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| 1 | Zircon U-Pb Ages and Hf Isotopes of Neoproterozoic Meta-Igneous Rocks in the Liansandao Area,Northern Sulu Orogen,Eastern China,and the Tectonic Implications显示文摘The Sulu Orogen preserves the Neoproterozoic tectonic-magmatic events,corresponding to the breaking up of the Rodinia supercontinent.The ages and petrogenesis of meta-igneous rocks in the Liansandao area in the northern Sulu Orogen are not well-constrained.This study reports zircon U-Pb ages and Hf isotopes of these rocks from the Liansandao area.Three meta-igneous rock samples give similar weighted mean 206 Pb/238 U ages of 744±11,767±12,and 762±15 Ma,respectively,indicating the Neoproterozoic crystallization ages.These rocks formed coevally with the Wulian and Yangkou intrusions that located along the Yantai-Qingdao-Wulian fault zone.The Neoproterozoic ages indicate that the meta-igneous rocks from the Liansandao area have affinity to the Yangtze Block.The three samples haveεHf(t)values of-7.2–-10.5,-6.0–-17.5,and-6.8–-12.0,respectively.These negativeεHf(t)values indicate a primarily crustal source.However,the widely variousεHf(t)values that are higher than the continental crust,suggesting magma mixing between mantle-derived materials and the continental crust or source heterogeneity.Combined with the Hf model ages and geochemical characteristics,the monzodiorite(sample LSD-2)is most likely to be mantle-derived magma then interacted with ancient continental crust,and the granitic protolith(samples LSD-1 and LSD-3)in the Liansandao area might derive from the re-melting of a Paleoproterozoic continental crust at^750 Ma,resulting from the upwelling and underplating of mantle-derived magma formed in an extensional setting due to the break-up of the Rodinia supercontinent. | Zhaojun Song Huimin Liu Fanxue Meng Xingyu Yuan Qiao Feng Dingwu Zhou Juan Ramon Vidal Romani Hongbo Yan | 2019 | Journal of Earth Science2019，30，6： | 4 |
| 2 | Methanol electro-oxidation to formate on iron-substituted lanthanum cobaltite perovskite oxides显示文摘Electrochemically producing formate by oxidizing methanol is a promising way to add value to methanol.Noble metal-based electrocatalysts,which have been extensively studied for the methanol oxidation reaction,can catalyze the complete oxidation of methanol to carbon dioxide,but not the mild oxidation to formate.As a result,exploring efficient and earth-abundant electrocatalysts for formate production from methanol is of interest.Herein,we present the electro-oxidation of methanol to formate,catalyzed by iron-substituted lanthanum cobaltite(LaCo_(1-x)Fe_(x)O_(3)).The Fe/Co ratio in the oxides greatly influences the activity and selectivity.This effect is attributed to the higher affinity of Fe and Co to the two reactants:CH3OH and OH,respectively.Because a balance between these affinities is favored,LaCo_(0.5)Fe_(0.5)O_(3) shows the highest formate production rate,at 24.5 mmol h^(-1) g_(oxide)^(-1),and a relatively high Faradaic efficiency of 44.4%in a series of(LaCo_(1-x)Fe_(x)O_(3))samples(x=0.00,0.25,0.50,0.75,1.00)at 1.6 V versus a reversible hydrogen electrode. | Fanxu Meng Chencheng Dai Zheng Liu Songzhu Luo Jingjie Ge Yan Duan Gao Chen Chao Wei Riccardo Ruixi Chen Jiarui Wang Daniel Mandler Zhichuan J.Xu | 2022 | eScience2022，2，1： | 1 |
| 3 | High-performance polarization-sensitive photodetectors on two-dimensionalβ-InSe显示文摘Two-dimensional(2D)indium selenide(InSe)has been widely studied for application in transistors and photodetectors,which benefit from its excellent optoelectronic properties.Among the three specific polytypes(γ-,ε-andβ-phase)of InSe,only the crystal lattice of InSe inβ-phase(β-InSe)belongs to a non-symmetry point group of D_(6 h)_^(4),which indicates stronger anisotropic transport behavior and potential in the polarized photodetection ofβ-InSe-based optoelectronic devices.Therefore,we prepare the stable p-type 2D-layeredβ-InSe via temperature gradient method.The anisotropic Raman,transport and photoresponse properties ofβ-InSe have been experimentally and theoretically proven,showing that theβ-InSe-based device has a ratio of 3.76 for the maximum to minimum dark current at two orthogonal orientations and a high photocurrent anisotropic ratio of 0.70 at 1 V bias voltage,respectively.The appealing anisotropic properties demonstrated in this work clearly identifyβ-InSe as a competitive candidate for filter-free polarization-sensitive photodetectors. | Zhinan Guo Rui Cao Huide Wang Xi Zhang Fanxu Meng Xue Chen Siyan Gao David KSang Thi Huong Nguyen Anh Tuan Duong Jinlai Zhao Yu-Jia Zeng Sunglae Cho Bing Zhao Ping-Heng Tan Han Zhang Dianyuan Fan | 2022 | National Science Review2022，9，5： | 1 |
| 4 | In-situ neutron-transmutation for substitutional doping in 2D layered indium selenide based phototransistor显示文摘Neutron-transmutation doping(NTD)has been demonstrated for the first time in this work for substitutional introduction of tin(Sn)shallow donors into two-dimensional(2D)layered indium selenide(InSe)to manipulate electron transfer and charge carrier dynamics.Multidisciplinary study including density functional theory,transient optical absorption,and FET devices have been carried out to reveal that the field effect electron mobility of the fabricated phototransistor is increased 100-fold due to the smaller electron effective mass and longer electron life time in the Sn-doped InSe.The responsivity of the Sn-doped InSe based phototransistor is accordingly enhanced by about 50 times,being as high as 397 A/W.The results show that NTD is a highly effective and controllable doping method,possessing good compatibility with the semiconductor manufacturing process,even after device fabrication,and can be carried out without introducing any contamination,which is radically different from traditional doping methods. | Zhinan Guo Yonghong Zeng Fanxu Meng Hengze Qu Shengli Zhang Shipeng Hu Sidi Fan Haibo Zeng Rui Cao Paras N.Prasad Dianyuan Fan Han Zhang | 2022 | eLight2022，2，1： | 1 |
| 5 | Performance improvement of inverted polymer solar cells thermally evaporating nickel oxide as an anode buffer layer显示文摘 | Wenjuan Yu Liang Shen Shengping Ruan Fanxu Meng Jialue Wang Enrui Zhang Weiyou Chen | 2011 | Solar Energy Materials and Solar Cells2011，，： | 1 |
| 6 | Decoupling of Lu-Hf and Sm-Nd Isotopic System in Deep-Seated Xenoliths from the Xuzhou-Suzhou Area,China: Differences in Element Mobility during Metamorphism显示文摘This paper presents whole-rock Hf isotopic data for a suite of eclogite and garnet clinopyroxenite xenoliths hosted in the Early Cretaceous dioritic intrusions from the Xuzhou-Suzhou area along the southeastern margin of the Eastern Block of the North China Craton(NCC).Six of the eight studied xenolith samples plot significantly above the terrestrial Hf-Nd isotopic array and haveεHf(0)value up to+60.All the samples define a well correlated 147 Sm/144 Nd-143 Nd/144 Nd age of 2081 Ma,which is considered to record the granulite-facies metamorphism.In contrast,the Lu-Hf isotope system faithfully records the protolith information.The mineralogical assemblage,especially garnet and/or zircon(rutile to some extent)mainly controlled the decoupling of Hf-Nd isotope.The metamorphic modification on protolith characteristics and the differences in element mobility during metamorphism may also reinforce the observed decoupling between the Sm-Nd and Lu-Hf isotope systems;i.e.,the absence of the correlations inεNd-εHf and also 87 Sr/86 Sr-143 Nd/144 Nd diagram.The Lu/Hf isochron age of 2424 Ma is similar to the zircon age peak of the studied xenoliths and the dominant age of NCC basement,indicating that the igneous protolith has an affinity to the Archean basement of the NCC.Furthermore,the positiveεHf(t)values at 2500 Ma indicate a crustal growth event of 2500 Ma in the NCC. | Fanxue Meng Wenliang Xu Qinglin Xu Jingliang Guo Yu Zhang | 2019 | Journal of Earth Science2019，30，6： | 1 |
| 7 | Interlayer sensitized van der Waals heterojunction photodetector with enhanced performance显示文摘Although photodetection based on two-dimensional(2D)van der Waals(vdWs)P-N heterojunction has attracted extensive attention recently,their low responsivity(R)due to the lack of carrier gain mechanism in reverse bias or zero bias operation hinders their applications in advanced photodetection area.Here,a black phosphorus/rhodamine 6G/molybdenum disulfide(BP/R6G/MoS_(2))photodiode with high responsivity at reverse bias or zero bias has been achieved by using interfacial charge transfer of R6G molecules assembled between heterojunction layers.The formed vdWs interface achieves high performance photoresponse by efficiently separating the additional photogenerated electrons and holes generated by R6G molecules.The devices sensitized by the dye molecule R6G exhibit enhanced photodetection performance without sacrificing the photoresponse speed.Among them,the R increased by 14.8-20.4 times,and the specific detectivity(D^(*))increased by 24.9-34.4 times.The strategy based on interlayer assembly of dye molecules proposed here may pave a new way for realizing high-performance photodetection based on 2D vdWs heterojunctions with high responsivity and fast response speed. | Huide Wang Yonghong Zeng FanXu Meng Rui Cao Yi Liu Zhinan Guo Tingting Wang Haiguo Hu Sidi Fan Yatao Yang SWageh Omar AAl-Hartomy Abul Kalam Yonghong Shao Yu-Jia Zeng Dianyuan Fan Han Zhang | 2023 | Nano Research2023，16，7： | 0 |
| 8 | Fully depleted vdW heterojunction based high performance photovoltaic photodetector显示文摘Van der Waals(vdW)heterojunctions,with their unique electronic and optoelectronic properties,have become promising candidates for photodetector applications.Amplifying the contribution of the depletion region in vdW heterojunction,which would enhance both of the collection efficiency and speed of the photogenerated carriers,presents an effective strategy for achieving high performance vdW heterojunction photodetectors.Herein,a fully depleted vdW heterojunction photodetector is built on two-dimensional(2D)semiconductor materials(GaTe and InSe)layered on a pattered bottom electrode in vertical structure,in which the generation and motion of carriers are exclusively achieved in the depletion region.Attributed to the intrinsic built-in electric field,the elimination of series resistance and the depletion region confinement of carriers,the as-fabricated photodetector exhibits prominent photovoltaic properties with a high open-circuit voltage of 0.465 V,as well as photoresponse characteristics with outstanding responsivity,detectivity and photoresponse speed of 63.7 A/W,3.88×10^(13)Jones,and 32.7 ms respectively.The overall performance of this fully depleted GaTe/InSe vdW heterojunctions photodetectors are ranking high among the top level of 2D materials based photodetectors.It indicates the device architecture can provide new opportunities for the fabrication of high-performance photodetectors. | Yonghong Zeng Fanxu Meng Sidi Fan Pengfei Wang Cuiyun Kou Mingyi Sun Haiguo Hu Rui Cao Swelm Wageh Omar A.Al-Hartomy Abul Kalam Bowen Du Wenchao Ding Songrui Wei Zhinan Guo Qiuliang Wang Han Zhang | 2023 | Journal of Materiomics2023，9，6： | 0 |
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