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25篇 您的检索式:作者名="Yufei Tan"
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1Ultrasensitive and stable X-ray detection using zero-dimensional lead-free perovskites显示文摘Sensitive and reliable X-ray detectors are essential for medical radiography,industrial inspection and security screening.Lowering the radiation dose allows reduced health risks and increased frequency and fidelity of diagnostic technologies for earlier detection of disease and its recurrence.Three-dimensional(3 D)organic-inorganic hybrid lead halide perovskites are promising for direct X-ray detection-they show improved sensitivity compared to conventional X-ray detectors.However,their high and unstable dark current,caused by ion migration and high dark carrier concentration in the 3 D hybrid perovskites,limits their performance and long-term operation stability.Here we report ultrasensitive,stable X-ray detectors made using zero-dimensional(0 D)methylammonium bismuth iodide perovskite(MA3Bi2I9)single crystals.The 0 D crystal structure leads to a high activation energy(Ea)for ion migration(0.46 e V)and is also accompanied by a low dark carrier concentration(~10^6 cm^-3).The X-ray detectors exhibit sensitivity of 10,620μC Gy-1 air cm-2,a limit of detection(Lo D)of 0.62 nG yairs-1,and stable operation even under high applied biases;no deterioration in detection performance was observed following sensing of an integrated X-ray irradiation dose of^23,800 m Gyair,equivalent to>200,000 times the dose required for a single commercial X-ray chest radiograph.Regulating the ion migration channels and decreasing the dark carrier concentration in perovskites provide routes for stable and ultrasensitive X-ray detectors.Xiaojia Zheng Wei Zhao Peng Wang Hairen Tan Makhsud I.Saidaminov Shujie Tie Ligao Chen Yufei Peng Jidong Long Wen-HuZhang 2020Journal of Energy Chemistry2020,29,10:7
2Tunable Syngas Synthesis from Photocatalytic CO2 Reduction Under Visible-Light Irradiation by Interfacial Engineering显示文摘Visible-light-driven CO2 photoreduction to achieve renewable materials,such as syngas,hydrocarbons,and alcohols,is a key process that could relieve environmental problems and the energy crisis simultaneously.Reduction of syngas products with diff erent H2:CO proportions is highly expected to produce high value-added chemicals in the industry.However,the development of technologies employing long-wavelength irradiation to achieve CO2 photoreduction and simultaneous tuning of the resultant H2:CO proportion remains a challenging endeavor.In this work,we carried out interfacial engineering by designing a series of heterostructured layered double-hydroxide/MoS2 nanocomposites via electrostatic self-assembly.The syngas proportion(H 2:CO)obtained from CO2 photoreduction could be modulated from 1:1 to 9:1 by visible-light irradiation(λ>400 nm)under the control of the interface-rich heterostructures.This work provides a cost-eff ective strategy for solar-tofuel conversion in an artificial photosynthetic system and describes a novel route to produce syngas with targeted proportions.Conghui Qiu Sha Bai Wenjing Cao Ling Tan Junyan Liu Yufei Zhao Yu-Fei Song 2020Transactions of Tianjin University2020,26,5:6
3Tuning the selectivity of photoreduction of CO2 to syngas over Pd/layered double hydroxide nanosheets under visible light up to 600 nm显示文摘Photocatalytic reduction of CO2 with H2 O to syngas is an effective way for producing high value-added chemical feedstocks such as methanol and light olefins in industry.Nevertheless,the precise control of CO/H2 ratio from photocatalytic CO2 reduction reaction still poses a great challenge for the further application.Herein,we prepared a series of highly efficient heterostructure based on highly dispersed palladium supported on ultrathin Co Al-layered double hydroxide(LDH).In conjunction with a Ru-complex sensitizer,the molar ratios of CO/H2 can be tuned from 1:0.74 to 1:3 under visible-light irradiation(λ>400 nm).More interestingly,the syngas can be obtained under light irradiation atλ>600 nm.Structure characterization and density functional theory calculations revealed that the remarkable catalytic activity can be due to the supported palladium,which improved the charge transfer efficiency.Meanwhile,more H atoms were used to generate H2 on the supported palladium for further tunable CO/H2 ratio.This work demonstrates a new strategy for harnessing abundant solar-energy to produce syngas from a CO2 feedstock.Xian Wang Zelin Wang Ya Bai Ling Tan Yanqi Xu Xiaojie Hao Jikang Wang Abdul Hanif Mahadi Yufei Zhao Lirong Zheng Yu-Fei Song 2020Journal of Energy Chemistry2020,29,7:5
4Intercalation Effect in NiAl-layered Double Hydroxide Nanosheets for CO2 Reduction Under Visible Light显示文摘Photocatalytic reduction of CO2(CO2PR)to valuable solar fuels is considered as a promising route to the amelioration of fossil fuel conundrum and the mitigation of greenhouse gases.Although progress has been made to enhance CO2PR performance,the available method that can promote the selectivity of CO2PR products remains to be a challenge.In this work,we synthesized NO3-or CO32-intercalated NiAl-layered double hydroxide(NiAl-LDH)photocatalysts and investigated the performance of CO2PR in the presence of an electron donor and a photosensitizer.Compared with Ni2Al-CO32-,Ni2Al-NO3-exhibited superior catalytic performance in the CO2PR,and the resulted selectivity of CH4 in Ni2Al-NO3-(6.1%)was 12.2 times that of Ni2Al-CO32-(0.5%)under visible light irradiation.X-Ray absorption fine structure(XAFS)result reveals a relative abundance of defects in Ni2Al-NO3-,which played as active sites and promoted charge transfer in CO2PR for the efficient CH4 evolution.KIPKORIR Peter TAN Ling REN Jing ZHAO Yufei SONG Yu-Fei 2020Chemical Research in Chinese Universities2020,36,1:4
5China Antihypertensive Trial in Acute Ischemic Stroke II (CATIS-2): rationale and design显示文摘Backgrounds Increased blood pressure(BP)for patients who had an acute ischaemic stroke is associated with poor functional outcome,however the optimal timing of antihypertensive therapy is unknown.Aims We aim to compare early antihypertensive treatment to delayed antihypertensive treatment for reducing the risk of composite major disability and mortality at 3 months in acute ischaemic stroke.Design The China Antihypertensive Trial in Acute Ischemic Stroke II(CATIS-2)trial is a multicentre,randomised,open-label,blinded-endpoints trial that will be conducted in 100 hospitals in China.The primary outcome is the composite of death and major disability(modified Rankin Scale score≥3)at 3 months of randomisation.Antihypertensive treatment will be received immediately after randomisation in the early treatment group,aimed at average systolic BP by 10%-20%reduction within the first 24 hours,and achieving an average BP level of<140/90 mm Hg within 5 days.Patients in the delayed treatment group will discontinue any antihypertension medications for the first 7 days of randomisation,and will receive antihypertensive therapy achieving a BP goal of<140/90 mm Hg after 7 days.Conclusion The CATIS-2 trial will be testing the hypotheses that early BP lowering leads to improved functional outcome without any other harms,and developing clinical guidelines of the BP management for patients who had an acute ischaemic stroke.Liping Liu Yilong Wang Xuewei Xie Dacheng Liu Aili Wang Penglian Wang Suwen Shen Chongke Zhong Yufei Wei Tan Xu Yuesong Pan Yong Jiang Xia Meng David Wang Yonghong Zhang Jiang He Yongjun Wang 2021Stroke & Vascular Neurology2021,6,2:3
6A core-shell structured COYID-19 mRNA vaccine with favorable biodistribution pattern and promising immunity显示文摘Although inoculation of COVID-19 vaccines has rolled out globally,there is still a critical need for safe and effective vaccines to ensure fair and equitable supply for all countries.Here,we report on the development of a highly efficacious mRNA vaccine,SW0123 that is composed of sequence-modified mRNA encoding the full-length SARS-CoV-2 Spike protein packaged in core-shell structured lipopolyplex(LPP)nanoparticles.SWOT 23 is easy to produce using a large-scale microfluidics-based apparatus.The unique core-shell structured nanoparticle facilitates vaccine uptake and demonstrates a high colloidal stability,and a desirable biodistribution pattern with low liver targeting effect upon intramuscular administration.Extensive evaluations in mice and nonhuman primates revealed strong immunogenicity of SW0123,represented by induction of Th1-polarized T cell responses and high levels of antibodies that were capable of neutralizing not only the wild-type SARS-CoV-2,but also a panel of variants including D614G and N501Y variants.In addition,SW0123 conferred effective protection in both mice and non-human primates upon SARS-CoV-2 challenge.Taken together,SW0123 is a promising vaccine candidate that holds prospects for further evaluation in humans.Ren Yang Yao Deng Baoying Huang Lei Huang Ang Lin Yuhua Li Wenling Wang Jingjing Liu Shuaiyao Lu Zhenzhen Zhan Yufei Wang Ruhan A Wen Wang Peihua Niu Li Zhao Shiqiang Li Xiaopin Ma Luyao Zhang Yujian Zhang Weiguo Yao Xingjie Liang Jincun Zhao Zhongmin Liu Xiaozhong Peng Hangwen Li Wenjie Tan 2021Signal Transduction and Targeted Therapy2021,6,6:3
7Prospect of China's ambient air quality standards显示文摘Ambient air quality standards are the core strategic goal of ambient air quality management.Countries worldwide have given importance to research on the development of ambient air quality standards.To understand the history of the development of China’s ambient air quality standards,this study analyzed the background associated with all previous formulations and revisions of the standards,classification of functional areas,standard grading,pollutants,and evolution of the standard limits over the past 40 years.The results show that since the initial release of the“Ambient Air Quality Standard”by China in 1982,it has been supplemented once,revised twice,and modified twice.The first ambient air quality standard specified the standard limits of six pollutants commonly found in ambient air.With the development of ambient air quality management,the number of pollutants has increased to ten.Since the release of the“Ambient Air Quality Standards”in 2012,the ambient air quality in China has significantly improved.However,the proportion of cities meeting these standards is still low.At present,China is suitably positioned to make the standards associated with 24 hr SO2concentrations more stringent such that it meets the values defined in the World Health Organization(WHO)interim target-2 and the WHO air quality guideline(AQG).We further suggested that the SO2standard should be revised promptly.Simultaneously,regions with a relatively high proportion of cities meeting the standard are encouraged to introduce more stringent interim target limits in due course to manage the local ambient air quality.Zongshuang Wang Yufei Tan Min Guo Miaomiao Cheng Yanyue Gu Siyu Chen Xuefang Wu Fahe Chai 2023Journal of Environmental Sciences2023,,1:2
8Comparison of inorganic chemical compositions of atmospheric TSP,PM10 and PM2.5 in northern and southern Chinese coastal cities显示文摘To compare the inorganic chemical compositions of TSP(total suspended paniculate),PM_(10)(particulate matter with an aerodynamic diameter less than 10 μm) and PM_(2.5)(particulate matter with an aerodynamic diameter less than 2.5 μm) in southern and northern cities in China,atmospheric particles were synchronously collected in Dalian(the northern city)and Xiamen(the southern city) in spring and autumn of 2004.The mass concentrations,twenty-three elements and nine soluble ions were assessed.The results show that in Dalian,the mass concentrations of Mg,Al,Ca,Mn and Fe in spring were 4.0-10.1,2.6-8.0,4.1-12,1.2-3.6 and 2.9-7.9 times higher,respectively,than those in Xiamen.The dust storm influence is more obvious in Dalian in spring.However,in Xiamen,heavy metals accounted for 13.9%-17.9%of TSP,while heavy metals contributed to 5.5%-9.3%of TSP in Dalian.These concentrations suggest that heavy metal pollution in Xiamen was more serious.In addition,the concentrations of Na^+,Cl^-,Ca^(2+) and Mg^(2+) were higher in Dalian due to the influence of marine aerosol,construction activities and soil dust.The NO^(3-)/SO_4^(2-) ratios in Dalian(0.25-0.49) were lower than those in Xiamen(0.51-0.62),indicating that the contributions of vehicle emission to particles in Xiamen were higher.Coefficient of divergence values was higher than 0.40,implying that the inorganic chemical composition profiles for the particles of Dalian and Xiamen were quite different from each other.Yiding Ma Zongshuang Wang Yufei Tan Shu Xu Shaofei Kong Gang Wu Xuefang Wu Hong Li 2017Journal of Environmental Sciences2017,29,5:2
9Scaled-up synthesis of defect-rich layered double hydroxide monolayers without organic species for efficient oxygen evolution reaction显示文摘The scaled-up synthesis of organic-free monolayer nanomaterials is highly desirable,especially in obtaining green energy by electrocatalysis.In this study,a method for the scaled-up synthesis of the series of monolayer layered double hydroxides(LDHs)without the addition of organic solvents is reported via the separate nucleation and aging steps process.The resulting monolayer LDHs with the thicknesses of less than 1 nm showed a narrow thickness distribution.X-ray absorption fine-structure revealed that monolayer NiFe-LDH nanosheets have a number of oxygen and metal vacancies defects.As a practical application,monolayer NiFe-LDH nanosheets containing defects showed an enhanced electrocatalytic water oxidation activity compared with that of bulk NiFe-LDH.Density functional theory calculations uncovered that excellent catalytic activity is attributed to vacancies defects.The proposed method is an economical and universally applicable strategy for the scaled-up production of monolayer LDHs.Haoyuan Chi Jingwen Dong Tian Li Sha Bai Ling Tan Jikang Wang Tianyang Shen Guihao Liu Lihong Liu Luyi Sun Yufei Zhao Yu-Fei Song 2022Green Energy & Environment2022,7,5:2
10Development of a widely targeted volatilomics method for profiling volatilomes in plants显示文摘Volatile organic compounds play essential roles in plant environment interactions as well as determining the fragrance of plants.Although gas chromatography-mass spectrometry-based untargeted metabolo-mics is commonly used to assess plant volatiles,it suffers from high spectral convolution,low detection sensitivity,a limited number of annotated metabolites,and relatively poor reproducibility.Here,we report a widely targeted volatilomics(WTV)method that involves using a“targeted spectra extraction”algorithm to address spectral convolution,constructing a high-coverage MS2 spectral tag library to expand volatile annotation,adapting a multiple reaction monitoring mode to improve sensitivity,and using regression models to adjust for signal drift.The newly developed method was used to profile the volatilome of rice grains.Compared with the untargeted method,the newly developed WTV method shows higher sensitivity(for example,the signal-to-noise ratio of guaicol increased from 4.1 to 18.8),high annotation coverage(the number of annotated volatiles increased from 43 to 132),and better reproducibility(the number of volatiles in quality control samples with relative standard deviation value below 30.0%increased from 14 to 92 after normalization).Using the WTV method,we studied the metabolic responses of tomato to environmental stimuli and profiled the volatilomes of different rice accessions.The results identified benzothiazole as a potential airborne signal priming tomato plants for enhanced defense and 2-nonanone and 2-heptanone as novel aromatic compounds contributing to rice fragrance.These case studies suggest that the widely targeted volatilomics method is more efficient than those currently used and may considerably promote plant volatilomics studies.Honglun Yuan Guangping Cao Xiaodong Hou Menglan Huang Pengmeng Du Tingting Tan Youjin Zhang Haihong Zhou Xianqing Liu Ling Liu Yiding Jiangfang Yufei Li Zhenhuan Liu Chuanying Fang Liqing Zhao Alisdair R.Fernie Jie Luo 2022Molecular Plant2022,15,1:2
11The spatial distribution of nitrogen removal functional genes in multimedia biofilters for sewage treatment 显示文摘Ji Guodong He Chunguang Tan Yufei 2013Ecological Engineering2013,55,:1
12Design, implemen- tation, and evaluation of a NUMA-Aware cache for iSCSI storage servers显示文摘Ren Yufei Li Tan Yu Dantong 2015IEEE Transactions on Parallel and Dis- tributed Systems2015,26,2:1
13Experimental test on Carbon Crystal Panel system and simulation research on its partial-heating program显示文摘Tiantian Zhang Yufei Tan Haiqiao Zhang 2011Building and Environment2011,,:1
14Wastewater treatment efficiency of a multi-media biological aerated filter(MBAF) containing clinoptilolite and bioceramsite in a brick-wall embedded design显示文摘Ji Guodong Tong Jingjing Tan Yufei 2011Bioresource Technology2011,102,2:1
15Experimental simulation of the relative contribution of volatile-N and char-N to NO_X formation from a low-capacity bituminous coal-fired industrial boiler显示文摘The conversion of fuel-N to NOx is the main contribution of NOx from coal-fired industrial boilers and is the least-studied modelling problem arising from coal combustion. This paper summarises the current understanding of the mechanisms that account for the formation of NOx from fuel-N during coal combustion. Further experimentation on NOx emissions during bituminous coal combustion was simulated with attention focused on the contribution of char-N and volatile-N to fuel-NOx through the Coal/Char combustion method. The critical analysis of this issue allowed for the identification of uncertainties and produced well-founded conclusions. The results indicated that fuel-NOx formation was a very complex physical-chemical process involving many competing mechanisms. These mechanisms included chemical reactions, convective mass transfer, heat transfer, adsorption and desorption. The contribution of char-N in this experiment varied between 30% and 70%. There may be a slight question as to the exact identity of the main contributor to fuel-NOx , and no definitive conclusion can be made as of yet. This uncertainty is because the contribution of char-N to fuel-NO x was heavily affected by the combustion conditions and the contribution of char-N increased monotonically as temperature increased. There was a critical point in the relationship between particle size, air flow, O2 concentration and the contribution of char-N. The contribution of char-N increased with the increase of particle size and air flow initially when less than the critical value, and decreased when more than thecritical value. The contribution of char-N initially decreased when the O2 concentration was increased from 10% to 15% and increased more with the further increase in O2 concentration.WU XueFang WANG Sheng WANG ZongShuang CHE Fei WANG ZhanShan XU Shu LI Qin TAN YuFei 2013Science China Chemistry2013,56,4:1
16BiO_(2-x)Nanosheets with Surface Electron Localizations for Efficient Electrocatalytic CO_(2)Reduction to Formate显示文摘To enhance the activity and selectivity of electrocatalytic CO_(2)reduction to formate is of great importance from both environmental and economical viewpoints.Herein,the BiO_(2-x)nanosheets with surface electron localizations were constructed and utilized for the efficient CO_(2)-to-formate conversion.The formate Faraday efficiency reaches 99.1%with current density of 12 mA cm^(−2)at^(−1).1 V versus the reversible hydrogen electrode(RHE)in an H-type cell while those in the flow cell are 91.3%and 319 mA cm^(−2)at^(−1).0 V versus RHE,respectively.Theoretical calculations indicate that the electron localization presenting in the BiO_(2-x)nanosheet favors OCHO*intermediate stabilization and suppresses H*intermediate adsorption,thus improving the CO_(2)-to-formate efficiency.The BiO_(2-x)electrocatalyst is nondopant,easily prepared,low-cost,highly active and selective for CO_(2)RR to formate,which has demonstrated potential for application in the Zn-CO_(2)battery.The maximum power density can reach 2.33 mW cm^(−2),and the charge/discharge cycling stability is>100 h(300 cycles)at 4.5 mA cm^(−2).Zhonghao Tan Jianling Zhang Yisen Yang Yufei Sha Ran Duan Jiajun Zhong Buxing Han Jingyang Hu Yingzhe Zhao 2023CCS Chemistry2023,5,1:0
17Vernier But Not Grating Acuity Contributes to an Early Stage of Visual Word Processing显示文摘The process of reading words depends heavily on efficient visual skills, including analyzing and decomposing basic visual features. Surprisingly, previous reading-related studies have almost exclusively focused on gross aspects of visual skills, while only very few have investigated the role of finer skills. The present study filled this gap and examined the relations of two finer visual skills measured by grating acuity(the ability to resolve periodic luminance variations across space) and Vernier acuity(the ability to detect/discriminate relative locations of features) to Chinese character-processing as measured by character form-matching and lexical decision tasks in skilled adult readers. The results showed that Vernier acuity was significantly correlated with performance in character form-matching but not visual symbol formmatching, while no correlation was found between grating acuity and character processing. Interestingly, we found no correlation of the two visual skills with lexical decisionperformance. These findings provide for the first time empirical evidence that the finer visual skills, particularly as reflected in Vernier acuity, may directly contribute to an early stage of hierarchical word processing.Yufei Tan Xiuhong Tong Wei Chen Xuchu Weng Sheng He Jing Zhao 2018Neuroscience Bulletin2018,34,3:0
18中国北京地区部分医院患者疼痛现状调查(英文)显示文摘Objective:This study aimed to survey the characteristics and treatments of cancer pain in Beijing hospitals,China.Methods:At 20:00 on December 22,2009,there conducted a questionnaire survey in 2238 patients with malignant tumors of 26 hospitals in Beijing,and the survey results were statistically analyzed.Results:The 531 cases in 2238 patients had pained and 121 cases (22.79%) had outbreak pain with one week.At 20:00 on December 22,2009,199 cases (38%) in the above-mentioned 531 pain patients suffered the moderate to severe pain (pain scores ≥ 4).The number of pain (pain scores ≥ 4) patients in the consecutive three days from December 20 to December 22 were 150.Conclusion:In the 531 cancer pain patients of the surveyed hospitals,38% of the patients were not satisfied with the pain control.Doctors believed that the main reason for pain not controlled was the non-standard treatment,but patients considered to be afraid of addiction.Shikai Wu Fang Li Pingping Li Jian Luo Xiaoming Wu Heling Shi Xiaohong Ning Yufei Yang Huangying Tan Ping Yang Guangqing Zhu Jianhua Zhu Guoqing Liao Huoming Chen Dapeng Lv Ye Fang Hong Dai Xiaoming Xi Xiuhua Li Yuan Qin Li Feng Su Wang Xiaoyan Chen Hongyong Wang Hongyan Li Duanqi Liu 2012The Chinese-German Journal of Clinical Oncology2012,11,6:0
19Heteroatom anchors Fe-Mn dual-atom catalysts with bi-functional oxygen catalytic activity for low-temperature rechargeable flexible Zn-air batteries显示文摘M-N-C(M=Fe,Co,Ni,etc.) catalyst owns high catalytic activity in the oxygen catalytic reaction which is the most likely to replace the Pt-based catalysts.But it is still a challenge to further increase the active site density.This article constructs the high-efficiency FeMn-N/S-C-1000 catalyst to realize ORR/OER bifunctional catalysis by hetero-atom,bimetal(Fe,Mn) doped simultaneously strategy.When evaluated it as bi-functional electro-catalysts,FeMn-N/S-C-1000 exhibits excellent catalytic activity(E_(1/2)=0.924 V,E_(j=10)=1.617 V) in alkaline media,outperforms conventional Pt/C,RuO_(2) and most non-precious-metal catalysts reported recently,Such outstanding performance is owing to N,S co-coordinated with metal to form multi-types of single atom,dual atom active sites to carry out bi-catalysis.Importantly,nitrite poison test provides the proof that the active sites of FeMn-N/S-C are more than that of single-atom catalysts to promote catalytic reactions directly.To better understand the local structure of Fe and Mn active sites,XAS and DFT were employed to reveal that FeMn-N_5/S-C site plays the key role during catalysis.Notably,the FeMn-N/S-C-1000 based low-temperature rechargeable flexible Zn-air also exhibits superior discharge performance and extraordinary durability at-40℃.This work will provide a new idea to design diatomic catalysts applied in low-temperature rechargeable batteries.Yuting He Hongtao Li Yi Wang Yufei Jia Yongning Liu Qiang Tan 2024Journal of Energy Chemistry2024,90,3:0
20Remote Synthesis of Layered Double Hydroxide Nanosheets Through the Automatic Chemical Robot显示文摘As a family of two-dimensional functional materials, layered double hydroxides(LDHs) have the characteristics of adjustable lamellar element type and proportion, variable interlamellar anion, controllable particle size and thickness, providing a robust platform for photo/electro/thermal-catalysis. With the continuous progress of materials science, the synthesis of LDHs is becoming more and more refined. Herein, to achieve the fine preparation of LDHs materials, especailly for the no-chemical/material researchers, we successfully assembled the automatic synthesis device and wrote corresponding computer software to control this device, and the automatic synthesis of bulk and monolayer LDHs nanosheets on a laboratory scale can be realized. This work paves a new labor-saving way for the fine synthesis of LDHs nanostructures, further improving the development of LDHs-based materials.WANG Zelin LIU Guihao SHEN Tianyang TAN Ling ZHAO Yufei SONG Yu-Fei 2022Chemical Research in Chinese Universities2022,38,1:0
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