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| 1 | Precise nanomedicine for intelligent therapy of cancer显示文摘Precise nanomedicine has been extensively explored for efficient cancer imaging and targeted cancer therapy, as evidenced by a few breakthroughs in their preclinical and clinical explorations. Here, we demonstrate the recent advances of intelligent cancer nanomedicine, and discuss the comprehensive understanding of their structure-function relationship for smart and efficient cancer nanomedicine including various imaging and therapeutic applications, as well as nanotoxicity. In particular, a few emerging strategies that have advanced cancer nanomedicine are also highlighted as the emerging focus such as tumor imprisonment, supramolecular chemotherapy, and DNA nanorobot. The challenge and outlook of some scientific and engineering issues are also discussed in future development. We wish to highlight these new progress of precise nanomedicine with the ultimate goal to inspire more successful explorations of intelligent nanoparticles for future clinical translations. | Huabing Chen Zhanjun Gu Hongwei An Chunying Chen Jie Chen Ran Cui Siqin Chen Weihai Chen Xuesi Chen Xiaoyuan Chen Zhuo Chen Baoquan Ding Qian Dong Qin Fan Ting Fu Dayong Hou Qiao Jiang Hengte Ke Xiqun Jiang Gang Liu Suping Li Tianyu Li Zhuang Liu Guangjun Nie Muhammad Ovais Daiwen Pang Nasha Qiu Youqing Shen Huayu Tian Chao Wang Hao Wang Ziqi Wang Huaping Xu Jiang-Fei Xu Xiangliang Yang Shuang Zhu Xianchuang Zheng Xianzheng Zhang Yanbing Zhao Weihong Tan Xi Zhang Yuliang Zhao | 2018 | Science China Chemistry2018，61，12： | 19 |
| 2 | Aggregation-enhanced emission and efficient electroluminescence of conjugated polymers containing tetraphenylethene units显示文摘Tetraphenylethene (TPE) is a popular luminogen characterized by aggregation-induced emission and has been widely used to construct solid-state emissive materials. In this work, two thermally stable polymers (P1 and P2) consisting of TPE conjugated to the 2,7-positions of fluorene and carbazole, respectively, are synthesized and characterized. Both polymers are weakly fluorescent in solutions but show greatly enhanced emission as the aggregate formation, presenting an aggregation-enhanced emission feature. Two kinds of polymer light-emitting diodes are fabricated utilizing P1 and P2 as emitters (EML) (device I: ITO/PEDOT:PSS (45 nm)/PVK:EML (1:1 wt%, 55 nm)/TPBI (38 nm)/Ca:Ag; device II: ITO/PEDOT:PSS (45 nm)/ PVK:OXD-7:EML (3:1:3 wt%, 55 nm)/TPBI (38 nm)/Ca:Ag). The device II of P2 shows the best performances, affording a maximum luminance of 6500 cd/m 2 and a high peak efficiency of 2.11 cd/A. | HE BaiRong YE ShangHui GUO YanJu CHEN Bin XU XiaoFei QIU HuaYu ZHAO ZuJin | 2013 | Science China Chemistry2013，56，9： | 2 |
| 3 | An Endotenon Sheath-Inspired Double-Network Binder Enables Superior Cycling Performance of Silicon Electrodes显示文摘Silicon(Si)has been regarded as an alternative anode material to traditional graphite owing to its higher theoretical capacity(4200 vs.372 m Ah g;).However,Si anodes suffer from the inherent volume expansion and unstable solid electrolyte interphase,thus experiencing fast capacity decay,which hinders their commercial application.To address this,herein,an endotenon sheathinspired water-soluble double-network binder(DNB)is presented for resolving the bottleneck of Si anodes.The as-developed binder shows excellent adhesion,high mechanical properties,and a considerable self-healing capability mainly benefited by its supramolecular hybrid network.Apart from these advantages,this binder also induces a Li;N/Li F-rich solid electrolyte interface layer,contributing to a superior cycle stability of Si electrodes.As expected,the DNB can achieve mechanically more stable Si electrodes than traditional polyacrylic acid and pectin binders.As a result,DNB delivers superior electrochemical performance ofSi/Li half cells and Li Ni;Co;Mn;O;/Si full cells,even with a high loading of Si electrode,to traditional polyacrylic acid and pectin binders.The bioinspired binder design provides a promising route to achieve long-life Si anode-assembled lithium batteries. | Meifang Jiang Pengzhou Mu Huanrui Zhang Tiantian Dong Ben Tang Huayu Qiu Zhou Chen Guanglei Cui | 2022 | Nano-Micro Letters2022，14，6： | 2 |
| 4 | Separation of the isomer compositions of oligomethylphenyl cyclosiloxane on capillary column and determination of the isomers by GC-MS 显示文摘 | Jiang Kezhi Ni Yong Qiu Huayu | 2006 | Chromatographia2006，64，1112： | 1 |
| 5 | A Highly Copper‐Selective Ratiometric Fluorescent Sensor Based on BODIPY显示文摘 | Jinlong Huang Bo Wang Jianguo Ye Bin Liu Huayu Qiu Shouchun Yin | 2012 | Chin J Chem2012，，8： | 1 |
| 6 | Separation of the isomer compositions of oligomethylphenyl cyclosiloxane on capillary column and determination of the isomers by GC MS显示文摘 | Jiang Kezhi Ni Yong Qiu Huayu | 2006 | Chromatographia2006，64，1112： | 1 |
| 7 | Exceptionally flame-retardant flexible polyurethane foam composites:synergistic effect of the silicone resin/graphene oxide coating显示文摘A facile strategy was developed to fabricate flexible polyurethane(PU)foam composites with exceptional flame retardancy.The approach involves the incorporation of graphene oxide(GO)into a silicone resin(SiR)solution,which is then deposited onto a PU foam surface via the dip-coating technique and cured.Fourier-transform infrared spectroscopy,scanning electron microscopy,and Raman spectroscopy measurements demonstrated that the SiR and GO were successfully coated onto the PU skeleton and the intrinsic porous structure of the PU foam remained intact.The effects of SiR and GO on the mechanical and thermal stability and flame retardancy of PU composites were evaluated through compression tests,thermogravimetric analysis,vertical combustion tests,and the limiting oxygen index.The measurement results revealed that the composites(PU@SiR-GO)showed superior flame retardancy and thermal and mechanical stability compared to pristine PU or PU coated with SiR alone.The mechanical and thermal stability and the flame-retardant properties of the PU composites were enhanced significantly with increasing GO content.Based on the composition,microstructure,and surface morphology of PU@SiR-GO composites before and after combustion tests,a possible flame-retardance mechanism is proposed.This work provides a simple and effective strategy for fabricating flame retardant composites with improved mechanical performance. | Qian Wu Jincheng Zhang Shengpeng Wang Bajin Chen Yijun Feng Yongbing Pei Yue Yan Longcheng Tang Huayu Qiu Lianbin Wu | 2021 | Frontiers of Chemical Science and Engineering2021，15，4： | 1 |
| 8 | Facile generation of highly durable thiol-functionalized polyhedral oligomeric silsesquioxane based superhydrophobic melamine foam显示文摘In this study,a durable superhydrophobic/superoleophilic melamine foam was fabricated by a facile and rapid one-step thiol-ene click chemistry and Michael addition reaction,which demonstrated excellent robustness in oil/water separation.First,1H,1H,2H-perfluoro-1-hexene reacted with thiol-functionalized polyhedral oligomeric silsesquioxane via the thiol-ene click chemistry to obtain a fluorinated thiol-functionalized polyhedral oligomeric silsesquioxane solution.Subsequently,the melamine foam was immersed to the solution system to form nanoaggregates on the melamine foam surface by the Michael addition reaction in the presence of ultraviolet light.The micro/nano rough structure and low surface energy of the nanoaggregates layer endowed the pristine melamine foam with superhydrophobicity;the water contact angle was greater than 150°.More importantly,the as-prepared melamine foam could withstand harsh conditions,such as a corrosive solution environment,strong ultraviolet light,mechanical compression,high and low temperature exposure,and ultrasonic washing.Driven by gravity,the as-prepared melamine foam could efficiently separate the oil/water mixtures and maintain 98%separation efficiency at high and low temperatures.In addition,it maintained the desirable absorption capability in different oil/organic solvents even after 15 absorption cycles.Accordingly,this facile,low-cost,and robust onestep method provides important support for the superhydrophobic oil/water separation field. | Meng Li Yuanfeng Fang Chun Liu Mengmeng Zhou Xiaomei Miao Yongbing Pei Yue Yan Wenjun Xiao Huayu Qiu Lianbin Wu | 2022 | Frontiers of Chemical Science and Engineering2022，16，8： | 0 |
| 9 | Quasi‑Solid Electrolyte Interphase Boosting Charge and Mass Transfer for Dendrite‑Free Zinc Battery显示文摘The practical applications of zinc metal batteries are plagued by the dendritic propagation of its metal anodes due to the limited transfer rate of charge and mass at the electrode/electrolyte interphase.To enhance the reversibility of Zn metal,a quasi-solid interphase composed by defective metal-organic framework(MOF)nanoparticles(D-UiO-66)and two kinds of zinc salts electrolytes is fabricated on the Zn surface served as a zinc ions reservoir.Particularly,anions in the aqueous electrolytes could be spontaneously anchored onto the Lewis acidic sites in defective MOF channels.With the synergistic effect between the MOF channels and the anchored anions,Zn^(2+)transport is prompted significantly.Simultaneously,such quasi-solid interphase boost charge and mass transfer of Zn^(2+),leading to a high zinc transference number,good ionic conductivity,and high Zn^(2+)concentration near the anode,which mitigates Zn dendrite growth obviously.Encouragingly,unprecedented average coulombic efficiency of 99.8%is achieved in the Zn||Cu cell with the proposed quasi-solid interphase.The cycling performance of D-UiO-66@Zn||MnO_(2)(~92.9%capacity retention after 2000 cycles)and D-UiO-66@Zn||NH_(4)V_(4)O_(10)(~84.0%capacity retention after 800 cycles)prove the feasibility of the quasi-solid interphase. | Xueer Xu Yifei Xu Jingtong Zhang Yu Zhong Zhongxu Li Huayu Qiu Hao Bin Wu Jie Wang Xiuli Wang Changdong Gu Jiangping Tu | 2023 | Nano-Micro Letters2023，15，4： | 0 |
| 10 | Correction to:An endotenon sheath‑inspired double‑network binder enables superior cycling performance of silicon electrodes显示文摘The original version of this article unfortunately contained some mistakes.1.The authors found that the data unit in Fig.3a–f is wrong.The corrected version of Fig.3 is given below:2.The authors found that explanation of the data lines in Fig.2e is wrong.The corrected version of the explanation of Fig.2e is given below:The DNB can endure approximately 300%stretching and withstand stress up to about 1.5 MPa,as shown in Fig.2e. | Meifang Jiang Pengzhou Mu Huanrui Zhang Tiantian Dong Ben Tang Huayu Qiu Zhou Chen Guanglei Cui | 2022 | Nano-Micro Letters2022，14，8： | 0 |
| 11 | Anti-corrosive Hybrid Electrolytes for Rechargeable Aqueous Zinc Batteries显示文摘Aqueous zinc(Zn)-metal cells with cost-effective components and high safety have long been a promising large-scale energy storage system,but Zn anodes are intrinsically unstable with common aqueous electrolytes,causing substantial underutilization of the theoretical capacity.In this work,we report a strictly neutral aqueous Zn electrolyte at a low cost by leveraging the dynamic hydrolysis equilibrium of a dual-salt Zn(Ac)2/NaAc(Ac:CH3COO−)formulation.With the pH regulation,the corrosion and hydrogen evolution encountered in Zn anodes can be suppressed significantly.This hybrid aqueous electrolyte not only enables dendrite-free Zn plating/stripping at a nearly 95%Coulombic efficiency[an increase of 24%compared to that of the single-salt 1 mol/L Zn(Ac)2 electrolyte],but also supports the reversible operation of Zn cells paired with either Na3V2(PO4)3 or iodine cathodes—the former delivers a high output voltage of 1.55 V with an energy level of 99.5 W·h/kg(based on the mass of the cathode),and the latter possesses a high specific capacity of 110.9 mA·h/g while yielding long-term cyclability(thousands of cycles).These findings open up a new avenue of modifying practical electrolytes having targeted properties to stabilize multivalent metal anodes. | WANG Jia QIU Huayu ZHAO Zhiming ZHANG Yuchen ZHAO Jingwen MA Yinglei LI Jiedong XING Min LI Guicun CUI Guanglei | 2021 | Chemical Research in Chinese Universities2021，37，2： | 0 |
| 12 | Structures and isomerization of cabenoids H_2CLiBr显示文摘ALTHOLIGH carbenoids as the active organometallic intermediates have been widely used in organic syntheses, up to now, only few simple saturated and unsaturated carbenoids, such as H2CLiF, Cl3CLi, HCLiF2 and HCCLiF, have been studied by theoretical methods. | QIU Huayu and DENG ConghaoTheoretical Chemistry Group, Shandong University, Jinan 250100, China | 1997 | Chinese Science Bulletin1997，42，3： | 0 |
| 13 | Aggregation-enhanced emission and efficient electroluminescence of conjugated polymers containing tetraphenylethene units显示文摘Tetraphenylethene(TPE)is a popular luminogen characterized by aggregation-induced emission and has been widely used to construct solid-state emissive materials.In this work,two thermally stable polymers(P1 and P2)consisting of TPE conjugated to the 2,7-positions of fluorene and carbazole,respectively,are synthesized and characterized.Both polymers are weakly fluorescent in solutions but show greatly enhanced emission as the aggregate formation,presenting an aggregation-enhanced emission feature.Two kinds of polymer light-emitting diodes are fabricated utilizing P1 and P2 as emitters(EML)(device I:ITO/PEDOT:PSS(45 nm)/PVK:EML(1:1 wt%,55nm)/TPBI(38 nm)/Ca:Ag;device II:ITO/PEDOT:PSS(45 nm)/PVK:OXD-7:EML(3:1:3 wt%,55 nm)/TPBI(38nm)/Ca:Ag).The device II of P2 shows the best performances,affording a maximum luminance of 6500 cd/m2and a high peak efficiency of 2.11 cd/A. | HE BaiRong YE ShangHui GUO YanJu CHEN Bin XU XiaoFei QIU HuaYu ZHAO ZuJin | 2013 | 中国科学:化学2013，43，9： | 0 |
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