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| 1 | Environmental application and ecological significance of nano-zero valent iron显示文摘Toxicity studies considering both the bare and stabilized forms of zero valent iron nanoparticles(nZVI) could be timely, given that ecological risks identified are minimized through modification or with substitution of approaches in the synthesis, development and environmental application of the nanoparticles before succeeding to volume production.This review is focused on the fate, transport and toxicological implications of the bare nZVI and surface modified particles used for environmental applications. | Biruck D.Yirsaw Mallavarapu Megharaj Zuliang Chen Ravi Naidu | 2016 | Journal of Environmental Sciences2016，28，6： | 13 |
| 2 | Spatio-temporal Pattern Characteristics of Relationship Between Urbanization and Economic Development at County Level in China显示文摘The relationship between China’s urbanization and economic development(RCUED) is an important concern nationwide. As important actors in regional strategy and policy, county-level regions have played an increasingly significant role in the development of China’s social economy. However, the existing research on the RCUED lacks the fine depiction of the county-level administrative units.Using 2000 and 2010 census data and the statistical analysis method, we uncovered the evolution characteristics of China’s urbanization and economic development and conducted a quantitative identification for the RCUED with improved methods using the quadrant map approach. In addition, we investigated the spatial correlation effect of the RCUED using the spatial autocorrelation analysis method. The results were as follows: 1) In general, a high degree of matching exists between China’s urbanization and economic development at the county level at the significance level of 0.01. The correlation coefficients between China’s urbanization and economic development in2000 and 2010 were 0.608 and 0.603, respectively. 2) A significant regional difference exists in the RCUED at the county level. Based on a comparative analysis of 2276 county units in China in the two years, we found that county units can be categorized as under-urbanized, basic coordination and over-urbanized in various areas. No situation was observed where urbanization seriously lagged behind the economic development level, so the levels of urbanization and economic development appear to be basically coordinated,and the coordination state may be gradually optimized over time. 3) Over time, the spatial dependency of the RCUED has weakened and the spatial heterogeneity has increased. Northeast China has always been an area characterized by over-urbanization. The number of county units classified as under-urbanized has begun to decline in eastern coastal urban agglomeration areas, while counties rich in resources have transformed from having point-shaped over-urbanization to plane-shaped under-urbanization along the northern border,and the number of over-urbanized county units has increased in the middle reaches of the Yangtze River. 4)’Lag-lag’ type and ’advance-advance’ type accounted for 68% of all counties in China, and these counties were shown to have obvious spatial differentiation characteristics. | YANG Zhen ZHANG Xiaolei LEI Jun DUAN Zuliang LI Jiangang | 2019 | Chinese Geographical Science2019，29，4： | 9 |
| 3 | Integrated transcriptomic and metabolomic analyses of a wax deficient citrus mutant exhibiting jasmonic acid-mediated defense against fungal pathogens显示文摘Naturally,resistant crop germplasms are important resources for managing the issues of agricultural product safety and environment deterioration.We found a spontaneous mutant of‘Newhall’navel orange(Citrus sinensis Osbeck)(MT)with broad-spectrum protections against fungal pathogens in the orchard,postharvest-storage,and artificial inoculation conditions.To understand the defense mechanism of MT fruit,we constructed a genome-scale metabolic network that integrated metabolome and transcriptome datasets.The coordinated transcriptomic and metabolic data were enriched in two sub-networks,showing the decrease in very long chain fatty acid(by 41.53%)and cuticular wax synthesis(by 81.34%),and increase in the synthesis of jasmonic acid(JA)(by 95.23%)and JA-induced metabolites such as 5-dimethylnobietin(by 28.37%)in MT.Furthermore,cytological and biochemical analyses confirmed that the response to fungal infection in MT was independent of wax deficiency and was correlated with the levels of jasmonates,and the expression of plant defensin gene PDF1.2.Results of exogenous application of MeJA and JA inhibitors such as propyl gallate proved that JA-mediated defense contributes to the strong tolerance against pathogens in MT.Our results indicated that jasmonate biosynthesis and signaling are stimulated by the fatty acid redirection of MT,and participate in the tolerance of pathogenic fungi. | Yizhong He Jingwen Han Runsheng Liu Yuduan Ding Jinqiu Wang Li Sun Xiaoming Yang Yunliu Zeng Weiwei Wen Juan Xu Hongming Zhang Xiang Yan Zhaoxing Chen Zuliang Gu Hong Chen Huanqing Tang Xiuxin Deng Yunjiang Cheng | 2018 | Horticulture Research2018，5，1： | 8 |
| 4 | IL-33 induces immunosuppressive neutrophils via a type 2 innate lymphoid cell/IL-13/STAT6 axis and protects the liver against injury in LCMV infection-induced viral hepatitis显示文摘Viral hepatitis is still a public health problem affecting several million people around the world.Neutrophils are polymorphonuclear cells that have a critical role in antibacterial infection.However,the role of neutrophils in viral infection is not fully understood.By using a mouse model of lymphocytic choriomeningitis virus infection-induced viral hepatitis,we observed increased neutrophil recruitment in the liver accompanied by enhanced CD8+T-cell responses.Liver neutrophils expressed high levels of immunomodulatory cytokines,such as C-X-C chemokine ligand 2,arginase-1,inducible nitric oxide synthase and interleukin(IL)-10,demonstrating immunosuppressive properties.Depletion of neutrophils in vivo by a neutralizing antibody resulted in the exacerbation of liver injury and the promotion of T-cell responses at the immune contraction stage.IL-33 significantly induced neutrophil recruitment in the liver and attenuated liver injury by limiting effector T-cell accumulation.Mechanistically,we found that IL-33 promoted the expression of arginase-1 in neutrophils through the type 2 innate lymphoid cell(ILC2)-derived IL-13.Additionally,IL-13 increased the inhibitory effect of neutrophils on CD8+T-cell proliferation in vitro,partially through arginase-1.Finally,we found that IL-13 induced arginase-1 expression,depending on signal transducer and activator of transcription factor 6(STAT6)signaling.Therefore,IL-33 induced immunosuppressive neutrophils via an ILC2/IL-13/STAT6 axis.Collectively,our findings shed new light on the mechanisms associated with IL-33-triggered neutrophils in the liver and suggest potential targets for therapeutic investigation in viral hepatitis. | Yuejin Liang Panpan Yi Denley Ming Kee Yuan Zuliang Jie Zakari Kwota Lynn Soong Yingzi Cong Jiaren Sun | 2019 | Cellular & Molecular Immunology2019，16，2： | 7 |
| 5 | Simultaneous removal of Cu(Ⅱ) and Cr(Ⅵ) by Mg–Al–Cl layered double hydroxide and mechanism insight显示文摘Mg–Al–Cl layered double hydroxide(Cl-LDH) was prepared to simultaneously remove Cu(Ⅱ)and Cr(VI) from aqueous solution. The coexisting Cu(Ⅱ)(20 mg/L) and Cr(VI)(40 mg/L) were completely removed within 30 min by Cl-LDH in a dosage of 2.0 g/L; the removal rate of Cu(Ⅱ) was accelerated in the presence of Cr(VI). Moreover, compared with the adsorption of single Cu(Ⅱ) or Cr(VI), the adsorption capacities of Cl-LDH for Cu(Ⅱ) and Cr(VI) can be improved by 81.05% and 49.56%, respectively, in the case of coexisting Cu(Ⅱ)(200 mg/L) and Cr(VI)(400 mg/L). The affecting factors(such as solution initial p H, adsorbent dosage, and contact time) have been systematically investigated. Besides, the changes of p H values and the concentrations of Mg^(2+) and Al^(2+)in relevant solutions were monitored. To get the underlying mechanism, the Cl-LDH samples before and after adsorption were thoroughly characterized by X-ray powder diffraction, transmission electron microscopy, Fourier transform infrared spectroscopy, and X-ray photoelectron spectroscopy. On the basis of these analyses, a possible mechanism was proposed. The coadsorption process involves anion exchange of Cr(VI) with Cl-in Cl-LDH interlayer, isomorphic substitution of Mg^(2+) with Cu^(2+), formation of Cu_2Cl(OH)_3precipitation, and the adsorption of Cr(VI) by Cu_2Cl(OH)_3. This work provides a new insight into simultaneous removal of heavy metal cations and anions from wastewater by Cl-LDH. | Xianyang Yue Weizhen Liu Zuliang Chen Zhang Lin | 2017 | Journal of Environmental Sciences2017，29，3： | 6 |
| 6 | Higher Order Triangular Mixed Finite Element Methods for Semilinear Quadratic Optimal Control Problems显示文摘In this paper,we investigate a priori error estimates for the quadratic optimal control problems governed by semilinear elliptic partial differential equations using higher order triangular mixed finite element methods.The state and the co-state are approximated by the order k Raviart-Thomas mixed finite element spaces and the control is approximated by piecewise polynomials of order k(k≥0).A priori error estimates for the mixed finite element approximation of semilinear control problems are obtained.Finally,we present some numerical examples which confirm our theoretical results. | Kang Deng Yanping Chen Zuliang Lu | 2011 | Numerical Mathematics(Theory,Methods and Applications)2011，4，2： | 4 |
| 7 | Synthesis of New Substituted 4-Amino-3,5-dinitropyridine Derivatives显示文摘为一些新 4-amino-3,5-dinitropyridine 衍生物的准备的灵巧的合成线路被揭示了。2-chloropyridin-4-amine (1 ) 的硝代作为开始的材料在意外一步舞反应,给 dinitrated 衍生物,由分别地,有钠叠氮化物,钾氟化物,氨,甲胺,和 4-nitroimidazol 的反应给了代替的 4-amino-3,5-dinitropyridine 衍生物的亲核的替换列在后面。同时,它的叠氮化物衍生物经历了戒指闭合变换进 7-amino-6-nitro-[1,2,5 ] oxadiazolo [3,4-b ] pyridine-1-oxide。是意义所有在温和条件下面亲核的替换反应被执行。 | Congming Ma Yongbin Wang Kehui Hou Zuliang Liu Qizheng Yao | 2013 | Chinese Journal of Chemistry2013，31，10： | 4 |
| 8 | Investigation of tribological properties of composite C_(60)-LB films显示文摘Composite C60-LB films were fabricated by the Langmuir-Blodgett (LB) technique, their micro- structures, micro- and macro-tribological properties were investigated using atomic force microscope/ friction force microscope (AFM/FFM). The results showed that in the confined C60-LB films there were two kinds of structures for the special C60 assembly: grain diameters of one kind were in the range of 150 -230 nm; the other was smaller than 20 nm. Mi- cro-tribological studies showed that topographical images of tiny C60 aggregates (<20 nm) were con- sistent with their frictional ones very well, namely, low friction occurred on tiny C60 aggregates compared with fatty chains LB monolayer, and ‘Micro-rolling effect’ was apparent; but for big large ones frictional forces were relatively high and ‘ratchet mechanism’ was seen apparently. Macro-tribological data proved large C60 aggregates had wear resistance and load-carrying capacities and anti-wear lives for com- posite C60-LB films were prolonged greatly with dis- persibility of C60 improved and its grain diameter re- duced. Tiny C60 aggregates were mainly the lubri- cating agents. Friction coefficients of composite C60-LB films gradually reduced with loads increasing having the same friction coefficient-load relations with boundary lubrication films. | YANG Guanghong ZHANG Xingtang XUN Jun JIANG Xiaohong ZHANG Pingyu DU Zuliang | 2006 | Chinese Science Bulletin2006，51，15： | 3 |
| 9 | Synthesis and Characterization of Some N-Aryl-4-nitroimidazoles as Potential Insensitive Energy Materials显示文摘4-nitroimidazole 的 N 芳基衍生物在优秀收益在 CuI/TBAB 催化系统下面被综合了,在 DMF 溶剂把 KOH 用作基础。 | Kehui Hou Zuliang Liu | 2013 | Chinese Journal of Chemistry2013，31，2： | 3 |
| 10 | Preventing abnormal NF-κB activation and autoimmunity by Otub1-mediated p100 stabilization显示文摘NF-κB, a family of transcription factors regulating diverse biological processes including immune responses, is activated by canonical and noncanonical pathways based on degradation of IκBα and processing of the IκB-like protein p100, respectively. Although p100 responds to noncanonical NF-κB stimuli for processing, it does not undergo degradation, but rather becomes accumulated, along with canonical NF-κB activation. We show here that the stability of p100 is tightly controlled by a deubiquitinase, Otub1. Otub1 deficiency not only promotes signal-induced p100 processing and noncanonical NF-κB activation but also causes steady-state p100 degradation, leading to aberrant NF-κB activation in the canonical pathway. B-cell-conditional deletion of Otub1 results in B-cell hyperplasia, antibody hyper-production, and lupus-like autoimmunity. Otub1-deficient B cells display aberrantly activated phenotypes and overproduce the cytokine IL-6, contributing to autoimmunity induction. Thus, maintenance of p100 stability by Otub1 serves as an unusual mechanism of NF-κB regulation that prevents autoimmunity. | Yanchuan Li Jin-Young Yang Xiaoping Xie Zuliang Jie Lingyun Zhang Jianhong Shi Daniel Lin Meidi Gu Xiaofei Zhou Haiyan S. Li Stephanie S. Watowich Antrix Jain Sung Yun Jung Jun Qin Xuhong Cheng Shao-Cong Sun | 2019 | Cell Research2019，29，6： | 3 |
| 11 | 高温合金差示扫描量热分析(DSC)的影响因素:粉末粒度和显微组织显示文摘对固溶强化型625镍基高温合金粉末进行升、降温差示扫描量热分析(DSC)试验,研究了不同粉末粒度(<37,45~53,75~105,105~150,150~355μm)对相变温度的影响。采用场发射扫描电镜(FESEM)、电子探针(EPMA)和同步辐射X射线衍射(SXRD)对625合金粉末的形貌、元素分布和相组成进行表征。结果表明:不同粒径PM625粉末均为树枝晶结构,枝晶间距在2~10μm范围,元素Ni和Cr倾向分布于枝晶干,Mo和Nb偏析于枝晶间。不同粒度的PM625粉末中均仅存在基体γ相。PM625粉末DSC加热曲线固相线附近区域拐点尖锐,表现为合金开始熔化温度(偏离基线的拐点)与名义固相线温度(切线交点)差异很小,不同粒度间的差异仅为2~5℃。合金完全熔化后重新冷却的过程中原始粉末的低偏析特性消失,冷却曲线固相线区域圆弧较大,名义固相线和终凝温度差较大,为53~65℃。DSC试验升温过程中不同粒径粉末的固、液相线以及初熔温度最大差异分别为3, 2和2℃,降温过程不同粒径粉末固、液相线温度差分别为6和2℃。0~355μm粉末粒径范围内,粒径对固溶强化型PM625高温合金粉末相变温度无明显影响。 | 郑亮 刘玉峰 Gorley Michael J Hong Zuliang DaySarah Tang Chiu C 李周 张国庆 | 2019 | 稀有金属材料与工程2019，48，5： | 3 |
| 12 | Synthesis and characterization of BiFeO_3 nanotube arrays and Y-junction BiFeO_3 nanotubes显示文摘Multiferroic BiFeO3 (BFO) nanotube arrays (~100 nm in diameter and ~50 μm in length) were synthesized by the sol-gel method utilizing the anodic aluminum oxide (AAO) membrane technique. The micro-structure and chemical components of the BFO nanotubes were investigated using scanning electron microscopy (SEM), transmission electron microscopy (TEM) and X-ray photoelectron spectrometer (XPS). The BFO nanotubes exhibited polycrystalline microstructures. The novel Y-junction BFO nano-tubes were simultaneously fabricated. | LI ChunYang LIU Bing ZHAO JianPo WANG JiangFeng HU BinBin DU ZuLiang | 2009 | Chinese Science Bulletin2009，54，5： | 3 |
| 13 | Synthesis of 2-Azido-4-nitroimidazole and Its Derivatives for High-Energy Materials显示文摘2-Azido-4-nitroimidazole 和它的衍生物为精力充沛的材料应用程序被综合了。综合混合物被 1H, 13C NMR 光谱学和元素的分析充分描绘。他们中的大多数被单个水晶 X 光检查衍射决定。混合物的计算密度在 1.71 和 1.92 g 牡汹祰慲潺敬 ? 典昊鰬[整之间变化吗? | Kehui Hou Congming Ma Zuliang Liu | 2013 | Chinese Journal of Chemistry2013，31，12： | 2 |
| 14 | CuInSe_2 thin films obtained by pulse-plating electrodeposition technique with novel pulse wave显示文摘CuInSe2 films were electrodeposited onto indium tin oxide(ITO) substrate in constant current mode using bell-like wave modulated square wave in aqueous solution.The films obtained at different pulse frequencies were characterized by scanning electron microscopy(SEM),X-ray energy dispersive spectroscopy(EDS) and X-ray diffraction(XRD).UV-Vis-NIR absorption spectro scopy was used to study the optical properties of these films.The results showed that the chalcopyrite phase CuInSe2 films with a smooth surface and stoichiometric composition could be obtained at appropriate pulse frequency.The crystallinity of CuInSe2 films could be further improved after annealing treatment.Despite this,we also found that the films obtained using the pulse-plating electrodeposition technique had a faster deposition rate and better film adhesion ability than that using the traditional CIS electrodeposition technique,which is significant to the low-cost CIS thin film solar cell production. | WANG XiaoLi WANG GuangJun TIAN BaoLi WAN ShaoMing DU ZuLiang | 2010 | Chinese Science Bulletin2010，55，18： | 2 |
| 15 | Synthesis of iron-based nanoparticles by green tea extract and their degradation of malachite显示文摘 | Xiulan Weng Lanlan Huang Zuliang Chen Mallavarapu Megharaj Ravendra Naidu | 2013 | Industrial Crops & Products2013，，： | 2 |
| 16 | Improved algorithm of atmospheric refraction error in Longley-Rice channel model显示文摘Longley-Rice channel model modifies the atmospheric refraction by the equivalent earth radius method,which is simple calculation but is not accurate.As it only uses the horizontal difference,but does not make use of the vertical section information,it does not agree with the actual propagation path.The atmospheric refraction error correction method of the Longley-Rice channel model has been improved.The improved method makes use of the vertical section information sufficiently and maps the distance between the receiver and transmitter to the radio wave propagation distance.It can exactly reflect the infection of propagation distance for the radio wave propagation loss.It is predicted to be more close to the experimental results by simulation in comparison with the measured data.The effectiveness of improved methods is proved by simulation. | Wang Zuliang Zheng Mao Wang Juan Zheng Linhua | 2008 | Journal of Systems Engineering and Electronics2008，19，4： | 2 |
| 17 | Chemical modification and the photoluminescence stabilization of titanic acid nanotubes显示文摘Titanic acid nanotubes (H2Ti2O4(OH)2) were surface-modified with cetyl alcohol through dehydration reaction because of existence of Ti–OH. The modified nanotubes were characterized by transmission electron microscopy (TEM), Fourier Transform Infrared (FT-IR) spectrometry and pho-toluminescence (PL) spectra. The results indicate that the modified nanotubes can be easily dis-persed into organic solvent such as chloroform and toluene in contrast with the unmodified nanotubes, which makes it easier to be assembled by LB technique. Moreover, the Ti-O-CH2(CH2)14CH3 on the surface of the nanotubes can hinder the adsorption of water and consequently the photoluminescence property of the nanotubes can be stabilized. Even though kept in humid condition or in air for a long time, the modified nanotubes also maintain the special photoluminescence property in the visible re-gion. | ZHANG Xingtang WANG Yumei ZHANG Chunmei JIANG Xiaohong TIAN Baoli LI Yuncai HUANG Yabin DU Zuliang | 2006 | Science China Chemistry2006，49，2： | 2 |
| 18 | Luminescent and photovoltaic properties of poly(9,9-dioctylfluorene-co-bithiophene) in organic electronic devices显示文摘We studied the luminescent and photovoltaic properties of poly(9,9-dioctylfluorene-co-bithiophene)(F8T2) based on ITO/PEDOT:PSS/F8T2/Bphen/LiF(0 or 1 nm)/Al and ITO/PEDOT:PSS/F8T2:PCBM/Bphen/Al.A stable and bright yellow emission was obtained from polymer F8T2,and the electroluminescence power reached 45 ?W at a 15 V driving voltage.Polymer F8T2 shows a broad absorption band from 400 to 500 nm,and has a shorter absorption edge at about 560 nm compared to that of the typical electron donor P3HT(650 nm).The photoluminescence quenching of F8T2 occurs with only a small fraction of blended PCBM due to the effective exciton dissociation at the interface between F8T2 and PCBM.Polymer solar cells(PSCs) using F8T2:PCBM as the active layer show a low power conversion efficiency(PCE) of 0.10% with an open circuit voltage(Voc) of 0.91 V and short circuit current density(Jsc) of 0.23 mA/cm2.The PSCs using F8T2:P3HT:PCBM as the active layer have a Voc of 0.85 V and Jsc of 3.02 mA/cm2,improving the PCE by about 0.90%.We attribute the improved cell performance to the higher number of photons harvested by P3HT molecules. | XU XiaoWei ZHU EnWei BIAN LinYi WANG ZiXuan WANG Jin ZHUO ZuLiang WANG Jian ZHANG FuJun TANG WeiHua | 2012 | Chinese Science Bulletin2012，57，9： | 2 |
| 19 | Raman scattering and photoluminescence of Fe-doped ZnO nanocantilever arrays显示文摘Single crystalline Fe-doped ZnO nanocantilever arrays have been synthesized by thermal evaporating amorphous Zn-Fe-C-O composite powder. The characterizations of composition, structure and phonon spectrum properties of the nanocantilevers have been performed. Arrays of uniform, perfectly aligned and single-crystal nanowires have been observed by electron microscopy. The results of the X-ray photo-electric spectra and the Raman spectrum provide the evidence that Fe is incorporated into the ZnO lattice at Zn site. Abnormally, the room temperature UV emission band of Fe-doped ZnO nanocan-tilevers disappears and the green one has a large red-shift, and the intensity of the green emission is strongly quenched because the Fe3+ enters the ZnO crystal lattice. | ZHANG Bin ZHOU ShaoMin WANG HaiWei DU ZuLiang | 2008 | Chinese Science Bulletin2008，53，11： | 2 |
| 20 | Solvothermal synthesis of CdS nanorods and photovoltaic characteristics of CdS/PVK composite system显示文摘Large quantities of CdS nanorods are successfully synthesized through Cd(CH3COO)2·2H2O reacting with Na2S·9H2O and EDA in aqueous solution. XRD result shows that the sample is of hexagonal structure. And TEM result shows that the morphologies of the resulting CdS are mainly in three-armed rod-like structure with a diameter of 10―15 nm and a length of 100 nm. The nanocomposites of CdS/PVK with different molar ratios are prepared by spin coating method on tin-doped indium oxide (ITO) substrate. A notable decrease of photoluminescence (PL) efficiency and a significant enhance-ment of surface photovoltage signal have been observed in CdS/PVK composites when the molar frac-tion of CdS increases. We interpret these results as the energy level matching between CdS and PVK in nanocomposites. This energy level matching facilitates fast interfacial charge transfer then increases the separation efficiency of electron-hole pairs and the carrier generation efficiency. The detailed charge transfer process has also been demonstrated. | JI YanLing CHENG Ke ZHANG HongMei ZHANG XingTang LI YunCai DU ZuLiang | 2008 | Chinese Science Bulletin2008，53，1： | 2 |
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