| 1 | Tailoring spontaneous infrared emission of HgTe quantum dots with laser-printed plasmonic arrays显示文摘Chemically synthesized near-infrared to mid-infrared(IR)colloidal quantum dots(QDs)offer a promising platform for the realization of devices including emitters,detectors,security,and sensor systems.However,at longer wavelengths,the quantum yield of such QDs decreases as the radiative emission rate drops following Fermi’s golden rule,while non-radiative recombination channels compete with light emission.Control over the radiative and non-radiative channels of the IR-emitting QDs is crucially important to improve the performance of IR-range devices.Here,we demonstrate strong enhancement of the spontaneous emission rate of near-to mid-IR HgTe QDs coupled to periodically arranged plasmonic nanoantennas,in the form of nanobumps,produced on the surface of glasssupported Au films via ablation-free direct femtosecond laser printing.The enhancement is achieved by simultaneous radiative coupling of the emission that spectrally matches the first-order lattice resonance of the arrays,as well as more efficient photoluminescence excitation provided by coupling of the pump radiation to the local surface plasmon resonances of the isolated nanoantennas.Moreover,coupling of the HgTe QDs to the lattice plasmons reduces the influence of non-radiative decay losses mediated by the formation of polarons formed between QD surface-trapped carriers and the IR absorption bands of dodecanethiol used as a ligand on the QDs,allowing us to improve the shape of the emission spectrum through a reduction in the spectral dip related to this ligand coupling.Considering the ease of the chemical synthesis and processing of the HgTe QDs combined with the scalability of the direct laser fabrication of nanoantennas with tailored plasmonic responses,our results provide an important step towards the design of IR-range devices for various applications. | A.A.Sergeev D.V.Pavlov A.A.Kuchmizhak M.V.Lapine W.K.Yiu Y.Dong N.Ke S.Juodkazis N.Zhao S.V.Kershaw A.L.Rogach | 2020 | Light(Science & Applications)2020，9，1： | 5 |
| 6 | Numerical simulation of effect of convection-diffusion on oxygen transport in microcirculation显示文摘The entire process of oxygen transport in microcirculation by developing a3 D porous media model is calculated numerically with coupled solid deformation-fluid seepage-convection and diffusion. The principal novelty of the model is that it takes into account volumetric deformation of both capillary and tissues resulting from capillary fluctuation. How solid deformation, fluid seepage, and convection-diffusion combine to affect oxygen transport is examined quantitatively:(1) Solid deformation is more significant in the middle of capillary, where the maximum value of volumetric deformation reaches about 0.5%.(2) Solid deformation has positive influence on the tissue fluid so that it flows more uniformly and causes oxygen to be transported more uniformly, and eventually impacts oxygen concentration by 0.1%–0.5%.(3) Convection-diffusion coupled deformation and seepage has a maximum(16%) and average(3%) increase in oxygen concentration,compared with pure molecular diffusion. Its more significant role is to allow oxygen to be transported more evenly. | N.ZHAO K.IRAMINA | 2015 | Applied Mathematics and Mechanics(English Edition)2015，36，2： | 0 |
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