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222篇 您的检索式:作者名="Synthesis"
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1Energy balance closure at ChinaFLUX sites显示文摘Network of eddy covariance observation is measuring long-term carbon and water fluxes in contrasting ecosystems and climates. As one important reference of independently evaluating scalar flux estimates from eddy covariance, energy balance closure is used widely in study of carbon and water fluxes. Energy balance closure in ChinaFLUX was evaluated by statistical regression of turbulent energy fluxes (sensible and latent heat) against available energy (net radiation, soil heat flux, canopy heat storage) and the energy balance ratio (EBR) and the frequency distribution of relative errors of energy balance (δ). The trends of diurnal and seasonal variation of energy balance in ChinaFLUX were analyzed. The results indicated that the imbalance was prevalent in all observation sites, but there were little differences among sites because of the properties variation of sites. The imbalance was greater during nocturnal periods than daytime and closure was improved with friction velocity intensifying. Generally the results suggested that estimates of the scalar turbulent fluxes of sensible and latent heat were underestimated and/or that available energy was overestimated. Finally, we discussed certain factors that are contributed to the imbalance of energy, such as systematic errors associated with the sampling mismatch, systematic instrument bias, neglected energy sinks, low and high frequency loss of turbulent fluxes and advection of heat and water vapor.LI Zhengquan, YU Guirui, WEN Xuefa, ZHANG Leiming, REN Chuanyou & FU Yuling Chinese Ecosystem Research Network Synthesis Research Center, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China Graduate School of the Chinese Academy of Sciences, Beijing 100039, China 2005Science China Earth Sciences2005,48,z1:50
2Advances in carbon flux observation and research in Asia显示文摘As an important component of FLUXNET, Asia is increasingly becoming the hotspot in global carbon research for its vast territory, complex climate type and vegetation diversity. The present three regional flux observation networks in Asia (i.e. AsiaFlux, KoFlux and ChinaFLUX)have 54 flux observation sites altogether, covering tropic rainforest, evergreen broad-leaved forest, broad-leaved and coniferous mixed forest, shrubland, grassland, alpine meadow and cropland ecosystems with a latitudinal distribution from 2°N to 63°N. Long-term and continuous fluxes of carbon dioxide, water vapor and energy between the biosphere and atmosphere are mainly measured with eddy covariance technique to (1) quantify and compare the carbon, water and energy budgets across diverse ecosystems; (2) quantify the environmental and biotic controlling mechanism on ecosystem carbon, water and energy fluxes; (3) validate the soil-vegetation-atmosphere model; and (4) serve the integrated study of terrestrial ecosystem carbon and water cycle. Over the last decades, great advancements have been made in the theory and technology of flux measurement, ecosystem flux patterns, simulation and scale conversion by Asian flux community. The establishment of ChinaFLUX has greatly filled the gap of flux observation and research in Eurasia. To further promote the flux measurement and research,accelerate data sharing and improve the data quality, it is necessary to present a methodological system of flux estimation and evaluation over complex terrain and to develop the integrated research that combines the flux measurement, stable isotope measurement, remote sensing observation and GIS technique. It also requires the establishment of the Joint Committee of Asian Flux Network in the Asia-Pacific region in order to promote the cooperation and communication of ideas and data by supporting project scientists, workshops and visiting scientists.YU Guirui, ZHANG Leiming, SUN Xiaomin, FU Yuling & LI Zhengquan Synthesis Center of Chinese Ecosystem Research Network (CERN), Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China Graduate School of the Chinese Academy of Sciences, Beijing 100039, China 2005Science China Earth Sciences2005,48,z1:16
3新型2-氨基-5-苯亚甲基-4H-咪唑啉-4-酮衍生物的合成及生物活性显示文摘通过烯基膦亚胺1与芳基异氰酸酯的aza-Witig反应得到碳二亚胺2,再用2与亲核试剂的成环反应制得10个新型的2-氨基-5-苯亚甲基-4H-咪唑啉-4-酮衍生物4.探讨了碳二亚胺2与不同亲核试剂反应的活性并分离得到了一个胍中间体3i.DING Ming Wu *, TU Hai Yang, LIU Zhao Jie, ZHUANG Nong Bo (Institute of Organic Synthesis, Central China Normal University, Wuhan, 430079) 1998高等学校化学学报1998,19,6:15
4Turbulence flux measurement above the overstory of a subtropical Pinus plantation over the hilly region in southeastern China显示文摘Continuous turbulence flux measurement using the eddy covariance (EC) technique was made from January 1 to December 31 in 2003 at two and three canopy heights of a subtropical Pinus plantation on the red earth hilly region in southeastern China. To be able to make sure that the measured turbulence flux will equal the net ecosystem/atmosphere exchange, the quality of the data has to be assessed. Three criteria were investigated here, including the power spectra and cospectra analyses, flux variance similarity (integral turbulence test) and energy balance closure. The spectral analyses suggested that above-canopy power spectral slopes for all velocity components and scalars such as CO2, H2O and air temperature followed the expected -2/3 power law in the inertial subrange, and their cospectral slopes were close to -4/3 power law in the inertial subrange. The important contribution of large-scale motions to energy and mass transfer above the canopy at higher measurement level was also confirmed by the spectral analyses. The eddy covariance systems have the ability to resolve fluctuations associated with small-scale eddies and did not induce an obvious underestimation of the measured turbulence flux. The Monin-Obukhov similarity functions for the normalized standard deviation of vertical wind speed and air temperature were well-defined functions of atmospheric stability at two heights above the forest canopy, which indicated that turbulence flux measurements made at two heights were within the surface layer. Nocturnal flux underestimation and departures of this normalized standard deviation of vertical wind speed similarity function from that expected from Monin-Obukhov theory were a function of friction velocity. Thus, an optimal criterion of friction velocity was determined to be greater than 0.2-0.3 m s-1 for nocturnal fluxes so that the eddy covariance flux measurement was under high turbulent mixing conditions. Energy balance closure reached about 72%-81% at the studied site, which was comparable to the 10%-30% of energy imbalance reported in the literature. However, the energy balance closure could be only used as a useful reference criterion.WEN Xuefa, YU Guirui, SUN Xiaomin & LIU Yunfen Chinese Ecosystem Research Network Synthesis Research Center, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China Graduate School of the Chinese Academy of Sciences, Beijing 100039, China 2005Science China Earth Sciences2005,48,z1:14
5Seasonal patterns and environmental control of ecosystem respiration in subtropical and temperate forests in China显示文摘Continuous measurement of carbon dioxide exchange using the eddy covariance (EC) technique was made at two ChinaFLUX forest sites including the young subtropical Pinus plantation (Qianyanzhou) and old temperate broad-leaved Korean pine mixed forest (Changbai Mountains) as part of the ChinaFLUX network. Seasonal patterns and environmental control of ecosystem respiration in the subtropical and temperate forests were evaluated by the often-used multiplicative model and Q10 model as a function of temperature and soil water content. The resuits suggested that ( i ) temperature was found to be a dominant factor in the ecosystem respiration, and most of the temporal variability of ecosystem respiration was explained by temperature. However, in the drought-stressed ecosystem, soil water content controlled the temporal variability of ecosystem respiration other than temperature effects, and soil water content became a dominat factor when severe drought affected the ecosystem respiration; (ii) the regression models analysis revealed that in the drier soil, ecosystem respiration was more sensitive to soil moisture than was expressed by the often-used multiplicative model. It was possible to accurately estimate the seasonal variation of ecosystem respiration based on the Q10 model; and (iii)annual ecosystem respiration derived from the often-used multiplicative model was 1209 g C m-2and 1303 g C m-2, and was consistently a little higher than the Q10 model estimates of 1197 g C m-2 and 1268 g C m-2 for Qianyanzhou and Changbai Mountains, respectively.YU Guirui, WEN Xuefa, LI Qingkang, ZHANG Leiming, REN Chuanyou, LIU Yunfen & GUAN Dexin Chinese Ecosystem Research Network Synthesis Research Center, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China Institute of Applied Ecology, Chinese Academy of Sciences, Shenyang 110016, China Graduate School of the Chinese Academy of Sciences, Beijing 100039, China 2005Science China Earth Sciences2005,48,z1:13
6Grain Size and Wettability of TiO_2/SiO_2 Photocatalytic Composite Thin Filing显示文摘The uniform transparent TiO2/SiO2 photocatalytic composite thin films are prepared by sol-gel method on the soda lime glass substrates, and characterized by UV-visible spectroscopy, X-ray diffraction (XRD), transmission electron microscopy (TEM), BET surface area, FTIR spectroscopy and X-ray photoelectron spectroscopy (XPS). It was found that the addition of SiO2 to TiO2 thin films can suppress the grain growth of TiO2 crystal, increase the hydroxyl content on the surface of TiO2 films, lower the contact angle for water on TiO2 films and enhance the hydrophilic property of TiO2 films. The super-hydrophilic TiO2/SiO2 photocatalytic composite thin films with the contact angle of 0° are obtained by the addition of 10%-20% SiO2 in mole fraction.Jiaguo Yu, Xiujian Zhao, Jimmy C Yu, Jun Lin (State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China Deportment of Chemised The Chinese University of Hong Kong, Hong Kong, 2001Rare Metals2001,20,2:11
7中国科学院生态系统网络观测与模拟重点实验室CERN综合研究中心研究成果与发展显示文摘介绍了中国生态系统研究网络(CERN)综合研究中心成立以来的发展历程和主要研究成果,以及未来研究方向及预期发展。取得的代表性研究成果主要有:CERN动态监测数据与生态系统空间信息数据管理和共享系统的开发、陆地生态系统碳和水热通量观测研究、陆地生态系统碳储量的时空格局特征研究、陆地生态系统多尺度模拟综合集成研究和青藏高原生态系统格局与全球变化相互作用关系研究等。未来的研究方向主要集中在陆地生态系统碳氮水循环及其耦合,区域碳汇功能动态,生态敏感区、脆弱区和过渡区对全球气候变化的响应与适应,生态监测、模拟与生态信息应用以及全球气候变化主要因子对生态系统关键过程的影响。未来除了履行CERN综合研究中心的基本职能外,争取在以上研究方向取得有国际影响的开拓性研究成果。Synthesis Research Center of Chinese Ecosystem Research Network,CAS(Institute of Geographic Sciences and Natural Resources Research,CAS,Beijing 100101,China) 2010自然资源学报2010,25,9:6
8Ruthenium(Ⅲ) chloride as an efficient catalyst for the synthesis of perimidine derivatives under mild conditions显示文摘Various biologically important perimidine derivatives have been synthesized efficiently from various ketones and naphthalene- 1,8-diamine by using a catalytic amount of RuCl3(1 mol%).This method is a very simple and high yielding reaction for the synthesis of perimidine derivatives.Jing Zhang~a Song Lin Zhang~(a,b,*) Jun Min Zhang~a a Key Laboratory of Organic Synthesis of Jiangsu Province,College of Chemistry and Chemical Engineering,Dushu Lake Campus,Suzhou University,Suzhou 215123,China b College of Chemistry and Environmental Science,Henan Normal University,Xinxiang 453007,China 2007Chinese Chemical Letters2007,18,9:5
9Phenomenon of “contact guidance” on the surface with nano-micro-groove-like pattern and cell physiological effects显示文摘The topography of material surface has important influence on cell behavior and physiological functions. Groove-like pattern has drawn much attention among various patterns, due to the phenomenon of 'contact guidance' induced by this kind of topography. This review mainly focuses on 'contact guidance' formation as well as its influence on cell behavior and physiological effects. The possible mechanisms of 'contact guidance' formation were discussed. The research trend and the potential applications were also suggested.ZHOU Feng 1,2, YUAN Lin 1,3, HUANG He 1,2 & CHEN Hong1,2 1 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan 430070, China 2 School of Materials Science and Engineering, Wuhan University of Technology, Wuhan 430070, China 3 Biomedical Materials Research Center, Wuhan University of Technology, Wuhan 430070, China 2009Chinese Science Bulletin2009,54,18:5
10Hydrothermal Synthesis and Characterization of a Novel Supramolecular Network Compound [Co(IN)_2(H_2O)_4](IN=Isonicotinate)显示文摘A novel supramolecular compound, [Co(IN)2(H2O)4](1), was synthesized by means of the hydrothermal method and its structure was characterized with elemental analysis, FT-IR spectrum, TGA and X-ray diffraction. Though the unit cell structure of the title compound is only monomeric, all these units as building blocks are assembled into a novel three-dimensional supramolecular network via the widely hydrogen-bonding and π-π stacking interactions.JIA Hong-bin 1,3, YU Jie-hui 1, DING Hong 1, XU Ji-qing 1**, YE Ling 2, JING Wei-jie 1WANG Tie-gang 1, XU Jia-ning 1, QU Xue-jian 1 and LI Zeng-chun 1,31. College of Chemistry and State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130023, P. R. China 2. Key Laboratory of Supramolecular Structure and Materials of Ministry of Education, Jilin University, Changchun 130023, P. R. China 3. Department of Chemistry, Inner Mongolia University for Nationalities, Tongliao 028000, P. R. China 2002Chemical Research in Chinese Universities2002,18,4:5
11Miktoarms hyperbranched polymer brushes:One-step fast synthesis by parallel click chemistry and hierarchical self-assembly显示文摘Spherical molecular brushes with amphiphilic heteroarms were facilely synthesized by grafting the arms of hydrophobic 2-azidoethyle palmitate and hydrophilic monoazide-terminated poly(ethylene glycol) onto the core of alkyne-modified hyperbranched polyglycerol (HPG) with high molecular weight (Mn=122 kDa) via one-pot parallel click chemistry.The parallel click grafting strategy was demonstrated to be highly efficient (~100%),very fast (~ 2 h) and well controllable to the amphilicity of molecular brushes.Through adjusting the feeding ratio of hydrophobic and hydrophilic arms,a series of brushes with different arm ratios were readily obtained.The resulting miktoarms hyperbranched polymer brushes (HPG-g-C16/PEG350) were characterized by hydrogen-nuclear magnetic resonance (1H NMR),Fourier transform infrared (FT-IR) spectroscopy,gel permeation chromatography (GPC),and differential scanning calorimetry (DSC) measurements.The spherical molecular brushes showed high molecular weights up to 230 kDa,and thus could be visualized by atomic force microscopy (AFM).AFM and dynamic laser light scattering (DLS) were employed to investigate the self-assembly properties of amphiphilic molecular brushes with closed proportion of hydrophobic and hydrophilic arms.The brushes could self-assemble hierarchically into spherical micelles,and network-like fibre structures,and again spherical micelles by addition of n-hexane into the dichloromethane or chloroform solution of brushes.In addition,this kind of miktoarms polymer brush also showed the ability of dye loading via host-guest encapsulation,which promises the potential application of spherical molecular brushes in supramolecular chemistry.HAN Yi & GAO Chao MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and Engineering,Zhejiang University,Hangzhou 310027,China 2010Science China Chemistry2010,53,12:5
12A Quantum Chemistry Study of Inhibition Properties of Imidazole and Its Derivatives on Iron Surface Corrosion显示文摘The geometries of imidazole and its derivatives were respectively optimized by using ab initio method, and the molecular orbital energy levels and the charge densities were obtained for their optimum geometries. The frontier orbital energy levels, and the net charges of N (1) atom and the imidazole ring of those molecules were obtained with ab initio and SCC-DV-Xα methods. It was found that the inhibition properties of those compounds change with the highest occupied molecular orbital energy levels, and the net charges of N(1) atom. We took four iron atoms on the crystal plane (100) of α-iron as the surface which was used to study the adsorption towards the inhibitors. The adsorption models of the inhibitor to be adsorbed on the Fe-cluster surface were optimized with SCC-DV-Xα method. It turns out that the most favorable model is that the inhibitor molecule is adsorbed on the Fe-cluster surface in an inclined state. The calculation shows that the stabilization energies of the systems are well correlated with the inhibition efficien cies.YAN Xiao-ci, XIA Wen-bing, LIU Jie, OU YANG-li, LUO Ming-dao~(**) and YANG Feng (Department of Chemistry, Wuhan University, Wuhan 430072, P. R. China) MIN Xin-min (National Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, P. R. China) To whom correspondence should be addressed. 2001Chemical Research in Chinese Universities2001,17,3:4
13Intramolecular aromatic-ring stacking interaction of ternary Zn(UTP)L^(2-) complexes显示文摘THE mechanism of the action of the classic platinum antitumor drugs can be interpreted accord-ing to their bidentate, bifunctional interaction with the DNA of the tumor cell, resulting in in-hibition of the DNA replication. Recently, it was found that a new class of compounds withthe general formula cis-[Pt(NH3)2(N-het)Cl]Cl(N-het is a heteroaromatic N-base like pyri-dine) show effective antitumor activities. However, two possible mechanisms of actionLE Xueyi, WU Fuhai, SONG Fenyun and Jl Liangnian1.Department of Chemistry, Zhongshan University, Guangzhou 510275, China State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China 2. Department of Hygienics, Guangdong Pharmaceutical School, Guangzhou 510224, China 1997Chinese Science Bulletin1997,42,14:4
14Delivery of surface-mediated non-viral gene nanoparticles from ultrathin layer-by-layer multilayers显示文摘An efficient and safe gene delivery system remains a challenge in the development of gene therapy.Polycation-based gene nanoparticles are a typical non-viral gene delivery system,which are able to transfect cells in vitro and in vivo.This paper reported a facile method for constructing biodegradable multilayers via layer-by-layer self-assembly,in which the polycation-based gene nanoparticles were loaded.Through this surface-mediated delivery system,adherent cells on the multilayer could be transfected in situ.Gene nanoparticles-loaded multilayers transfect cells with higher efficiency than naked DNA-loaded multilayers because of the complex configuration of the DNA.DNA nanoparticles/PGA multilayers constructed on the scaffold surface could also realize in situ transfection on the adherent cells.The well-structured,easy-processed multilayers may provide a novel approach to precisely controlled delivery of gene nanoparticles,which may have potential applications for gene therapy in tissue engineering and medical implants.WANG XueFei,REN KeFeng,LIN QuanKui & JI Jian Key Laboratory of Macromolecule Synthesis and Functionalization,Ministry of Education Department of Polymer Science and Engineering,Zhejiang University,Hangzhou 310027,China 2010Science China Chemistry2010,53,3:4
15Ice core dust particulate by XPS-SEM/EDAX——Impact of dust particulate on SO_4^(2-) record in ice cores显示文摘The ice core dust particulate sampled from Mt. Xixabangma has been analyzed by means of X-ray photoelectron spectrometer (XPS) and scanning electron microscope with energy dispersion X-ray analysis (SEM/EDAX). The results show that the contents of SO42- and SO32- in the surface layer of the dust are significantly higher than those in the subsurface layer (with the exception of organic sulfide). This difference indicates that the surface SOx has been captured and then chemically converted by the atmospheric dust particulate before its deposition with snow, which is obviously different from those inner layer sulfates and sulfites contained by dust itself. In addition, it has been determined by SEM/EDAX that the dust contains relatively high concentrations of transition metal elements such as Fe and Ti oxides which could function as photocatalysts to the conversion of SOx adhered on the surface of the dust, and consequently accelerate the deposition of SOx to snow. Our research alsoLI Zhongqin , LU Gongxuan , LIU Baozhong , FU Hongxiang LIU YuTianshan Glaciological Station , Lanzhou Institute of Glaciology and Geocryology , Chinese Academy of Sciences , Lanzhou 730000,China State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics , Chinese Academy ofSciences , Lanzhou 730000, China, 1999Chinese Science Bulletin1999,44,15:4
16Hydrothermal synthesis and characterization of rare-earth ruthenate pyrochlore compounds R_2Ru_2O_7(R=Pr_(3+),Sm(3+)-Ho(3+))显示文摘A series of pyrochlore oxides, R2Ru2O7 (R=Pr3+, Sm3+–Ho3+) were synthesized under mild hydrothermal conditions. All the samples crystallize in uniform octahedron characteristically. The products were characterized by powder X-ray diffraction, scanning electron microscopy, energy-disperse X-ray spectroscopy, and dc susceptibility, and the factors that affected the crystallization were discussed. It was found that the purity of products depends strongly on the raw materials and the amount of alkalinity in the initial reaction mixtures. The ZFC and FC susceptibilities of all of the compounds R2Ru2O7 at low temperature were also measured and discussed.YAO LinRan, WANG Dong, PENG Wen, HU WeiWei, YUAN HongMing & FENG ShouHua State key Laboratory of Inorganic Synthesis and Preparative Chemistry College of Chemistry, Jilin University, Changchun 130023, China 2011Science China Chemistry2011,54,6:3
17Microstructure and Temperature Distribution in ZnAl_2O_4 Sintered Body by Pulse Electric Current显示文摘Microstructure of reaction sintering of ZnAl2O4 at 1500℃ by hot-pressing(HP) and pulse electric current was investigated. The results indicated that the existed cracks in sintered body were caused by structure mismatch. lt is the evidence that periodical temperature field existed during pulse electric current sintering of nonconductive materials.The distance between high temperature areas was related to die diameter.Dongming ZHANG, Zhengyi FU and Jingkun GUOState Key Lab. of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China 2003Journal of Materials Science & Technology2003,19,6:3
18A Novel Bimetallic Tetrahedron Cobalt Complex Promoting the Addition of Diethylzinc to Benzaldehyde显示文摘Our recent work found a novel bimetallic tetrahedron cobalt complex which can cataly- ze the addition of diethylzinc to benzaldehyde effectively.Wei Qiang ZHANG, Zhi CHEN, Yu Hua ZHANG, Xin Yi ZHU, Yu Gang CHEN, Huan Wang JING, Yuan Qi YIN* State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000 2001Chinese Chemical Letters2001,12,5:3
19Long-period Gratings in-situ Sensing for Flow Monitoring in Liquid Composite Molding显示文摘Liquid composite moulding (LCM) processes are used to manufacture high quality and complex-shaped composite parts in the automotive, marine, aerospace and civil industries. On-line sensing plays an important role in controlling the quality of the final product in the LCM manufacturing environment. The long-period fiber grating (LPG)technology, a new real-time fiber optic sensor system, was developed to monitor the flow front progression. The sensor operation and characterization under various process conditions were discussed in detail. The experimental results showed that LPG sensors were robust and reliable to detect the arrival of resin at pre-selected locations in structures with low-medium fiber volume fraction; however were limited at different depths in structures with high fiber volume fraction.Yingdan ZHU, Chang WANG, Jihui WANG, Wei HE and Guoqiang GAO State Key Laboratory of Advanced Technology for Materials Synthesis and Proceeding, Wuhan University of Technology, Wuhan 430070, China 2005Journal of Materials Science & Technology2005,21,2:3
20WETTABILITY BETWEEN TiB_2 CERAMIC AND METALS显示文摘Self consistent Field discrete variational Xα( SCF Xα DV) method was used to study the wettabilitybetween TiB2 Ceramic and Metals. The Metals were Ni, Mo, Ni+ Mo, and etc. microstructureof TiB2/ Fe, TiB2/ Niand TiB2/ NiMoinvestigatedby TEM werechosen toidentify the calculation model. The result shows the wetting in the above systems were chemicalreactive wetting ,and can becalculated by SCF Xα DV . Theeffectof active ele ment( Mo) to TiB2/ Ni wettability wasstudied too.J.Y. Zhang, Z.Y. Fu , W.M Wang , H. Wang and X.M. Min State Key Lab .of Advanced Technologyfor Materials Synthesis and Processing, Wuhan University of Technolo gy, Wuhan 430070 ,China 1999Acta Metallurgica Sinica(English Letters)1999,12,4:3
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