|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Cloud point extraction and flame atomic absorption spectrometry analysis of palladium, platinum, and gold ions from industrial polluted soil显示文摘Cloud point extraction (CPE) with Tergitol TMN-6 was applied for the extraction of trace amounts of palladium (Pd(Ⅱ)), platinum (Pt(Ⅳ)), and gold (Au(Ⅲ)) in the soil of industrial sewage. Ammonium pyrolysine dithiocarbamate (APDC) was adopted as the chelating agent prior to CPE and then was detected by atomic absorption spectrometry (AAS). Different parameters such as the concentration of surfactants, chelating agent and salt, sample pH, equilibration temperature and time, centrifugation time and rates, and the effect of foreign ions were studied. Under optimum conditions, the low limits of detections are 1.4, 2.8 and 1.2 ng·ml^-1 and the enrichment factors are 21, 12, and 24 for Pd(Ⅱ), Pt(Ⅳ), and Au(Ⅲ, respectively. The relative standard deviations vary from 0.6% to 1.0% (n=11). All correlation coefficients of the calibration curves are >0.9960. The proposed method was successfully applied for the determination of Pd(Ⅱ), Pt(Ⅳ), and Au(Ⅲ) in the real soil of industrial sewage samples. | LIAN Yuanpei ZHEN Wei TAI Zhigang YANG Yaling SONG Jun LI Zonghao | 2012 | Rare Metals2012，31，5： | 5 |
| 2 | Solvent engineering towards scalable fabrication of high-quality perovskite films for efficient solar modules显示文摘Over the last decade,remarkable progress has been made in metal halide perovskite solar cells(PSCs),which have been a focus of emerging photovoltaic techniques and show great potential for commercialization.However,the upscaling of small-area PSCs to large-area solar modules to meet the demands of practical applications remains a significant challenge.The scalable production of high-quality perovskite films by a simple,reproducible process is crucial for resolving this issue.Furthermore,the crystallization behavior in the solution-processed fabrication of perovskite films can be strongly influenced by the physicochemical properties of the precursor inks,which are significantly affected by the employed solvents and their interactions with the solutes.Thus,a comprehensive understanding of solvent engineering for fabricating perovskite films over large areas is urgently required.In this paper,we first analyze the role of solvents in the solution-processed fabrication of large-area perovskite films based on the classical crystal nucleation and growth mechanism.Recent efforts in solvent engineering to improve the quality of perovskite films for solar modules are discussed.Finally,the basic principles and future challenges of solvent system design for scalable fabrication of high-quality perovskite films for efficient solar modules are proposed. | Zhaoyi Jiang Binkai Wang Wenjun Zhang Zhichun Yang Mengjie Li Fumeng Ren Tahir Imran Zhenxing Sun Shasha Zhang Yiqiang Zhang Zhiguo Zhao Zonghao Liu Wei Chen | 2023 | Journal of Energy Chemistry2023，，5： | 4 |
| 3 | Mars Orbiter magnetometer of China’s First Mars Mission Tianwen-1显示文摘As one of the seven scientific payloads on board the Tianwen-1 orbiter,the Mars Orbiter Magnetometer(MOMAG)will measure the magnetic fields of and surrounding Mars to study its space environment and the interaction with the solar wind.The instrument consists of two identical triaxial fluxgate magnetometer sensors,mounted on a 3.19 meter-long boom with a seperation of about 90 cm.The dual-magnetometers configuration will help eliminate the magnetic field interference generated by the spacecraft platform and payloads.The sensors are controlled by an electric box mounted inside the orbiter.Each magnetometer measures the ambient vector magnetic field over a wide dynamic range(to 10,000 nT per axis)with a resolution of 1.19 pT.Both magnetometers sample the ambient magnetic field at an intrinsic frequency of 128 Hz,but will operate in a model with alternating frequency between 1 and 32 Hz to meet telemetry allocations. | Kai Liu XinJun Hao YiRen Li TieLong Zhang ZongHao Pan ManMing Chen XiaoWen Hu Xin Li ChengLong Shen YuMing Wang | 2020 | Earth and Planetary Physics2020，4，4： | 2 |
| 4 | Core - sheath functional polymer nanofibers perpared by co - electrospinning 显示文摘 | Xin Yi Huang Zonghao Li Wenwen | 2008 | European Polymer Journal2008，44，4： | 1 |
| 5 | Core-sheath functional polymer nanofibers prepared by ec-eleetrospinning 显示文摘 | YiXin Zonghao Huang Wenwen Li | 2008 | European Polymer Journal2008，44，： | 1 |
| 6 | Core-sheath functional polymer nanofibers prepared by co-e1ectrospinning显示文摘 | XIN Yi HUANG Zonghao LI Wen wen et a1 | 2008 | European Polymer Journal2008，44，： | 1 |
| 7 | Trial of antiepilepsirine (AES) in children with epilepsy 显示文摘 | Li Wang Dayao Zao Zonghao Zhang | 1999 | Brain & Development1999，21，： | 1 |
| 8 | A low-energy ion spectrometer with half-space entrance for three-axis stabilized spacecraft显示文摘A low-energy ion spectrometer(LEIS) for use aboard three-axis stabilized spacecraft has been developed to measure ion energy per charge distribution in three-dimensional space with good energy-, angular-and temporal-resolutions. For the standard top-hat electrostatic analyzer used widely in space plasma detection, three-axis stabilized spacecraft makes it difficult to obtain complete coverage of all possible ion arrival directions. We have designed angular scanning deflectors supplementing to a cylindrically symmetric top-hat electrostatic analyzer to provide a half-space field of view as 360°×90°(–45°–+45°), and fabricated the LEIS flight model for detecting magnetospheric ions in geosynchronous orbit. The performance of this payload has been evaluated in detail by a series of simulation and environmental tests, and the payload has also been calibrated through laboratory experiments using a low-energy ion source. The results show that capabilities of the LEIS payload are in accordance with the requirements of a magnetospheric mission. | HU RenXiang SHAN Xu YUAN GuangYuan WANG ShuWen ZHANG WeiHang QI Wei CAO Zhe LI YiRen CHEN ManMing YANG XiaoPing WANG Bo SHAO SiPei LI Feng ZHONG XiaoQing FAN Dan HAO XinJun FENG ChangQing SU ZhenPeng SHEN ChengLong LI Xin DAI GuYue QIU BingLin PAN ZongHao LIU Kai XU ChunKai LIU ShuBin AN Qi ZHANG TieLong WANG YuMing CHEN XiangJun | 2019 | Science China(Technological Sciences)2019，62，6： | 1 |
| 9 | Core-sheath func- tional polymer nanofibers prepared by co-electrospinning 显示文摘 | Xin Yi Huang Zonghao Li Wenwen | 2008 | Eur Polym J2008，44，4： | 1 |
| 10 | Core–sheath functional polymer nanofibers prepared by co-electrospinning显示文摘 | Yi Xin Zonghao Huang Wenwen Li Zijiang Jiang Yanbin Tong Cheng Wang | 2008 | European Polymer Journal2008，，4： | 1 |
| 11 | Characteristics of microbial communities in water from CBM wells and biogas production potential in eastern Yunnan and western Guizhou, China显示文摘The study of microbial communities in the produced water of coalbed methane(CBM)wells is an important aspect of microbial-enhanced methane production.Water produced from 15 CBM wells in four synclines in eastern Yunnan and western Guizhou was collected.Through the use of 16S ribosomal RNA(16S rRNA)amplicon sequencing and realtime fluorescence quantitative polymerase chain reaction(PCR),the characteristics of bacterial and archaeal communities before and after enrichment culture were studied.The methanogenic pathways of secondary biogas were discussed,and potential microbial-enhanced methane production was preliminarily evaluated.The results showed that the bacterial DNA content in uncultured produced water was low,so it is difficult to detect.After enrichment,the dominant bacteria phyla were Proteobacteria,Bacteroidetes,and Firmicutes.A total of seven phyla were detected in the uncultured produced water,and the dominant archaeal phylum was Euyarchaeota.Methanogens were the main component of archaea.The dominant archaeal genera were Methanobacterium,Methanoculleus and Methanobrevibacter.The community structure of the archaea changed noticeably after four days of enrichment culture.The relative abundance of Euryarchaeota increased to 99%in most samples after enrichment culture.It was found that there was a transition from Methanoregula to Methanobacterium within genera.The relative abundance of Methanobacterium increased,which can produce hydrogenotrophic methane.Combined with the isotopic composition of the produced water and gas,it is considered that the CBM in the Tucheng and Enhong synlines consists of a mixture of thermogenic gas and biogas.The proportion of secondary biogas in the Tucheng and Enhong synlines are estimated to range from 10.89% to 49.62%.There are mainly hydrogentrophic methanogens in the study area,and CO_(2) reduction is the main way of microbial gas production.After enrichment culture of produced water in the study area,the hydrogenotrophic methanogens were enriched.These two areas have strong potential for microbial-enhanced methane production. | Wenguang TIAN Zhaobiao YANG Zonghao QIN Yong QIN Cunlei LI Benju LU Yongchen LI | 2023 | Frontiers of Earth Science2023，17，1： | 0 |
| 12 | First results of the low energy ion spectrometer onboard a Chinese geosynchronous satellite显示文摘A Chinese geosynchronous satellite was launched on June 23,2020.It carried a plasma detection package to monitor the space environment around the orbit.Here we report the inflight performance of a low energy ion spectrometer(LEIS),one of the primary instruments in the plasma detection package,and its initial observations in flight.Benefiting from the state-of-the-art design of a top-hat electrostatic analyzer cooperated with angular scanning deflectors,three-dimensional measurement of ions in space with a large field of view of 360°×90°and a wide energy range from 50 eV to 25 keV per charge has been achieved.The differential energy flux spectra of ions around the orbit have shown clear signatures of surface charging and storm/substorm ion injections.The occurrence of surface charging could be caused by the lack of photoemission at the Earth's eclipse(near the midnight)or the storm energetic electron injection at the dawn sector.The present results demonstrated a good performance of the LEIS payload in flight for monitoring the space ion environment around the orbit.In situ measurements of the LEIS payload provide us an opportunity to understand the magnetospheric ion dynamics and forecast the associate space weather impacts. | SHAN Xu MIAO Bin CAO Zhe SUN ZhenYu LI YiRen LIU Kai GUO XingYu QU SanBiao SU ZhenPeng SHEN ChengLong PAN ZongHao LI Xin HAO XinJun YANG XiaoPing TIAN Chao JIANG Yu LIU ShuBin AN Qi CHEN XiangJun WANG YuMing | 2023 | Science China(Technological Sciences)2023，66，5： | 0 |
| 13 | In-flight calibration of the magnetometer on the Mars orbiter of Tianwen-1显示文摘Mars orbiter magnetometer(MOMAG)is one of seven science payloads onboard Tianwen-1’s orbiter.Unlike most of the satellites,Tianwen-1’s orbiter is not magnetically cleaned,and the boom where placed the magnetometer’s sensors is not long enough.These pose many challenges to the magnetic field data processing.In this study,we introduce the in-flight calibration process of the Tianwen-1/MOMAG.The magnetic interference including spacecraft generated dynamic field and the slowlychanging zero offsets are cleaned in sequence.Then the calibrated magnetic field data are compared with the data from the Mars atmosphere and volatile Evolutio N(MAVEN).We find that some physical structures in the solar wind are consistent between the two data sets,and the distributions of the magnetic field strength in the solar wind are very similar.These results suggest that the in-flight calibration of the MOMAG is successful and the MOMAG provides reliable data for scientific research. | ZOU ZhuXuan WANG YuMing ZHANG TieLong WANG GuoQiang XIAO SuDong PAN ZongHao ZHANG ZhouBin YAN Wei DU Yang CHI YuTian CHENG Long WU ZhiYong HAO XinJun LI YiRen LIU Kai CHEN ManMing SU ZhenPeng SHEN ChengLong XU MengJiao GUO JingNan | 2023 | Science China(Technological Sciences)2023，66，8： | 0 |
| 14 | On the Construction of n-Electron States with Symplectic Symmetry显示文摘Under quasispin scheme, a complete group theoretical classification of fermion states with symplectlc symmetry is proposed. Furthermore, the first and second order irreducible tensor operators are investigated in detail to approach the fermion states with explicit forms. | Sun Jiazhong(Sun Chiachung), Li Baifu, Zeng Zonghao and Liu Chengbu (Institute of Theoretical Chemistry, Jilin University, Changchun) | 1989 | Chemical Research in Chinese Universities1989，5，4： | 0 |
| 15 | Ground calibration of the Mars orbiter magnetometer onboard Tianwen-1显示文摘Ground calibration experiments of the Mars orbiter magnetometer(MOMAG)onboard the orbiter of Tianwen-1 were performed to determine the sensitivity,misalignment angle,and offset of the sensors.The linearity of the applied calibrated magnetic fields and the output from the sensors were confirmed to be better than 10^(-4),and the sensor axes were orthogonal to each other within 0.5 degrees.The temperature dependencies of the sensitivity and misalignment angle were examined,but no clear signatures of temperature dependencies could be seen.Sensor offset and the stability of sensor offset drift with a temperature change were also determined by the rotation method.The stability of the sensor offset drift was less than 0.01 nT/℃.The ground calibration of MOMAG determines all the calibration parameters of the sensors for accurate magnetic field measurements in orbit with the appropriate corrections. | ManMing Chen Kai Liu XiaoWen Hu YiRen Li XinJun Hao ZongHao Pan | 2023 | Earth and Planetary Physics2023，7，3： | 0 |
| 16 | Multifunctional AIE Molecules Possessing Long-lasting Room Temperature Phosphorescence, Thermally Activated Delayed Fluorescence and Dual-mode Mechanochromism显示文摘Two simple donor-acceptor multifunctional pure organic light-emitting molecules[(9H-carbazol-9-yl)(4-hydroxyphenyl)-methanone(CzMP)and(4-hydroxyphenyl)(10H-phenothiazin-10-yl)methanone(PTZMP)]with distinct aggregation-induced emission(AIE)properties were synthesized.Surprisingly,CzMP showed a long room temperature phosphorescence lifetime(>900 ms),and PTZMP exhibited triple emission of prompt fluorescence(PF),room temperature phosphorescence(RTP)and thermally activated delayed fluorescence(TADF).Furthermore,CzMP effectively responded to mechanical external forces and solvent fumigation,exhibiting dual-mode mechanochromic luminescence(MCL)including multiple fluorescence color shifts and phosphorescence switching.Time-dependent density functional theory(TDDFT)calculations were investigated to explain different luminescence properties of the two molecules,and the single crystal of CzMP was obtained and analyzed to demonstrate the unique molecular stacking pattern and strong intermolecular interactions in close association with phosphorescence emission.The multifunctional luminescent properties of the emitters explored in this work could be more effectively applied to a wide range of applications,such as information encryption and anti-counterfeiting. | ZHANG Xiaokun LI Xiaolong WANG Zonghao BAI Lulu QU Hongmei XU Songlin | 2023 | Chemical Research in Chinese Universities2023，39，6： | 0 |
| 17 | The Mars orbiter magnetometer of Tianwen-1:in-flight performance and first science results显示文摘The Mars Orbiter MAGnetometer(MOMAG)is a scientific instrument onboard the orbiter of China’s first mission for Mars—Tianwen-1.Since November 13,2021,it has been recording magnetic field data from the solar wind to the magnetic pile-up region surrounding Mars.Here we present its in-flight performance and first science results,based on its first one and one-half months’data.Comparing these early MOMAG observations to the magnetic field data in the solar wind from NASA’s Mars Atmosphere and Volatile EvolutioN(MAVEN)mission,we report that the MOMAG magnetic field data are at the same level in magnitude,and describe the same magnetic structures with similar variations in three components.We recognize 158 clear bow shock(BS)crossings in these MOMAG data;their locations match well statistically with the modeled average BS.We also identify and compare five pairs of datasets collected when Tianwen-1’s orbiter and the MAVEN probe made simultaneous BS crossings.These BS crossings confirm the global shape of modeled BS,as well as the south-north asymmetry of the Martian BS.Two cases presented in this paper suggest that the BS is probably more dynamic at flank than near the nose.So far,MOMAG performs well,and provides accurate magnetic field vectors.MOMAG is continuously scanning the magnetic field surrounding Mars.Data from MOMAG’s measurements complement data from MAVEN and will undoubt edly advance our understanding of the plasma environment of Mars. | YuMing Wang TieLong Zhang GuoQiang Wang SuDong Xiao ZhuXuan Zou Long Cheng ZongHao Pan Kai Liu XinJun Hao YiRen Li ManMing Chen ZhouBin Zhang Wei Yan ZhenPeng Su ZhiYong Wu ChengLong Shen YuTian Chi MengJiao Xu JingNan Guo Yang Du | 2023 | Earth and Planetary Physics2023，7，2： | 0 |
| 18 | Rational design of nanocarriers for mitochondria-targeted drug delivery显示文摘Well-developed mitochondria-targeted nanocarriers for function regulation are highly desirable.Numerous studies have been conducted on the treatment of mitochondria-related diseases;however,further improvements are required to develop more effective drug delivery methods.Herein,we comprehensively introduce recent developments progress in rational design of mitochondria-targeted nanocarriers,and discuss the different strategies of available nanocarriers for targeting mitochondria.We also highlight the advantages and disadvantages of various carrier systems that are currently in use.Finally,perspective on new generation for mitochondria-targeted delivery systems in the emerging area of drug-based therapeutics is also discussed. | Lihua Huang Zonghao Sun Qian Shen Zhongxi Huang Shuangxi Wang Naidi Yang Gongqiang Li Qiong Wu Wei Wang Lin Li Changmin Yu | 2022 | Chinese Chemical Letters2022，33，9： | 0 |
| 19 | β-decay study of neutron-rich nucleus ^(34)Al显示文摘The'island of inversion'has been known for over a quarter century,since Warburton et al.[1]proposed that nuclei with intruder ground states would constitute a 3×3 square with Z=10-12,N=20-22 in 1990.Uncovering the underlying inversion mechanism and exploring the scope of the island have attracted significant theoretical and experimental efforts in the following years.Now it is well known that the reduction of N=20 shell gap,which is likely caused by the | Rui Han XiangQing Li WeiGuang Jiang ZhiHuan Li Hui Hua ShuangQuan Zhang CenXi Yuan DongXing Jiang YanLin Ye Jing Li ZongHao Li FuRong Xu QiBo Chen Jie Meng JianSong Wang Chuan Xu YeLei Sun ChunGuang Wang HongYi Wu ChenYang Niu ChenGuang Li Chao He Wei Jiang PengJie Li HongLiang Zang Jun Feng SiDong Chen Qiang Liu XiaoChi Chen HuShan Xu ZhengGuo Hu YanYun Yang Peng Ma JunBing Ma ShiLun Jin Zhen Bai MeiRong Huang Yuan Jie Zhou WeiHu Ma Yong Li XiaoHong Zhou YuHu Zhang GuoQing Xiao WenLong Zhan | 2017 | Science China(Physics,Mechanics & Astronomy)2017，60，4： | 0 |
| 20 | Nitrogen deposition mediates more stochastic processes in structuring plant community than soil microbial community in the Eurasian steppe显示文摘Anthropogenic environmental changes may affect community assembly through mediating both deterministic(e.g.,competitive exclusion and environmental filtering)and stochastic processes(e.g.,birth/death and dispersal/colonization).It is traditionally thought that environmental changes have a larger mediation effect on stochastic processes in structuring soil microbial community than aboveground plant community;however,this hypothesis remains largely untested.Here we report an unexpected pattern that nitrogen(N)deposition has a larger mediation effect on stochastic processes in structuring plant community than soil microbial community(those<2 mm in diameter,including archaea,bacteria,fungi,and protists)in the Eurasian steppe.We performed a ten-year nitrogen deposition experiment in a semiarid grassland ecosystem in Inner Mongolia,manipulating nine rates(0–50 g N m^(-2)per year)at two frequencies(nitrogen added twice or 12 times per year)under two grassland management strategies(fencing or mowing).We separated the compositional variation of plant and soil microbial communities caused by each treatment into the deterministic and stochastic components with a recently-developed method.As nitrogen addition rate increased,the relative importance of stochastic component of plant community first increased and then decreased,while that of soil microbial community first decreased and then increased.On the whole,the relative importance of stochastic component was significantly larger in plant community(0.552±0.035;mean±standard error)than in microbial community(0.427±0.035).Consistently,the proportion of compositional variation explained by the deterministic soil and community indices was smaller for plant community(0.172–0.186)than microbial community(0.240–0.767).Meanwhile,as nitrogen addition rate increased,the linkage between plant and microbial community composition first became weaker and then became stronger.The larger stochasticity in plant community relative to microbial community assembly suggested that more stochastic strategies(e.g.,seeds addition)should be adopted to maintain above-than below-ground biodiversity under the pressure of nitrogen deposition. | Wei Yang Shuhan Zhang Ang Li Junjie Yang Shuang Pang Zonghao Hu Zhiping Wang Xingguo Han Ximei Zhang | 2024 | Science China(Life Sciences)2024，67，4： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员