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| 1 | Adsorption of VOCs on reduced graphene oxide显示文摘A modified Hummer's method was adopted for the synthesis of graphene oxide(GO) and reduced graphene oxide(rGO). It was revealed that the modified method is effective for the production of GO and rGO from graphite. Transmission electron microscopy(TEM) images of GO and rGO showed a sheet-like morphology. Because of the presence of oxygenated functional groups on the carbon surface, the interlayer spacing of the prepared GO was higher than that of rGO. The presence of \OH and C_O groups in the Fourier transform infrared spectra(FTIR) spectrum and G-mode and 2D-mode in Raman spectra confirmed the synthesis of GO and rGO. rGO(292.6 m^2/g) showed higher surface area than that of GO(236.4 m^2/g). The prepared rGO was used as an adsorbent for benzene and toluene(model pollutants of volatile organic compounds(VOCs)) under dynamic adsorption/desorption conditions. rGO showed higher adsorption capacity and breakthrough times than GO. The adsorption capacity of rGO for benzene and toluene was 276.4 and 304.4 mg/g, respectively.Desorption experiments showed that the spent rGO can be successfully regenerated by heating at 150.0°C. Its excellent adsorption/desorption performance for benzene and toluene makes rGO a potential adsorbent for VOC adsorption. | Lian Yu Long Wang Weicheng Xu Limin Chen Mingli Fu Junliang Wu Daiqi Ye | 2018 | Journal of Environmental Sciences2018，30，5： | 10 |
| 2 | Toluene decomposition performance and NOx by-product formation during a DBD-catalyst process显示文摘Characteristics of toluene decomposition and formation of nitrogen oxide(NOx) by-products were investigated in a dielectric barrier discharge(DBD) reactor with/without catalyst at room temperature and atmospheric pressure. Four kinds of metal oxides, i.e., manganese oxide(Mn Ox), iron oxide(Fe Ox), cobalt oxide(Co Ox) and copper oxide(Cu O), supported on Al2O3/nickel foam, were used as catalysts. It was found that introducing catalysts could improve toluene removal efficiency, promote decomposition of by-product ozone and enhance CO2 selectivity. In addition, NOx was suppressed with the decrease of specific energy density(SED) and the increase of humidity, gas flow rate and toluene concentration, or catalyst introduction. Among the four kinds of catalysts, the Cu O catalyst showed the best performance in NOx suppression. The Mn Ox catalyst exhibited the lowest concentration of O3 and highest CO2 selectivity but the highest concentration of NOx. A possible pathway for NOx production in DBD was discussed. The contributions of oxygen active species and hydroxyl radicals are dominant in NOx suppression. | Yufang Guo Xiaobin Liao Mingli Fu Haibao Huang Daiqi Ye | 2015 | Journal of Environmental Sciences2015，27，2： | 7 |
| 3 | Highly efficient Cu/anatase TiO2 {001}-nanosheets catalysts for methanol synthesis from CO2显示文摘Anatase TiO_2 nanosheets(-ns-) with dominant exposed {001} facets were used as support to load copper,and the synthesized Cu/TiO_2-ns catalysts were evaluated for CO_2 hydrogenation to methanol. Under the reaction conditions, P = 3.0 MPa, T = 260 ℃, V(N_2):V(H_2):V(CO_2) = 8:69:23 and gas hourly space velocity(GHSV) = 3600 mL g^(-1)h^(-1), the methanol yield reached an appealing high value, 5.6%. Copper-loading amount, calcination temperature and reduction atmosphere have been investigated in this work, which significantly influence the particle sizes of copper and/or the defect concentration in TiO_2, then leading to different catalytic performance. Characterizations of XRD, EPR, CO_2-TPD and FTIR demonstrate that higher specific surface area of Cu is good for the hydrogenation of CO_2 and adequate amount of Ti^(3+) plays important roles in CO_2 activation. Both of them facilitate high turnover frequency(TOF) of methanol formation. | Yunfeng Bao Chunlei Huang Limin Chen Yu dong Zhang Long Liang Jinjun Wen Mingli Fu Junliang Wu Daiqi Ye | 2018 | Journal of Energy Chemistry2018，27，2： | 7 |
| 4 | Macroporous Ni foam-supported Co_3O_4 nanobrush and nanomace hybrid arrays for high-efficiency CO oxidation显示文摘Herein, we reported the synthesis of well-defined Co_3O_4 nanoarrays(NAs) supported on a monolithic three-dimensional macroporous nickel(Ni) foam substrate for use in highefficiency CO oxidation. The monolithic Co_3O_4 NAs catalysts were obtained through a generic hydrothermal synthesis route with subsequent calcination. By controlling the reaction time,solvent polarity and deposition agent, these Co_3O_4 NAs catalysts exhibited various novel morphologies(single or hybrid arrays), whose physicochemical properties were further characterized by using several analytical techniques. Based on the catalytic and characterization analyses, it was found that the Co_3O_4 NAs-6 catalyst with nanobrush and nanomace arrays displayed enhanced catalytic activity for CO oxidation, achieving an efficient 100% CO oxidation conversion at a gas hourly space velocity(GHSV) 10,000 hr^(-1) and 150°C with longterm stability. Compared with the other Co_3O_4 NAs catalysts, it had the highest abundance of surface-adsorbed oxygen species, excellent low-temperature reducibility and was rich in surface-active sites(Co^(3+)/Co^(2+)= 1.26). | Shengpeng Mo Hui He Quanming Ren Shuangde Li Weixia Zhang Mingli Fu Limin Chen Junliang Wu Yunfa Chen Daiqi Ye | 2019 | Journal of Environmental Sciences2019，31，1： | 4 |
| 5 | Post-marketing safety surveillance and reevaluation of Motherwort injection:A clinical study of 10094 cases显示文摘OBJECTIVE:To investigate the safety profiles of Motherwort injection(MI).METHODS:A multi-center,prospective and drugderived hospital intensive monitoring method was conducted to assess the safety of MI in real world applications.This study was based on a very large population after the injection was approved and marketed in China.All patients using the injection in participating hospitals were monitored to determine the incidence,pattern,severity and outcome of associated adverse events.RESULTS:The post-marketing surveillance was performed in 10 094 female patients from April to December,2015.The incidence of adverse drug reactions(ADRs) was 0.79‰(8/10 094).Among the 8 patients,the reported adverse events mainly included systemic abnormalities,such as fever,chills and eyelid edema;skin and appendages disorders,such as pruritus and rash;gastrointestinal disorders,such as nausea,abdominal distension and pain;heart rate and rhythm disorders,such as palpitation and increased heart rate.All of these ADRs were mild in severity.CONCLUSION:In this study the ADRs incidence rate of MI is very low,which supports that it is generally safe for use in obstetric and gynecological diseases.However,the total number of 8 ADRs recorded over a relatively short time span seems limited,and the low number of reports could not represent an absolute guarantee of safety. | Cao Shan Zhang Wenhao Zhao Ziwei Heng Mingli Bu Huaien Wang Hongwu Liu Xinghui Wang Zhong Cai Yan Ma Yuyan Cui Shihong Deng Jihong Ding Guifeng Ding Yajuan Dong Linhong Duan Zhentao Fan Ling Fan Yang Fu Fen He Jing Ji Shuying Jin Lin Li Hong Li Hongying Liao Tao Lu Wei Luo Xiucui Lü Zhihui Ma Fengchun Ma Dafeng Shi Tianyun Sun Juying Sun Xiaotong Teng Hong Wang Jinhua Wang Ruihua Wang Ying Wang Zhengling Xi Jie Xu Minjuan Xu Zhihong Yan Qian Yang Cuirong Yang Yimei Yin Jie Yu Jinhua Yuan Wenjun Zhang Guanli Zhang Meihua Zhao Renfeng Zhong Yonghong Zhou Jian | 2018 | Journal of Traditional Chinese Medicine2018，38，4： | 4 |
| 6 | Experimental study on the partial discharge and AC breakdown properties of C_(4)F_(7)N/CO_(2)mixture显示文摘As an environmental friendly insulating medium,C_(4)F_(7)N has received extensive attention in the past two years.In this study,the partial discharge(PD)and breakdown characteristics of C_(4)F_(7)N/CO_(2)gas mixture were investigated using the gas insulation performance test platform.The influence of gas pressure and mixing ratio on the PD initial voltage(PDIV)and breakdown voltage of C_(4)F_(7)N/CO_(2)gas mixture in different electric fields was tested.It was found that the PDIV and breakdown voltage of gas mixture with 2-8%C_(4)F_(7)N in the highly non-uniform field showed a linear saturation increasing trend with the change of gas pressure and mixing ratio.The breakdown voltage of gas mixture increases linearly with gas pressure in the quasi-uniform electric field.The relative breakdown voltage of gas mixture in the highly non-uniform field under high-pressure conditions is inferior to those of low-pressure conditions.The C_(4)F_(7)N/CO_(2)gas mixture containing 2-8%C_(4)F_(7)N is sensitive to the non-uniformity of electric field.According to the PD and breakdown tests results,C_(4)F_(7)N/CO_(2)gas mixture with 2-8%C_(4)F_(7)N has the potential to replace SF6 using in gas-insulated equipment. | Yi Li Xiaoxing Zhang Ji Zhang Mingli Fu Ran Zhuo Yi Luo Dachang Chen Song Xiao | 2019 | High Voltage2019，4，1： | 4 |
| 7 | Unraveling specific role of carbon matrix over Pd/quasi-Ce-MOF facilitating toluene enhanced degradation显示文摘Metal organic frameworks(MOFs)derivatives represented by quasi-MOFs have excellent physical and chemical properties and can be applied for the catalytic combustion of volatile organic compounds(VOCs).In this work,Pd/quasi-Ce-BTC synthesized by simple one-step Npyrolysis was applied to the oxidation of toluene,showing excellent toluene catalytic activity(T_(90)=175℃,30000 mL/(g·h)).Microscopic analyses indicate the formation and interaction of a carbon matrix composite quasi-MOF structure interface.The results show that the amorphous carbon matrix formed during the partial pyrolysis of Ce-BTC significantly improves the adsorption and activation capacity of toluene in the reaction,and constructs a reductive system to maintain high concentrations of Ce^(3+)and Pd^(0),which can facilitate the activation and utilization of oxygen in reaction.Quasi in-situ XPS proves that carbon matrix is indirectly involved in the activation and storage of oxygen,and Pd^(0)is the crucial active site for the activation of oxygen.Stability and water resistance tests display good stability of Pd/quasi-Ce-BTC.This work provides a potential method for designing quasi-MOF catalysts towards VOCs effective abatement. | Chunjing Su Zhi Li Mengqi Mao Wenhua Ye Jinping Zhong Quanming Ren Hairong Cheng Haomin Huang Mingli Fu Junliang Wu Yun Hu Daiqi Ye Haihong Xu | 2022 | Journal of Rare Earths2022，40，11： | 2 |
| 8 | Construction of Cu-Ce interface for boosting toluene oxidation:Study of Cu-Ce interaction and intermediates identified by in situ DRIFTS显示文摘A facile hydrothermal method was applied to gain stably and highly efficient CuO-CeO_(2)(denoted as Cu1Ce2)catalyst for toluene oxidation.The changes of surface and inter properties on Cu1Ce2 were investigated comparing with pure CeO_(2)and pure CuO.The formation of Cu-Ce interface promotes the electron transfer between Cu and Ce through Cu^(2+)+Ce^(3+)↔Cu^(+)+Ce^(4+)and leads to high redox properties and mobility of oxygen species.Thus,the Cu1Ce2 catalyst makes up the shortcoming of CeO_(2)and CuO and achieved high catalytic performance with T_(50)=234°C and T_(99)=250°C(the temperature at which 50%and 90%C_(7)H_(8)conversion is obtained,respectively)for toluene oxidation.Different reaction steps and intermediates for toluene oxidation over Cu1Ce2,CeO_(2)and CuO were detected by in situ DRIFTS,the fast benzyl species conversion and preferential transformation of benzoates into carbonates through C=C breaking over Cu1Ce2 should accelerate the reaction. | Jiahui Lu Jinping Zhong Quanming Ren Jiaqi Li Linghe Song Shengpeng Mo Mingyuan Zhang Peirong Chen Mingli Fu Daiqi Ye | 2021 | Chinese Chemical Letters2021，32，11： | 2 |
| 9 | Research progress of semiconductive shielding layer of HVDC cable显示文摘As an indispensable part of high-voltage direct current(HVDC)cable,the semiconductive shielding layer plays the role of uniforming electric field in the cable.However,cable shielding materials>35 kV mainly rely on foreign imports in China,which belongs to the technical weak issues in the field of electrical materials.At present,there are few systematic reports on semiconductive shielding material of HVDC cable.In the work,the mechanisms of charge conduction and thermal conduction of semiconductive material have been introduced.Effect of raw material,carbon black content and the second conductive filler on the resistance characteristics of the semiconductive layer,the charge accumulation characteristics of the insulating layer and the interface characteristics have been studied.A kind of semiconductive layer as a high voltage terminal charge emission method has been proposed to study charge emission from the semiconducting layer to the insulation layer.This work can provide theoretical guidance for the research of semiconductive shielding materials. | Yanhui Wei Wang Han Guochang Li Qingquan Lei Mingli Fu Chuncheng Hao Guanjun Zhang | 2020 | High Voltage2020，5，1： | 2 |
| 10 | Space charge behav- ior in multi-layer oil-paper insulation under different dc voltages and temperatures 显示文摘 | TANG Chao CHEN G FU Mingli | 2010 | IEEE Transactions on Dielectrics and E- lectrical Insulation2010，17，3： | 1 |
| 11 | Elects of cupping therapy on the pulmonary functions in asthmatic children 显示文摘 | Hong Jiaxuan Fu Mingli Wang Xiaoyuan | 2006 | Journal of Tra- ditional Chinese Medicine2006，26，1： | 1 |
| 12 | Soot oxidation via CuO doped CeO2 catalysts prepared using coprecipitation and citrate acid complex-combustion synthesis显示文摘 | Fu Mingli Yue Xianghui Ye Daiqi | 2010 | Catalysts Today2010，，3： | 1 |
| 13 | Plasma-Catalytic Oxidation of Toluene on Mn x O y at Atmospheric Pressure and Room Temperature显示文摘 | Meijuan Lu Rong Huang Peitao Wang Limin Chen Junliang Wu Mingli Fu William Wen Bichun Huang Daiqi Ye | 2014 | Plasma Chemistry and Plasma Processing2014，，5： | 1 |
| 14 | On the performance and mechanisms of toluene removal by FeO x /SBA-15-assisted non-thermal plasma at atmospheric pressure and room temperature显示文摘 | Meijuan Lu Rong Huang Junliang Wu Mingli Fu Limin Chen Daiqi Ye | 2014 | Catalysis Today2014，，： | 1 |
| 15 | Immobilizing ultrafine bimetallic PtAg alloy onto uniform MnO_(2) microsphere as a highly active catalyst for CO oxidation显示文摘Herein,a facile glycol reduction route is successful employed to synthesize bimetallic Pt Ag alloys with homogeneous distribution of sizes and elements.Experimental studies reveal that the ultrafine Pt Ag alloys with well-defined sizes from around 3.3 nm to 5.8 nm are immobilized onto MnO_(2)microsphere,which remarkably enhances the catalytic performances for CO oxidation.Importantly,quasi in-situ X-ray photoelectron spectroscopy(XPS)result reveals that both Mn and Pt ions on the surface of catalysts would realize alternating reduction-oxidation by CO and O_(2)molecules,and the oxygen vacancy sites could be replenished and excited by gas-phase O_(2). | Shengpeng Mo Peng Peng Yinchang Pei Taiming Shen Qinglin Xie Mingli Fu Yunfa Chen Daiqi Ye | 2021 | Chinese Chemical Letters2021，32，6： | 1 |
| 16 | Broadband impedance spectrum detection of buffer layer defects in 110 kV crosslinked polyethylene cable with corrugated aluminium sheath显示文摘The buffer layer defects of high‐voltage crosslinked polyethylene(XLPE)cable occur frequently,which makes the detection method become the focus to be studied.Here,the broadband impedance detection technology for the buffer layer defects of high‐voltage XLPE cables with corrugated aluminium sheath is investigated.There are nine cable samples,including new and defective ones.Some of the defective cables are artificial,and the other is retired cables.The influence of wiring mode,the circumferential relative position of electrodes,cable length,artificial white powder,artificial damp,and retired defective cables on the impedance spectrum is studied.It is found that the wiring mode of the insulation shield/aluminium sheath at the end of the cable can effectively detect the buffer layer defects.And the broadband impedance amplitude spectrum of the buffer layer in defective cable,measuring at various circumferential relative positions,is obviously different.When there are white powders,air gaps,or ablation in the buffer layer,the broadband impedance spectrum(BIS)will increase by several times.When the buffer layer is damped,the BIS will reduce.The research here provides theoretical support and technical methods for the buffer layer defects of XLPE cable with corrugated aluminium sheath. | Yanpeng Hao Peng Zhao Baojun Hui Yanting Cheng Wenbo Zhu Mingli Fu Xiaodong Li | 2023 | High Voltage2023，8，5： | 0 |
| 17 | Corrigendum to ‘Adsorption of VOCs on reduced graphene oxide’ [J. Environ. Sci. 67 (2018) 171-178]显示文摘The authors regret“In the whole text,ppm and mg/L was confusing.As in aqueous phase,1 ppm=1 mg/L,but in gaseous phase,1 ppm=0.001%o.In this paper,in text and figures,the concentration units were ppm,but when calculating the adsorption ca-pacity,the concentration units ppm were mistakenly used as mg/L.As for benzene,1 ppm=3.4871 x 10^-3 mg/L,as for toluene。 | Lian Yu Long Wang Weicheng Xu Limin Chen Mingli Fu Junliang Wu Daiqi Ye | 2020 | Journal of Environmental Sciences2020，32，4： | 0 |
| 18 | An evolving trajectory-from PD,logistics,SCM to the theory of material flow显示文摘The growing interest in the material flow(MF)theory has invoked much interesting research in recent years.Although the MF theory is relatively new,a review of the related literature from a historical perspective shows that MF theory represents a new stage of the evolutionary development of interrelated subjects such as Physical Distribution(PD),Logistics,and Supply Chain Management(SCM).The purpose of this paper is to provide a summative review of the evolution of the subjects of PD,Logistics,and SCM,and their new development,MF theory.The paper aims at tracing how concepts and findings in PD,Logistics,SCM,and MF have been developed and have evolved.The study shows that PD evolved to Logistics in middle of the 1980s;starting from the late 1990s,Logistics has evolved to SCM;and today PD,Logistics,and SCM can be considered to be under the umbrella provided by a new theory called MF theory.This paper points out that MF theory is a necessity to deal with the overwhelming complexity of material flow systems in the global economy of the twenty-first century. | Hanping Hou Mikhail Yu Kataev Zuopeng(Justin)Zhang Sohail Chaudhry Huiqi Zhu Liuliu Fu Mingli Yu | 2015 | Journal of Management Analytics2015，2，2： | 0 |
| 19 | Synergistic catalytic ozonation of toluene with manganese and cerium varies at low temperature显示文摘The temperature of waste gas in refuse transfer station,airport smoking area,and RTO terminal is low,which needs deep oxidation.Catalytic ozonation is one of the most effective treatment techniques in these scenarios.In this study,we reported that catalysts were modified under the condition of mag-netic field to simulate the low temperature dynamic conditions of low concentration toluene for catalytic ozonation.This paper aims to explore the relationship between oxygen vacancy and active oxygen species,and the specific pathways of toluene oxidation.The study found that citric acid can enhance the syner-gistic effect between Mn and Ce,and promote the generation of oxygen vacancies.The surface molecule adsorption oxygen is more conducive to catalytic oxidation than subsurface atom adsorption oxygen.Fi-nally,we proposed the main pathways of toluene in this reaction system,which runs through the whole process of the reaction. | Qi Gan Mingli Fu Peng Liu Yuchen Zhang Juxia Xiong Jinping Zhong Lei Liu Junliang Wu Xiaojun Niu Yun Hu Daiqi Ye | 2022 | Chinese Chemical Letters2022，33，5： | 0 |
| 20 | Effects of Zr substitution on soot combustion over cubic fluorite-structured nanoceria:Soot-ceria contact and interfacial oxygen evolution显示文摘Ceria is widely used as a catalyst for soot combustion,but effects of Zr substitution on the reaction mechanism is ambiguous.The present work elucidates effects of Zr substitution on soot combustion over cubic fluorite-structured nanoceria.The nanostructured CeO_(2),Ce_(0.92)Zr_(0.08)O_(2),and Ce_(0.84)Zr_(0.16)O_(2)composed of 5-6 nm crystallites display T_(m-CO2)(the temperature at maximum CO_2 yield)at 383,355,and 375℃under 10 vol.%O_(2)/N_(2),respectively.The size of agglomerate decreases from 165.5 to 51.9-57.3 nm,which is beneficial for the sootceria contact.Moreover,Zr increases the amount of surface oxygen vacancies,generating more active oxygen(O_(2)^-and O^(-))for soot oxidation.Thus,the activities of Ce_(0.92)Zr_(0.08)O_(2)and Ce_(0.84)Zr_(0.16)O_(2)in soot combustion are better than that of CeO_(2).Although oxygen vacancies promote the migration of lattice O~(2-),the enriched surface Zr also inhibits the mobility of lattice O^(2-).Therefore,the T_(m-CO2)of Ce_(0.84)Zr_(0.1)6 O_(2)is higher than that of Ce_(0.92)Zr_(0.08)O_(2).Based on reaction kinetic study,soot in direct contact with ceria preferentially decomposes with low activation energy,while the oxidation of isolated soot occurs through diffusion with high activation energy.The obtained findings provide new understanding on the soot combustion over nanoceria. | Peng Liu Xiaoliang Liang Yanliu Dang Junkai He Alireza Shirazi-Amin Laura A.Achola Shanka Dissanayake Hanlin Chen Mingli Fu Daiqi Ye Steven L.Suib | 2021 | Journal of Environmental Sciences2021，33，3： | 0 |
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