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| 1 | CFD study on double-to single-loop flow pattern transition and its influence on macro mixing efficiency in fully baffled tank stirred by a Rushton turbine显示文摘For a fully baffled tank stirred by a Rushton turbine (RT), the flow pattern will change from double- to single-loop as the off bottom clearance (C) of the RT decreases from one third of the tank diameter. Such a flow pattern transition as well as its influence on the macro mixing efficiency was investigated via CFD simulation. The transient sliding mesh approach coupled with the standard k-s turbulence model could correctly and efficiently reproduce the reported critical C range where the flow pattern changes. Simulation results indicated that such a critical C range varied hardly with the impeller rotation speed but decreased significantly with increasing impeller diameter. Small RTs are preferable to generating the single-loop flow pattern. A mechanism of the flow pattern transition was further proposed to explain these phe no mena. The discharge stream from the RT deviates down wards from the horizontal direction for small C values;if it meets the tank wall first, the double-loop will form;if it hits the tank bottom first, the single-loop will form. With the flow pattern transition, the mixing time decreased by about 35% at the same power input (P), indicating that the single-loop flow pattern was more efficient than the double-loop to enhance the macro mixing in the tank. A comparison was further made between the single-loop RT and pitched blade turbine (PBT, 45°) from macro mixing perspective. The single-loop RT was found to be less efficient than the PBT and usually required 60% more time to achieve the same level of macro mixing at the same P. | Quanhong Zhu Hang Xiao Aqiang Chen Shujun Geng Qingshan Huang | 2019 | Chinese Journal of Chemical Engineering2019，27，5： | 6 |
| 2 | Impacts of solid physical properties on the performances of a slurry external airlift loop reactor integrating mixing and separation显示文摘Solid physical properties are vital for the design, optimization, and scale-up of gas–liquid–solid multiphase reactors. The complex and interactional effects of the solid physical properties, including particle diameter, density, wettability, and sphericity, on the hydrodynamic behaviors in a new external airlift loop reactor(EALR) integrating mixing and separation are decoupled in this work. Two semi-empirical equations are proposed and validated to predict the overall gas holdup and liquid circulating velocity satisfactorily, and then the individual influence of such solid physical properties is further investigated. The results demonstrate that both the overall gas holdup in the riser and the liquid circulating velocity in the downcomer increase with the contact angle, but decrease with particle size, density, and sphericity.Additionally, the impact of the particle size on the liquid circulating velocity is also profoundly revealed on a micro-level considering the particle size distribution. Moreover, the axial solid concentration distribution is discussed, and the uniformity of the slurry is described by the mixing index of the solid particles. The results show that a more homogeneous mixture can be achieved by adding finer particles other than attaining violent turbulence. Therefore, this work lays a foundation for the design, scale-up, and industrialization of the EALRs. | Tian Zhang Qingshan Huang Shujun Geng Aqiang Chen Yan Liu Haidong Zhang | 2023 | Chinese Journal of Chemical Engineering2023，55，3： | 0 |
| 3 | Advances in the Application of Perovskite Materials显示文摘Nowadays, the soar of photovoltaic performance of perovskite solar cells has set off a fever in the study of metal halide perovskite materials. The excellent optoelectronic properties and defect tolerance feature allow metal halide perovskite to be employed in a wide variety of applications. This article provides a holistic review over the current progress and future prospects of metal halide perovskite materials in representative promising applications, including traditional optoelectronic devices(solar cells, light-emitting diodes, photodetectors, lasers), and cutting-edge technologies in terms of neuromorphic devices(artificial synapses and memristors) and pressure-induced emission. This review highlights the fundamentals, the current progress and the remaining challenges for each application, aiming to provide a comprehensive overview of the development status and a navigation of future research for metal halide perovskite materials and devices. | Lixiu Zhang Luyao Mei Kaiyang Wang Yinhua Lv Shuai Zhang Yaxiao Lian Xiaoke Liu Zhiwei Ma Guanjun Xiao Qiang Liu Shuaibo Zhai Shengli Zhang Gengling Liu Ligang Yuan Bingbing Guo Ziming Chen Keyu Wei Aqiang Liu Shizhong Yue Guangda Niu Xiyan Pan Jie Sun Yong Hua Wu‑Qiang Wu Dawei Di Baodan Zhao Jianjun Tian Zhijie Wang Yang Yang Liang Chu Mingjian Yuan Haibo Zeng Hin‑Lap Yip Keyou Yan Wentao Xu Lu Zhu Wenhua Zhang Guichuan Xing Feng Gao Liming Ding | 2023 | Nano-Micro Letters2023，15，10： | 0 |
| 4 | Influences of fluid physical properties,solid particles,and operating conditions on the hydrodynamics in slurry reactors显示文摘Slurry reactors are popular in many industrial processes,involved with numerous chemical and biological mixtures,solid particles with different concentrations and properties,and a wide range of operating conditions.These factors can significantly affect the hydrodynamic in the slurry reactors,having remarkable effects on the design,scale-up,and operation of the slurry reactors.This article reviews the influences of fluid physical properties,solid particles,and operating conditions on the hydrodynamics in slurry reactors.Firstly,the influence of fluid properties,including the density and viscosity of the individual liquid and gas phases and the interfacial tension,has been reviewed.Secondly,the solid particle properties(i.e.,concentration,density,size,wettability,and shape)on the hydrodynamics have been discussed in detail,and some vital but often ignored features,especially the influences of particle wettability and shape,as well as the variation of surface tension because of solid concentration alteration,are highlighted in this work.Thirdly,the variations of physical properties of fluids,hydrodynamics,and bubble behavior resulted from the temperature and pressure variations are also summarized,and the indirect influences of pressure on viscosity and surface tension are addressed systematically.Finally,conclusions and perspectives of these notable influences on the design and scale-up of industrial slurry reactors are presented. | He Yang Aqiang Chen Shujun Geng Jingcai Cheng Fei Gao Qingshan Huang Chao Yang | 2022 | Chinese Journal of Chemical Engineering2022，35，4： | 0 |
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