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| 1 | Abundant Production of Reactive Water Radical Cations under Ambient Conditions显示文摘Water radical cations,the crucial intermediates in many aqueous reactions and biochemical processes,are difficult to investigate experimentally due to their short lifetime andlowabundance.Herein,ahomemade device based on energy-tunable discharge was employed to deposit suitable amounts of energy to atmospheric pressure pure water vapor for abundant production of water radical cations,stabilized as(H_(2)O)n^(+·)(n=2-5)with a maximal abundance of≥8.3×10^(6) cps for(H_(2)O)_(2)^(+·),characterized by mass spectrometry(MS).The abundance of water radical cations was optimized by adjusting the experimental parameters such as the discharge voltage(2.5 kV),temperature of the MS inlet(140℃),carrier gas flow(20mL/min),and the distance between the discharge tip and MS inlet(12 mm).The ambient formation of water radical cationswas further confirmedby thehigh reactivity of as-prepared water radical cations,which reacted with benzene,ethyl acetate,and dimethyl disulfide instantly,showing rich chemistry with ionic and radical characteristics.Moreover,the computations usingCCSD(T)//MP2 method and density functional theory confirmed that the O-O single-electron bound dimer(B),as well as the hydronium hydroxyl radical complex(A),accounted for the unusual chemistry of the water radical cations,providing a facile approach to access the high reactivity ofwater radical cations under the ambient conditions. | Meng Wang Xiao-Fei Gao Rui Su Peng He Yuan-Yuan Cheng Ke Li Dongbo Mi Xiaoping Zhang Xinglei Zhang Huanwen Chen R.Graham Cooks | 2022 | CCS Chemistry2022，4，4： | 3 |
| 2 | Modulation of the effector functions of a human lgGI through engineering of its hinge region显示文摘 | DALL'ACQUA WF COOK KE Damschroder MM | 2006 | J Immunol2006，177，2： | 1 |
| 3 | Comparing the effective- ness of an inverted classroom to a traditional classroom in an Up- per-Division engineering course 显示文摘 | MASON GS SHUMAN TR COOK KE | 2013 | IEEE Transac Educ2013，56，4： | 1 |
| 4 | Delp An Overview of Parallel Processing Approaches to Image and Video Compression显示文摘 | Gregory W Cook Leah H Jamieson Edward J | 1994 | Proceedings of SPIE-The International Society for Optical Engineering1994，2186，： | 1 |
| 5 | The risk of bleeding in thrombocytopenic patients with acute myeloid leukemia显示文摘 | Webert KE Cook RJ Sigouin CS | 2006 | Haematological2006，91，11： | 1 |
| 6 | Timing of heparin and perfusion temperature during procurement of organs with extracorporeal support in donors after circulatory determination of death显示文摘 | Rojas-Pena A Hall CM Cook KE | 2011 | ASAIO J2011，57，： | 1 |
| 7 | Platelet and leukocyte activation and design consequences for thoracic artificial lungs显示文摘 | Cook KE Maxhimer J Leonard DJ | 2002 | ASAIO J2002，48，6： | 1 |
| 8 | Timing of heparin and perfusion temperature during proeurement of organs with extracorporeal support in donors after circulatory determination of death显示文摘 | Rojas-Pena A Hall CM Cook KE | 2011 | ASAIO J2011，57，5： | 1 |
| 9 | Modulation of the effector functions of a human IgG1 through engineering of its hinge region 显示文摘 | Dall'Aequa WF Cook KE Damschroder MM | 2006 | J Immunol2006，177，： | 1 |
| 10 | Timing of heparinand perfusion temperature during procurement of organs withextracorporeal support indonors after circulatory determination ofdeath 显示文摘 | Rojas-Pena A Hall CM Cook KE | 2011 | ASAIO J2011，57，5： | 1 |
| 11 | Timing of heparin andperfusion temperature during procurement of organs withextracorporeal support in donors after circulatory determination ofdeath 显示文摘 | Rojas-Pena A Hall CM Cook KE | 2011 | ASAIO J2011，57，5： | 1 |
| 12 | Primary structure of the human platelet serotmxin 5 - HT2A receptor: identify with frontal cortex serotonin 5 - HT2A receptor显示文摘 | Cook EH Fletcher KE Wainwright M | 1994 | Journal of Neurochemistry1994，63，2： | 1 |
| 13 | In vivo hemodynamic re- sponses to thoracic artificial lung attachment显示文摘 | Perlman CE Cook KE Seipelt JR | 2005 | ASAIO J2005，51，4： | 1 |
| 14 | Use of probiotics to prevent ventilator-associated pneumonia:a survey of pharmacists′attitudes显示文摘 | Wheeler KE Cook DJ Mehta S | 2016 | J Crit Care2016，31，1： | 1 |
| 15 | Recommendations for Tele- phone Counseling显示文摘 | Ormond KE Haun J Cook L | 2000 | J Cenet Couns2000，9，1： | 1 |
| 16 | Urinary 8-oxo-2V- deoxyguanosine-source, significance and supplements 显示文摘 | Cooke MS Evans MD Herbert KE | 2000 | Free Radic Res2000，32，： | 1 |
| 17 | Timing of heparin and peffusion temperature during procurement of organs with extracorporeal support in donors after circulatory determination of death显示文摘 | Rojas-Pena A Hall CM Cook KE | 2011 | ASAIO J2011，57，5： | 1 |
| 18 | Methodologic issues in the use of bleeding as an outcome in transfusion medicine studies显示文摘 | Heddle NM Cook R J Webert KE | 2003 | Transfusion2003，43，6： | 1 |
| 19 | Hair product use and the risk of breast cancer in young women 显示文摘 | Cook IS Malone KE Daling JR | 1999 | Cancer Causes Control1999，10，6： | 1 |
| 20 | Timing of heparin and perfusion temperature during procurement of organs with extracorporeal support in donors after circulatory determination of death显示文摘 | Rojas-Pena A Hall CM Cook KE | | 0，，： | 1 |
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