|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Enhanced aromatic selectivity by the sheet-like ZSM-5 in syngas conversion显示文摘Aromatics are important basic chemicals. However, direct conversion of syngas via the conventional Fischer-Tropsch synthesis produces little aromatics. We presented herein that a bifunctional composite of ZSM-5 in combination with Zn Cr Oxcatalyzes syngas conversion to aromatics. Particularly, ZSM-5 crystals with a sheet-like morphology can enhance significantly the aromatization activity. The lower length ratio of the b/a axes of the crystals, the more aromatics form but without influencing the selectivity of small molecules such as CH4 and C2–C4. Since the acid properties and the Al chemical environment were not altered while the morphology changed, the enhanced aromatic selectivity is likely attributed to the favored diffusion of aromatics in these sheet-like crystals. | Junhao Yang Ke Gong Dengyun Miao Feng Jiao Xiulian Pan Xiangju Meng Fengshou Xiao Xinhe Bao | 2019 | Journal of Energy Chemistry2019,28,8: | 10 |
| 2 | Mesoporous zeolites as efficient catalysts for oil refining and natural gas conversion显示文摘 | Jie ZHU Xiangju MENG Fengshou XIAO | 2013 | Frontiers of Chemical Science and Engineering2013,7,2: | 8 |
| 3 | Templating route for synthesizing mesoporous zeolites with improved catalytic properties 显示文摘 | Meng Xiangiu Nawaz Faisal Xiao Fengshou | 2009 | Nano Today2009,4,4: | 1 |
| 4 | Hydrothermally stable ordered mesoporous titano silicates with highly active catalytic sites显示文摘 | Xiao Fengshou Han Yu Yu Yi | 2002 | J Am Chem Soc2002,124,6: | 1 |
| 5 | Organosilane surfactant-assisted synthesis of mesoporous SSZ-39 zeolite with enhanced catalytic performance in the methanol-to-olefins reaction显示文摘SSZ-39 zeolite with AEI framework structure is a good catalyst candidate for the methanol-to-olefins(MTO)reaction.However,the diffusion limitation and coke formation often results in fast deactivation of the SSZ-39 zeolite catalyst.One solution for this challenge is to introduce mesoporosity in the SSZ-39 zeolite.Herein,we report the synthesis of mesoporous SSZ-39 zeolite using an organosilane surfactant,,-dimethyl--(3-(trimethoxysilyl)propyl)octan-1-aminium chloride,as a mesopore template and,-dimethyl--2,6-dimethylpiperidinium as a micropore template.The obtained zeolites were characterized by X-ray diffraction,N sorption,scanning electron microscopy,temperature programmed desorption of ammonia,and magic angle spinning nuclear magnetic resonance of Al.The results show that the mesoporous SSZ-39 zeolite has high crystallinity,meso/microporosity,high surface area,cuboid morphology,and abundant acidic sites.More importantly,this mesoporous SSZ-39 zeolite exhibits enhanced catalyst lifetime in the MTO reaction due to the presence of mesoporosity for fast mass transfer,compared with a conventional SSZ-39 zeolite without mesoporosity. | Hao Xu Chi Lei Qinming Wu Qiuyan Zhu Xiangju Meng Daniel Dai Stefan Maurer Andrei-Nicolae Parvulescu Ulrich Muller Fengshou Xiao | 2020 | Frontiers of Chemical Science and Engineering2020,14,2: | 1 |
| 6 | Templating Route for Synthesizing Mesoporous Zeolites with Improved Catalytic Properties显示文摘 | Meng Xiangju Nawaz Faisal Xiao Fengshou | 2009 | Nano Today2009,4,4: | 1 |
| 7 | Templating route for synthesizing mesopomus zeolites with improved catalytic properties显示文摘 | Xiangju Meng Faisal Nawaz Fengshou Xiao | 2009 | Nano Today2009,4,4: | 1 |
| 8 | Synthesis and Structure of Copper Hydroxyphosp - hate and Its High Catalyti - Activity in Hydroxylation of Phenol by H2O2 显示文摘 | Fengshou Xiao Jianmin Sun Ranbo Yu | 2001 | J Catal2001,199,: | 1 |
| 9 | A novel catalyst of copper hydroxyphosphate with high activity in wet oxidation of aromatics 显示文摘 | Fengshou Xiao Jianmin Sun Xiangju Meng | 2001 | Applied Catalysis A: General2001,207,: | 1 |
| 10 | Selective catalytic oxidati on of napht hol to 2-hydroxyl-1,4- naphthoquinone by hydrogen peroxide overmetalloporphyrin catal ysts显示文摘 | YAN Yan XIAO Fengshou ZHENG Guodong | 2000 | Journal of Molecular Catalysis A : Chemical2000,157,: | 1 |
| 11 | Catalytic Performance in Phenol Hydroxylation by Hydrogen Peroxide over a Catalyst of V-Zr-O Complex显示文摘 | Xiao Fengshou Wang Dan | 1999 | Catal Today1999,51,1: | 1 |
| 12 | Green Routes for synthesis of zeolites显示文摘 | Meng Xiangju Xiao Fengshou | 2014 | Chem Rev2014,114,2: | 1 |
| 13 | Design and size control of uniform zeolite nanocrystals synthesized in adjustable con- fined voids formed by recyclable monedisperse polymer spheres 显示文摘 | Yang Xiaoyu Tian Ge Xiao Fengshou | 2005 | Angew Chem Int Ed2005,44,: | 1 |
| 14 | Syn- thesis and Structure of Copper Hydroxyphoshata and Its High Catalytic Activity in Hydroxylation of Phenol by H:O2 显示文摘 | Xiao Fengshou Sun Jianmin Meng Xiangju | 2001 | J Catal2001,199,2: | 1 |
| 15 | Hydrothermally stahle ordered mesoporous titanosilicates with highly active catalytic sites显示文摘 | XIAO Fengshou HAN Yu YU Yi | 2002 | J Am Chem Soc2002,124,6: | 1 |
| 16 | Green Routes for Synthesis of Zeolites显示文摘 | Meng Xiangju Xiao Fengshou | 2014 | Chem Rev2014,114,2: | 1 |
| 17 | Green routes for syn- thesisofzeolites显示文摘 | Meng Xiangju Xiao Fengshou | 2013 | ChemRev2013,114,2: | 1 |
| 18 | In-situ transmission electron microscopy observation of particle size effect of nanoscale platinum catalysts on the formation of fullerenelike carbon shells显示文摘 | Xin Ge Binhai Peng Xiabai Ying Ran Wang Xiaoyang Liu Fengshou Xiao Shilun Qiu Jixue Li | 2008 | Carbon2008,,11: | 1 |
| 19 | Mesoporous aluminosilicates with ordered hexagonal structure, strong acidity, and extraordinary hydrothermal stability at high temperatures显示文摘 | Zhang Zongtao Han Yu Xiao Fengshou | 2001 | J Am Chem Soc2001,123,21: | 1 |
| 20 | Design and size con- trol of uniform zeolite nanocrystals synthesized in adjustable confined voids formed by recyclable monodisperse polymer spheres 显示文摘 | Yang Xiaoyu Tian Ge Xiao Fengshou | 2005 | Angew Chem Int Ed2005,44,: | 1 |