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| 1 | Enhancing hydrogen evolution on the basal plane of transition metal dichacolgenide van der Waals heterostructures显示文摘Recent years have seen a surge in the use of low-dimensional transition metal dichacolgenides,such as MoS_(2),as catalysts for the electrochemical hydrogen evolution reaction.In particular,sulfur vacancies in MoS_(2)can activate the inert basal plane,but that requires an unrealistically high defect concentration(~9%)to achieve optimal activity.In this work,we demonstrate by firstprinciples calculations that assembling van der Waals heterostructures can enhance the catalytic activity of MoS_(2)with low concentrations of sulfur vacancies.We integrate MoS_(2)with various two-dimensional nanostructures,including graphene,h-BN,phosphorene,transition metal dichacolgenides,MXenes,and their derivatives,aiming to fine-tune the free energy of atomic hydrogen adsorption.Remarkably,an optimal free energy can be achieved for a low sulfur vacancy concentration of~2.5%in the MoS_(2)/MXene-OH heterostructure,as well as high porosity and tunability.These results demonstrate the potential of combining two-dimensional van der Waals assembly with defect engineering for efficient hydrogen production. | Faling Ling Wei Kang Huirong Jing Wen Zeng Yankun Chen Xiaoqing Liu Yixin Zhang Lin Qi Liang Fang Miao Zhou | 2019 | npj Computational Materials2019，，1： | 2 |
| 2 | The assimilation and degradation of carbohydrates by yeast cells显示文摘 | Fales F W | 1951 | Journal of Biological Chemistry1951，193，1： | 1 |
| 3 | Hydroxypropy-β- cyclodextrin: preparationand characterization; effects on solubility of drugs显示文摘 | PITHA J MILECKI J FALES H | 1986 | International Journal of Pharma- ceutics1986，29，1： | 1 |
| 4 | Modeling and Control of a Wheel Loader With a Human - in - the - Loop Assessment Using Virtual Reality 显示文摘 | Roger Fales Erik Spencer Kurt Chipperfield Frank Wagner Atul Kelkar | 2005 | Journal of Dynamic Systems Measurement and Control2005，127，3： | 1 |
| 5 | Decision criteria for the exploration of ornamental-stone deposits: Application to the marbles of the Portuguese estremoz anticline 显示文摘 | CARVALHO J F HENRIQUES P FALE P LUIS G | 2008 | International Journal of Rock Mechanics and Mining Sciences2008，45，8： | 1 |
| 6 | Chemical Composition and Biodegradability of Crop Residues Colonized by White-rot Fungi 显示文摘 | Karunanandaa K Fales S L Varga G A | 1992 | J Sci Food Agric1992，60，： | 1 |
| 7 | Surface-enhanced Raman scattering molecular sentinel nanoprobes for viral infection diagnostics显示文摘 | Wang H Fales A M Zaas A K | 2013 | Analytica Chimiea Acta2013，786，： | 1 |
| 8 | Anxiety and cognitive efficiency:Differential modulation of transient and sustained neural activity during a working memory task显示文摘 | Fales C.L Barch D.M Burgess G.C Schaefer A Mennin D.S Gray J.R & Braver T.S | | 0，，03： | 1 |
| 9 | Antioxidant capacity and phenolic contents of some Mediterranean medicinal plants and their potential role in the inhibition of cyclooxygenase-I and acetylcholinesterase activities 显示文摘 | Ouchemoukh NA Madani K Fale PLV | 2014 | Industrial Crops and Products2014，53，1： | 1 |
| 10 | Emotional-stimulus processing in trait anxiety is modulated by stimulus valence during neuroimaging of a working-memory task显示文摘 | Fales C.L Becerril K.E Luking K.R Barch D.M | | 0，，02： | 1 |
| 11 | Information-Theoretic Assessment of Sampled Imaging System显示文摘 | Huck F O Fales C l Alter-Gratenberg R | 1999 | Optional Engineering1999，38，5： | 1 |
| 12 | A fiberoptic bronchoscopy technique to obtain uncontaminated lower airway secretions for bacterial culture 显示文摘 | Wimberley N Faling LJ Bartlett JG | 1979 | Am Rev Respir Dis1979，119，3： | 1 |
| 13 | Design and analysis of a two stage poppet valve for flow control显示文摘 | Muller M T Fales R C | 2014 | International Journal of Fluid Power2014，9，1： | 1 |
| 14 | Control-theoretic Analysis of a Closed Loop PPC System显示文摘 | Duffle N Fale I | 2002 | Annals of the CIRP2002，52，1： | 1 |
| 15 | Reducing moisture induced error associated with measuring forage quality using near infrared reflectance显示文摘 | FALES S L CUMMINS D G | 1982 | Agronomy Journal1982，74，： | 1 |
| 16 | Fluid stress measurements of magnetorheological fluids in tubes显示文摘 | Dang A Ooi L Fales J | 2000 | Industr Eng Chem Res2000，39，7： | 1 |
| 17 | Uncertainty modeling and predicting the probability of stability and performance in the manufacture of dynamic systems显示文摘 | Fales R | 2010 | Isa Transactions2010，49，4： | 1 |
| 18 | Information-theoretical assessment of sampled imaging systems显示文摘 | HUCK F O FALES C L ALTER-GARTENBERG R | 1999 | SPIE Optical Engineering1999，38，5： | 1 |
| 19 | Yield and composition of herbaceous biomass harvested from naturalized grassland in southern Iowa显示文摘 | Florine S E Moore K J Fales S L | 2006 | Biomass and Bioenergy2006，30，6： | 1 |
| 20 | Image-gathering system design for information and fidelity显示文摘 | HUCK F O FALES C L McCormick J A | 1988 | J Opt Soc Am1988，5，： | 1 |
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