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| 1 | One-step strategy to graphene/Ni(OH)2 composite hy- drogels as advanced three-dimensional supercapacitor electrode materials显示文摘基于 Graphene 三维(3D ) 宏观的材料最近在电气化学的精力变换和存储由他们的令人激动的潜力的优点吸引了增加的兴趣。这里,我们报导灵巧的一步舞策略准备机械地强壮、电子上传导性的 graphene/Ni (哦) 有一个互连的多孔的网络的 2 合成 hydrogels。没有增加任何另外的文件夹或传导性的添加剂,合成 hydrogels 直接被用作 3D supercapacitor 电极材料。包含 82 wt.% Ni 的优化合成 hydrogel (哦) 2 与优秀骑车在 40 mV/s (63% 电容保留) 以 5 mV/s 和 785 F/g 的扫描率展出了 1,247 F/g 的一个特定的电容稳定性。3D hydrogels 的能力极大地超过 graphene 表和 Ni 的物理混合物的(哦) 2 nanoplates (在 40 mV/s 的 309 F/g ) 。一样的策略也被使用制作 graphene 碳 nanotube/Ni (哦) 有进一步改进的特定的电容(在 5 mV/s 的 1,352 F/g ) 和率能力(在 40 mV/s 的 66% 电容保留) 的 2 第三的合成 hydrogels。这里获得的两合成 hydrogels 能交付高精力密度(43 和 47 Wh/kg,分别地) 并且力量密度(8 和 9 kW/kg,分别地) ,为 supercapacitor 应用使他们成为吸引人的电极材料。这研究打开一条新小径到功能的 3D graphene 的设计和制造合成材料,和罐头显著地包括精力存储并且在以外影响宽广区域。 | Yuxi Xu Xiaoqing Huang Zhaoyang Lin Xing Zhong Yu Huang Xiangfeng Duan | 2013 | Nano Research2013，6，1： | 28 |
| 2 | Chemical vapor deposition growth of monolayer MoSe2 nanosheets显示文摘 | Jonathan C. Shaw Hailong Zhou Yu Chen Nathan O. Weiss Yuan Liu Yu Huang Xiangfeng Duan | 2014 | Nano Research2014，7，4： | 26 |
| 3 | Progress of the key materials for organic solar cells显示文摘Organic solar cells have attracted academic and industrial interests due to the advantages like lightweight,flexibility and roll-to-roll fabrication.Nowadays,18%power conversion efficiency has been achieved in the state-of-the-art organic solar cells.The recent rapid progress in organic solar cells relies on the continuously emerging new materials and device fabrication technologies,and the deep understanding on film morphology,molecular packing and device physics.Donor and acceptor materials are the key materials for organic solar cells since they determine the device performance.The past 25 years have witnessed an odyssey in developing high-performance donors and acceptors.In this review,we focus on those star materials and milestone work,and introduce the molecular structure evolution of key materials.These key materials include homopolymer donors,D-A copolymer donors,A-D-A small molecular donors,fullerene acceptors and nonfullerene acceptors.At last,we outlook the challenges and very important directions in key materials development. | Yang Tong Zuo Xiao Xiaoyan Du Chuantian Zuo Yuelong Li Menglan Lv Yongbo Yuan Chenyi Yi Feng Hao Yong Hua Ting Lei Qianqian Lin Kuan Sun Dewei Zhao Chunhui Duan Xiangfeng Shao Wei Li Hin-Lap Yip Zhengguo Xiaol Bin Zhang Qingzhen Bian Yuanhang Cheng Shengjian Liu Ming Cheng Zhiwen Jin Shangfeng Yang Liming Ding | 2020 | Science China Chemistry2020，63，6： | 15 |
| 4 | Effects of dietary protein restriction on muscle fiber characteristics and m TORC1 pathway in the skeletal muscle of growing-finishing pigs显示文摘Background: To investigate the effects of dietary crude protein(CP) restriction on muscle fiber characteristics and key regulators related to protein deposition in skeletal muscle, a total of 18 growing-finishing pigs(62.30 ± 0.88 kg)were allotted to 3 groups and fed with the recommended adequate protein(AP, 16 % CP) diet, moderately restricted protein(MP, 13 % CP) diet and low protein(LP, 10 % CP) diet, respectively. The skeletal muscle of different locations in pigs, including longissimus dorsi muscle(LDM), psoas major muscle(PMM) and biceps femoris muscle(BFM) were collected and analyzed.Results: Results showed that growing-finishing pigs fed the MP or AP diet improved(P < 0.01) the average daily gain and feed: gain ratio compared with those fed the LP diet, and the MP diet tended to increase(P = 0.09) the weight of LDM. Moreover, the ATP content and energy charge value were varied among muscle samples from different locations of pigs fed the reduced protein diets. We also observed that pigs fed the MP diet up-regulated(P < 0.05) muscular m RNA expression of all the selected key genes, except that myosin heavy chain(My HC) IIb,My HC IIx, while m RNA expression of ubiquitin ligases genes was not affected by dietary CP level. Additionally, the activation of mammalian target of rapamycin complex 1(m TORC1) pathway was stimulated(P < 0.05) in skeletal muscle of the pigs fed the MP or AP diet compared with those fed the LP diet.Conclusion: The results suggest that the pigs fed the MP diet could catch up to the growth performance and the LDM weight of the pigs fed the AP diet, and the underlying mechanism may be partly due to the alteration in energy status, modulation of muscle fiber characteristics and m TORC1 activation as well as its downstream effectors in skeletal muscle of different locations in growing-finishing pigs. | Yinghui Li Fengna Li Li Wu Hongkui Wei Yingying Liu Tiejun Li Bie Tan Xiangfeng Kong Kang Yao Shuai Chen Fei Wu Yehui Duan Yulong Yin | 2017 | Journal of Animal Science and Biotechnology2017，8，1： | 13 |
| 5 | Three-dimensional graphene framework with ultra-high sulfur content for a robust lithium-sulfur battery显示文摘 | Benjamin Papandrea Xu Xu Yuxi Xu Chih-Yen Chen Zhaoyang Lin Gongming Wang Yanzhu Luo Matthew Liu yu Huang Liqiang Mai Xiangfeng Duan | 2016 | Nano Research2016，9，1： | 13 |
| 6 | Chemical vapor deposition growth of single-crystalline cesium lead halide microplatelets and heterostructures for optoelectronic applications显示文摘Organic-inorganic hybrid halide perovskites, such as CH3NH3PbI3, have emerged as an exciting class of materials for solar photovoltaic applications; however, they are currently plagued by insufficient environmental stability. To solve this issue, all-inorganic halide perovskites have been developed and shown to exhibit significantly improved stability. Here, we report a single-step chemical vapor deposition growth of cesium lead halide (CsPbX3) microcrystals. Optical microscopy studies show that the resulting perovskite crystals predominantly adopt a square-platelet morphology. Powder X-ray diffraction (PXRD) studies of the resulting crystals demonstrate a highly crystalline nature, with CsPbCl3, CsPbBr3, and CsPbI3 showing tetragonal, monoclinic, and orthorhombic phases, respectively. Scanning electron microscopy (SEM) and atomic force microscopy (AFM) studies show that the resulting platelets exhibit well-faceted structures with lateral dimensions of the order of 10-50 μm, thickness around 1 μm, and ultra-smooth surface, suggesting the absence of obvious grain boundaries and the single-crystalline nature of the individual microplatelets. Photoluminescence (PL) images and spectroscopic studies show a uniform and intense emission consistent with the expected band edge transition. Additionally, PL images show brighter emission around the edge of the platelets, demonstrating a wave-guiding effect in high-quality crystals. With a well-defined geometry and ultra-smooth surface, the square platelet structure can function as a whispering gallery mode cavity with a quality factor up to 2,863 to support laser emission at room temperature. Finally, we demonstrate that such microplatelets can be readily grown on a variety of substrates, including silicon, graphene, and other two-dimensional materials such as molybdenum disulfide, which can readily allow the construction of heterostructure optoelectronic devices, including a graphene/perovskite/graphene vertically-stacked photodetector with photoresponsivity > 105 A/W. The extraordinary optical properties of CsPbX3 platelets, combined with their ability to be grown on diverse materials to form functional heterostructures, can lead to exciting opportunities for broad optoelectronic applications. | Yiliu Wang Xun Guan Dehui Li Hung-Chieh Cheng Xidong Duan Zhaoyang Lin Xiangfeng Duan | 2017 | Nano Research2017，10，4： | 8 |
| 7 | Pt3Ag alloy wavy nanowires as highly effective electrocatalysts for ethanol oxidation reaction显示文摘Direct ethanol fuel cell(DEFC)has received tremendous research interests because of the more convenient storage and transportation of ethanol vs.compressed hydrogen.However,the electrocatalytic ethanol oxidation reaction typically requires precious metal catalysts and is plagued with relatively high over potential and low mass activity.Here we report the synthesis of Pt3Ag alloy wavy nanowires via a particle attachment mechanism in a facile solvothermal process.Transmission microscopy studies and elemental analyses show highly wavy nanowire structures with an average diameter of 4.6±1.0 nm and uniform Pt3Ag alloy formation.Electrocatalytic studies demonstrate that the resulting alloy nanowires can function as highly effective electrocatalysts for ethanol oxidation reactions(EOR)with ultrahigh specific activity of 28.0 mA/cm^2 and mass activity of 6.1 A/mg,far exceeding that of the commercial Pt/carbon samples(1.10 A/mg).The improved electrocatalytic activity may be partly attributed to partial electron transfer from Ag to Pt in the Pt3Ag alloy,which weakens CO binding and the CO poisoning effect.The one-dimensional nanowire morphology also contributes to favorable charge transport properties that are critical for extracting charge from catalytic active sites to external circuits.The chronoamperometry studies demonstrate considerably improved stability for long term operation compared with the commercial Pt/C samples,making the Pt3Ag wavy nanowires an attractive electrocatalyst for EOR. | Xiaoyang Fu Chengzhang Wan Aixin Zhang Zipeng Zhao Huaixun Huyan Xiaoqing Pan Shuaijing Du Xiangfeng Duan Yu Huang | 2020 | Nano Research2020，13，5： | 5 |
| 8 | In situ development of highly concave and compositionconfined PtNi octahedra with high oxygen reduction reaction activity and durability显示文摘有为催化氧减小反应(ORR ) 的唯一的结构的 PtNi 金属 nanocrystals 的控制综合体吸引了大兴趣。这里,我们报导单个水晶的 PtNi octahedra 的一步舞合成与在里面开发 situ 高度为 ORR 是最佳的凹面特征和自我限制的作文。揭示的详细研究充满磅的播种、随后的 Pt/Ni 合作减小,和 PtNi 融合导致了一致单个水晶的 PtNi octahedra,并且 Ni 富有的表面蚀刻的 Ni 方面分离和氧的联合导致了凹度并且限制了 Ni 内容。凹面 PtNi nanocrystals 以两个比商业地可得到的 Pt/C 催化剂展出了高得多的 ORR 性能特定的活动(高 29.1 倍) 并且集体活动(高 12.9 倍) 在 0.9 V (对可逆的氢电极(RHE )) 。没有凹度,表演也比 PtNi octahedra 的高,证实更高的活动是仔细与它的形态学有关。而且,凹面 octahedra 也由于不稳定的地点的钝化在 ORR (在在 0.6 和 1.1 V 对 RHE 之间的 10,000 个周期以后仍然是的 93% 集体活动) 展出了显著稳定性。 | Enbo Zhu Yongjia Li Chin-Yi Chiu Xiaoqing Huang Mufan Li Zipeng Zhao Yuan Liu Xiangfeng Duan Yu Huang | 2016 | Nano Research2016，9，1： | 4 |
| 9 | Ultrafast growth of large single crystals of monolayer WS2 and WSe2显示文摘Monolayer transition metal dichalcogenides(TMDs)have attracted considerable attention as atomically thin semiconductors for the ultimate transistor scaling.For practical applications in integrated electronics,large monolayer single crystals are essential for ensuring consistent electronic properties and high device yield.The TMDs available today are generally obtained by mechanical exfoliation or chemical vapor deposition(CVD)growth,but are often of mixed layer thickness,limited single crystal domain size or have very slow growth rate.Scalable and rapid growth of large single crystals of monolayer TMDs requires maximization of lateral growth rate while completely suppressing the vertical growth,which represents a fundamental synthetic challenge and has motivated considerable efforts.Herein we report a modified CVD approach with controllable reverse flow for rapid growth of large domain single crystals of monolayer TMDs.With the use of reverse flow to precisely control the chemical vapor supply in the thermal CVD process,we can effectively prevent undesired nucleation before reaching optimum growth temperature and enable rapid nucleation and growth of monolayer TMD single crystals at a high temperature that is difficult to attain with use of a typical thermal CVD process.We show that monolayer single crystals of 450μm lateral size can be prepared in 10 s,with the highest lateral growth rate up to 45μm/s.Electronic characterization shows that the resulting monolayer WSe2 material exhibits excellent electronic properties with carrier mobility up to 90 cm^2 V^-1 s^-1,comparable to that of the best exfoliated monolayers.Our study provides a robust pathway for rapid growth of high-quality TMD single crystals. | Zhengwei Zhang Peng Chen Xiangdong Yang Yuan Liu Huifang Ma Jia Li Bei Zhao Jun Luo Xidong Duan Xiangfeng Duan | 2020 | National Science Review2020，7，4： | 4 |
| 10 | Three-dimensional graphene membrane cathode for high energy density rechargeable lithium-air batteries in ambient conditions显示文摘锂空气电池在活动电源供应的高精力密度为应用吸引了重要兴趣,还对有在周围的条件下面的稳定的骑车性能的可充电的 Li 空气电池的发展有可观的挑战。这里,我们报导一三维(3D ) 恐水病的 graphene 膜作为为高效 Li 空气电池的潮湿抵抗的阴极。 3D graphene 膜为有效电荷运输展示一个高度互连的 graphene 网络,为氧和电解质离子的有效散开的高度多孔的结构,为绝缘的分泌物产品的高能力存储的一个大特定的表面区域,并且为 O 2/H2 O 选择。当延迟时,这些隧道便于 O 2 ingression 潮湿散开并且保证优秀控告 / 解除骑车在周围的条件下面的稳定性。膜能因此与非凡的性能启用柔韧的 Li 空气电池,包括超过 5,700 mAh/g 的一个最大的阴极能力并且优秀再装骑车行为(> 在 140 mAh/g 的 2,000 个周期,并且 > 在 1,400 mAh/g 的 100 个周期) 。graphene 膜空气阴极能交付 100,000-300,000 mAh/g 的一个一生能力,比得上典型的锂离子电池阴极的。有显著地改进的单个费用能力和 Li 离子电池的比得上那些的一生能力的 Li 空气电池的稳定的操作可以为为未来其他的吸引人的高精力密度存储提供活动电源供应。这些电池可以提供长得多的电池生活并且极大地减少再装频率。 | Xing Zhong Benjamin Papandrea Yuxi Xu Zhaoyang Lin Hua Zhang Yuan Liu Yu Huang Xiangfeng Duan | 2017 | Nano Research2017，10，2： | 4 |
| 11 | Reduced graphene oxide/silicon nanowire hetero- structures with enhanced photoactivity and superior photoelectrochemical stability显示文摘Silicon nanowires (SiNWs) have been widely studied as light harvesting antennas in photocatalysts due to their ability to absorb broad-spectrum solar radiation, but they are typically limited by poor photoelectrochemical stability. Here, we report the synthesis of reduced graphene oxide-SiNW (rGO-SiNW) heterostructures to achieve greatly improved photocatalytic activity and stability. The SiNWs were synthesized through a metal-assisted electroless etching process and functionalized with reduced graphene oxide (rGO) flakes through a chemical absorption process. Here, the rGO not only functions as a physical protection layer to isolate the SiNWs from the harsh electrochemical environment but also serves as a charge mediator to facilitate the charge separation and transport processes. Furthermore, the rGO may also function as a redox catalyst to ensure efficient utilization of photo-carriers for the desired chemical reactions. Photocatalytic dye degradation studies show that the photoactivity of the heterostructures can be significantly enhanced with an initial activation process and maintained without apparent decay over repeated reaction cycles. Electrochemical and photo- electrochemical studies indicate that the enhanced photoactivity and photostability can be attributed to the more efficient separation of photoexcited charge carriers in SiNWs and the reduced self-oxidation of the surface of the SiNWs during the photocatalytic dye degradation process. The ability to significantly improve the photocatalytic activity and stability in rGO-SiNW heterostructures can not only lead to more opportunities for the application of silicon-based photocatalysts/ photoelectrodes for solar energy harvesting but also provide new insights into the stabilization of other unstable photocatalytic | Xing Zhong Gongming wang Benjamin Papandrea Mufan Li Yuxi Xu Yu Chen Chih-Yen Chen Hailong Zhou Teng Xue Yongjia Li Dehui Li Yu Huang Xiangfeng Duan | 2015 | Nano Research2015，8，9： | 4 |
| 12 | Highly-anisotropic optical and electrical properties in layered SnSe显示文摘因为他们极化依赖者或方向依赖者的唯一的联合,各向异性的材料具有可观的兴趣电、光、热电的性质。低对称二维(2D ) covalently 结合的原子层叠的货车 der Waals 形成的材料内在地是各向异性的。分层的 SnSe 展出格子对称的低度,与弄歪的 NaCl 结构和在里面飞机 anisotropy。这里,我们报导在里面飞机的系统的研究在分层的 SnSe 的各向异性的性质用散布的解决角度的拉曼,光吸收,和电的运输学习。光、电的描述是方向依赖者,并且成功地在分层的 SnSe 识别了水晶的取向。而且, SnSe 薄片厚度和刺激波长上的 Raman 紧张 anisotropy 的依赖被实验和理论计算调查。最后,电的运输研究证明很少层 SnSe 地效果晶体管(联邦货物税) 有在扶手椅和之字形方向之间的搬运人活动性(5.8 ) 的大各向异性的比率,它是高价值为 2D 报导了的一个记录各向异性的材料。分层的 SnSe 的高度各向异性的性质在新窗户中为各向异性的光学,电子学,和 optoelectronics.Open | Shengxue Yang Yuan Liu Minghui Wu Li-Dong Zhao Zhaoyang Lin Hung-chieh Cheng Yiliu Wang Chengbao Jiang Su-Huai Wei Li Huang Yu Huang Xiangfeng Duan | 2018 | Nano Research2018，11，1： | 4 |
| 13 | A Silicon Monoxide Lithium-Ion Battery Anode with Ultrahigh Areal Capacity显示文摘Silicon monoxide(SiO)is an attractive anode material for next-generation lithium-ion batteries for its ultra-high theoretical capacity of 2680 mAh g−1.The studies to date have been limited to electrodes with a rela-tively low mass loading(<3.5 mg cm^(−2)),which has seriously restricted the areal capacity and its potential in practical devices.Maximizing areal capacity with such high-capacity materials is critical for capitalizing their potential in practi-cal technologies.Herein,we report a monolithic three-dimensional(3D)large-sheet holey gra-phene framework/SiO(LHGF/SiO)composite for high-mass-loading electrode.By specifically using large-sheet holey graphene building blocks,we construct LHGF with super-elasticity and exceptional mechanical robustness,which is essential for accommodating the large volume change of SiO and ensuring the structure integrity even at ultrahigh mass loading.Additionally,the 3D porous graphene network structure in LHGF ensures excellent electron and ion transport.By systematically tailoring microstructure design,we show the LHGF/SiO anode with a mass loading of 44 mg cm^(−2)delivers a high areal capacity of 35.4 mAh cm^(−2)at a current of 8.8 mA cm^(−2)and retains a capacity of 10.6 mAh cm^(−2)at 17.6 mA cm^(−2),greatly exceeding those of the state-of-the-art commercial or research devices.Furthermore,we show an LHGF/SiO anode with an ultra-high mass loading of 94 mg cm^(−2)delivers an unprecedented areal capacity up to 140.8 mAh cm^(−2).The achievement of such high areal capacities marks a critical step toward realizing the full potential of high-capacity alloy-type electrode materials in practical lithium-ion batteries. | Jiang Zhong Tao Wang Lei Wang Lele Peng Shubin Fu Meng Zhang Jinhui Cao Xiang Xu Junfei Liang Huilong Fei Xidong Duan Bingan Lu Yiliu Wang Jian Zhu Xiangfeng Duan | 2022 | Nano-Micro Letters2022，14，3： | 4 |
| 14 | Holey graphene hydrogel with in-plane pores for high- performance capacitive desalination显示文摘电容的 deionization 是一条吸引人的途径浇脱盐和治疗。完成有效 capacitative 脱盐,有高特定的电容的讲道理地设计的电极,传导性,和稳定性是必要的。这里,我们报导构造一三维(3D ) 有穴的 graphene hydrogel (HGH ) 。这材料包含丰富的在里面飞机毛孔,提供有效离子运输小径。而且,它形成 graphene 表的一个高度互连的网络,提供层次多孔的结构能提供的有效电子运输小径,和它的 3D 为离子的吸附和存储的一个大特定的表面区域。因而, HGH 与优秀电的电导率用作没有文件夹的电极材料。周期的 voltammetry (CV ) 大小显示优化 HGH 能由于他们的分解完成 358.4 Femovable | Weiqing Kong Xidong Duan Yongjie Ge Hongtao Liu Jiawen Hu Xiangfeng Duan | 2016 | Nano Research2016，9，8： | 3 |
| 15 | Ultrathin wavy Rh nanowires as highly effective electrocatalysts for methanol oxidation reaction with ultrahigh ECSA显示文摘Direct methanol fuel cells (DMFCs) have received tremendous research interests because of the facile storage of liquid methanol vs.hydrogen.However,the DMFC today is severely plagued by the poor kinetics and rather high overpotential in methanol oxidation reaction (MOR).Here we report the investigation of the ultrathin Rh wavy nanowires as a highly effective MOR electrocatalyst.We show that ultrathin wavy Rh nanowires can be robustly synthesized with 2-3 nm diameters.Electrochemical studies show a current peak at the potential of 0.61 V vs.reversible hydrogen electrode (RHE),considerably lower than that of Pt based catalysts (~ 0.8-0.9 V vs.RHE).Importantly,with ultrathin diameters and favorable charge transport,the Rh nanowires catalysts exhibit an ultrahigh electrochemically active surface area determined from CO-stripping (ECSAco) of 144.2 m2/g,far exceeding that of the commercial Rh black samples (20 m2/g).Together,the Rh nanowire catalysts deliver a mass activity of 722 mA/mg at 0.61 V,considerably higher than many previously reported electrocatalysts at the same potential.The chronoamperometry studies also demonstrate good stability and CO-tolerance compared with the Rh black control sample,making ultrathin Rh wavy nanowires an attractive electrocatalyst for MOR. | Xiaoyang Fu Zipeng Zhao Chengzhang Wan Yiliu Wang Zheng Fan Frank Song Bocheng Cao Mufan Li Wang Xue Yu Huang Xiangfeng Duan | 2019 | Nano Research2019，12，1： | 3 |
| 16 | Enhancement of oxygen reduction reaction activity by grain boundaries in platinum nanostructures显示文摘Systematic control of grain boundary densities in various platinum(Pt)nanostructures was achieved by specific peptide-assisted assembly and coagulation of nanocrystals.A positive quadratic correlation was observed between the oxygen reduction reaction(ORR)specific activities of the Pt nanostructures and the grain boundary densities on their surfaces.Compared to commercial Pt/C,the grain-boundary-rich strain-free Pt ultrathin nanoplates demonstrated a 15.5 times higher specific activity and a 13.7 times higher mass activity.Simulation studies suggested that the specific activity of ORR was proportional to the resident number and the resident time of oxygen on the catalyst surface,both of which correlate positively with grain boundary density,leading to improved ORR activities. | Enbo Zhu Wang Xue Shiyi Wang Xucheng Yan Jingxuan Zhou Yang Liu Jin Cai Ershuai Liu Qingying Jia Xiangfeng Duan Yujing Li Hendrik Heinz Yu Huang | 2020 | Nano Research2020，13，12： | 3 |
| 17 | A field-effect approach to directly profiling the localized states in monolayer MoS2显示文摘A fundamental understanding of the charge transport mechanism in two-dimensional semiconductors(e.g., MoS2) is crucial for fully exploring their potential in electronic and optoelectronic devices. By using monolayer graphene as the barrier-free contact to MoS2, we show that the field-modulated conductivity can be used to probe the electronic structure of the localized states. A series of regularly distributed plateaus were observed in the gate-dependent transfer curves. Calculations based on the variable-range hopping theory indicate that such plateaus can be attributed to the discrete localized states near mobility edge. This method provides an effective approach to directly profiling the localized states in conduction channel with an ultrahigh resolution up to 1 meV. | Hao Wu Yuan Liu Zeyu Deng Hung-Chieh Cheng Dehui Li Jian Guo Qiyuan He Sen Yang Mengning Ding Yun-Chiao Huang Chen Wang Yu Huang Xiangfeng Duan | 2019 | Science Bulletin2019，64，15： | 2 |
| 18 | Hot graphene sponge cleans viscous crude-oil spill显示文摘Ocean crude oil spill can cause instant and lasting damage to marine ecosystem,leading to disastrous environmental,economical and social consequences[1,2].The 2010 Gulf oil spill has cost British Petroleum over $60 billion,and will impact the local fishing and tourism industry | Xiangfeng Duan | 2017 | Science China Materials2017，60，7： | 2 |
| 19 | Direct van der Waals epitaxial growth of 1D/2D Sb2Se3/WS2 mixed-dimensional p-n heterojunctions显示文摘The mixed-dimensional integration of two-dimensional (2D) materials with non-2D materials can give rise to prominent advances in performance or function.To date,the mixed-dimensional one-dimensional (1D)/2D heterostructures have been fabricated using various physical assembly approaches.However,direct epitaxial growth method which has notable advantages in preparing large-scale products and obtaining perfect interfaces is rarely investigated.Herein,we demonstrate for the first time the direct synthesis of the 1D/2D mixed-dimensional heterostructures by sequential vapor-phase growth of Sb2Se3 nanowires on WS2 monolayers.X-ray diffraction (XRD) pattern and Raman spectrum confirm the composition of the Sb2Se3/NS2 heterostructures.Transmission electron microscope (TEM) measurement demonstrates high quality of the heterostructures.Electrical transport characterization reveals that Sb2Se3 nanowire exhibits p-type characteristic and that WS2 monolayer exhibits n-type behavior,and that the p-n diode from 1D/2D mixed-dimensional Sb2Se3/WS2 heterostructure possesses obvious current rectification behavior.Optoelectronic measurements of the heterostructures show apparent photovoltaic response with an open-circuit voltage of 0.19 V,photoresponsivity of 1.51 A/W (Vds =5 V) and fast response time of less than 8 ms.The van der Waals epitaxial growth mode of Sb2Se3 nanowires on WS2 monolayers is verified by stripping the Sb2Se3 nanowire from the heterostructures using tape.Together,the direct van der Waals epitaxy opens a facile pathway to 1D/2D mixed-dimensional heterostructures for functional electronic and optoelectronic devices. | Guangzhuang Sun Bo Li Jia Li Zhengwei Zhang Huifang Ma Peng Chen Bei Zhao Ruixia Wu Weiqi Dang Xiangdong Yang Xuwan Tang Chen Dai Ziwei Huang Yuan Liu Xidong Duan Xiangfeng Duan | 2019 | Nano Research2019，12，5： | 2 |
| 20 | Selective growth of wide band gap atomically thin Sb2O3 inorganic molecular crystal on WS2显示文摘Heterostructures combined by different individual two-dimensional(2D)materials are essential building blocks to realize unique electronic,optoelectronic properties and multifunctional applications.To date,the direct growth of 2D/2D atomic van der Waals heterostructures(vdWHs)have been extensively investigated.However,the heterostructures from 2D inorganic molecular crystals and atomic crystals have been rarely reported.Here we report two-step direct epitaxial growth of the inorganic molecular-atomic Sb2O3/WS2 vdWHs.The thickness of Sb2O3 nanosheets on WS2 nanosheets can be tuned by variable growth temperatures.Oriented growth behavior of Sb2O3 on WS2 was determined through statistics.Optical images,Raman spectra,Raman mappings and selected-area electron diffraction(SAED),etc.,reveal that Sb2O3/WS2 heterostructures are vertically stacked with high crystal quality.Electrical transport measurements demonstrate that the heterotransistors based on the heterostructures possess high current on/off ratio of 5 × 10^5,obvious gate-tunable and current rectification output characteristics.Optoelectronic characterizations show that the heterostructures have a clear photoresponse with high responsivity of 16.4 AW.The growth of vdWHs from 2D inorganic molecular-atomic crystals may open up new opportunities in 2D functional electronics and optoelectronics. | Guangzhuang Sun Bo Li Shifa Wang Zhengwei Zhang Jia Li Xidong Duan Xiangfeng Duan | 2019 | Nano Research2019，12，11： | 2 |
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