| 1 | One-step multi-compositional oxidation of YSi alloy:Experiments and ab initio computation显示文摘YSi alloy is a promising candidate as oxidation resistant coatings for both the bond coat of environmental barrier coatings(EBCs)and anti-ablation coatings at a high temperature of∼1300℃.In this study,a one-step multi-compositional oxidation by rapid heating oxidation mode is proposed to reduce the oxidation rate by 3.6 times compared to conventional slow heating oxidation mode.Results show that preferentially formed Y_(2)O_(3) oxide initiates a multi-step oxidation,produces a cracking and porous oxides,and thereby resulting in a fast oxidation with pesting.The one-step multi-compositional oxidation with a compact and dense Y_(2)Si_(2)O_(7)scale contributes to the much better oxidation resistance for rapid heating oxidation mode of YSi alloy.The stable formation of Y_(2)Si_(2)O_(7)scale is comprehensively understood by the energy barrier,charge density and electronic level based on density functional theory.This study demonstrates a promising application of YSi alloy by rapid heating oxidation mode. | W.J.Wang J.C.Luo L.Chen G.J.Yang | 2023 | Journal of Materials Science & Technology2023，，27： | 0 |
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