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| 1 | ZIF-8/LiFePO4 derived Fe-N-P Co-doped carbon nanotube encapsulated Fe2P nanoparticles for efficient oxygen reduction and Zn-air batteries显示文摘Iron-based oxygen reduction reaction(ORR)catalysts have been the focus of research,and iron sources play an important role for the preparation of efficient ORR catalysts.Here,we successfully use LiFePO4 as ideal sources of Fe and P to construct the heteroatom doped Fe-based carbon materials.The obtained Fe-N-P co-doped coral-like carbon nanotube arrays encapsulated Fe2P catalyst(C-ZIF/LFP)shows very high half-wave potential of 0.88 V in alkaline electrolytes toward ORR,superior to Pt/C(0.85 V),and also presents a high half-wave potential of 0.74 V in acidic electrolytes,comparable to Pt/C(0.8 V).When further applied into a home-made Zn-air battery as cathode,a peak power density of 140 mW·cm^-2 is reached,exceeds commercial Pt/C(110 mW·cm^-2).Besides,it also presents exceptional durability and methanol resistance compared with Pt/C.Noticeably,the preparation method of such a high-performance catalyst is simple and easy to optimize,suitable for the large-scale production.What’s more,it opens up a more sustainable development scenario to reduce the hazardous wastes such as LiFePO4 by directly using them for preparing high-performance ORR catalysts. | Huihui Jin Huang Zhou Pengxia Ji Chengtian Zhang Jiahuan Luo Weihao Zeng Chenxi Hu Daping He Shichun Mu | 2020 | Nano Research2020，13，3： | 8 |
| 2 | Broadband mid-infrared molecular spectroscopy based on passive coherent optical–optical modulated frequency combs显示文摘Mid-infrared dual-comb spectroscopy is of great interest owing to the strong spectroscopic features of trace gases,biological molecules,and solid matter with higher resolution,accuracy,and acquisition speed. However,the prerequisite of achieving high coherence of optical sources with the use of bulk sophisticated control systems prevents their widespread use in field applications. Here we generate a highly mutually coherent dual midinfrared comb spectrometer based on the optical–optical modulation of a continuous-wave (CW) interband or quantum cascade laser. Mutual coherence was passively achieved without post-data processes or active carrier envelope phase-locking processes. The center wavelength of the generated mid-infrared frequency combs can be flexibly tuned by adjusting the wavelength of the CW seeds. The parallel detection of multiple molecular species,including C_(2)H_(2),CH_(4),H_(2)CO,H_(2)S,COS,and H_(2)O,was achieved. This technique provides a stable and robust dual-comb spectrometer that will find nonlaboratory applications including open-path atmospheric gas sensing,industrial process monitoring,and combustion. | ZHONG ZUO CHENGLIN GU DAOWANG PENG XING ZOU YUANFENG DI LIAN ZHOU DAPING LUO YANG LIU WENXUE LI | 2021 | Photonics Research2021，9，7： | 3 |
| 3 | Tunable optical frequency comb from a compact and robust Er:fiber laser显示文摘We report on a compact and robust self-referenced optical frequency comb with a tunable repetition rate,generated by an all-polarization-maintaining(PM)mode-locked Er-doped fiber laser.The spacing between comb teeth can be tuned above 300 kHz at a repetition rate of 101 MHz.The repetition rate and the carrier-envelope offset of the laser are stabilized separately,and the relative residual phase noises are determined to be 336µrad and 713 mrad(1 Hz-1 MHz).The accurate frequency characteristics and the stable structure show great potential for the use of such a comb in applications of precision measurements. | Zhiwei Zhu Yang Liu Daping Luo Chenglin Gu Lian Zhou Gehui Xie Zejiang Deng Wenxue Li | 2020 | High Power Laser Science and Engineering2020，8，2： | 2 |
| 4 | Doppler velocimeter based on dual-comb absorption spectroscopy显示文摘The determination of airflow parameters is essential to the research of critical information on environment monitoring,chemical kinetics,and aerodynamic and propulsion applications.During the past few decades,tunable diode laser absorption spectroscopy has become a common and efficient tool for the flow velocity measurement based on the Doppler shift of the absorption line.Dual-comb absorption spectroscopy(DCAS),as a state-of-theart Fourier-transform broadband spectroscopic technique,not only can detect multiple trace molecules in parallel but also can extract Doppler shifts to derive the flow velocity through the analysis of dozens of molecular absorption lines simultaneously with high precision.Here,we report a proof-of-principle demonstration of the velocity measurements of acetylene at various flow velocities by means of a high-resolution and broadband DCAS.Mode-resolved Doppler-shifted rotational-vibrational lines in the P branch of acetylene molecules are obtained.A model for multiline Doppler frequency determination is investigated and experimentally verified.The flow velocity measurements with a measuring uncertainty down to the submeter per second over the range from 8.7 m/s to 44.8 m/s at an effective time resolution of 1 s and a measuring uncertainty of 1.97 m/s at 0.1 s are demonstrated.With broadband mid-infrared frequency combs covering atmospheric transmission windows,the open-path measurement for monitoring diffusion of the weak pollutant source would be realized. | CHENGLIN GU XING ZOU ZHONG ZUO DAOWANG PENG YUANFENG DI YANG LIU DAPING LUO WENXUE LI | 2020 | Photonics Research2020，8，12： | 2 |
| 5 | Optimizing noise characteristics of mode-locked Yb-doped fiber laser using gain-induced RIN-transfer dynamics显示文摘Gain-parameter-dependent transfer functions and phase-noise performances in a mode-locked Yb-doped fiber laser are measured in this study.It is discovered that the corner frequency in the amplitude and phase domains is determined by the absorption coefficient of the gain fiber,when the total absorption and other cavity parameters are fixed.This shows that an oscillator using gain fiber with higher dopant concentration accumulates more phase noise.Furthermore,we present net cavity dispersion-dependent transfer functions to verify the effect of dispersion management on the frequency response.We derive a guideline for optimizing mode-locked fiber laser design to achieve low phase noise and timing jitter. | Jiangshuoxue Han Yang Liu Zejiang Deng Gehui Xie Daping Luo Chenglin Gu Lian Zhou Wenxue Li | 2021 | High Power Laser Science and Engineering2021，9，3： | 1 |
| 6 | Mid-infrared optical frequency comb in the 2.7-4.0μm range via difference frequency generation from a compact laser system显示文摘We report on the generation of a mid-infrared(mid-IR)frequency comb with a maximum average output power of250 mW and tunability in the 2.7-4.0μm region.The approach is based on a single-stage difference frequency generation(DFG)starting from a compact Yb-doped fiber laser system.The repetition rate of the near-infrared(NIR)comb is locked at 75 MHz.The phase noise of the repetition rate in the offset-free mid-IR comb system is measured and analyzed.Except for the intrinsic of NIR comb,environmental noise at low frequency and quantum noise at high frequency from the amplifier chain and nonlinear spectral broadening are the main noise sources of broadening the linewidth of comb teeth,which limits the precision of mid-IR dual-comb spectroscopy. | Lian Zhou Yang Liu Gehui Xie Chenglin Gu Zejiang Deng Zhiwei Zhu Cheng Ouyang Zhong Zuo Daping Luo Bin Wu Kunfeng Chen Wenxue Li | 2020 | High Power Laser Science and Engineering2020，8，4： | 1 |
| 7 | Dual-comb spectroscopy from the ultraviolet to mid-infrared region based on high-order harmonic generation显示文摘Dual-comb spectroscopy(DCS)has revolutionized numerous spectroscopic applications due to its high spectral resolution and fast measurement speed.Substantial efforts have been made to obtain a coherent dual-comb source at various spectral regions through nonlinear frequency conversion,where the preservation of coherence has become a problem of great importance.In this study,we report the generation of coherent dual-comb sources covering from the ultraviolet to mid-infrared region based on high-order harmonic generation.Driven by high-repetition-rate femtosecond mid-infrared dual-comb pump pulses,up to ninth-order harmonic was generated from the ultraviolet to mid-infrared region using an aperiodically poled lithium niobate waveguide.To investigate the coherence property of the high-order harmonic generation,DCS was performed at every generated spectral region from 450 to 3600 nm.The measured dual-comb spectra with distinctive tooth-resolved structures show the well-preserved coherence without apparent degradation after the cascaded quadratic nonlinear processes.The subsequent methane absorption spectroscopy at multiple spectral regions of different harmonics was carried out to characterize the spectroscopic capability of the system.These results demonstrate the potential of our scheme to generate compact and coherent broadband optical frequency combs for simultaneous multi-target detections. | YUANFENG DI ZHONG ZUO DAOWANG PENG DAPING LUO CHENGLIN GU WENXUE LI | 2023 | Photonics Research2023，11，8： | 0 |
| 8 | Tunable compact asynchronous optical sampling system using Er-doped fiber laser显示文摘We report a compact,tunable,self-starting,all-fiber laser-based asynchronous optical sampling(ASOPS)system.Two Er-doped fiber oscillators were used as the pulsed-laser source,whose repetition rate could be set at 100 MHz with a tuning range of 1.25 MHz through a fiber delay line.By employing phase-locked and temperature control loops,the repetition rate offset of the two lasers was stabilized with 7.13×10^(−11)fractional instability at an average time of 1 s.Its capabilities in the terahertz regime were demonstrated by terahertz time-domain spectroscopy,achieving a spectral bandwidth of 3 THz with a dynamic range of 30 dB.The large range of repetition rate adjustment in our ASOPS system has the potential to be a powerful tool in the terahertz regime. | Zilin Zhao Daping Luo Yang Liu Zejiang Deng Lian Zhou Gehui Xie Chenglin Gu Yanzhao Yang BinWu Wenxue Li | 2023 | High Power Laser Science and Engineering2023，11，2： | 0 |
| 9 | Shear mechanical properties and energy evolution of rock-like samples containing multiple combinations of non-persistent joints显示文摘Discontinuities are often considered as important factors responsible for the instability caused by shear failure in engineering rock mass,and energy-driven instability is the root cause of rock failure.However,few studies focus on the energy evolution during the failure process using a three-dimensional(3D)numerical model.In this study,a series of laboratory direct shear tests on rock-like samples is numer-ically simulated using bonded particle models(BPMs)with multiple combinations of discontinuous in the particle flow code(PFC3D),in which the location and size of the particles conform to the uniform distribution.The effects of joint row number and inclination on the stress-strain characteristics and failure mode of rock were studied from the perspective of microcrack growth and energy evolution.The results showed that,when the number of joint rows Nr>1,the shear failure region does not change with the increase of Nr for the type B(2-columnn multiple-row at center)and the type C(2-column multiple-row at edge)as compared to the type A(1-column multiple-row at center)joint models.Notably,joints significantly increase the post-peak energy dissipation but have little effect on the proportion of energy before the peak.Friction consumes most of the energy while kinetic energy accounts for less than 1%of total energy during the shear process.Peak elastic strain energy follows the variation trend of peak shear displacement.The development and accumulation of microcracks directly affect the energy dissipation,and there is a significant linear relationship between the cumulative number of critical microcracks and the critical dissipated energy at the failure,when the dip direction of joints is opposite to the shear direction,more microcracks will be accumulated at the peak time,resulting in more energy dissipation.The results contribute to deeply understanding the shear failure process of non-persistent jointed mass. | Daping Tai Shengwen Qi Bowen Zheng Chonglang Wang Songfeng Guo Guangming Luo | 2023 | Journal of Rock Mechanics and Geotechnical Engineering2023，15，7： | 0 |
| 10 | Decellularized Extracellular Matrix Containing Electrospun Fibers for Nerve Regeneration:A Comparison Between Core–Shell Structured and Preblended Composites显示文摘Advanced biomaterial-based strategies for treatment of peripheral nerve injury require precise control over both topological and biological cues for facilitating rapid and directed nerve regeneration.As a highly bioactive and tissue-specifc natural material,decellularized extracellular matrix(dECM)derived from peripheral nerves(decellularized nerve matrix,DNM)has drawn increasing attention in the feld of regenerative medicine,due to its outstanding capabilities in facilitating neurite outgrowth and remyelination.To induce and maintain sufcient topological guidance,electrospinning was conducted for fabrication of axially aligned nanofbers consisting of DNM and poly(ε-caprolactone)(PCL).Core–shell structured fbers were prepared by coaxial electrospinning using DNM as the shell and PCL as the core.Compared to the aligned electrospun fbers using preblended DNM/PCL,the core–shell structured fbers exhibited lower tensile strength,faster degradation,but considerable toughness for nerve guidance conduit preparation and relatively intact fbrous structure after long-term degradation.More importantly,the full DNM surface coverage of the aligned core–shell fbers efectively promoted axonal extension and Schwann cells migration.The DNM contents further triggered neurite bundling and myelin formation toward nerve fber maturation and functionalization.Herein,we not only pursue a multi-functional scafold design for nerve regeneration,a detailed comparison between core–shell structured and preblended electrospinning of DNM/PCL composites was also provided as an applicable paradigm for advanced tissue-engineered strategies using dECM-based biomaterials. | Rongli Deng Ziling Luo Zilong Rao Zudong Lin Shihao Chen Jing Zhou Qingtang Zhu Xiaolin Liu Ying Bai Daping Quan | 2022 | Advanced Fiber Materials2022，4，3： | 0 |
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