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		题名	作者	年代	出处	被引量
	1	Fluorinated Covalent Organic Frameworks Coupled with Molecular Cobalt Cocatalysts for Efficient Photocatalytic CO_(2)Reduction显示文摘The combination of covalent organic framework(COF)photosensitizers with molecular cocatalysts is a promising avenue for photocatalytic carbon dioxide(CO_(2))reduction.Here,a series of isostructural COFs was synthesized using linkers of different lengths,with or without partial fluorination.These COFs were investigated for photocatalytic CO_(2)reduction under visible-light irradiation when combined with cobalt(II)bipyridine complexes as a cocatalyst.Fluorination was found to enhance both CO_(2)affinity and catalytic activity,and a partially fluorinated COF,FBP-COF,achieved the highest CO_(2)-to-CO conversion efficiency,showing a carbon monoxide(CO)generation rate of 2.08 mmol h−1 g−1 and a 90%CO selectivity.FBP-COF also showed good stability under sacrificial conditions,generating CO for 50 h with a turnover number of 91.5.This activity is much higher than a homogeneous system using ruthenium bipyridine complexes as the photosensitizer combined with the same cobalt bipyridine complexes.	Zhiwei Fu Chang Shu Xiaoyan Wang Linjiang Chen Xue Wang Lunjie Liu Kewei Wang Rob Clowes Samantha Y.Chong Xiaofeng Wu Andrew I.Cooper	2023	CCS Chemistry2023，5，10：	0

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