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    题名 作者 年代 出处 被引量
1Preparation and microstructure characterization of a nano-sized Ti^(4+)-doped AgSnO_2 electrical contact material显示文摘A Ti4+-doped nano-structured AgSnO2 material was prepared using sol-gel method and characterized by X-ray diffraction (XRD), transmis-sion electron microscopy (TEM), and scanning electron microscopy (SEM). The results show that Ti4+ cations are successfully doped into the crystal lattice of SnO2, and thus significantly improve the electrical conductivity of the sample. Furthermore, the coating of Ag on Ti4+-doped SnO2 nano-sized particles enhances the surface wettability and enables the resulting AgSnO2 material to have better mechanical properties.ZHENG Ji LI Songlin DOU Fuqi LI Tonghui 2009Rare Metals2009,28,1:24
2First observation of tropospheric nitrogen dioxide from the Environmental Trace Gases Monitoring Instrument onboard the GaoFen-5 satellite显示文摘The Environmental Trace Gases Monitoring Instrument(EMI)is the first Chinese satellite-borne UV–Vis spectrometer aiming to measure the distribution of atmospheric trace gases on a global scale.The EMI instrument onboard the GaoFen-5 satellite was launched on 9 May 2018.In this paper,we present the tropospheric nitrogen dioxide(NO2)vertical column density(VCD)retrieval algorithm dedicated to EMI measurement.We report the first successful retrieval of tropospheric NO_(2) VCD from the EMI instrument.Our retrieval improved the original EMI NO_(2) prototype algorithm by modifying the settings of the spectral fit and air mass factor calculations to account for the on-orbit instrumental performance changes.The retrieved EMI NO_(2) VCDs generally show good spatiotemporal agreement with the satellite-borne Ozone Monitoring Instrument and TROPOspheric Monitoring Instrument(correlation coefficient R of ~0.9,bias<50%).A comparison with ground-based MAX-DOAS(Multi-Axis Differential Optical Absorption Spectroscopy)observations also shows good correlation with an R of 0.82.The results indicate that the EMI NO_(2) retrieval algorithm derives reliable and precise results,and this algorithm can feasibly produce stable operational products that can contribute to global air pollution monitoring.Chengxin Zhang Cheng Liu Ka Lok Chan Qihou Hu Haoran Liu Bo Li Chengzhi Xing Wei Tan Haijin Zhou Fuqi Si Jianguo Liu 2020Light(Science & Applications)2020,9,1:11
3Effect of nitrogen levels on photosynthetic parameters,morphological and chemical characters of saplings and trees in a temperate forest显示文摘Exploring the response differences of leaf physiology parameters to enhanced nitrogen deposition between saplings and trees is vital for predicting the variations of terrestrial ecosystem structure and function under future global climate change. In this study, the ecophysiological parameters of saplings and trees of Fraxinus mandshurica Rupr. were measured at different levels of nitrogen addition in a temperate forest. The results show that ecophysiological parameters maximum net photosynthetic rate(P_(max)), apparent quantum efficiency(a), dark respiration(R_d), light saturation point(L_(sp)), photosynthetic nitrogen use efficiency(PNUE),specific leaf area(SLA)and stomatal conductance under saturated light intensity(G_(smax)) were higher in saplings than in trees. These physiological parameters and not N_(leaf)(leaf nitrogen content)led to relatively lower P_(max) and R_d in trees. For both saplings and trees, low and median nitrogen addition(23 and 46 kg ha^(-1)a^(-1)) resulted in significant increases in Pmax, Rd, Lsp, Chl, PNUE, SLA and Gsmax. These parameters tended to decline under high additions of nitrogen(69 kg ha^(-1)a^(-1)),whereas Nleaf was always enhanced with increasing nitrogen. Variations in Pmax and Rd with increasing nitrogen were attributed to variations in the strongly related parameters of, Lsp, Chl, PNUE, SLA and Gsmax. Overall, the response sensitivity of physiological parameters to enhanced nitrogen levels was lower in trees compared with saplings.Jinwei Sun Fuqi Yao Jiabing Wu Pingcang Zhang Wensheng Xu 2018Journal of Forestry Research2018,29,6:3
4Biogas charging and dissipating process and its accumulation in the Sebei gasfield,Qaidam Basin,China显示文摘The Sebei gasfield is the largest biogas accumulation found in China and many reservoirs and seal rocks superposed on a syndepositional anticline in Quaternary.The biogas charging and dissipating process and its distribution have been a research focus for many years.The authors suggest a diffusing and accumulating model for the biogas,as they find that the shallower the gas producer,the more methane in the biogas,and the lighter stable carbon isotope composition of methane.Based on the diffusing model,diffused biogas is quantitatively estimated for each potential sandy reservoir in the gasfield,and the gas charging quantity for the sandy reservoir is also calculated by the diffused gas quantity plus gas reserve in-place.A ratio of diffusing quantity to charging quantity is postulated to describe biogas accumulating state in a sandy reservoir,if the ratio is less than 0.6,the reservoir forms a good gas-pool and high-production layer in the gasfield,which often occurs in the reservoirs deeper than 900 m;if the ratio is greater than 0.6,a few gas accumulated in the reservoir,which frequently exists in the reservoirs shallower than 900 m.Therefore,a biogas accumulation model is built up as lateral direct charging from gas source for the sands deeper than 900 m and indirect charging from lower gas-bearing sands by diffusion at depth shallower than 900 m.With this charging and diffusion quantitative model,the authors conducted re-evaluation on each wildcat in the central area of the Qaidam Basin,and found many commercial biogas layers.JIN Qiang 1,CHENG FuQi 1,2 ,SU AiGuo 3 ,ZHU GuangYou 3 ,WANG Li 1 &CAO Qian 1 1 China University of Petroleum,Dongying,Shandong 257061,China 2 Geological Institute of Shengli Oilfield,SINOPEC,Dongying,Shandong 257015,China 3 Petroleum Exploration and Development Institute,PetroChina,Beijing 100083,China 2008Science China Earth Sciences2008,51,S1:2
5Nonlinear Optical Properties of Perfectly Polarized KIO_(3) Single Crystal显示文摘The nonlinear optical properties of a perfectly polarized KIO^single crystal were investigated.The principal refractive indices and nonlinear optical coefficients have been measured.The results are as follows:n1=1.6967,n2=1-8329,n3=1.8358 for 0.5893μm;d_(31)=1.2|d_(31)(LiIO_(3))|,d_(32)=1.8|d_(31)(LiIO_(3))|.The in tensity of the frequency-doubled light of the KIO_(3 )single crystal with 2.96 mm thickness is 1.2 times as large as that of the KTP single crystal with the same thickness.YIN Xin LU Mengkai ZHANG Shaojun LI Fuqi 1992Chinese Physics Letters1992,9,2:2
6Non-dispersive infrared in-strument based on gas filter correlation technology for atmosphere monitoring显示文摘Si Fuqi Liu Jianguo Liu Wenqing Chinese Journal Of Quantum Electronics0,21,4:1
7Discriminating hydrocarbon generation potential of coaly source rocks and their contribution:a case study from the Upper Paleozoic of Bohai Bay Basin,China显示文摘Although various coaly source rocks widely developed in the Carboniferous-Permian(C-P)of the Bohai Bay Basin,their geochemical characteristics and hydrocarbon generation potential are poorly understood.This study aims to discriminate the contribution of hydrocarbon generation from different C-P coaly source rocks and clarify the differences within generated oils using organic geochemistry,organic petrology,and thermal simulation experiments.The coaly source rocks containt coal clarain and durain,carbonaceous shale,and shale deposited in deltaic and lagoonal environment.The results indicated that clarain,durain,and carbonaceous shale exhibited higher hydrogen index and liquid-gas hydrocarbon yields than lagoonal and deltaic shales,which was mainly associated with the concentrations of sporinite,cutinite,and hydrogen-rich collodetrinite.Aliphatic hydro-carbons originated firom coal and carbonaceous shale presented lower Ts/(Ts+Tm),Ga/17α(H)21β(H)-C_(30)hopane,18α(H)-oleanane/17α(H)21β(H)-C_(30)hopane ratios,and higher 17β3(H)21α(H)-C_(30)Morane/17α(H)21β(H)-C_(30)hopane than deltaic lagoonal shales.Parameters of aromatic hydrocarbons generated from five lithologies of coaly source rocks trended as clear group distribution,e.g.,clarain and durain showing lower MNR,DBT/Fluorene(F)ratios and higher DBF/F ratio than coaly shales.The distinct descending trend of hydrocarbon potential is obtained from clarain,durain,carbonaceous shale to lagoonal and deltaic shales,implying dominated the petroleum and natural gas supplement from coal and carbonaceous shale.The difference between aliphatic and aromatic hydrocarbons provides a significant contribution to analyze the generic relationship between coaly source rock and lacustrine shale.Our results illustrate the importance of coaly source rocks for the in-depth oil-gas exploration of the Bohai Bay Basin and understanding hydrocarbon generation potential of source rocks in coal bearing strata.Jinjun XU Da LOU Qiang JIN Lixin FU Fuqi CHENG Shuhui ZHOU Xiuhong WANG Chao LIANG Fulai LI 2021Frontiers of Earth Science2021,15,4:1
8PD Pattern Recognition for Stator Bar Models with Six Kinds of Characteristic Vectors using BP Networks显示文摘Kai Gao Kexiong Tan Fuqi Li 2002IEEE Transaction on Dielectrics and Electrical Insulation2002,9,3:1
9PD monitor system for power generators显示文摘Zhenyuan Wang Deheng Zhu Kexiong Tan Fuqi Li 0,,06:1
10Effects of trace element supplementation on the inflammatory response in a rabbit model of major trauma 显示文摘Yuan Wanan Yu Xiaojun Liu Fuqi 2010J Trace Elem Med Biol2010,24,1:1
11On-line partial discharge monitoring and diagnostic system for power transformer显示文摘Du Lin Jiang lei Li Fuqi 2005Journal of Ts- inghua University(Science and Technology)2005,10,5:1
12Estimating Daily Dew Point Temperature Based on Local and Cross-StationMeteorological Data Using CatBoost Algorithm显示文摘Accurate estimation of dew point temperature(Tdew)plays a very important role in the fields of water resource management,agricultural engineering,climatology and energy utilization.However,there are few studies on the applicability of local Tdew algorithms at regional scales.This study evaluated the performance of a new machine learning algorithm,i.e.,gradient boosting on decision trees with categorical features support(Cat Boost)to estimate daily Tdew using limited local and cross-station meteorological data.The random forests(RF)algorithm was also assessed for comparison.Daily meteorological data from 2016 to 2019,including maximum,minimum and average temperature(Tmax,Tmin and Tmean),maximum,minimum and average relative humidity(RHmax,RHmin and RHmean),maximum,minimum and average global solar radiation(Rsmax,Rsmin and Rsmean)from three weather stations in Hunan of China were used to evaluate the CatBoost and RF algorithms.The results showed that both algorithms achieved satisfactory estimation accuracy at the target stations(on average RMSE=1.020℃,R^(2)=0.969,MAE=0.718℃and NRMSE=0.087)in the absence of complete meteorological parameters(with only temperature data as input).The Cat Boost algorithm(on average RMSE=1.900℃and R^(2)=0.835)was better than the RF algorithm(on average RMSE=2.214℃andR^(2)=0.828).The accuracy and stability of the CatBoost and RF algorithms were positively correlated with the number of input parameters,and the three-parameter algorithms achieved higher estimation accuracy than the two-parameter algorithms.The developed methodology is helpful to predict Tdew at regional scale.Fuqi Yao Jinwei Sun Jianhua Dong 2022Computer Modeling in Engineering & Sciences2022,,2:1
13Preliminary research of pressure and phase change on containing gas (oil) fluid system 显示文摘HuWenxuan(胡文瑄) FuQi(符琦) LuXiancai(陆现彩) 1996高校地质学报1996,,4:1
14Effect of spectral resolution on the measurement of monoaromatic hydrocarbons by DOAS显示文摘有低得多的运作的费用和能力的优秀反应特征和察觉敏感使微分光吸收光谱学( DOAS )成为在某单音的芳族烃( MAHC )的异构体之间区别一个强大的工具由于化学结构的类似跟踪 MAHCs.But 的集中变化,那些 MAHC 有类似的重叠典型吸收结构,它使仪器的参数的选择批评到精确察觉 MAHCs.Firstly ,光谱在 DOAS 系统使用的分辨率决定 O2 的非线性的吸收和典型吸收结构的集体依赖;从而,它为察觉在大气的系列决定 O2 吸收的 ehmination 错误的效果 MAHCs.Secondly ,光谱分辨率决定在在汽车工业和光谱的重叠的干扰使用的技术溶剂代表主要成分的 12 MAHC 的微分吸收特征。第三,光谱分辨率决定敏感,时间决定和线性范围。那么光谱有到噪音的信号的最好的比率的分辨率范围被用来决定最合适光谱分辨率范围,以及光谱分辨率变化保证 MAHC 的典型吸收结构和 O2 吸收干扰的 rninimization。最后, 0.15-0.16 nm (在半最大值的 FWHM:full 宽度) 被假定接近最佳光谱分辨率和它被 DOAS 被 MAHC 的实际测量的结果证实。PENG Fumin XIE Pinhua ZHANG Yinghua ZHU Yanwu SI Fuqi LIU Wenqing WANG Junde 2008Journal of Environmental Sciences2008,20,5:1
15A Step Optimum Configuration Method for PBG/EBG Design Based on S-parameters显示文摘SHAN Fuqi GAO Baoxin ZHANG Xuexia 2006Chinese Journal of Electronics2006,15,2:0
16Synergy of first-and second-sphere interactions in a covalent organic framework boosts highly selective platinum uptake显示文摘Platinum recovery from waste electrical and electronic equipment(WEEE) in highly acidic solutions is significant to the electronics industry and environmental remediation. However, the lack of ingenious design and synergetic coordination gives rise to unsatisfied PtCl_(4)^(2-)extraction capacities and selectivities in most previously reported adsorbents(e.g., polymeric and inorganic materials). Herein, we proposed a synergistic strategy that realizes highly selective PtCl_(4)^(2-)uptake through first-and second-sphere coordinations. The proof-of-concept imine-linked covalent organic framework(SCU-COF-3) was found to chelate Pt Cl42-via the direct N…Pt coordination and the synergistically interlaminar N–H…Cl hydrogen bonds, which was disclosed by the comprehensive analysis of extended X-ray adsorption fine structure(EXAFS) characterizations and density functional theory(DFT) calculations. The unique adsorption mechanism imparts a superior adsorption capacity(168.4 mg g-1)and extraordinary Pt(II) selectivity to SCU-COF-3 under static conditions. In addition, SCU-COF-3 exhibits an upgraded distribution coefficient of 1.62 × 10^(5)mL· g^(-1), one order of magnitude higher than those of reported natural adsorbents. Specifically, SCU-COF-3 can extract PtCl_(4)^(2- )quantitatively from a simulated acidic waste solution coexisting with other 12 competitive ions, suggesting its promising application in practical scenarios.Linwei He Baoyu Li Zhonglin Ma Lixi Chen Shicheng Gong Mingxing Zhang Yaoyao Bai Qi Guo Fuqi Wu Fuqiang Zhao Jie Li Duo Zhang Daopeng Sheng Xing Dai Long Chen Jie Shu Zhifang Chai Shuao Wang 2023Science China Chemistry2023,66,3:0
17Superior Iodine Uptake Capacity Enabled by an Open Metal-Sulfide Framework Composed of Three Types of Active Sites显示文摘Efficient adsorption of gaseous radioiodine is pivotal for the sustainable development of nuclear energy and the long-termradiation safety of the ecological system.However,state-of-the-art adsorbents(e.g.metal-organic frameworks and covalent-organic frameworks)currently under exploration suffer severely from limited adsorption capacity,especially under a real-world scenariowith extremely lowradioiodine concentration and elevated temperature.This mostly originates from the relatively weak sorption driving forces mainly determinedby the iodine-adsorbent interaction consistingof noncovalent interactionswith a small fraction of strong chemical bonding.Here,we document the discovery of an open metal-sulfide framework((NH_(4))_(2)(Sn_(3)S_(7)),donated as SCU-SnS)constructed by three different types of active sites as a superior iodine adsorbent.Benefiting from the ability of iodine for pre-enrichment into the framework by charge-balancing NH_(4)^(+)through N-H···I interaction,the efficient reduction of I^(2)affording I^(-)by S^(2-),and extremely high binding affinity between Sn_(4)^(+)and I^(-),SCU-SnS exhibit a record-breaking iodine adsorption capacity(2.12 g/g)under dynamic breakthrough conditions and the highest static capacity(6.12 g/g)among all reported inorganic adsorbents,both at 348 K.Its facile synthesis and low cost endow SCU-SnS with powerful application potential for the nuclear industry.Yugang Zhang Linwei He Tingting Pan Jian Xie Fuqi Wu Xinglong Dong Xia Wang Lixi Chen Shicheng Gong Wei Liu Litao Kang Junchang Chen Lanhua Chen Long Chen Yu Han Shuao Wang 2023CCS Chemistry2023,5,7:0
18Observations of stratospheric ozone above Ny-?lesund in the Arctic, 2010–2011显示文摘Stratosphere ozone depletion above the Arctic region has drawn increased attention recently. Here we present stratospheric ozone column densities above Ny-?lesund in the Arctic during summer 2010 and 2011, based on a self-developed passive differential optical absorption spectroscopy(DOAS) technique. By analyzing the received scattered solar spectrum, daily variations of ozone vertical column densities(VCDs) were obtained and correlated with satellite-borne ozone monitoring results and ozone sonde data. The comparisons showed good correlation, confirming the feasibility of DOAS in high-latitude Arctic regions. The preliminary analysis also demonstrated that abnormal low-level ozone columns found in spring 2011 had negative impacts on total ozone column densities over the entire year. The loss of stratospheric ozone may be correlated with low stratospheric temperatures, where heterogeneous atmospheric reactions were active.LUO Yuhan SI Fuqi LIU Wenqing SUN Liguang LIU Yi 2015Advances in Polar Science2015,26,3:0
19An efficient atomic cross-chain commitment resisting fork fraud显示文摘1 Introduction Cross-chain transaction,as an essential component of blockchain technology,enables value exchange cross blockchains[1].Atomic cross-chain transaction technology has mainly encountered two challenges:efficiency and security.Efficiency challenges usually include the pressures on storage,transaction fees(e.g.,gas)or throughput,etc.Security challenges refer to the requirement that the assets traded must be obtained by the intended person for an intended amount.Among which fork fraud is one of the specialized problems,which refers to attackers obtaining assets that should not be obtained by manipulating blockchain forks.Many cross-chaining solutions today are not aware of such malicious attacks.In this study,we propose EAC3,an Efficient Atomic CrossChain Commitment that can resist fork fraud.By introducing a new resource multiplexing strategy,and redesigning the crosschain transaction process,EAC3 can effectively reduce various transaction overheads,and keep the possibility that attackers obtaining assets through secretly manipulating a chain fork at a safe level.Fuqi JIN Wenquan LI Lanju KONG Qingzhong LI 2023Frontiers of Computer Science2023,17,5:0
20Differential structure of Ordovician karst zone and hydrocarbon enrichment in paleogeomorphic units in Tahe area,Tarim Basin,NW China显示文摘Based on a large number of drilling,logging,seismic and production data,the differential structures of karst zone and hydrocarbon distribution in different paleogeomorphic units of the Tahe area,Tarim Basin,are discussed by analyzing the karst drainages and flowing channels.The karst paleogeomorphy of Ordovician in Tahe area is composed of watershed,karst valley and karst basin.The watershed has epikarst zone of 57.8 m thick on average and vadose karst zone of 115.2 m thick on average with dense faults,fractures and medium-small fracture-caves,and 76.5%of wells in this area have cumulative production of more than 5×10^(4) t per well.The karst valleys have epikarst zone,vadose karst zone and runoff karst zone,with an average thickness of 14.6,26.4 and 132.6 m respectively.In the runoff karst zone,the caves of subsurface river are mostly filled by fine sediment,with a filling rate up to 86.8%,and 84.9%of wells in this area have cumulative production of less than 2×10^(4) t per well.The karst basin has no karst zone,but only fault-karst reservoirs in local fault zones,which are up to 600 m thick and closely developed within 1 km around faults.Different karst landforms have different water flowing pattern,forming different karst zone structures and resulting in differential distribution of oil and gas.The watershed has been on the direction of oil and gas migration,so medium-small sized connected fracture-caves in this area have high filling degree of oil and gas,and most wells in this area have high production.Most caves in subsurface river are filled due to strong sedimentation and transportation of the river,so the subsurface river sediment has low hydrocarbon abundance and more low production oil wells.The faults linking source rock are not only the water channels but also the oil-gas migration pathways,where the karst fractures and caves provide huge reservoir space for oil and gas accumulation.ZHANG San JIN Qjang HU Mingyi HAN Qichao SUN Jianfang CHENG Fuqi ZHANG Xudong 2021Petroleum Exploration and Development2021,48,5:0
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