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| 1 | Controlling the gelation temperature of biomimetic polyisocyanides显示文摘Thermosensitive polymers show an entropy-driven transition from a well-solvated to a poorly solvated polymer chain, resulting in a more compact globular conformation. The transition at the lower critical solution temperature(LCST) is often sharp, which allows for a wide range of smart material applications.At the LCST, oligo(ethylene glycol)-substituted polyisocyanides(PICs) form soft hydrogels, composed of polymer bundles similar to biological gels, such as actin, fibrin and intermediate filaments. Here, we show that the LCST of PICs strongly depends linearly on the length of the ethylene glycol(EG) tails; every EG group increases the LCSTand thus the gelation temperature by nearly 30 ℃. Using a copolymerisation approach, we demonstrate that we can precisely tailor the gelation temperature between 10 ℃ and 60 ℃and, consequently, tune the mechanical properties of the PIC gels. | Paul H.J. Kouwer Paula de Almeida Onno ven den Boomen Zaskia H. Eksteen-Akeroyd Roel Hammink Maarten Jaspers Stijn Kragt Mathijs F.J. Mabesoone RoelandJ.M. Nolte Alan E. Rowan Martin G.T.A. Rutten Vincent A.A. Le Sage Daniel C. Schoenmakers Chengfen Xing Jialiang xu | 2018 | Chinese Chemical Letters2018，29，2： | 2 |
| 2 | Practical application of sigma metrics QC procedures in clinical chemistry显示文摘 | Schoenmakers CH Naus AJ Vermeer HJ | 2011 | Clin Chem Lab Med2011，49，11： | 1 |
| 3 | Completeness of lung cancer surgery: is mediastinal dis- section common practice 显示文摘 | VERHAGEN AF SCHOENMAKERS MC BARENDREGT W | 2012 | Eur J Cardiothorac Surg2012，41，4： | 1 |
| 4 | Linear reconstruction of perceived images from human brain activity显示文摘 | SCHOENMAKERS S BARTH M HESKES T | 2013 | Neuroimage2013，83，： | 1 |
| 5 | A chal- lenge with Porphyromonas gingivalis differentially affects the os- teoclastogenesis potential of periodontal ligament fibroblasts from periodontitis patients and non-periodontitis donors显示文摘 | SOKOS D SCHERES N SCHOENMAKER T | 2014 | Journal of Clinical Periodontology2014，41，2： | 1 |
| 6 | A mutation in the thyroid hormone receptor alpha gene显示文摘 | Bochukova E Schoenmakers N Agostini M | 2012 | N Engl J Med2012，366，： | 1 |
| 7 | Chromo- some 3 translocations and familial renal cell cancer 显示文摘 | Bonne A C Bodmer D Schoenmakers E F | 2004 | Current molecular medicine2004，4，8： | 1 |
| 8 | Sequence analysis of 21 genes located in the Kartagener syndrome linkage region on chromosome 15q显示文摘 | Geremek M Schoenmaker F Zeitkiewicz E | 2008 | Eur J Hum Genet2008，16，1： | 1 |
| 9 | Effect of thrombin peptide 508 (TPS08) on bone healing during distraction osteogenesis in rabbit tibia显示文摘 | Amir LR Li G Schoenmaker T | 2007 | Cell Tissue Res2007，330，1： | 1 |
| 10 | Chronic amiodarone evokes no torsade de pointes arrhythmias despite QT lengthening in an animal model of acquired long-QT syndrome显示文摘 | van Opstal JM Schoenmakers M Verduyn SC | 2001 | Circulation2001，104，22： | 1 |
| 11 | Sequence analysis of 21 genes located in the kartagener syndrome likage region on chromosome 15 显示文摘 | GEREMEK M SCHOENMAKER E ZEITKIEWICZ E | 2008 | Eur J Hum Genet2008，16，： | 1 |
| 12 | Distillation of formaldehyde containing mixture:laboratoty experiments,equilibrium stage modeling and simulation显示文摘 | Michael Ott Hartmust Schoenmakers Hans Hasse | 2005 | Chemical Engineering and Process2005，44，6： | 1 |
| 13 | Fast and efficient size-based separations of polymers using ultra-high-pressure liquid chromatography显示文摘 | ULIYANCHENKO E SCHOENMAKERS P J VAN DER WAL S | 2011 | Journal of Chromatography A2011，1218，11： | 1 |
| 14 | Sequence analysis of 21 genes located in the kartagener syndrome likage region on chromosome 15 q 显示文摘 | Geremek M Schoenmaker F Zeitkiewicz E | 2008 | Eur J Hum Genet2008，16，6： | 1 |
| 15 | Prognostic significance of tissue polypeptide-specific antigen(TPS)in patients with advanced non-small cell lung cancar显示文摘 | Vander GA Schoenmakers CH Koktc | 2006 | Eur J csncer2006，30，： | 1 |
| 16 | Model predictivecontrol of integrated unit operations:Control of a dividedwall column显示文摘 | ADRIAN T SCHOENMAKER S H BOLL M | 2004 | Chem Eng Process2004，43，： | 1 |
| 17 | Sequence analysis of genes located in the kartagener syndrome likage region on chromosome 15 q显示文摘 | Geremek M Schoenmaker F Zeitkiewicz E | 2008 | Eur J Hum Genet2008，16，6： | 1 |
| 18 | The spatial dimension of pa- tenting by multinational firms in Europe 显示文摘 | VERSPAGEN B SCHOENMAKERS W | 2004 | Journal of Economic Geography2004，，11： | 1 |
| 19 | Exploration and exploitation in innovation: Refraining the interpretation显示文摘 | Li Y Vanhaverbeke W and Schoenmakers W | 2008 | Cre- ativity and Innovation Management2008，17，2： | 1 |
| 20 | Chronic amiodarone evokes no tor- sade de points arrhythmias despite QT lengthening in a animal model of acquired long QT syndrome显示文摘 | VAN OPSTAL J M SCHOENMAKERS M VER- DUYN SC | 2001 | Circulation2001，104，： | 1 |
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