant Molecular Biology2005，，5： | 1 |
| 12 | Monitoring of Gene Expression Profiles and Isolation of Candidate Genes Involved in Pollination and Fertilization in Rice (Oryza Sativa L.) with a 10K cDNA Microarray显示文摘 | Lefu Lan Wei Chen Ying Lai Jinfeng Suo Zhaosheng Kong Can Li Ying Lu Yujun Zhang Xiangyu Zhao Xiansheng Zhang Yansheng Zhang Bin Han Jing Cheng Yongbiao Xue | 2004 | Plant Molecular Biology2004，，4： | 1 |
| 13 | Microarray Analysis of Gene Expression Involved in Anther Development in rice (Oryza sativa L.)显示文摘 | Zhen Wang Yu Liang Chijun Li Yunyuan Xu Lefu Lan Dazhong Zhao Changbin Chen Zhihong Xu Yongbiao Xue Kang Chong | 2005 | Plant Molecular Biology2005，，5： | 1 |
| 14 | Preparation of Mg2Ni intermetallic compound from nanoparticles显示文摘 | Shao Huaiyu Liu Tong Zhang Lefu | 2003 | Scr Mater2003，49，： | 1 |
| 15 | Sartrolides A-G and bissartrolide, new cembranolides from the South China Sea soft coral Sarcophyton trocheliophorum Marenzeller 显示文摘 | LIANG Linfu LAN Lefu GUO Yuewei | 2013 | Tetrahedron2013，69，35： | 1 |
| 16 | Physical and chemical characteristic of particulate matter from biodiesel exhaust e- mission using non - thermal plasma technology 显示文摘 | Wang Pan Cai Yixi Zhang Lefu | 2010 | Energy and Fuels2010，24，5： | 1 |
| 17 | Corrosion behavior of ferritic/martensitic steel P92 in supercritical water显示文摘 | Kaiju Yin Shaoyu Qiu Rui Tang Qiang Zhang Lefu Zhang | 2009 | The Journal of Supercritical Fluids2009，，3： | 1 |
| 18 | Selection and corrosion evaluation tests of candidate SCWR fuel cladding materials显示文摘 | Lefu Zhang Yichen Bao Rui Tang | 2012 | Nuclear Engineering and Design2012，，： | 1 |
| 19 | Effect of Preadsorption and Shape Selective Desorption on Methanol Amination Product Distribution显示文摘 | Guo Jianwei Wang Lefu Cui Yingde | 2001 | Journal of South China University of Technology (Natural Science Edition)2001，29，10： | 1 |
| 20 | Structure and luminescence properties of color-tunable phosphor Sr_(2)La_(3)(SiO_(4))_(3)F:Tb^(3+),Sm^(3+)显示文摘A series of single-phase and color-tunable phosphors Sr_(2)La_(3)(SiO_(4))_(3)F:0.15Tb^(3+),xSm^(3+)(SLSOF:0.15Tb^(3+),xSm^(3+)) was prepared using solid-state route.The X-ray diffraction(XRD) was used to characterize the phase of the as-prepared samples.The synthesized phosphors have apatite-type structure without other impurities.Sm^(3+) and Tb^(3+) ions substitute La^(3+) into the lattice and form a single-phase solid solution.The elements are evenly distributed in the sample according to the scanning electron microscopy(SEM) results.The crystal structure of the host phosphor was refined by the Rietveld method.The optical properties were studied in detail by investigation of the luminescence and diffuse spectra,fluorescence decay curves and energy transfer efficiency.The phosphor color can be changed from green(0.29,0.48) to yellow/orange and red(0.57,0.42) via adjusting the doping ratio of Sm^(3+).The SLSOF:0.15Tb^(3+),xSm^(3+)phosphors can emit typical multicolor light such as green,yellow,orange and red with gradually increasing Sm^(3+)doping concentration.All results indicate the occurrence of the energy transfer which results in the color-tunable properties of the phosphors. | Haikun Liu Kun Nie Yuanyuan Zhang Lefu Mei Dina V.Deyneko Xiaoxue Ma | 2023 | Journal of Rare Earths2023，41，9： | 1 |
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