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| 1 | Advances of Electrochemical and Electrochemiluminescent Sensors Based on Covalent Organic Frameworks显示文摘Covalent organic frameworks(COFs),a rapidly developing category of crystalline conjugated organic polymers,possess highly ordered structures,large specific surface areas,stable chemical properties,and tunable pore microenvironments.Since the first report of boroxine/boronate ester-linked COFs in 2005,COFs have rapidly gained popularity,showing important application prospects in various fields,such as sensing,catalysis,separation,and energy storage.Among them,COFs-based electrochemical(EC)sensors with upgraded analytical performance are arousing extensive interest.In this review,therefore,we summarize the basic properties and the general synthesis methods of COFs used in the field of electroanalytical chemistry,with special emphasis on their usages in the fabrication of chemical sensors,ions sensors,immunosensors,and aptasensors.Notably,the emerged COFs in the electrochemiluminescence(ECL)realm are thoroughly covered along with their preliminary applications.Additionally,final conclusions on state-of-the-art COFs are provided in terms of EC and ECL sensors,as well as challenges and prospects for extending and improving the research and applications of COFs in electroanalytical chemistry. | Yue Cao Ru Wu Yan‑Yan Gao Yang Zhou Jun‑Jie Zhu | 2024 | Nano-Micro Letters2024，16，2： | 0 |
| 2 | 金属有机框架材料的合成及在电催化反应中的应用显示文摘电催化反应在现代储能和转化中扮演关键角色,先进的电催化剂有助于降低电化学反应过程的能耗并提高反应效率。金属有机框架材料(MOFs)由有机连接体和金属节点构建而成,因其具备高比表面积、大孔隙率、可调谐孔径和灵活功能,成为备受瞩目的多孔晶体材料之一,同时在电催化研究领域获得广泛的探索。介绍了MOFs材料的设计理念和合成方法,探讨其在电催化反应中的应用和提升相应领域内MOFs材料活性的主要研究方向,主要涵盖HER、OER、ORR和CO_(2)RR领域。此外,还总结了提高MOFs材料电催化性能的基本原则,探讨了该快速发展领域面临的挑战和未来发展方向。 | 徐广坡 刘欧阳 | 2023 | 化肥设计2023，61，4： | 0 |
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