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| 1 | Facile synthesis of poly(aroxycarbonyltriazole)s with aggregation-induced emission characteristics by metal-free click polymerization显示文摘Regioseletive 1,3-dipolar polycycloadditions of 4,4'-isopropylidenediphenyl dipropiolate (1) and tetraphenylethene (TPE)-containing diazides (2) are carried out in polar solvents such as DMF/toluene at a moderate temperature of 100℃ for 6 h,producing poly(aroxycarbonyltriazole)s (PACTs) P3 with high molecular weights (Mw up to 23900) and regioregularities (F1,4 up to ~90%) in high yields (up to ~99%).These metal-free click polymerizations can propagate smoothly in an open atmosphere without protection from oxygen and moisture.The obtained polymers are soluble in common organic solvents and thermally stable at temperatures up to 375℃.Thanks to their contained TPE moieties,the PACTs show aggregation-induced emission and can serve as fluorescent chemosensors for superamplified detection of explosives. | LI HongKun MEI Ju WANG Jian ZHANG Shuang ZHAO QiuLi WEI Qiang QIN AnJun SUN JingZhi TANG Ben Zhong | 2011 | Science China Chemistry2011，54，4： | 8 |
| 2 | Partial eharaeterization and anti - tumor activity of an acidic polysaccharides from Gracilaria Lemaneifor- m/s 显示文摘 | Yanli Fan Wenhang Wang Wei Song Hongshuo Chen An- guo Teng Anjun Liu | 2012 | Carbohydrate Polymers2012，88，： | 1 |
| 3 | Partial characterization and anti-tumor activity of an acidic polysaccharide from Gracilaria lemaneiformis显示文摘 | Yanli Fan Wenhang Wang Wei Song Hongshuo Chen Anguo Teng Anjun Liu | 2012 | Carbohydrate Polymers2012，，4： | 1 |
| 4 | The performance of kapok/down blended wadding显示文摘 | Peng Cui Fumei Wang Anjun Wei Kongwei Zhao | 2010 | Textile Research Journal2010，80，6： | 1 |
| 5 | 3,4,5-Triphenyl-1,2,4-triazole-based multifunctional n-type AIEgen显示文摘The luminogens with aggregation-induced emission(AIEgens) characteristics have been widely applied in diverse areas. However,the n-type AIEgens are to be further developed. In this paper, we designed and synthesized an n-type multifunctional AIEgen of tetraphenylethene-substituted 3,4,5-triphenyl-4H-1,2,4-triazole(BTPE-TAZ). This AIEgen can serve as both light-emitting and electron-transporting layers in organic light-emitting devices. Moreover, it also exhibits the interesting optical waveguide and reversible mechanochromic luminescence properties, which are of great potential for practical applications. | Yang Shi Yuanjing Cai Yi Jia Wang Ming Chen Han Nie Wei Qin Haoke Zhang Jing Zhi Sun Anjun Qin Ben Zhong Tang | 2017 | Science China Chemistry2017，60，5： | 1 |
| 6 | Challenges and advances on low-temperature rechargeable lithiumsulfur batteries显示文摘Lithium-sulfur(Li-S)batteries have demonstrated the potential to conquer the energy storage related market due to the extremely high energy density.However,their performances at low temperature are still needed to be improved to broaden their applications.Therefore,in this review,the basic failure mechanisms and major challenges of Li-S battery at low temperature are categorized as the high desolvation barrier of Li^(+),uncontrolled nucleation and deposition of lithium,polysulfides clustering,and passivation of cathode by film like Li_(2)S.Targeting these major issues,strategies,and advances concerning the design of optimized electrolyte,composite cathode and functional separator are highlighted and discussed.Finally,the suggestions are proposed for the future development of practical Li-S battery working at low temperature scenarios,hoping to accelerate the commercialization process and bring revolution to the energy storage market. | Yu Jiao Fan Wang Yuhong Ma Sangang Luo Yaoyao Li Anjun Hu Miao He Fei Li Dongjiang Chen Wei Chen Tianyu Lei Yin Hu | 2023 | Nano Research2023，16，6： | 0 |
| 7 | Synergy of in-situ heterogeneous interphases tailored lithium deposition显示文摘The implementation of a robust artificial solid electrolyte interphase(ASEI)to replace the unstable natural SEI can regulate lithium deposition behaviors and avoid the safety hazards caused by dendrites permeation in lithium metal batteries.Despite of devoted efforts in tailoring components of ASEI,the intrinsic mechanism of interfacial synergy within the heterogeneous interphases has not been well elucidated yet.Herein,we show that the lithium plating/striping behaviors can be substantially enhanced(over 900 h with an overpotential of less than 20 mV at 1 mA·cm^(−2)in Li|Li symmetric cells and 146 cycles in anode-free cells)by regulating the heterogeneous interphases.This favorable ASEI composed of LiF and Li_(3)N components can be in-situ generated during cycling by large-scale fabricated fluorinated boron nitride coatings.Further,the synergy of each heterogeneous component within ASEI was explored theoretically and experimentally.Li_(3)N has high adsorption energy and low ion diffusion barrier,which facilitates the transport of lithium ions and avoids its local accumulation to evolve into dendrites.Both the substrate and LiF are interfacially stable with high electron tunneling barriers,preventing the electrolyte decomposition and parasitic reactions.Finally,the high stiffness of the boron nitride also ensures lithium dendrites are suppressed once they grow,providing a stable environment for long-term cycling of lithium metal batteries. | Yinuo Li Anjun Hu Xingdong Gan Miao He Jun Zhu Wei Chen Yin Hu Tianyu Lei Fei Li Yaoyao Li Yuxin Fan Fan Wang Mingjie Zhou An Wen Baihai Li | 2023 | Nano Research2023，16，6： | 0 |
| 8 | Manipulating the ion-transference and deposition kinetics by regulating the surface chemistry of zinc metal anodes for rechargeable zinc-air batteries显示文摘Aqueous zinc-air battery(ZAB)has attractive features as the potential energy storage system such as high safety,low cost and good environmental compatibility.However,the issue of dendrite growth on zinc metal anodes has seriously hindered the development of ZAB.Herein,the N-doped carbon cloth(NC)prepared via magnetron sputtering is explored as the substrate to induce the uniform nucleation of zinc metal and suppress dendrite growth.Results show that the introduction of heteroatoms accelerates the migration and deposition kinetics of Zn^(2+)by boosting the desolvation process of Zn^(2+),eventually reducing the nucleation overpotential.Besides,theoretical calculation results confirm the zincophilicity of N-containing functional group(such as pyridine N and pyrrole N),which can guide the nucleation and growth of zinc uniformly on the electrode surface by both promoting the redistribution of Zn^(2+) in the vicinity of the surface and enhancing its interaction with zinc atoms.As a result,the half-cell assembled with magnetron sputtered carbon cloth achieves a high zinc stripping/plating coulombic efficiency of 98.8%and long-term stability of over 500 cycles at 0.2 mA cm^(-2).And the Coulombic efficiency reached about 99.5%at the 10th cycle and maintained for more than 210 cycles at a high current density of 5.0 mA cm^(-2).The assembled symmetrical battery can deliver 220 plating/stripping cycles with ultra-low voltage hysteresis of only 11 mV.In addition,the assembled zinc-air full battery with NC-Zn anode delivers a high special capacity of about 429 mAh g_(Zn)^(-1) and a long life of over 430 cycles.The effectiveness of surface functionalization in promoting the transfer and deposition kinetics of Zn^(2+) presented in this work shows enlightening significance in the development of metal anodes in aqueous electrolytes. | Miao He Chaozhu Shu Ruixing Zheng Wei Xiang Anjun Hu Yu Yan Zhiqun Ran Minglu Li Xiaojuan Wen Ting Zeng Jianping Long | 2023 | Green Energy & Environment2023，8，1： | 0 |
| 9 | A novel silver-doped nickel oxide hole-selective contact for crystalline silicon heterojunction solar cells显示文摘Based on its band alignment,p-type nickel oxide(NiO_(x))is an excellent candidate material for hole transport layers in crystalline silicon heterojunction solar cells,as it has a smallΔEV and largeΔEC with crystalline silicon.Herein,to overcome the poor hole selectivity of stoichiometric NiO_(x) due to its low carrier concentration and conductivity,silver-doped nickel oxide(NiO_(x):Ag)hole transport layers with high carrier concentrations were prepared by co-sputtering high-purity silver sheets and pure NiO_(x) targets.The improved electrical conductivity of NiO_(x) was attributed to the holes generated by the Ag^(+)substituents for Ni^(2+),and moreover,the introduction of Ag^(+)also increased the amount of Ni^(3+)present,both of which increased the carrier concentration in NiO_(x).Ag^(+)doping also reduced the c-Si/NiO_(x) contact resistivity and improved the hole-selective contact with NiO_(x).Furthermore,the problems of particle clusters and interfacial defects on the surfaces of NiO_(x):Ag films were solved by UV-ozone oxidation and high-temperature annealing,which facilitated separation and transport of carriers at the c-Si/NiO_(x) interface.The constructed c-Si/NiO_(x):Ag solar cell exhibited an increase in open-circuit voltage from 490 to 596 mV and achieved a conversion efficiency of 14.4%. | Junfeng Zhao Xudong Yang Zhongqing Zhang Shengpeng Xie Fangfang Liu Anjun Han Zhengxin Liu Yun Sun Wei Liu | 2024 | Frontiers of Chemical Science and Engineering2024，18，2： | 0 |
| 10 | AIEgen configuration transition and aggregation enable dual prompt emission for single-component nondoped white OLEDs显示文摘The dual emission(DE)feature in materials holds great potential to revolutionize the development of one-component system white organic lightemitting diodes(WOLEDs).However,the reported DE materials remain scarce owing to the formidable challenge of breaking Kasha’s rule and managing the intricate energy/charge transfer processes.Herein,we have introduced a groundbreaking DE AIEgen,2CzAn-TPE,which possesses a simple structure and undergoes Z-to-E isomerization and exhibits yellow and red fluorescence powders for pre-and post-sublimation,respectively.With relatively lower potential energy,Z-conformation((Z)-1,2-diphenyl-1,2-bis(4-(10-(9-phenyl-9H-carbazol-3-yl)anthracen-9-yl)phenyl)ethene)of 2CzAn-TPE can be readily transformed into E-conformation((E)-1,2-diphenyl-1,2-bis(4-(10-(9-phenyl-9Hcarbazol-3-yl)anthracen-9-yl)phenyl)ethene)via vacuum sublimation.The utilization of X-ray diffraction and grazing-incidence-wide-angle X-ray scattering techniques confirms the structural transformation,while the crystallographic analysis reveals the establishment of numerous intermolecular CH⋅⋅⋅πinteractions between the tetraphenylethene(TPE)moiety and both the anthracene and carbazole units.This allows a densely packed molecular arrangement,thereby offering propitious conditions for excimer generation in the E-conformation aggregated state.By utilizing the sublimated 2CzAn-TPE as an emitter,a nondoped one-component WOLED was prepared,exhibiting an exceptionally high external quantum efficiency(EQE)of 5.0%,which represents one of the highest performances among all one-componentWOLEDs.This research introduces a novel,simple,and efficient approach to realize highly efficient one-molecule WOLEDs. | Jiasen Zhang Qiang Wei Wei Li Hao Chen Xiangyu Zhu Yongqi Bai Nannan Fei Liang Cao Zujin Zhao Anjun Qin Ben Zhong Tang Ziyi Ge | 2024 | Aggregate2024，5，1： | 0 |
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