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| 1 | A synchronous nucleation and passivation strategy for controllable synthesis of Au36(PA)24: unveiling the formation process and the role of Au22(PA)18 intermediate显示文摘Despite the recent progress on controllable synthesis of alkynyl-protected Au nanoclusters,the effective synthetic means are very limited and the cluster formation process still remains puzzling.Here,we develop a novel synchronous nucleation and passivation strategy to fabricate Au36(PA)24(PA=phenylacetylenyl) nanoclusters with high yield.In Au36(PA)24formation process,Au22(PA)18as key intermediate was identified.Meanwhile,Au22(PA)18can be synthesized under a low amount of reductant,and by employing more reductants,Au22(PA)18can turn into Au36(PA)24eventually.Moreover,the structure evolution from Au22(PA)18to Au36(PA)24is proposed,where four Au13cuboctahedra can yield one Au28kernel.Finally,the ratiocination is verified by the good accordance between the predicted intermediate/product ratio and the experimental value.This study not only offers a novel synthetic strategy,but also sheds light on understanding the structural evolution process of alkynyl-protected Au nanoclusters at atomic level. | Xiaoshuang Ma Guanyu Ma Lubing Qin Guangxu Chen Shaowei Chen Zhenghua Tang | 2020 | Science China Chemistry2020，63，12： | 4 |
| 2 | Corrigendum to“Fenton cleaning strategy for ceramic membrane fouling in wastewater treatment”[J Environ Sci 85(2019)189-199]显示文摘The authors regret that one author should be also on the author list given his contribution.The changed author list is shown below.The authors would like to apologise for any inconvenience caused. | Tang Shengyin Zhang Lixun Peng Yi Liu Jing Zhang Xihui Zhang Zhenghua | 2019 | Journal of Environmental Sciences2019，31，12： | 3 |
| 3 | Recent diagnostic developments at the 100 kJ-level laser facility in China显示文摘A 100 kJ-level laser facility has been designed to study inertial confinement fusion physics in China.This facility incorporates various diagnostic techniques,including optical,x-ray imaging,x-ray spectrum,and fusion product diagnostics,as well as general diagnostics assistance systems and central control and data acquisition systems.This paper describes recent developments in diagnostics at the facility. | Feng Wang Shaoen Jiang Yongkun Ding Shenye Liu Jiamin Yang Sanwei Li Tianxuan Huang Zhurong Cao Zhenghua Yang Xin Hu Wenyong Miao Jiyan Zhang Zhebin Wang Guohong Yang Rongqing Yi Qi Tang Longyu Kuang Zhichao Li Dong Yang Yulong Li Xiaoshi Peng Kuan Ren Baohan Zhang | 2020 | Matter and Radiation at Extremes2020，5，3： | 2 |
| 4 | Carrier recombination suppression and transport enhancement enable high-performance self-powered broadband Sb_(2)Se_(3) photodetectors显示文摘Antimony selenide(Sb_(2)Se_(3))is a promising candidate for photodetector applications boasting unique material benefits and remarkable optoelectronic properties.Achieving high-performance self-powered Sb_(2)Se_(3)photodetector through a synergistic regulation of absorber layer and heterojunction interface demonstrates great potential and needs essential investigation.In this study,an effective two-step thermodynamic/kinetic deposition technique containing sputtered and selenized Sb precursor is implemented to induce self-assembled growth of Sb_(2)Se_(3)light absorbing thin film with large crystal grains and desirable[hk1]orientation,presenting considerable thin-film photodetector performance.Furthermore,aluminum(Al^(3+))cation dopant is introduced to modify the optoelectronic properties of CdS buffer layer,and further optimize the Sb_(2)Se_(3)/CdS(Al)heterojunction interface quality.Thanks to the suppressed carrier recombination and enhanced carrier transport kinetics,the champion Mo/Sb_(2)Se_(3)/CdS(Al)/ITO/Ag photodetector exhibits self-powered and broadband characteristics,accompanied by simultaneously high responsivity of 0.9 A W^(-1)(at 11 nW cm^(-2)),linear dynamic range of 120 dB,impressive ON/OFF switching ratio over 10^(6)and signal-to-noise ratio of 10^(9),record total noise determined realistic detectivity of 4.78×10^(12)Jones,and ultra-fast response speed with rise/decay time of 24/75 ns,representing the top level for Sb_(2)Se_(3)-based photodetectors.This intriguing work opens up an avenue for its selfpowered broadband photodetector applications. | Shuo Chen Yi Fu Muhammad Ishaq Chuanhao Li Donglou Ren Zhenghua Su Xvsheng Qiao Ping Fan Guangxing Liang Jiang Tang | 2023 | InfoMat2023，5，4： | 1 |
| 5 | Bimetallic(Iron or Cobalt) Complexes Bearing 2-methyl-2,4-bis (6- iminopyridin-2-yl)-I H-1, 5-benzodiazepines for Ethylene Reactivity 显示文摘 | ZH ANG Shu VYSTOROP I TANG Zhenghua | 2007 | Organometallics2007，26，： | 1 |
| 6 | The role of molybdenum additions and prior deformation on acicular ferrite formation in microalloyed Nb-Ti low-carbon linepipe steels显示文摘 | Tang Zhenghua and Stumpf Waldo | 2008 | Materials Characterization2008，59，6： | 1 |
| 7 | Fenton cleaning strategy for ceramic membrane fouling in wastewater treatment显示文摘Membrane fouling is an obstacle impeding the wide applications of ceramic membranes and organics are responsible for most of the membrane fouling issues in wastewater treatment.In this study,Fenton cleaning strategy was firstly proposed to clean ceramic membrane fouling in wastewater treatment.Fe2+ efficiently catalyzed fouling cleaning with H2O2 (1.5%) to recover the filterability of ceramic membrane.The maximum ΔTMP recovery (over 99%) was achieved at an optimal Fe2+ dosage of 124 mg/L after 6 hr of immersion cleaning.The total residual membrane fouling resistance decreased gradually from this optimum value as the Fe2+ dosage increased above 124 mg/L.The residual hydraulically reversible fouling resistance accounted for most of the membrane fouling and was basically removed (≤3.0 × 109 m-1) when Fe2+ dosages higher than 124 mg/L were used.The foulants responsible for the formation of a residual hydraulically reversible fouling layer (DOC (dissolved organic carbon),proteins,polysaccharides,EEM (fluorescence excitationemission matrix spectra),SS (suspended solids),and VSS (volatile suspended solids)) were gradually removed as the Fe2+ dosage increased.These residual organic foulants were degraded from biopolymers (10-200 kDa) to low molecular weight substances (0.1-1 kDa),and the particle size of these residual foulants decreased significantly as a result.The strong oxidation power of hydrogen peroxide/hydroxy radicals towards organic foulants was enhanced by Fe2+.Fe2+ played a significant role in the removal of hydraulically reversible fouling and irreversible fouling from the ceramic membrane.However,Fe2+(≥124 mg/L) increased the likelihood of forming secondary iron-organics aggregates. | Shengyin Tang Lixun Zhang Yi Peng Jing Liu Zhenghua Zhang | 2019 | Journal of Environmental Sciences2019，31，11： | 1 |
| 8 | Bimetallic (Fe or Co) complexes bearing 2-methyl-24-bis(6-iminopyridin-2-yl)-1H-15-benzodiazepines for ethylene reactivity显示文摘 | Zhang Shu Vystorop 1 Tang Zhenghua | 2007 | Organometallics2007，26，9： | 1 |
| 9 | t H-NMR study of the hydrolysis of some model pyrimidyl reactive dyes 显示文摘 | Tang Wei Zhu Zhenghua Chen Kongchang | 1989 | Dyes and Pigment1989，11，4： | 1 |
| 10 | Multiplex detection of KRAS and BRAF mutations using cationic conjugated polymers显示文摘The mutation detections of KRAS and BRAF genes are of significant importance to predict the responses to anti-cancer therapy and develop new drugs. In this paper, we developed a multi-step fluorescence resonance energy transfer (FRET) assay for multiplex detection of KRAS and BRAF mutations using cationic conjugated polymers (CCP). The newly established detection system could detect as low as 2% mutant DNAs in DNA admixtures. By triggering the emission intensity change of CCP and the dyes labeled in the DNA, four possible statuses (three mutations and one wildtype) can be differentiated in one extension reaction. The detection efficiency of this new method in clinical molecular diagnosis was validated by determining KRAS and BRAF mutations of 51 formalin-fixed paraffin-embedded (FFPE) ovary tissue samples. Furthermore, the result of the CCP-based multi-step FRET assay can be directly visualized under UV light so that no expensive instruments and technical expertise are needed. Thus, the assay provides a sensitive, reliable, cost-effective and simple method for the detection of disease-related gene mutations. | XING BaoLing SONG JinZhao GE SuMei TANG ZhengHua LIU MengLu YANG Qiong Lü FengTing LIU LiBing WANG Shu | 2013 | Chinese Science Bulletin2013，58，8： | 1 |
| 11 | Carbon Fiber Reinforced Epoxy Resin Matrix Composites显示文摘Carbon fiber reinforced polymer matrix composites have been the focus of research.As the most widely used epoxy resin in all matrix materials,it is also the most studied.In this paper,the modification of TDE-85 epoxy resin,the curing properties of curing agent and the preparation method of prepreg were reviewed.The progress and application of carbon fiber reinforced epoxy resin composites at home and abroad were reviewed,made carbon fiber/epoxy resin composite materials in the automotive fuel cell application prospects. | Zhiyuan Yu Rongchang Li Zhenghua Peng Yonglian Tang | 2017 | Materials Science(Advanced Composite Materials)2017，1，1： | 1 |
| 12 | The effect of microstructure and processing variables on the yield to ultimate tensile strength ratio in a Nb–Ti and a Nb–Ti–Mo line pipe steel显示文摘 | Zhenghua Tang Waldo Stumpf | 2008 | Materials Science & Engineering A2008，，1： | 1 |
| 13 | The role of molybdenum additions and prior deibnnation on acieular ferrite tormalion in mieroalloyed Nb-Ti low-carbon line-pipe steels 显示文摘 | Tang Zhenghua Stumpf W | 2008 | Materials Chm''aeterization2008，59，6： | 1 |
| 14 | The role of molyb denum additions and prior deformation on acicular ferrite forma tion in microalloyed Nb Ti low carbon line pipe steels显示文摘 | TANG ZHENGHUA STUMPF WALDO | 2008 | Mate rials Characterization2008，59，： | 1 |
| 15 | The effect of transportation on the expression of heat shock proteins and meat quality of M. longissimus dorsi in pigs显示文摘 | Jimian Yu Shu Tang Endong Bao Miao Zhang Qingqing Hao Zhenghua Yue | 2009 | Meat Science2009，，3： | 1 |
| 16 | The Role of Molybdenum Additions and Prior Deformation on Acicular Ferrite Formation in Microalloyed Nb-Ti Low-Carbon Line-Pipe Steels显示文摘 | Tang Zhenghua Stumpf W | 2008 | Materials Characterization2008，59，6： | 1 |
| 17 | The role of molybdenum additions and prior deformation on acicular ferrite formation in microalloyed Nb-Ti low carbon pipeline steels显示文摘 | Tang Zhenghua Waldo Stumpy | 2008 | Materials Characterization2008，59，： | 1 |
| 18 | Atomically precise metal nanoclusters for(photo)electroreduction of CO_(2): Recent advances, challenges and opportunities显示文摘To alleviate the global warming by removing excess CO_(2) and converting them into value-added chemicals,(photo)electrochemical reduction has been recognized as a promising strategy.As the CO_(2) reduction reaction(CO_(2) RR) is involved with multiple electrons and multiple products,plus the complexity of the surface chemical environment of the catalyst,it is extremely challenging to establish the structure/function relationship.Atomically precise metal nanoclusters(NCs),with crystallographically resolved structure,molecule-like characters and strong quantum confinement effects,have been emerging as a new type of catalyst for CO_(2) RR,and more importantly,they can provide an ideal platform to unravel the comprehensive mechanistic insights and establish the structure/function relationship eventually.In this review,the recent advances regarding employing molecular metal NCs with well-defined structure including Au NCs,Au-based alloy NCs,Ag NCs,Cu NCs for CO_(2) RR and relevant mechanistic studies are discussed,and the opportunities and challenges are proposed at the end for paving the development of CO_(2) RR by using atomically precise metal NCs. | Lubing Qin Guanyu Ma Likai Wang Zhenghua Tang | 2021 | Journal of Energy Chemistry2021，30，6： | 0 |
| 19 | Result of proton beam energy calibration of GECAM satellite charged particle detector显示文摘Purpose A charged particle detector(CPD)is one of two main detectors on the GECAM satellite.It was designed to detect charged particles.Electrons and protons are space’s mainly charged particles.So,a research on the proton detection ability of a CPD and deriving the energy response to charged particles of the CPD in the two designed operating modes is important.Method The proton calibration tests of the CPD under diferent working modes were carried out at the Heavy Ion Research Facility in Lanzhou.Result and conclusion Through testing and analysis,it was concluded that when CPD works in semi-component mode,it can detect the maximum energy,and when working in full-component mode,it can provide better energy resolution. | Chaoyue Zhang Xiaohua Liang Yanbing Xu Wenxi Peng Jianjian He Dongya Guo Ke Gong Yaqing Liu Zhenghua An Dali Zhang Sheng Yang Xiaojing Liu Xiangyang Wen Rui Qiao Jinzhou Wang Min Gao Shaolin Xiong Fan Zhang Xinqiao Li Xingzhu Cui Chaoyang Li Jilong Tang Xiaohua Wang Dengkui Wang Zhipeng Wei | 2022 | Radiation Detection Technology and Methods2022，6，1： | 0 |
| 20 | Homoleptic alkynyl-protected Ag_(32 )nanocluster with atomic precision: Probing the ligand effect toward CO_(2) electroreduction and 4-nitrophenol reduction显示文摘We report a superatomic homoleptic alkynyl-protected Ag_(32)L_(24)(L=3,5-bis(trifluoromethylbenzene)acetylide,Ag_(32) for short)nanocluster with atomic precision,which possesses eight free electrons.Ag_(32) is formed by an Ag17 core with C3 symmetry and the remaining 15 Ag atoms bond to each other and coordinate with the 24 surface ligands.When applied as electrocatalyst for CO_(2) reduction reaction(CO_(2)RR),Ag_(32) exhibited the highest Faradaic efficiency(FE)of CO up to 96.44%at−0.8 V with hydrogen evolution being significantly suppressed in a wide potential range,meanwhile it has a reaction rate constant of 0.242 min−1 at room temperature and an activation energy of 45.21 kJ·mol−1 in catalyzing the reduction of 4-nitrophenol,both markedly superior than the thiolate and phosphine ligand co-protected Ag_(32) nanocluster.Such strong ligand effect was further understood by density functional theory(DFT)calculations,as it revealed that,one single ligand stripping off from the intact cluster can create the undercoordinated Ag atom as the catalytically active site for both clusters,but alkynyl-protected Ag_(32) nanocluster possesses a smaller energy barrier for forming the key*COOH intermediate in CO_(2)RR,and favors the adsorption of 4-nitrophenol.This study not only discovers a new member of homoleptic alkynyl-protected Ag nanocluster,but also highlights the great potentials of employing alkynyl-protected Ag nanoclusters as bifunctional catalysts toward various reactions. | Leyi Chen Fang Sun Quanli Shen Lubing Qin Yonggang Liu Liang Qiao Qing Tang Likai Wang Zhenghua Tang | 2022 | Nano Research2022，15，10： | 0 |
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