|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Polymer-based EMI shielding composites with 3D conductive networks:A mini-review显示文摘High-frequency electromagnetic waves and electronic products can bring great convenience to people’s life,but lead to a series of electromagnetic interference(EMI)problems,such as great potential dangers to the normal operation of elec-tronic components and human safety.Therefore,the research of EMI shield-ing materials has attracted extensive attention by the scholars.Among them,polymer-based EMI shielding materials with light weight,high specific strength,and stable properties have become the current mainstream.The construction of 3D conductive networks has proved to be an effective method for the prepara-tion of polymer-based EMI shielding materials with excellent shielding effective-ness(SE).In this paper,the shielding mechanism of polymer-based EMI shield-ing materials with 3D conductive networks is briefly introduced,with emphasis on the preparation methods and latest research progress of polymer-based EMI shielding materials with different 3D conductive networks.The key scientific and technical problems to be solved in the field of polymer-based EMI shielding materials are also put forward.Finally,the development trend and application prospects of polymer-based EMI shielding materials are prospected. | Lei Wang Zhonglei Ma Yali Zhang Lixin Chen Dapeng Cao Junwei Gu | 2021 | SusMat2021，1，3： | 22 |
| 2 | A perspective on sustainable energy materials for lithium batteries显示文摘Lithium ion battery has achieved great success in portable electronics and even recently electronic vehicles since its commercialization in 1990s.However,lithium-ion batteries are confronted with several issues in terms of the sustainable development such as the high price of raw materials and electronic products,the emerging safety accidents,etc.The recent progresses are herein emphasized on lithium batteries for energy storage to clearly understand the sustainable energy chemistry and emerging energymaterials.The Perspective presents novel lithium-ion batteries developed with the aims of enhancing the electrochemical performance and sustainability of energy storage systems.First,revolutionary material chemistries,including novel low-cobalt cathode,organic electrode,and aqueous electrolyte,are discussed.Then,the characteristics of safety performance are analyzed and strategies to enhance safety are subsequently evaluated.Battery recycling is considered as the key factor for a sustainable society and related technologies are present as well.Finally,conclusion and outlook are drawn to shed lights on the further development of sustainable lithium-ion batteries. | Xin-Bing Cheng He Liu Hong Yuan Hong-Jie Peng Cheng Tang Jia-Qi Huang Qiang Zhang | 2021 | SusMat2021，1，1： | 14 |
| 3 | Progress in the sustainable recycling of spent lithium-ion batteries显示文摘Lithium-ion batteries(LIBs)are booming in multiple fields due to a rapid devel-opment in the last decade.However,limited by operational lifespans,a grow-ing number of spent LIBs reaching the end of their lives are consequently faced with serious accumulation and descended to hazardous waste.Without proper disposal,the spent LIBs will inevitably cause negative influence on the ecol-ogy and undermine the sustainable manufacture of LIBs.The initial research of recycling strategies mainly focused on the optimization of metallurgical pro-cesses.Recently,the sustainability of the recycling process has attracted much more attention and become an important factor.Here,we summarize the recent progress of the spent LIBs recycling from a sustainable perspective,especially discussing the green innovations in recycling strategies for spent LIBs.Through this article,we expect to reveal the challenges and developing tendency of the recycling strategies and provide a guideline for future researches on process-ing spent LIBs and beyond,like the recycling of the solid-state lithium metal batteries. | Min Fan Xin Chang Qinghai Meng Li-Jun Wan Yu-Guo Guo | 2021 | SusMat2021，1，2： | 7 |
| 4 | Demystifying the catalysis in lithium–sulfur batteries:Characterizationmethods and techniques显示文摘Lithium–sulfur(Li-S)batteries are promising next-generation energy storage systems with ultrahigh energy density.However,the intrinsic sluggish“solid–liquid–solid”reaction between S8 and Li2S causes unavoidable shuttling of polysulfides,severely limiting the practical energy density and cycling performance.Recently,the catalysis process has been introduced for the sulfur redox reaction to accelerate the conversion of polysulfides,providing a positive remedy for the polysulfides shuttling.Nevertheless,in-depth understanding of the catalyst evaluation criteria and catalytic mechanism still lies in the“black box”,and precise characterization technique is the key to unlock this puzzle.In this review,we provide a comprehensive overview of characterization techniques on the catalyst in Li-S batteries from two aspects of catalytic performance and catalytic mechanism,highlighting their significance and calling for more efforts to develop precise and fast techniques for Li-S catalysis.Moreover,we envision the future development of characterization for better understanding the catalysis toward practical Li-S battery. | Chuannan Geng Wuxing Hua DaweiWang Guowei Ling Chen Zhang Quan-Hong Yang | 2021 | SusMat2021，1，1： | 6 |
| 5 | Dendrite-accelerated thermal runaway mechanisms of lithium metal pouch batteries显示文摘High-energy-density lithium metal batteries(LMBs)are widely accepted as promising next-generation energy storage systems.However,the safety features of practical LMBs are rarely explored quantitatively.Herein,the thermal runaway behaviors of a 3.26 Ah(343 Wh kg^(−1))Li|LiNi_(0.5)Co_(0.2)Mn_(0.3)O_(2)pouch cell in the whole life cycle are quantitatively investigated by extended volume-accelerating rate calorimetry and differential scanning calorimetry.By thermal failure analyses on pristine cell with fresh Li metal,activated cell with once plated dendrites,and 20-cycled cell with large quantities of dendrites and dead Li,dendrite-accelerated thermal runaway mechanisms including reaction sequence and heat release contribution are reached.Suppressing dendrite growth and reducing the reactivity between Li metal anode and electrolyte at high temperature are effective strategies to enhance the safety performance of LMBs.These findings can largely enhance the understanding on the thermal runaway behaviors of Li metal pouch cells in practical working conditions. | Xiang-Qun Xu Xin-Bing Cheng Feng-Ni Jiang Shi-Jie Yang Dongsheng Ren Peng Shi HungJen Hsu Hong Yuan Jia-Qi Huang Minggao Ouyang Qiang Zhang | 2022 | SusMat2022，2，4： | 6 |
| 6 | Recent progress on precious metal single atom materials for water splitting catalysis显示文摘Electrochemical water splitting for hydrogen production has sparked intensive interests because it provides a new approach for sustainable energy resources and the avoidance of environmental problems.The precious metal-based sin-gle atomic catalysts(PMSACs)have been widely employed in water splitting catalysis by virtue of their maximum atom utilization and unique electronic structure,which can reduce metal amounts and remain high catalytic perfor-mance simultaneously.In this review,we will summarize recent research efforts toward developing SACs based on precious metals with excellent performance for electrochemical water splitting catalysis.First,the synthesis strategies for PMSACs will be classified and introduced including high-temperature pyrolysis,electrochemical method,photochemical reduction,wet chemistry method,etc.Then,a short description of characterization techniques for SACs will be given,which mainly involves the aberration-corrected scanning-transmission electron microscopy(AC-STEM)and X-ray absorption spectroscopy(XAS).In particular,the relationship between the electronic structure of the precious metal atomic sites and performance for water splitting will be discussed according to the the-oretical and experimental results.Finally,a brief perspective will be provided to highlight the challenges and opportunities for the development of novel PMSACs suitable for electrochemical water splitting applications. | Lei Zhou Shi-Yu Lu Shaojun Guo | 2021 | SusMat2021，1，2： | 6 |
| 7 | Advances in metal phosphides for sodium-ion batteries显示文摘Sodium-ion batteries(SIBs)have been extensively studied as the potential alter-native to lithium-ion batteries(LIBs)due to the abundant natural reserves and low price of sodium resources.Nevertheless,Na+ions possess a larger radius than Li+,resulting in slow diffusion dynamics in electrode materials,and thus seeking appropriate anode materials to meet high performance standards has become a trend in the field of SIBs.In this context,owing to the advantages of high theoretical capacity and proper redox potential,metal phosphides(MPs)are considered to be the promising materials to make up for the gap of SIBs anode materials.In this review,the recent development of MPs anode materials for SIBs is reviewed and analyzed comprehensively and deeply,including the synthesis method,advanced modification strategy,electrochemical performance,and Na storage mechanism.In addition,to promote the wide application of the emerg-ing MPs anodes for SIBs,several research emphases in the future are pointed out to overcome challenges toward the commercial application. | Qifei Li Dan Yang Haoliang Chen Xiang Lv Yu Jiang Yuezhan Feng Xianhong Rui Yan Yu | 2021 | SusMat2021，1，3： | 5 |
| 8 | Mechanism understanding for stripping electrochemistry of Li metal anode显示文摘The pursuit of sustainable energy has a great request for advanced energy stor-age devices.Lithium metal batteries are regarded as a potential electrochemi-cal storage system because of the extremely high capacity and the most nega-tive electrochemical potential of lithium metal anode.Dead lithium formed in the stripping process significantly contributes to the low efficiency and short lifespan of rechargeable lithium metal batteries.This review displays a critical review on the current research status about the stripping electrochemistry of lithium metal anode.The significance of stripping process to a robust lithium metal anode is emphasized.The stripping models in different electrochemical scenarios are discussed.Specific attention is paid to the understanding for the electrochemical principles of atom diffusion,electrochemical reaction,ion dif-fusion in solid electrolyte interphase(SEI),and electron transfer with the pur-pose to strengthen the insights into the behavior of lithium electrode stripping.The factors affecting stripping processes and corresponding solutions are sum-marized and categorized as follows:surface physics,SEI,operational and exter-nal factors.This review affords fresh insights to explore the lithium anode and design robust lithium metal batteries based on the comprehensive understand-ing of the stripping electrochemistry. | Feng-Ni Jiang Shi-Jie Yang He Liu Xin-Bing Cheng Lei Liu Rong Xiang Qiang Zhang Stefan Kaskel Jia-Qi Huang | 2021 | SusMat2021，1，4： | 5 |
| 9 | Recent advances in high-loading catalysts for low-temperature fuel cells: From nanoparticle to single atom显示文摘Low-temperature fuel cells(LTFCs)are considered to be one of the most promising power sources for widespread application in sustainable and renew-able energy conversion technologies.Although remarkable advances have been made in the mass activity of catalysts,mass transport impedance needs to be urgently addressed at a well-designed membrane electrode assembly(MEA)scale.Increasing the loading of electrocatalysts is conducive to prepare thinner and more efficient MEAs owing to the resulting enhanced reactant permeability,better proton diffusion,and lower electrical resistance.Herein,recent progress in high-loading(≥40 wt.%)Pt nanoparticle catalysts(NPCs)and high-loading(≥2 wt.%)single-atom catalysts(SACs)for LTFC applications are reviewed.A summary of various synthetic approaches and support materials for high-loading Pt NPCs and SACs is systematically presented.The influences of high surface area and appropriate surface functionalization for Pt NPCs,as well as coordina-tion environment,spatial confinement effect,and strong metal-support interac-tions(SMSI)for SACs are highlighted.Additionally,this review presents some ideas regarding challenges and future opportunities of high-loading catalysts in the application of LTFCs. | Lixiao Shen Miao Ma Fengdi Tu Zigang Zhao Yunfei Xia Kokswee Goh Lei Zhao Zhenbo Wang Guangjie Shao | 2021 | SusMat2021，1，4： | 3 |
| 10 | Recent advances in vacancy engineering of metal-organic frameworks and their derivatives for electrocatalysis显示文摘The efficient electrocatalysis plays the key role in the development of electrochemical energy conversion technologies to alleviate energy crisis.Given their multiple active sites and large specific surface areas as electrocatalysts,metalorganic frameworks(MOFs)and their derivatives have attracted considerable interests in recent years.Specially,exploring the roles of the enhanced active sites inMOFs and their derivatives is significant for understanding and developing new effective electrocatalysts.Recently,the vital role of vacancies has been proven to promote electrocatalytic processes(such as H2 or O2 evolution reactions,O2 reduction reactions,and N2 reduction reactions).In order to in-depth exploring the effect of vacancies in electrocatalysts,the vacancies classification,synthetic strategy,and the recent development of various vacancies inMOFs and their derivatives for electrocatalysis are reviewed.Also,the perspectives on the challenges and opportunities of vacancies inMOFs and their derivatives for electrocatalysis are presented. | Yuhang Wu Yuwen Li Junkuo Gao Qichun Zhang | 2021 | SusMat2021，1，1： | 3 |
| 11 | Recent advances in highly integrated energy conversion and storage system显示文摘The vigorous development in the field of energy conversion and storage devices directly contributes to the full utilization and convenient use of clean energy.However,some drawbacks of independent energy conversion and storage devices,including unstable,insufficient energy output and dependence on external power supply,are difficult to overcome by self-optimization,thus,hindering their further development and direct application.Coincidentally,the combination of above two devices can solve these problems,which conforms to their intrinsic needs for development.At the same time,the pursuit of portability and miniaturization also promotes the development of the power system toward a highly integrated direction.Therefore,we introduce several integration modes of energy conversion and storage systems,with emphasis on all-in-one power system,possessing the highest integration in this review.From the aspect of device configuration,working mechanisms and their performances,the all-inone power systems based on different energy sources(e.g.,mechanical,solar,thermal,and chemical energy)are discussed and analyzed.Finally,the design strategies are summarized and the potential development directions in the future are proposed.This review aims to provide a comprehensive overview of highly integrated energy conversion and storage system,and seeks to point out the opportunities and orientations of future research in this field. | Changxiang Shao Yang Zhao Liangti Qu | 2022 | SusMat2022，2，2： | 3 |
| 12 | Recent advances in functional fiber electronics显示文摘Rapid development ofwearable electronicswith various functionalities has stimulated the demand to construct functional fiber devices due to their merits of mechanical flexibility,weavability,miniaturization,and integrability.To this end,fiber components which can realize the functions of energy storage and conversion,actuating plus sensing have gained increasing concerns.Herein,we summarize the recent progress with respect to fiber material preparation,innovative structure design,and device performance in this review,also highlighting the possibility of integrated fiber electronics as an extension of application,the remaining challenges and future perspectives toward next-generation smart systems and to facilitate their commercialization. | Xiaopei Zhang Huijuan Lin Huan Shang Jingsan Xu Jixin Zhu Wei Huang | 2021 | SusMat2021，1，1： | 3 |
| 13 | Issues and rational design of aqueous electrolyte for Zn-ion batteries显示文摘Aqueous Zn-ion batteries(AZIBs)are regarded as a promising alternative to the widely used lithium-ion batteries in large-scale energy storage systems.The researches on the development of novel aqueous electrolyte to improve battery performance have also attracted great interest since the electrolyte is a key com-ponent for Zn2+migration between cathode and anode.Herein,we briefly sum-marized and illuminated the recent development tendency of aqueous electrolyte for AZIBs,then deeply analyzed its existing issues(water decomposition,cathode dissolution,corrosion and passivation,and dendrite growth)and discussed the corresponding optimization strategies(pH regulation,concentrated salt solution,electrolyte composition design,and functional additives).The internal mecha-nisms of these strategies were further revealed and the relationships between issues and solutions were clarified,which could guide the future development of aqueous electrolytes for AZIBs. | Qi Zhang Zefang Yang Huimin Ji Xiaohui Zeng Yougen Tang Dan Sun Haiyan Wang | 2021 | SusMat2021，1，3： | 3 |
| 14 | Renewable biomass-derived carbons for electrochemical capacitor applications显示文摘Biomass is rich,renewable,sustainable,and green resources,thereby excellent raw material for the fabrication of carbon materials.The diversity in structure and morphology of biomass are relevant in obtaining carbon materials with dif-ferent structures and performances.The inherent ordered porous structure of biomass also benefits the activation process to yield porous carbons with ultra-high specific surface area and pore volume.Besides,obtained biomass-derived carbons(BDCs)are hard carbon with porous morphology,stable structure,supe-rior hardness/strength,and good cycling performances when used in electro-chemical capacitors(ECs).The inherent N,S,P,and O elements in biomass yield naturally self-doped N,S,P,and O BDCs with unique intrinsic structures.In this paper,the synthesis approaches and applications of BDCs in ECs are reviewed.It shows that BDCs electrochemical performances are highly determined by their pore structures,specific surface areas,heteroatoms doping,graphitization degree,defects,and morphologies.The electrochemical performances of BDCs can further be improved by compositing with other materials,such as graphene,carbon nanofibers/nanotubes,transition metal oxides or hydroxides,and con-ducting polymers.The future challenges and outlooks of BDCs are also provided. | Xianyou Luo Shaorui Chen Tianzhao Hu Yong Chen Feng Li | 2021 | SusMat2021，1，2： | 3 |
| 15 | Electrolyte and anode-electrolyte interphase in solid-state lithium metal polymer batteries:A perspective显示文摘The interest for solid-state lithium metal(Li◦)batteries(SSLMBs)has been growing exponentially in recent years in view of their higher energy density and eliminated safety concerns.Solid polymer electrolytes(SPEs)are soft ionic conductors which can be easily processed into thin films at industrial level;these unique features confer solid-state Li◦polymer batteries(SSLMPBs,i.e.,SSLMBs utilizing SPEs as electrolytes)distinct advantages compared to SSLMBs containing other electrolytes.In this article,we briefly review recent progresses and achievements in SSLMPBs including the improvement of ionic conductivity of SPEs and their interfacial stability with Li◦anode.Moreover,we outline several advanced in-situ and ex-situ characterizing techniques which could assist in-depth understanding of the anode-electrolyte interphases in SSLMPBs.This article is hoped not only to update the state-of-the-art in the research on SSLMPBs but also to bring intriguing insights that could improve the fundamental properties(e.g.,transport,dendrite formation,and growth,etc.)and electrochemical performance of SSLMPBs. | Heng Zhang Yuhui Chen Chunmei Li Michel Armand | 2021 | SusMat2021，1，1： | 2 |
| 16 | Interface science in polymer-based composite solid electrolytes in lithium metal batteries显示文摘Solid-state lithium metal batteries(SSLMBs)have attracted considerable attention as one of the most promising energy storage systems owing to their high safety and energy density.Solid electrolytes,particularly polymer-based composite solid electrolytes(CSEs),are considered promising electrolyte candidates for SSLMBs.However,theirwide application is inhibited by various electrochemical issues,such as low ionic conductivity,the growth of lithium dendrites,and poor cycling stability,which are related to interface issues within SSLMBs.In this review,the parameters related to various interfaces in the CSE of SSLMBs,including the interfaces between the polymer matrix and inorganic fillers,between the CSEs and the cathode,and between the CSEs and the lithium metal anode,are examined.Relevant issues and corresponding remediation strategies are proposed.Finally,future perspectives based on interfacial engineering and the characterization of polymer/inorganic filler interactions are proposed for building high-performance CSEs for use in SSLMBs. | Lingqiao Wu Yongtao Wang Xianwei Guo Peipei Ding Zhiyuan Lin Haijun Yu | 2022 | SusMat2022，2，3： | 2 |
| 17 | A facile,scalable,high stability Lithium metal anode显示文摘Li has garnered enormous attention for next-generation Limetal batteries owing to its remarkable theoretical capacity.Unfortunately,as an anode,Li suffers from serious safety issues and fast capacity fading due to the formation of Li dendrites,which hinders the practical application of Li anode.Herein,a LiAlO_(2)-PVDF composite modification layer is fabricated on the surface of Li metal to enhance its stability and electrochemical performance.Benefitting fromthe synergetic effects of high Li+conductivity,high Li+transference number,excellent mechanical properties,superior chemical durability,and compactness of the modification layer,the LiAlO_(2)-PVDF@Li electrode delivers an ultra-long lifespan and a high capacity retention rate in the LiAlO2-PVDF@Li│LiFePO_(4) full cell.The proposed strategy provides a new alternative anode for Li metal batteries with high performance and scalable production. | Qiang Zhao Xin Chen Wang Hou Beirong Ye Yongqi Zhang Xinhui Xia Jinshu Wang | 2022 | SusMat2022，2，1： | 2 |
| 18 | Carbon dioxide copolymers:Emerging sustainable materials for versatile applications显示文摘Carbon dioxide(CO_(2))is cheap,renewable,abundant,and nontoxic carbon feedstocks in chemical reactions.In the past two decades,utilization of CO_(2)in polymer science has become a meaningful topic bridging two separate subjects,namely CO_(2)valorization and sustainable polymer synthesis.This review summarizes the recent progress in CO_(2)copolymer materials from synthesis to material performance adjustment,focusing on commercialized or potential commodity sustainable materials such as biodegradable polycarbonates and new structure polyurethanes from CO_(2)-polyol building blocks. | Han Cao Xianhong Wang | 2021 | SusMat2021，1，1： | 2 |
| 19 | Recent advances in fire-retardant carbon-based polymeric nanocomposites through fighting free radicals显示文摘Polymeric materials are ubiquitously utilized in modern society and continuously improve quality of life.Unfortunately,most of them suffer from intrinsic flammability,significantly limiting their practical applications.Fundamentally,free-radical reaction is a critical“trigger”for their thermal pyrolysis and following combustion process regardless of the anaerobic thermal pyrolysis in the condensed phase or aerobic combustion of polymers in the gaseous phase.The addition of free radical scavengers represents a promising and effective means to enhance the fire safety of polymeric materials.This review aims to offer a state-of-the-art overview on the creation of fire-retardant polymeric nanocomposites by adding fire retardants with an ability to trap free radicals.Their specific modes of action(condensed-phase action,gaseous-phase action,and dual-phases action)and performances in some typical polymers are reviewed and discussed in detail.Following this,some key challenges associated with these free-radical capturers are discussed,and design strategies are also proposed.This review provides some insights into the modes of action of free radical capturing agents and paves the avenue for the design of advanced fire-retardant polymeric nanocomposites for expanded real-world applications in industries. | Ting Sai Shiya Ran Zhenghong Guo Pingan Song Zhengping Fang | 2022 | SusMat2022，2，4： | 2 |
| 20 | Regulating closed pore structure enables significantly improved sodium storage for hard carbon pyrolyzing at relatively low temperature显示文摘The closed pore has been considered as the key structure for Na ion storage in hard carbon.However,the traditional view is that closed pores can only be formed by the curling of graphite-like crystallites in the case of high temperature carbonization.Ingenious designing of closed pore structures at lower temperature is still blank.Herein,for the first time,engineering the wall thickness and number of closed pores in waste rosewood-derived hard carbon was successfully achieved at a low temperature of 1100℃ by removing the lignin and hemicellulose components in wood precursor.When applied as an anode material,the optimum sample exhibits a high capacity of 326 mAh/g at 20 mA/g and a remarkable rate capability of 230mAh/g at 5000 mA/g,significantly higher than those of the untreated sample(only 33 mAh/g at 5000 mA/g).The significantly improved Na storage performance should be attributed to abundant closed pores that provide sufficient spaces forNa storage and thin porewall structure that is beneficial to the diffusion of Na^(+)in the bulk phase.This work provides a new idea for the future application of biomass-based hard carbon for advanced Na ion batteries. | Siyu Zhou Zheng Tang Zhiyi Pan Yuancheng Huang Le Zhao Xi Zhang Dan Sun Yougen Tang Abdelghaffar S.Dhmees Haiyan Wang | 2022 | SusMat2022，2，3： | 2 |
您所在的机构暂未开通此部分的功能，请联系管理员