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| 1 | Vertically Aligned Silicon Carbide Nanowires/Boron Nitride Cellulose Aerogel Networks Enhanced Thermal Conductivity and Electromagnetic Absorbing of Epoxy Composites显示文摘With the innovation of microelectronics technology, the heat dissipation problem inside the device will face a severe test. In this work, cellulose aerogel(CA) with highly enhanced thermal conductivity(TC) in vertical planes was successfully obtained by constructing a vertically aligned silicon carbide nanowires(SiC NWs)/boron nitride(BN) network via the ice template-assisted strategy. The unique network structure of SiC NWs connected to BN ensures that the TC of the composite in the vertical direction reaches 2.21 W m^(-1) K^(-1) at a low hybrid filler loading of 16.69 wt%, which was increased by 890% compared to pure epoxy(EP). In addition, relying on unique porous network structure of CA, EP-based composite also showed higher TC than other comparative samples in the horizontal direction. Meanwhile, the composite exhibits good electrically insulating with a volume electrical resistivity about 2.35 × 10^(11) Ω cm and displays excellent electromagnetic wave absorption performance with a minimum reflection loss of-21.5 dB and a wide effective absorption bandwidth(<-10 dB) from 8.8 to 11.6 GHz. Therefore, this work provides a new strategy for manufacturing polymer-based composites with excellent multifunctional performances in microelectronic packaging applications. | Duo Pan Gui Yang Hala MAbo-Dief Jingwen Dong Fengmei Su Chuntai Liu Yifan Li Ben Bin Xu Vignesh Murugadoss Nithesh Naik Salah MEl-Bahy Zeinhom MEl-Bahy Minan Huang Zhanhu Guo | 2022 | Nano-Micro Letters2022，14，7： | 7 |
| 2 | Manipulation of blue TADF top-emission OLEDs by the first-order optical cavity design:toward a highly pure blue emission and balanced charge transport显示文摘The broad luminescence spectrum of a thermally activated delayed fluorescence(TADF)organic light-emitting diode(OLED)is a critical issue to overcome for its application in high-color-purity displays.Herein,a novel device structure that utilizes the first-order microcavity optical mode with a high radiance intensity is demonstrated to solve this problem by considering the charge transport properties through the analysis of hole-only and electron-only devices.In addition,by tuning the optical interference near the semitransparent top cathode layers consisting of thin silver and organic capping layers,light extraction is increased by nearly 2 times compared to the device without a capping layer.Consequently,the optimized blue TADF top-emission OLED exhibits much lower full width at half-maximum,higher maximum current efficiency,and external quantum efficiency compared to the device before optimization.This approach is expected to provide a simple but effective way to further enhance the spectral purity of the conventional TADF-based OLEDs. | WANQI REN KYUNG ROCK SON TAE HOON PARK VIGNESH MURUGADOSS TAE GEUN KIM | 2021 | Photonics Research2021，9，8： | 3 |
| 3 | Highly transmitted silver nanowires-SWCNTs conductive flexible film by nested density structure and aluminum-doped zinc oxide capping layer for flexible amorphous silicon solar cells显示文摘Indium tin oxide(ITO)is widely used in transparent conductive films(TCFs);however,several disadvan-tages,such as high cost and toxicity of indium,limit its applications.Therefore,it is necessary to develop other materials that can replace ITO.Silver nanowires or single walled carbon nanotubes(SWCNTs)have attracted considerable interest owing to their unique electrical,optical,and thermal stabilities,and thus,they are ideal for transparent electrodes for flexible or stretchable devices.In this study,we develop a novel architecture of composite TCFs on a polyethylene naphthalate(PEN)flexible substrate.Herein,the silver nanowires-SWCNTs films with nested density structure were fabricated through ultrasonic spraying technology by varying the spraying width.For achieving enhanced transmittance,we combined the larger irregular grids and holes with fewer nanowires stacked in the longitudinal direction,more optical chan-nels,and good carrier transport.Thereafter,aluminum-doped zinc oxide(AZO)was used as capping to the structure for enhancing the optical properties of the TCFs.The silver nanowires-SWCNTs/AZO(ASA)bilayer was obtained in the optimized architecture,which showed superior optoelectronic performance to that shown by commercial ITO with a high optical transmittance of 92%at the wavelength of 550 nm and low sheet resistance of 17/sq.In the specially structured conductive film,the significant improvement in the transmittance and uniformity of the sheet resistance was attributed to the effective nanowire junc-tion contact compared to that in ordinary structure of silver nanowires,which reduced the mean density of small clusters of nanowires.Compared with the silver nanowires-SWCNTs films,the ASA bilayer film exhibited excellent resistance to boiling,mechanical bending(10,000 cycles),and CO_(2)plasma.Moreover,the sheet resistance of ASA changed slightly after the tape tests,thereby illustrating a strong adhesion to the PEN substrate after the enclosure of AZO.Meanwhile,the AZO capping layer can enhance the op-tical transmittance between 600 and 1500 nm.In addition,the amorphous silicon photovoltaic devices with flexible ASA TCFs exhibited a power conversion efficiency(PCE)of 8.67%.After bending for 3000 times,the PCE was decreased to 8.20%,thereby demonstrating the potential of developed films to replace traditional ITO. | Shunliang Gao Xiaohui Zhao Qi Fu Tianchi Zhang Jun Zhu Fuhua Hou Jian Ni Chengjun Zhu Tiantian Li Yanlai Wang Vignesh Murugadoss Gaber A.M.Mersal Mohamed M.Ibrahim Zeinhom M.El-Bahy Mina Huang Zhanhu Guo | 2022 | Journal of Materials Science & Technology2022，，31： | 2 |
| 4 | Interface Engineered Microcellular Magnetic Conductive Polyurethane Nanocomposite Foams for Electromagnetic Interference Shielding显示文摘Lightweight microcellular polyurethane(TPU)/carbon nanotubes(CNTs)/nickel-coated CNTs(Ni@CNTs)/polymerizable ionic liquid copolymer(PIL)composite foams are prepared by non-solvent induced phase separation(NIPS).CNTs and Ni@CNTs modified by PIL provide more heterogeneous nucleation sites and inhibit the aggregation and combination of microcellular structure.Compared with TPU/CNTs,the TPU/CNTs/PIL and TPU/CNTs/Ni@CNTs/PIL composite foams with smaller microcellular structures have a high electromagnetic interference shielding effectiveness(EMI SE).The evaporate time regulates the microcellular structure,improves the conductive network of composite foams and reduces the microcellular size,which strengthens the multiple reflections of electromagnetic wave.The TPU/10CNTs/10Ni@CNTs/PIL foam exhibits slightly higher SE values(69.9 dB)compared with TPU/20CNTs/PIL foam(53.3 dB).The highest specific EMI SE of TPU/20CNTs/PIL and TPU/10CNTs/10Ni@CNTs/PIL reaches up to 187.2 and 211.5 dB/(g cm^(−3)),respectively.The polarization losses caused by interfacial polarization between TPU substrates and conductive fillers,conduction loss caused by conductive network of fillers and magnetic loss caused by Ni@CNT synergistically attenuate the microwave energy. | Guolong Sang Pei Xu Tong Yan Vignesh Murugadoss Nithesh Naik Yunsheng Ding Zhanhu Guo | 2021 | Nano-Micro Letters2021，13，10： | 1 |
| 5 | Influence of mass ratio and calcination temperature on physical and photoelectrochemical properties of ZnFe-layered double oxide/cobalt oxide heterojunction semiconductor for dye degradation applications显示文摘A visible light-active photoelectrocatalyst,ZnFe-layered double oxide(LDO)/cobalt(II,III)oxide(Co_(3)O_(4))composites were obtained by calcining the Co loaded ZnFe-layered double hydroxide(LDH)prepared by a hydrothermal and microwave hydrothermal method.The morphological studies revealed that the ZnFe-LDO/Co_(3)O_(4) composites exhibited a flower-like structure comprising Co_(3)O_(4) nanowires and ZnFe-LDO nanosheets.Further,when the mass ratio of Co(NO_(3))_(2)·6H_(2)O/LDH was 1:1.8 and the calcination temperature was 550℃,the ZnFe-LDO/Co_(3)O_(4) composite exhibited 93.3%degradation efficiency for methylene blue(MB)at the applied voltage of 1.0 V under visible light after 3 h.Furthermore,the Mott-Schottky model experiments showed that the formation of a p-n heterojunction between ZnFe-LDO and Co_(3)O_(4) could effectively inhibit the recombination of electrons and holes in the photoelectrocatalytic process.Meanwhile,free radical scavenging experiments showed that the active radicals of⋅OH played an important role in the degradation of MB.Therefore,the photoelectrocatalytic effect of ZnFe-LDO/Co_(3)O_(4) provides a simple and effective strategy for the removal of organic pollutants. | Yufei Zhang Junjie Zheng Jiejie Nan Chengjie Gai Qian Shao Vignesh Murugadoss Srihari Maganti Nithesh Naik Hassan Algadi Mina Huang Ben Bin Xu Zhanhu Guo | 2023 | Particuology2023，，3： | 0 |
| 6 | Cavity-Suppressing Electrode Integrated with Multi-Quantum Well Emitter:A Universal Approach Toward High-Performance Blue TADF Top Emission OLED显示文摘A novel device structure for thermally activated delayed fluorescence(TADF)top emission organic light-emitting diodes(TEOLEDs)that improves the viewing angle characteristics and reduces the efficiency roll-off is presented.Furthermore,we describe the design and fabrication of a cavity-suppressing electrode(CSE),Ag(12 nm)/WO_(3)(65 nm)/Ag(12 nm)that can be used as a transparent cathode.While the TADF-TEOLED fabricated using the CSE exhibits higher external quantum efficiency(EQE)and improved angular dependency than the device fabricated using the microcavity-based Ag electrode,it suffers from low color purity and severe efficiency roll-off.These drawbacks can be reduced by using an optimized multi-quantum well emissive layer(MQW EML).The CSE-based TADF-TEOLED with an MQW EML fabricated herein exhibits a high EQE(18.05%),high color purity(full width at half maximum~59 nm),reduced efficiency roll-off(~46%at 1000 cd m^(−2)),and low angular dependence.These improvements can be attributed to the synergistic effect of the CSE and MQW EML.An optimized transparent CSE improves charge injection and light outcoupling with low angular dependence,and the MQW EML effectively confines charges and excitons,thereby improving the color purity and EQE significantly.The proposed approach facilitates the optimization of multiple output characteristics of TEOLEDs for future display applications. | Il Gyu Jang Vignesh Murugadoss Tae Hoon Park Kyung Rock Son Ho Jin Lee WanQi Ren Min Ji Yu Tae Geun Kim | 2022 | Nano-Micro Letters2022，14，4： | 0 |
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