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| 1 | Heterogeneous degradation of toxic organic pollutants by hydrophobic copper Schiff-base complex under visible irradiation显示文摘A hydrophobic complex of Cu2+[bis-salicylic aldehyde-o-phenylenediamine],Cu-SPA,was prepared and used as a heterogeneous photocatalyst to degrade organic pollutants in water under visible irradiation(420 nm)at neutral pH.The structure of complex was characterized by using nuclear magnetic resonance(NMR),elemental analysis,IR and UV-vis spectrometries.Degradation of Rhodamine B(RhB),Sulforhodamine B(SRB)and Benzoic acid(BA)in water were used as model reactions to evaluate the photocatalytic activities of Cu-SPA.The results indicated that RhB and SRB were easily adsorbed on the hydrophobic surface of Cu-SPA from aqueous solution(the maximum adsorption amount:Qmax=11.09 and 8.05μmol/g,respectively).Under visible irradiation,RhB and SRB were decolorized completely after 210 and 240 min,respectively,and BA was removed completely after 5 h.The efficiency of H2O2was>95%,in contrast to that of the reaction without catalyst or light(<20%).In water soluble medium,the hydrophobic Cu-SPA can be used more than 6 cycles.ESR results and the behavior of cyclic voltammetry showed that,in the reaction process,Cu2+-SPA was reduced to intermediate state Cu+-SPA firstly,which was extremely unstable and reacted rapidly with H2O2,leading to high reactive oxygen species(·OH radical)to degrade the substrate. | SONG Quan JIA ManKe MA WanHong FANG YanFen HUANG YingPing | 2013 | Science China Chemistry2013，56，12： | 5 |
| 2 | Photocatalytic properties of hierarchical BiOXs obtained via an ethanol-assisted solvothermal process显示文摘In this study, bismuth oxyhalide(Bi OXs(X_Cl, Br, I)) semiconductors were prepared by a simple solvothermal method, with ethanol serving as solvent and a series of tetrabutylammonium halide surfactants as halogen sources. Under identical synthetic conditions, Bi OBr was more readily constructed into regular flower-like hierarchical architectures. The photocatalytic properties of the materials were studied by monitoring the degradation of rhodamine B(Rh B),with visible light absorption, and colorless salicylic acid(SA). It was found that both Rh B and SA were rapidly degraded on the surface of Bi OBr. Bi OCl was rather active for the degradation of Rh B,but ineffective toward the degradation of SA. However, neither Rh B nor SA could be degraded effectively in the case of Bi OI. Further experiments such as UV–visible spectroscopy and detection of U OH and O2 Uradicals suggest that the electronic structure of the Bi OX photocatalysts is responsible for the difference in their activities. | Manke Jia Xiaolong Hu Shulian Wang Yingping Huang Lirong Song | 2015 | Journal of Environmental Sciences2015，27，9： | 5 |
| 3 | Synthesis of a magnetic micro/nano Fe_xO_y-CeO_2 composite and its application for degradation of hexachlorobenzene显示文摘A micrometer-sized nanostructured,magnetic,ball-like FexOy-CeO2 composite was synthesized through an ethylene-glycol mediated process.The synthesized samples were characterized by scanning electron microscopy combined with energydisperse X-ray analysis,transmission electron microscopy and X-ray powder diffraction.In the synthesis system,polyethylene glycol (PEG) and urea were found to play significant roles in the formation of the micrometer-sized spherical architecture of the precursor.The details of morphology and particle size could be changed with the initial concentration of Fe(NO3)3-9H2O and Ce(NO3)3-6H2O as the reactants.The magnetic FexOy-CeO2 composite with a similar morphology was readily obtained by calcination from the precursor.The characterization of transmission electron microscopy showed the calcined ball-like architecture was a highly porous structure consisting of many nanoparticles.Because of the micrometer-sized nanostructure and the multi-components as well as the magnetism,the as-obtained FexOy-CeO2 composite showed better activity and potentially easy recovery for the harmless degradation of hexachlorobenzene (HCB). | JIA ManKe,SU GuiJin,ZHENG MingHui,ZHANG Bing & LIN ShiJing State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences,Chinese Academy of Sciences,Beijing 100085,China | 2010 | Science China Chemistry2010，53，6： | 3 |
| 4 | 天然恒牙列的动态咬合接触形式显示文摘目的:在既往研究中.从未停止过关于修复和正畸治疗中进行咬合重建时.应该建立何种形式的咬合接触的讨论。对天然恒牙列的动态咬合的流行病学调查将有助于走出这种持续讨论的困境。本研究的目的就是要通过调查研究.总结年青群体和老年群体天然牙列的特征性动态咬合接触形式,并且分析动态咬合接触形式与性别和年龄之间的相关性。材料和方法:本研究共调查了834人。所有的调查对象都具有天然牙列.并且没有修复体存在。调查对象的年龄范围是20--63岁。在调查对象进行牙诱导的侧方和前伸运动过程中,检查天然牙的动态咬合接触形式。结果:结果发现存在以下的动态咬合接触形式:双侧和单侧的尖牙保护[牙合],组牙功能[牙合].平衡[牙合]以及“其他[牙合]型”。男性和女性之间不同类型的动态咬合接触形式的出现概率相同。但是.一些咬合接触形式的出现率与年龄有相关性。随着年龄的增加.双侧和单侧尖牙保护耠的出现率出现下降趋势,而组牙功能[牙合]的出现率上升。平衡[牙合]以及“其他[牙合]型”的出现率很低.并且没有呈现与年龄相关的变化趋势。结论:双侧尖牙保护[牙合]和组牙功能[牙合]是年青患者的特征性咬合接触形式.而老年患者中组牙功能[牙合]的接触形式更加普遍。当年青患者接受修复和正畸手段的咬合重建时.尖牙保护[牙合]是一种最适合的咬合接触形式,而对于老年患者来说.组牙功能[牙合]则更加适合。需要进一步的研究来探讨[牙合]型和牙周炎、磨牙症或者颞下颌关节紊乱病之间的关系。 | Halina Panek Teresa Matthews-Brzozowska Danuta Nowakowska Beata Panek Grzegorz Bielicki Slawomir Makacewicz Malgorzata Mank iewicz 李健(译) 姜婷(审) | 2009 | 中国口腔医学继续教育杂志2009，12，6： | 2 |
| 5 | Experimental Investigation of Runawayelectron Generation in Textor显示文摘 | Jaspers R Finken K H Mank G | 1993 | Nucl Fusion1993，，12： | 1 |
| 6 | Toe blood pressure:A valuable adjunct to ankle pressure measurement for assessing peripheral arterial disease显示文摘 | Ramsey DE Manke DA Sumner DS | 1983 | J Cardiovasc Surg1983，24，1： | 1 |
| 7 | Nurse-stuff levels and the quality of care in hospitals显示文摘 | Needleman J Ruerhaus P Manke S | 2002 | N Engl J Med2002，346，22： | 1 |
| 8 | Some chemistry in the Li/SOCl2 cell显示文摘 | Abraham K M Mank R M | 1980 | J Electrochem Soc1980，127，10： | 1 |
| 9 | Glucagon-like peptid infusion impmves left ventricular ejection fraction and functional status in patients with chronic heartfailure显示文摘 | Sokes GG Nikolaidis LA Manked S | | 0，，09： | 1 |
| 10 | In situ Raman analysis of gas formation in NiMH batteries显示文摘 | Mank a J G Belfadhel-Ayeb a Krüsemann P V E | 2005 | Applied Spectroscopy2005，59，1： | 1 |
| 11 | Self-association and chaperone activity of I-Isp27 are thermally activated 显示文摘 | Lelj-Garolla B Mank A G | 2006 | J Biol Chem2006，281，12： | 1 |
| 12 | Peptide nucleic acid fluorescence in situ hybridization-based identification of Candida albicans and its impact on mortality and antifugal therapy costs显示文摘 | Forrest G N Mankes K Jabra-Rizk M A | 2006 | J Clin Microbiol2006，44，9： | 1 |
| 13 | Two high-density AFLP? linkage maps of Zea mays L.: analysis of distribution of AFLP markers显示文摘 | M. Vuylsteke R. Mank R. Antonise E. Bastiaans M. L. Senior C. W. Stuber A. E. Melchinger T. Lübberstedt X. C. Xia P. Stam M. Zabeau M. Kuiper | 1999 | TAG Theoretical and Applied Genetics1999，，6： | 1 |
| 14 | The BTB and CNC homology 1 (BACH1) target genes are involved in the oxidative stress response and in control of the cell cycle 显示文摘 | Warnatz H J Schmidt D Manke T | 2011 | J Biol Chem2011，286，23： | 1 |
| 15 | Serial peripheral blood interleukin - 18 and pertorin fene expression measurements for prediction of acute kidney graft rejection 显示文摘 | Tania Simon Gerhard Opelz Manked Wiesel | 2004 | Transplantation2004，10，77： | 1 |
| 16 | The long and winding road leading to the successful introgression of downy mildew resistance into onion 显示文摘 | Scholten O van Heusden A Khrustaleva L Burger-Meijer K Mank R Antonise R Harrewijn J van Haecke W Oost E Peters R Kik C | 2007 | Euphytica2007，156，： | 1 |
| 17 | Development of a fast valve for mitigating disrup- tions in Tokamaks显示文摘 | SAVTCHKOV A FINKEN K H MANK G | 2002 | Review of Scientic Instru- ments2002，73，34： | 1 |
| 18 | High resolution map of eggplant ( Solanum melongena ) reveals extensive chromosome rearrangement in domesticated members of the Solanaceae显示文摘 | Sami Do?anlar Amy Frary Marie-Christine Daunay Koen Huvenaars Rolf Mank Anne Frary | 2014 | Euphytica2014，，2： | 1 |
| 19 | 2,5-DihydroxyBenzoic Acid Butylamine and Other Ionic Liquid Matrixes for Enhanced MALDI-MS Analysis of Biomolecules显示文摘 | Mank M Stahl B Boehm G | 2004 | Anal Chem2004，76，10： | 1 |
| 20 | QTL hotspots in eggplant ( Solanum melongena ) detected with a high resolution map and CIM analysis显示文摘 | Amy Frary Anne Frary Marie-Christine Daunay Koen Huvenaars Rolf Mank Sami Do?anlar | 2014 | Euphytica2014，，2： | 1 |
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