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| 1 | Microbial diversity in cold seep sediments from the northern South China Sea显示文摘华南海(SCS ) 是最大的西方的和平的边缘的海。然而,微生物引起的研究从来没在寒冷被执行过渗出在 SCS 的沉积。在 2004, SONNE 177 巡航发现二冷渗出有在北 SCS 的不同的水深度的区域。在水深度在 3000 m 附近的地方, Haiyang 4 区域已经为在 seafloor 上的活跃渗出被证实了,例如微生物引起的地席, authigenic 碳酸盐外壳和瓣鳃类。我们在从这感冒收集的一个 5.55-m 沉积核心调查了微生物引起的丰富和差异渗出区域。一条综合途径包括地球化学和 16S rRNA 基因被采用种系发生的分析。这里,我们证明与沉积核心的地球化学侧面一起的微生物引起的丰富和差异揭示了在硫酸盐减小和甲烷氧化之间的 a coupled 反应。直接计数结果显示出的氮蒽橘子那微生物引起的丰富从 105 ~ 106 cells/g 沉积(湿重量)。丰富的深度相关的变化显示出象甲烷集中侧面的一样的趋势。种系发生的分析显示了减少硫酸盐的细菌和厌氧的氧化甲烷的 archaea 的存在。差异在表面是高得多的,但是处于沉积的 geochemical 条件响应变化与深度严厉地减少了,例如甲烷,硫酸盐集中和全部的器官的碳。海洋的 Benthic 组 B, Chloroflexi 和 JS1 分别地是 archaeal 和细菌的图书馆的占优势的 phylotypes。 | Yong Zhang Xin Su Fang Chen Yuanyuan Wang Lu Jiao Hailiang Dong Yongyang Huang Hongchen Jiang | 2012 | Geoscience Frontiers2012，3，3： | 9 |
| 2 | Room temperature phosphorescence from natural products: Crystallization matters显示文摘Efficient room temperature phosphorescence is observed in natural compounds and polymers such as starch, cellulose, bovine serum albumin (BSA), and some other carbohydrates. Whereas being practically nonluminescent in solutions and TLC plates, they emit bright phosphorescence in the crystalline states with lifetime up to microseconds, exhibiting crystallization-induced phosphorescence (CIP) characteristics. The CIP of these natural products without any conventional chromophores offers a new platform for the exploration of conceptually novel luminogens. | GONG YongYang TAN YeQiang MEI Ju ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG Ben Zhong | 2013 | Science China Chemistry2013，56，9： | 8 |
| 3 | Crystallization-induced phosphorescence of benzils at room temperature显示文摘Efficient room temperature phosphorescence (RTP) is rarely observed in pure organic luminogens. However, we have newly observed that benzil and its derivatives are nonluminescent in solvents and thin layer chromatography (TLC) plates, but become highly phosphorescent in crystal state at room temperature, exhibiting typical crystallization-induced phosphorescence (CIP) characteristics. The CIP phenomenon is ascribed to the restriction of intramolecular rotations in crystals owing to effective intermolecular interactions. Such intermolecular interactions greatly rigidify the molecular conformation and significantly decrease the nonradiative deactivation channels of the triplet excitons, thus giving boosted phosphorescent emission at room temperature. | GONG YongYang TAN YeQiang LI Hong ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG Ben Zhong | 2013 | Science China Chemistry2013，56，9： | 6 |
| 4 | Interacting effects of multiple factors on the morphological evolution of the meandering reaches downstream the Three Gorges Dam显示文摘阐明河的过程上的水坝的影响能通知河保护和盆管理。然而,相对,很少研究集中了多重因素怎么交往影响蜿蜒地流的活动范围的词法进化。用水文学和地形学的数据,我们分析了下游地影响并且调整蜿蜒地流的活动范围的因素三个峡水坝(TGD ) 。我们的结论如下。(1 ) 蜿蜒地流的活动范围能在预先建水坝时期期间基于他们的进化被分类进二种类型:G1 活动范围,由侵蚀和凹面隧道免职(CECD ) ,和 G2 到达的凸的点酒吧描绘了,由凸的点酒吧免职和凹面隧道侵蚀(CDCE ) 描绘了。两种活动范围类型在水坝以后的时期期间展出了 CECD 特征。(2 ) 流动过程和沉积运输是引起了位于凸的点酒吧的低沙滩的严肃的侵蚀的因素。然而,在河政体,河边界和东廷·莱克的 jacking 的变化不对蜿蜒地流的活动范围的词法进化作为主要控制起作用。(3 ) 充满在凸的点酒吧的更大的侵蚀从 20,000 ~ 25,000 m 3/s 结果的分泌物。如果这些流动的持续时间,接近满满的分泌物,超过 20 天,点酒吧变得搜索。另外,在水流带来的碎石的减小引起在 water-falling 时期点酒吧 siltation 减少。(4 ) 在水坝以后的经期,洪水消退,分泌物从 20,000 ~ 25,000 m 3/s,的增加的持续时间和在沉积的重要减小期间,运输是引起了蜿蜒地流的活动范围显示出 CECD 特征的主要因素。在他们能通知估计河床变化,河管理策略和河保护的地方,我们的结果与另外的蜿蜒地流的活动范围相关。 | HAN Jianqiao ZHANG Wei FAN Yongyang YU Mengqing | 2017 | Journal of Geographical Sciences2017，27，10： | 3 |
| 5 | Channel evolution under changing hydrological regimes in anabranching reaches downstream of the Three Gorges Dam显示文摘 | Jianqiao HAN Wei ZHANG Jing YUAN Yongyang FAN | 2018 | Frontiers of Earth Science2018，12，3： | 2 |
| 6 | A gelable pure organic luminogen with fluorescence-phosphorescence dual emission显示文摘Pure organic luminogens with room temperature phosphorescence(RTP) have drawn much attention due to their fundamental importance and promising applications in optoelectronic devices, bioimaging, sensing, etc. Fluorescence-phosphorescence dual emission at room temperature, however, is rarely observed in pure organic materials. Herein, we reported a metal-and heavy-atom free pure organic luminogen with tert-butyl groups, DtBuCZBP, which is ready to form organogels in dimethylsulfoxide(DMSO).It emits prompt and delayed fluorescence, as well as RTP, namely dual emission in as-prepared solid, gels and polymeric films.To the best of our knowledge, it is the first example of metal-and heavy-atom free pure organic gelator with RTP emission. Such unique RTP and moreover dual emission properties in different states make DtBuCZBP a potential material for diverse applications. | Kaixuan Li Lifang Zhao Yongyang Gong Wang-Zhang Yuan Yongming Zhang | 2017 | Science China Chemistry2017，60，6： | 2 |
| 7 | Recent Progress of Mussel-Inspired Underwater Adhesives显示文摘 | Ke Zhang Feilong Zhang Yongyang Song Jun-Bing Fan Shutao Wang | 2017 | Chinese Journal of Chemistry2017，35，6： | 2 |
| 8 | Seismic response of multiple-anchor connections to concrete 显示文摘 | Zhang Yongyang Klingner R E Graves H L | 2001 | ACI Structural Journal2001，98，6： | 1 |
| 9 | Prediction of decline in shale gas well production using stable carbon isotope technique显示文摘Prediction of shale gas production is a challenging task because of the complex fracture-pore networks and gas flow mechanisms in shale reservoirs.Empirical methods,which are used in the industry to forecast the future production of shale gas,have not been assessed sufficiently to warrant high confidence in their results.Methane carbon isotopic signals have been used for producing gas wells,and are controlled by physical properties and physics-controlling production;they serve as a unique indicator of the gas production status.Here,a workable process,which is combined with a gas isotope interpretation tool(also known as a numerical simulator),has been implemented in Longrnaxi shale gas wells to predict the production decline curves.The numerical simulator,which takes into account a convection-diffu-sion-adsorption model for the matrix and a convection model for fractures in^(13)CH_(4) and ^(12)CH_(4) isotopologues,was used to stabilize the carbon isotope variation in the produced gas to elucidate gas recovery.Combined with the production rates of the four developing wells,the total reserves ranged from 1.72×10^(8) to 2.02×10^(8) m^(3),which were used to constrain the trend of two-segment produc-tion decline curves that exhibited a transition from a hyperbolic equation to an exponential one within 0.82-0.89 year.Two-segment production decline curves were used to forecast future production and estimate ultimate recovery. | Shengxian ZHAO Shujuan KANG Majia ZHENG Shuangfang LU Yunfeng YANG Huanxu ZHANG Yongyang LIU Ziqiang XIA Chenglin ZHANG Haoran HU Di ZHU | 2021 | Frontiers of Earth Science2021，15，4： | 1 |
| 10 | An almost sure central limit theorem for products of sums of partial sums under association显示文摘 | ZHANG Yongyang XIAO Yun DONG Zhishan | 2009 | J Math Anal Appl2009，35，5： | 1 |
| 11 | Gas hydrate occurrence on the continental slope of the northern South China Sea显示文摘 | WU SHIGUO ZHANG GUANGXUE HUANG YONGYANG | 2005 | Mar Petrol Geol2005，22，4： | 1 |
| 12 | Engineering subcellular-patterned biointerfaces to regulate the surface wetting of multicellular spheroids显示文摘 | Luying Wang Pingqiang Cai Jing Luo Feilong Zhang Jian Liu Yupeng Chen Zhongpeng Zhu Yongyang Song Bingquan Yang Xi Liu Xiaodong Chen Shutao Wang | 2018 | Nano Research2018，11，10： | 1 |
| 13 | High efficiency D-A structured luminogen with aggregation-induced emission and mechanochromic characteristics显示文摘A novel luminogen, CZ2TPAN, with typical D-A architecture was obtained. It shows intramolecular charge transfer and aggregation-induced emission characteristics with high solid-state efficiency of 65.3%. Moreover, it exhibits reversible mechanochromic behavior between crystalline and amorphous states with remarkable emission color change from green (504 nm) to yellow (545nm). | LU YaWei TAN YeQiang GONG YongYang LI Hong YUAN WangZhang ZHANG YongMing TANG Ben Zhong | 2013 | Chinese Science Bulletin2013，58，22： | 1 |
| 14 | Leakage of nuclear material powder from pressure container through a small orifice显示文摘Because of the radioactivity and toxic nature of nuclear materials,their containment within oxide matrices,encased in sealed containers,has been proposed as a suitable means for storage and transportation.However,container failures because of cracks or small orifices present a major leakage risk for nuclear materials,consequently posing a significant hazard to the environment and human beings.In this study,terbium oxide powder was used as a nuclear material representative to examine the leakage of nuclear material powder through orifices located at the base of a pressure container.The dependence of the orifice diameter,the powder layer thickness,and the internal pressure of the container on the leakage mechanism and amount was examined.A simplified model correlating the dependence of the above-mentioned parameters to determine the utmost leakage amount was also developed based on the present results.The leakage of the nuclear material powder was assessed by measuring its concentration using an optical particle counter.The diameter of the orifice determined the powder leakage mechanism,which in turn influenced the amount of leakage produced.Comparison studies showed that unlike the changes in the differential pressure,the volume of the container has little effect on the leakage amount.Under sufficiently high internal pressures,the oxide powder can be released as a fine aerosol.The work is not only crucial from the nuclear safety aspect,but is also beneficial for the safe application of powder and nanoparticles. | Longbo Liu Yanmin Wu Yongyang Su Hanbing Tang Zhihong Zhang Ping Huang Lili Zhang Lixing Zhang | 2014 | Particuology2014，12，3： | 0 |
| 15 | Flexible Dry Hydrogel with Lamella-Like Structure Engineered via Dehydration in Poor Solvent显示文摘Hydrogels are among the most promising biologic materials in recent technology with numerous desired applications,including serving as biosensors,drug delivery vehicles,and tissue-engineered products for cell matrices.However,they often dehydrate,and become stiff and brittle in air,causing loss of flexibility and functions.Several layered structures have been proven to increase the strength,toughness,and even flexibility of these materials,which might provide a new clue for the sustenance of the flexibility of drying gels.Herein,we report a novel solvent-dehydrated hydrogel engineering approach,aimed to change the inner structure and keep the flexibility of a dehydrated hydrogel in the air via solvent-induced dehydration,for example,acetonedehydrated polyacrylic acid hydrogel.This flexible dry gel could be folded,twisted,and stretched without any damage due to the assumed lamella-like structures,contrary to dry gels without these microstructures or those with porous structures,which retain brittle consistency.The flexible dry gel also exhibited excellent self-healing capability with the assistance of solvents.Fascinatingly,this flexible gel film displayed strain-visualizing paper writing/erasing performance properties,with water acting as invisible ink.Thus,this fabricated flexible hydrogel film might function as confidential information storage material.Our current approach is versatile,hence applicable to other hydrogels,and provides insight into the engineering of other functional gels for extended future applications. | Feilong Zhang Jiajia Zhou Zhen Gu Man Yang Siheng Li Yongyang Song Jun-Bing Fan Jingxin Meng Peiyi Wu Lei Jiang Shutao Wang | 2020 | CCS Chemistry2020，2，1： | 0 |
| 16 | Crystallization-induced phosphorescence, remarkable mechanochromism, and grinding enhanced emission of benzophenone-aromatic amine conjugates显示文摘Pure organic luminogens with efficient room temperature phosphorescence(RTP) and remarkable mechanochromism are highly desired in view of their fundamental significance and technical applications. Herein, four twisted pure organic luminogens based on benzophenone and aromatic amines were synthesized and their photophysical properties were thoroughly investigated. They exhibit crystallization-induced phosphorescence(CIP), giving bright fluorescence and phosphorescence dual emission in crystals. Upon grinding, they become amorphous and emit predominantly red-shifted fluorescence, demonstrating remarkable mechanochromism. Furthermore, three of them even demonstrate greatly enhanced emission upon grinding, which is rarely observed in twisted D-A structured luminogens. | Weijian Luo Yiren Zhang Yongyang Gong Qing Zhou Yongming Zhang Wangzhang Yuan | 2018 | Chinese Chemical Letters2018，29，10： | 0 |
| 17 | Building block copolymer particles via self‐assembly within a droplet显示文摘The self‐assembly of block copolymers(BCPs)within emulsion droplets is a flexible strategy for the preparation of polymer particles.This strategy permits the finetuning of shapes,internal structures,and surface nanostructures of the polymer particles,thus allowing many applications.Although some literature has reviewed the BCP preparation via self‐assembly within a droplet,a comprehensive summary including in‐depth understanding,controllable preparation,and application is lacked.In this review,we systematically delve into the multiple mechanisms that drive BCP self‐assembly within emulsion droplets,such as commensurability effects for minimizing total free energy,interfacial instability,organized spontaneous emulsification,phase separation of multiple components,and entropy effects between BCPs and nanoparticles.Additionally,a strategy combining selective cross‐linking and disassembly can further generate Janus particles featuring unique structures.Next,various applications across multiple disciplines are discussed,including drug delivery,display,biomedical imaging,macromolecular separation,and fuel cells.Finally,we present an overview of the current challenges and future directions for BCP emulsion self‐assembly,covering mechanism investigation,molecular design,stability control,and application exploration.We anticipate deeper understanding,more varieties,enhanced performance,and broader applications can be achieved with BCP emulsion self‐assembly after addressing the challenge. | Sen Zhang Han Bao Xinyi Shen Yongyang Song Shutao Wang | 2023 | Droplet2023，2，4： | 0 |
| 18 | Intrinsic emission and tunable phosphorescence of perfluorosulfonate ionomers with evolved ionic clusters显示文摘Intrinsic emission from unorthodox luminogens without traditional conjugated building blocks is drawing increasing attention.However,the emission mechanism is still controversial.Herein,we demonstrate the intriguing emission from perfluorosulfonate ionomers(PFSIs),which can be explained by the clustering triggered emission(CTE)mechanism.Despite being free of any conventional chromophores,PFSIs exhibit bright emission and multi-color phosphorescence(77 K)in concentrated solutions,powders and membranes with obvious aggregation-induced emission(AIE)characteristics.Clustered sulfonic acids are responsible for the light emission,and their connection and evolution are deeply explored via X-ray diffraction(XRD)and small angel X-ray scattering(SAXS),in which the electron overlap determined by the clustered status results in the extended conjugation and simultaneously rigidified conformations.These results demonstrate that it is feasible to use fluorescence analysis to explore the ionic cluster structure and evolution of PFSI,and it can be applied in the pure organic luminescent field as well. | Qing Zhou Jia Cui Tianjia Yang Changlu Hu Zihao Zhong Zhenhua Sun Yongyang Gong Supeng Pei Yongming Zhang | 2020 | Science China Chemistry2020，63，6： | 0 |
| 19 | Room temperature phosphorescence from natural products: Crystallization matters显示文摘Efficient room temperature phosphorescence is observed in natural compounds and polymers such as starch,cellulose,bovine serum albumin(BSA),and some other carbohydrates.Whereas being practically nonluminescent in solutions and TLC plates,they emit bright phosphorescence in the crystalline states with lifetime up to microseconds,exhibiting crystallization-induced phosphorescence(CIP)characteristics.The CIP of these natural products without any conventional chromophores offers a new platform for the exploration of conceptually novel luminogens. | GONG YongYang TAN YeQiang MEI Ju ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG BenZhong | 2013 | 中国科学:化学2013，43，9： | 0 |
| 20 | Crystallization-induced phosphorescence of benzils at room temperature显示文摘Efficient room temperature phosphorescence(RTP)is rarely observed in pure organic luminogens.However,we have newly observed that benzil and its derivatives are nonluminescent in solvents and thin layer chromatography(TLC)plates,but become highly phosphorescent in crystal state at room temperature,exhibiting typical crystallization-induced phosphorescence(CIP)characteristics.The CIP phenomenon is ascribed to the restriction of intramolecular rotations in crystals owing to effective intermolecular interactions.Such intermolecular interactions greatly rigidify the molecular conformation and significantly decrease the nonradiative deactivation channels of the triplet excitons,thus giving boosted phosphorescent emission at room temperature. | GONG YongYang TAN YeQiang LI Hong ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG Ben Zhong | 2013 | 中国科学:化学2013，43，9： | 0 |
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