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| 1 | One-step synthesis of N-doped metal/biochar composite using NH_3-ambiance pyrolysis for efficient degradation and mineralization of Methylene Blue显示文摘A series of new biochar-supported composite based on the combination of biochar and metallic nanoparticles(NPs)were produced through single-step pyrolysis of FeCl_3–Ti(OBu)_4 laden agar biomass under NH_3 environment.The physiochemical properties of composites were characterized thoroughly.It has found that heating temperature and N-doping through NH_3-ambiance pyrolysis significantly influence the visible-light sensitivity and bandgap energy of composites.The catalytic activities of composites were measured by degradation of Methylene Blue(MB)in the presence or absence of H_2O_2 and visible-light irradiation.Our best catalyst(N–TiO_2–Fe_3O_4-biochar)exhibits rapid and high MB removal competency(99.99%)via synergism of adsorption,photodegradation,and Fenton-like reaction.Continuous production of O_2U^-and UOH radicles performs MB degradation and mineralization,confirmed by scavenging experiments and degradation product analysis.The local trap state Ti^(3+),Fe_3O_4,and N-carbon of the catalyst acted as active sites.It has suggested that the Ti^(3+)and N-doped dense carbon layer improve charge separation and shuttle that prolonged photo-Fenton like reaction.Moreover,the catalyst is highly stable,collectible,and recyclable up to 5 cycles with high MB degradation efficiency.This work provides a new insight into the synthesis of highly visible-light sensitized biocharsupported photocatalyst through NH_3-ambiance pyrolysis of NPs-laden biomass. | Md Manik Mian Guijian Liu Balal Yousaf Biao Fu Rafay Ahmed Qumber Abbas Mehr Ahmed Mujtaba Munir Liu Ruijia | 2019 | Journal of Environmental Sciences2019，31，4： | 8 |
| 2 | Plasma concentration of interleukin-6 and the risk of future myocardial infarction among apparently health men 显示文摘 | Ridker PM Rafai N Stampfer MJ | 2000 | Circulation2000，101，15： | 1 |
| 3 | Hub location–allocation in intermodal logistic networks显示文摘 | Rafay Ishfaq Charles R. Sox | 2010 | European Journal of Operational Research2010，，2： | 1 |
| 4 | Clinical and electrophysiological aspects of acute organophosphate intoxication显示文摘 | Rafai MA Boulaajaj FZ Bourezgui M | 2007 | Neurophysiol Clin2007，37，1： | 1 |
| 5 | Effect of an intermittent lighting schedule on doe and suckling rabbit's performance显示文摘 | Virág Gy Papp Z Rafai P | | 0，，01： | 1 |
| 6 | Craniocervical arterial dissection in children: clinical and radiographic presentation and outcome显示文摘 | Rafay MF Armstrong D Deveber G Domi T Chan A MacGregor DL | 2006 | J Child Neurol2006，21，1： | 1 |
| 7 | Interrelationships among circulating interleukin-6 ,C-reactive protein,and traditional cardio- vascular risk factor in women显示文摘 | Bvermudez EA Rafai N Buring J | 2002 | Arterioscler Thromb Vasc Biol2002，22，： | 1 |
| 8 | Clinical results oflithium- disilicate crowns after up to 9 years of service显示文摘 | Gehrt M Wolfart S Rafai N | 2013 | Clin Oral Investig2013，17，1： | 1 |
| 9 | Clearance kinetics,biodistribution,and organ saturability of phosphorothioate oligodeoxynucleotides in mice 显示文摘 | Rafai A Brysch W Fadden K | 1996 | Am J Pathol1996，149，2： | 1 |
| 10 | Coordination properties of tris (2 - carboxy ethyl) phosphine, a newly introduced thiol reductant and its oxide 显示文摘 | Artur Krezel Rafai Latajka Grzegorz D Bujaez | 2003 | Inorg Chem2003，42，6： | 1 |
| 11 | Comparison of effects of protein kinase A,mitogen-activated protein kinase,and cyclin-dependent kinase blockers on rabbit ovarian granulosa cell functions显示文摘 | MAKAREVICH A V SIROTKIN A V RAFAY J | 2010 | Horm Metab Res2010，42，13： | 1 |
| 12 | Neurologicalmanifestations revealing primitive Gougerot-Sjogren syndrome :9cases 显示文摘 | Rafai MA Boulaajaj FZ Moutawakil F | 2009 | Joint Bone Spine2009，76，2： | 1 |
| 13 | Current surgical therapy of orbronchiectasis显示文摘 | Ashour M Kattan K Rafay MA | 1999 | World J Surg1999，23，3： | 1 |
| 14 | C-reactive protein, interleukin-6, and risk of developing type 2 diabetes mellitus 显示文摘 | Pradhan AD Manson J E Rafai N | 2001 | JAMA2001，286，： | 1 |
| 15 | Rapid redu- cation in Creactive protein with cerivastatin among 785 patients with primary hypercholesterolemia 显示文摘 | RIDKER P M RAFAI N LOWENTHAL S P | 2001 | Circula- tion2001，103，： | 1 |
| 16 | Currenl Surgical therapy for bronchiectasis显示文摘 | Ashour M AL-Kattan K Rafay MA | 1999 | World J Surg1999，23，11： | 1 |
| 17 | Mode of onset predicts etiological diagnosis of arterial ischemic stroke in children 显示文摘 | Braun KP Rafay MF Uiterwaal CS | 2007 | Stroke2007，38，2： | 1 |
| 18 | Comparison of C-reactive protein and low-density lipoprotein cholesterol levels in the prediction of first cardiovascular events显示文摘 | Ridker PM Rafai N Rose L | 2002 | N Engl J Med2002，347，20： | 1 |
| 19 | High-sensitivity C-reactive protein:a novel and promising marker of coronary hear disease显示文摘 | Rafai N Ridker PM | 2001 | Clin Chem2001，47，3： | 1 |
| 20 | Non-HDL cholesterol,Apo lipoprotein A-1 and B100 standard lipid measures,lipid ratio and CRP at risk factors for cardiovascular disease in women显示文摘 | Ridker PM Rafai N Cook NR | 2005 | JAMA2005，294，3： | 1 |
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