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| 1 | Experimental and mechanism studies on seawater flue gas desulfurization显示文摘Seawater flue gas desulfurization (Seawater FGD) process has a number of advantages, but the study on mechanism of seawater FGD is little. The effects of absorbing efficiency of SO 2 by the constant component and part of trace transition elements in seawater are studied by the experiment. The results indicate that the effect factors of absorption of SO 2 by seawater are alkaline, ion intensity, catalysis of Cl - and transition metal ions Fe 2+ , Mn 2+ . The degree of effect is alkaline > the catalysis of Cl -, Fe 2+ and Mn 2+ >ion intensity. The mechanisms of catalysis oxidation for S(IV) by Cl -, Fe 2+ and Mn 2+ are discussed. According to the results, some measures can be used to improve the capability of desulfurization. | ZHAOYi WANGXiao-ming 等 | 2003 | Journal of Environmental Sciences2003，15，1： | 17 |
| 2 | Machine learning guided appraisal and exploration of phase design for high entropy alloys显示文摘High entropy alloys(HEAs)and compositionally complex alloys(CCAs)have recently attracted great research interest because of their remarkable mechanical and physical properties.Although many useful HEAs or CCAs were reported,the rules of phase design,if there are any,which could guide alloy screening are still an open issue.In this work,we made a critical appraisal of the existing design rules commonly used by the academic community with different machine learning(ML)algorithms.Based on the artificial neural network algorithm,we were able to derive and extract a sensitivity matrix from the ML modeling,which enabled the quantitative assessment of how to tune a design parameter for the formation of a certain phase,such as solid solution,intermetallic,or amorphous phase.Furthermore,we explored the use of an extended set of new design parameters,which had not been considered before,for phase design in HEAs or CCAs with the ML modeling.To verify our ML-guided design rule,we performed various experiments and designed a series of alloys out of the Fe-Cr-Ni-Zr-Cu system.The outcomes of our experiments agree reasonably well with our predictions,which suggests that the ML-based techniques could be a useful tool in the future design of HEAs or CCAs. | Ziqing Zhou Yeju Zhou Quanfeng He Zhaoyi Ding Fucheng Li Yong Yang | 2019 | npj Computational Materials2019，，1： | 16 |
| 3 | Experimental study on the simultaneous desulfurization and denitrification by duct injection显示文摘The highly active absorbent with oxidization based on fly ash, lime and additive was prepared. Experiments of simultaneous desulfurization and denitrification were carried out using fixture bed and duct injection. The influencial factors for the absorptive capacity of the absorbent were studied. The absorptive capacities of 120.7 mg for SO 2 and 43.7 mg for NOx were achieved at a Ca/(S+N) molar ratio 1.2, respectively, corresponding removal efficiencies of 87% and 76%, while spent absorbent appeared in the form of dry powder. The optimal temperature and humidity of flue gas treated with this process were shown to be approximately 50℃, and 5% respectively. The mechanism of removal for SO 2 and NOx was investigated. In comparison with traditional dry FGD, this process appears to have lower cost, less complicated configuration and simpler disposal of used absorbent. The valuable references can be provided for industrial application by this process. The foreground of application will be vast in China and in the world. | ZHAOYi FUYan-chun MAShuang-chen HUANGJian-jun | 2004 | Journal of Environmental Sciences2004，16，4： | 9 |
| 4 | Conversion of confined metal@ZIF-8 structures to intermetallic nanoparticles supported on nitrogen-doped carbon for electrocatalysis显示文摘 | Zhiyuan Qi Yuchen Pei Tian Wei Goh Zhaoyi Wang Xinle Li Mary Lowe Raghu V. Maligal-Ganesh Wenyu Huang | 2018 | Nano Research2018，11，6： | 6 |
| 5 | Quantitative study of protein coronas on gold nano- particles with different surface modifications显示文摘 | Menghua Cui Renxiao Liu Zhaoyi Deng Guanglu Ge Ying Liu Liming Xie | 2014 | Nano Research2014，7，3： | 6 |
| 6 | Optical conductivity-based ultrasensitive mid-infrared biosensing on a hybrid metasurface显示文摘Optical devices are highly attractive for biosensing as they can not only enable quantitative measurements of analytes but also provide information on molecular structures.Unfortunately,typical refractive index-based optical sensors do not have sufficient sensitivity to probe the binding of low-molecular-weight analytes.Non-optical devices such as field-effect transistors can be more sensitive but do not offer some of the significant features of optical devices,particularly molecular fingerprinting.We present optical conductivity-based mid-infrared(mid-IR)biosensors that allow for sensitive and quantitative measurements of low-molecular-weight analytes as well as the enhancement of spectral fingerprints.The sensors employ a hybrid metasurface consisting of monolayer graphene and metallic nano-antennas and combine individual advantages of plasmonic,electronic and spectroscopic approaches.First,the hybrid metasurface sensors can optically detect target molecule-induced carrier doping to graphene,allowing highly sensitive detection of low-molecular-weight analytes despite their small sizes.Second,the resonance shifts caused by changes in graphene optical conductivity is a well-defined function of graphene carrier density,thereby allowing for quantification of the binding of molecules.Third,the sensor performance is highly stable and consistent thanks to its insensitivity to graphene carrier mobility degradation.Finally,the sensors can also act as substrates for surfaceenhanced infrared spectroscopy.We demonstrated the measurement of monolayers of sub-nanometer-sized molecules or particles and affinity binding-based quantitative detection of glucose down to 200 pM(36 pg/mL).We also demonstrated enhanced fingerprinting of minute quantities of glucose and polymer molecules. | Yibo Zhu Zhaoyi Li Zhuang Hao Christopher DiMarco Panita Maturavongsadit Yufeng Hao Ming Lu Aaron Stein Qian Wang James Hone Nanfang Yu Qiao Lin | 2018 | Light(Science & Applications)2018，7，1： | 6 |
| 7 | Numerical study and prediction of nuclear contaminant transport from Fukushima Daiichi nuclear power plant in the North Pacific Ocean显示文摘On March 11,2011,a large earthquake and subsequent tsunami near the east coast of Japan destroyed the Fukushima Daiichi nuclear power plant(FD-NPP),causing a massive release of nuclear contaminants.In this paper,a Pacific basin-wide physical dispersion model is developed and used to investigate the transport of nuclear contaminants.The Pacific circulation model,based on the Regional Ocean Modeling System(ROMS),is forced with air-sea flux climatology derived from COADS(the Comprehensive Ocean-Atmosphere Data Set).It is shown that ocean current dominates nuclear contaminant transport.Following the Kuroshio Extension and North Pacific Current,nuclear contaminants at the surface will move eastward in the Pacific as far as 140°W,thereafter dividing into two branches.For the south branch,nuclear contaminants will be transported westward by the equatorial current,and can reach the Philippines after 10 years' time.In contrast,the north branch will arrive at the American west coast and then migrate to the Bering Sea.At 200 m water depth,part of the nuclear materials will move southwestward along with deep ocean circulation,which could potentially reach the east coast of Taiwan.The other part will move to the west coast of America and separate into two branches.One will move northward along the west coast of Alaska,while the other will travel southward to the Hawaiian Islands.The transport of radiation contaminants below 500 m is slow,and will primarily remain in the central Pacific.The physical dispersion model results show that high concentrations of the radioactive isotope cesium-137(137 Cs) will move eastward and reach the central Pacific and west coast of North America in two and eight years,respectively.The sea areas influenced by the nuclear contaminants continue to expand,while peak concentrations decrease in the North Pacific. | WANG Hui WANG ZhaoYi ZHU XueMing WANG DaKui LIU GuiMei | 2012 | Chinese Science Bulletin2012，57，26： | 6 |
| 8 | Ecotoxicological effect of zinc oxide nanoparticles on soil microorganisms显示文摘最近的年里的锌氧化物 nanoparticles (ZnO-NPs ) 的普遍生产和使用形成了潜在的威胁到生态系统。这研究试图用实验室缩影测试在土壤微生物上调查 ZnO-NPs 的 ecotoxicological 效果。呼吸,加氨,脱氢酶(DH ) 活动,并且荧光灯 diacetate hydrolase (FDAH ) 活动被用作 ecotoxicological 参数。结果在每 g 土壤与 1 mg ZnO-NPs 对待的中立土壤显示出那(新鲜,中立) ,加氨显著地在三的学习时期期间被禁止月,而是抑制率在增加时间上减少了。在呼吸的抑制在测试的第一个月内被观察。在各种各样的 ZnO-NPs 治疗(1 mg, 5 mg,和每 g 土壤的 10 mg ZnO-NPs ) , DH 活动和 FDAH 活动在一个月的学习经期期间被禁止。为两项酶活动,在 ZnO-NPs 和抑制率的集中之间有积极 doseresponse 关系,但是曲线由于 ZnO-NPs 毒性的变化随着时间的过去变化了。土壤类型在土壤影响了 ZnONPs 的毒性。毒性在酸土壤是最高的,由中立土壤列在后面。毒性在碱的土壤是相对低的。毒性没被说明因为由 Zn 2+ 免除了 ZnO-NPs。有生物学的目标的 ZnO-NPs 的直接相互作用可能是原因之一。在中立、酸的土壤的土壤微生物上的 ZnO-NPs 的不利效果值得注意。 | Zhaoyi SHEN Zhuo CHEN Zhen HOU Tingting LI Xiaoxia LU | 2015 | Frontiers of Environmental Science & Engineering2015，9，5： | 5 |
| 9 | Soil erosion assessment by RUSLE with improved P factor and its validation:Case study on mountainous and hilly areas of Hubei Province,China显示文摘The Revised Universal Soil Loss Equation(RUSLE)is widely used to estimate regional soil erosion.However,quantitative impacts of soil and water conservation(SWC)measures on conservation practice factor(P)of the RUSLE remain largely unclear,especially for the mountainous and hilly areas.In this study,we improved the RUSLE by considering quantitative impacts of different SWC measures on the P factor value.The improved RUSLE was validated against the long-term(2000-2015)soil erosion monitoring data obtained from 96 runoff plots(15—35°)in mountainous and hilly areas of Hubei Province,China;the result presented a high accuracy with the determination coefficient of 0.89.Based on the erosion monitoring data of 2018 and 2019,the Root Mean Square Error of the result by the improved RUSLE was 28.0%smaller than that by the original RUSLE with decrement of 19.6%—24.0%in the average P factor values,indicating that the soil erosion modelling accuracy was significantly enhanced by the improved RUSLE.Relatively low P factor values appeared for farmlands with tillage measures(P<0.53),grasslands with engineering measures(P<0.23),woodlands with biological measures(P<0.28),and other land use types with biological measures(P<0.51).The soil erosion modulus showed a downward trend with the corresponding values of 1681.21,1673.14,1594.70,1482.40 and 1437.50 t km^(-2)a-1 in 2000,2005,2010,2015 and 2019,respectively.The applicability of the improved RUSLE was verified by the measurements in typical mountainous and hilly areas of Hubei Province,China,and arrangements of SWC measures of this area were proposed. | Pei Tian Zhanliang Zhu Qimeng Yue Yi He Zhaoyi Zhang Fanghua Hao Wenzhao Guo Lin Chen Muxing Liu | 2021 | International Soil and Water Conservation Research2021，9，3： | 4 |
| 10 | Single copper sites dispersed on hierarchically porous carbon for improving oxygen reduction reaction towards zinc-air battery显示文摘The demand for high-performance non-precious-metal electrocatalysts to replace the noble metal-based catalysts for oxygen reduction reaction(ORR)is intensively increasing.Herein,single-atomic copper sites supported on N-doped three-dimensional hierarchically porous carbon catalyst(Cu_(1)/NC)was prepared by coordination pyrolysis strategy.Remarkably,the Cu_(1)/NC-900 catalyst not only exhibits excellent ORR performance with a half-wave potential of 0.894 V(vs.RHE)in alkaline media,outperforming those of commercial Pt/C(0.851 V)and Cu nanoparticles anchored on N-doped porous carbon(CuNPs/NC-900),but also demonstrates high stability and methanol tolerance.Moreover,the Cu_(1)/NC-900 based Zn-air battery exhibits higher power density,rechargeability and cyclic stability than the one based on Pt/C.Both experimental and theoretical investigations demonstrated that the excellent performance of the as-obtained Cu_(1)/NC-900 could be attributed to the synergistic effect between copper coordinated by three N atoms active sites and the neighbouring carbon defect,resulting in elevated Cu d-band centers of Cu atoms and facilitating intermediate desorption for ORR process.This study may lead towards the development of highly efficient non-noble metal catalysts for applications in electrochemical energy conversion. | Wenjie Wu Yan Liu Dong Liu Wenxing Chen Zhaoyi Song Ximin Wang Yamin Zheng Ning Lu Chunxia Wang Junjie Mao Yadong Li | 2021 | Nano Research2021，14，4： | 4 |
| 11 | THEATMENT OF WASTEWATER FROM PRODUCTION PROCESS OF 2,3-ACID显示文摘Wastewater from production process of 2,3-acid was treated by adsorption usingmacroporous resin NDA-708. After only one-step treatment by resin adsorption, removalefficiency of three kinds of naphthalene chemicals was above 99%, removal efficiency ofCODcr was above 96% Under proper operating condition, desorption efficiency wasaround 100%. The running records of the industrial facility showed that the naphthlenechemicals in desorption effluent could be reused without obvious influence on the qualityOf the product. | FENG Wenguo ZHANG Quanxing CHEN Jinlong XU Zhaoyi PAN Bingcai SU Xing(Dept. of Environ. Sci. & Techn., Nanjing Univ ersity Nanjing 210093, ChinaDitong Chemical Corporation, Suzhou, 215124) | 1999 | Chinese Journal of Reactive Polymers1999，8，1： | 4 |
| 12 | Solvent engineering towards scalable fabrication of high-quality perovskite films for efficient solar modules显示文摘Over the last decade,remarkable progress has been made in metal halide perovskite solar cells(PSCs),which have been a focus of emerging photovoltaic techniques and show great potential for commercialization.However,the upscaling of small-area PSCs to large-area solar modules to meet the demands of practical applications remains a significant challenge.The scalable production of high-quality perovskite films by a simple,reproducible process is crucial for resolving this issue.Furthermore,the crystallization behavior in the solution-processed fabrication of perovskite films can be strongly influenced by the physicochemical properties of the precursor inks,which are significantly affected by the employed solvents and their interactions with the solutes.Thus,a comprehensive understanding of solvent engineering for fabricating perovskite films over large areas is urgently required.In this paper,we first analyze the role of solvents in the solution-processed fabrication of large-area perovskite films based on the classical crystal nucleation and growth mechanism.Recent efforts in solvent engineering to improve the quality of perovskite films for solar modules are discussed.Finally,the basic principles and future challenges of solvent system design for scalable fabrication of high-quality perovskite films for efficient solar modules are proposed. | Zhaoyi Jiang Binkai Wang Wenjun Zhang Zhichun Yang Mengjie Li Fumeng Ren Tahir Imran Zhenxing Sun Shasha Zhang Yiqiang Zhang Zhiguo Zhao Zonghao Liu Wei Chen | 2023 | Journal of Energy Chemistry2023，，5： | 4 |
| 13 | Exploring the design of eutectic or near-eutectic multicomponent alloys: From binary to high entropy alloys显示文摘Eutectic and near-eutectic high entropy alloys(HEAs) have recently attracted a great deal of interest because of their promising properties, such as an excellent castability and unique combination of good ductility and high strength. However, in the absence of a phase diagram, it remains a non-trivial task to find a eutectic or near-eutectic composition for a HE A system, which usually demands a tremendous amount of efforts if a trial-and-error approach is followed. In this paper, we briefly review the thermodynamics that governs the eutectic solidification in regular binary and ternary alloys, and proceed to the discussion for the design of eutectic HEAs. Based on the data reported, we then propose an improved strategy which may enable an efficient search for the eutectic or near eutectic HEA compositions. | ding zhaoyi he quanfeng yang yong | 2018 | Science China(Technological Sciences)2018，61，2： | 4 |
| 14 | Effect of inhibitors on macroscopical oxidation kinetics of calcium sulfite显示文摘In the presence of inhibitors, the macroscopical oxidation kinetics of calcium sulfite, the main byproduct in wet limestone scrubbing, was studied for the first time by adding different inhibitors and varying pH, concentration of calcium sulfite, oxygen partial pressure, concentration of inhibitors and temperature. The mathematical model about the general oxidation reaction was established, which was controlled by three steps involving dissolution of calcium sulfite, mass transfer of oxygen and chemical reaction in the solution. It was concluded that the general reaction was controlled by mass transfer of oxygen under uncatalyzed conditions, while it was controlled by dissolution of calcium sulfite after adding three kinds of inhibitors. Thus, the theory was provided for investigating the mechanism and oxidation kinetics of sulfite. The beneficial references were also supplied for design of oxidation technics in the wet limestone scrubbing. | ZHAOYi WANGLi-dong WANGXiao-ming LIQiang-wei XUPei-yao | 2005 | Journal of Environmental Sciences2005，17，3： | 3 |
| 15 | Numerical modeling of radionuclide migration in porous media with nonequilibrium sorption显示文摘Numericalmodelingofradionuclidemigrationinporousmediawithnonequilibriumsorption￥ChenJiajun;DaiJie(DepartmentofEnvironmentalEn... | Chen Jiajun Dai Jie(Department of Environmental Engineering,Tsinghua University,Beijing 100084,China)(Tianjin Institute of Geological Investigation and Research,Tianjin 300191,China)Xu Zhaoyi Tian Kaiming(Changchun University of Earth Sciences,Changchun 1 | 1996 | Journal of Environmental Sciences1996，8，1： | 3 |
| 16 | Hydrogel-based flexible materials for diabetes diagnosis,treatment,and management显示文摘Diabetes is a chronic metabolic disease characterized by high glucose concentration in blood.Conventional management of diabetes requires skin pricking and subcutaneous injection,causing physical pain and physiological issues to diabetic individuals.Hydrogels possess unique advantages such as lightweight,stretchability,biocompatibility,and biodegradability,offering the opportunities to be integrated as flexible devices for diabetes management.This review highlights the development of hydrogels as flexible materials for diabetes applications in glucose monitoring,insulin delivery,wound care,and cell transplantation in recent years.Challenges and prospects in the development of hydrogel-based flexible devices for personalized management of diabetes are discussed as well. | Jiang Song Yanni Zhang Siew Yin Chan Zhaoyi Du Yinjia Yan Tengjiao Wang Peng Li Wei Huang | 2021 | npj Flexible Electronics2021，5，1： | 2 |
| 17 | Intense single-band red upconversion emission in BiOCl:Er3+ layered semiconductor via co-doping Ho3+显示文摘Exploring a new tuning way to facilely realize single-band red emission in trivalent rare-earth ions(RE3+) doped upconversion(UC) materials is still desirable.In this work,the intense single-band red emission is achieved by co-doping only Ho3+in the BiOCl:Er3+ under 1550 nm excitation.In the BiOCl layered host,co-doping Ho3+can further enhance the red emission and simultaneously suppress the green emission of Er3+,and thus obviously improve the red-to-green(R/G) ratio.It is found that Ho3+does not se rve as ene rgy trapping through the 5 I6 state as in traditional UC materials but acts as ET bridge(4 S3/2,2 H11/2(Er3+)→5 F4,5 S2(Ho3+)→4 F9/2(Er3+)).The tuning mechanism of Ho3+is discussed in detail and further confirms through a comparative experiment.Our research gives an unusual perspective to tune the UC behavior of Er3+through co-doping Ho3+,which might be inspiring for achievement of single-band red UC emission. | Yuehong Peng Jincai Peng Jiajun Han Tianhui Wang Zhaoyi Yin Jianbei Qiu Qi W ang Zhengwen Yang Zhiguo Song | 2020 | Journal of Rare Earths2020，38，6： | 2 |
| 18 | 基于中国全球海洋预报系统(CGOFS)的全球高分辨率再分析产品评估显示文摘通过同化系统将观测资料与海洋数值模式融合得到的海洋再分析产品为海洋科学研究提供了重要的资料基础.本文采用WOA,SODA,AVISO和GLORS四种数据资料与我国自主研发的中国全球海洋预报系统(CGOFS)的气候态结果进行了对比,结果表明:CGOFS和SODA的全球海表面温度与WOA的均方根误差分别为0.51和0.43℃.CGOFS和SODA的海表面盐度与WOA的均方根误差分别为0.48和0.40 PSU;海流方面,CGOFS能较好的刻画主要大洋环流分布及赤道潜流的垂向结构;CGOFS的全球海表面高度异常与AVISO的均方根误差为0.018m;多年月平均海冰外缘线覆盖面积介于SODA和GLORS之间,海冰体积的生消规律与SODA和GLORS一致.总体来看,CGOFS全球高分辨率海洋再分析产品的气候态结果与国际同类产品基本一致,可为提升我国海洋综合科技实力提供可靠的资料保障. | Zhijie Li Zhaoyi Wang Yun Li Yu Zhang Jingjing Zheng Shan Gao | 2021 | Atmospheric and Oceanic Science Letters2021，14，5： | 2 |
| 19 | Finite element analysis of field pattern in multiple groove guide 显示文摘 | Lu Mai Lu Zhaoyi | 2002 | International Journal of Infrared and Millimeter Waves2002，23，12： | 2 |
| 20 | Application of SO4^2-TiO2 solid super acid in decontaminating radioactive pollutants 显示文摘 | Yin Hongling Tan Zhaoyi Liao Yantai | 2006 | Journal of Environmental Radioactivity2006，87，： | 1 |
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