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| 1 | Self-assembly tungsten selenide hybrid ternary MOF derived magnetic alloys via multi-polarization to boost microwave absorption显示文摘Confronted with severe electromagnetic wave pollution,the development of high-performance electromagnetic wave shielding or absorbing materials is an effective way to deal with it.Notably,double transition metal alloys and transition metal dichalcogenides have attracted extensive attention in electromagnetic wave absorption,but few reports have studied the effects of these two materials on electromagnetic wave absorption at the same time.In this work,cobalt-based alloy with magnetic loss mechanism was selected for composition optimization.The ternary metal-organic framework was prepared by the one-step method,and then CoCu/C was prepared by high temperature annealing.Finally,in the hydrothermal process,ultra-thin tungsten selenide nanosheets were coated on the surface of magnetic component,and the final polyhedral WSe_(2)/CoCu/C composites with multiple heterogeneous interfaces were obtained.The synergistic effect of dielectric and magnetic components optimizes impedance matching and allows more electromagnetic waves to enter the absorber.Subsequently,through the conduction loss of high conductivity graphitized carbon,interfacial polarization,and dipole polarization of heterogeneous interfaces between the components,the magnetic loss provided by CoCu alloy can work together to maximize the attenuation ability of electromagnetic waves.Exactly,the minimum reflection loss(RLmin)value of the composite reaches-53.43 dB when the matched thickness is 2.1 mm,while the maximum effective absorption bandwidth(EABmax)reaches 6.0 GHz at a thin thickness of 1.8 mm.This work provides some support and reference for the design of novel electromagnetic wave absorbing materials via the dielectric/magnetic loss synergistic mechanism. | Tianbao Zhao Tingting Zheng Di Lan Yan Zhang Zhengshuo Sun Chao Wang Zirui Jia Guanglei Wu | 2024 | Nano Research2024，17，3： | 0 |
| 2 | Three-dimensional macroscopic absorbents: From synergistic effects to advanced multifunctionalities显示文摘The accelerated arriving of 5G era has brought a new round of intelligent transformation which will completely emancipate smart terminal devices.While the subsequent deleterious effect of electromagnetic wave on electronic devices is increasingly serious,driving the growth of next-generation electromagnetic wave absorbents.As a tactful combination of components and structures,three-dimensional(3D)macroscopic absorbents with fascinating synergy afford exceptional electromagnetic wave absorption,and tremendous efforts have been devoted to this investigation.However,in terms of macroscopic absorbents and their synergistic effect,few reviews are proposed to comb the latest achievements and detailed synergy.This review article focuses on the synergistic effect of macro-architectured absorbents mainly including structure-induced synergy,structure-components synergy,and multiple-components induced synergy.And then the potential construction principles and strategies of macroscopic absorbents are combed.Significantly,the key information for structures and components manipulation including nano-micro design and components regulation is further dissected by critically selected cutting-edge 3D macroscopic absorbents.Moreover,a brief summary of multifunctional electromagnetic wave absorbents(EWAs)-based macroscopic structures is presented.Finally,the development prospects and challenges of these materials are discussed. | Shijie Zhang Di Lan Xingliang Chen Yueyuan Gu Junwen Ren Suxuan Du Shichang Cai Xiaomiao Zhao Zhiwei Zhao Guanglei Wu | 2024 | Nano Research2024，17，3： | 0 |
| 3 | Polymorphic cerium-based Prussian blue derivatives with in situ growing CNT/Co heterojunctions for enhanced microwave absorption via polarization and magnetization显示文摘In this paper,the structure evolution of cerium cobaltohexanoate(Ce[Co(CN)6],Ce-Co Prussian blue analog(PBA))has been realized by solvent catalysis at room temperature.The hexagonal bipyramidal microcrystals of Ce-Co PBA can be gradually transformed into dendrites by different proportions of ethanol(EtOH)and water.At the same time,the porous dendrites CeO_(2)/Co@carbon nanotub(CNT)with oxygen-rich vacancies(OVs)can be obtained by annealing Ce-Co PBA at 700℃.The microstructure study shows that carbon nanotubes will be catalyzed after annealing at high temperature,and the cobalt metal particles encapsulated in carbon nanotubes will be anchored in the matrix,regulating the impedance matching and multi-polarization suppression of the material,and its unique structure,vacancies,and strong interface effect make the material exhibit excellent electromagnetic wave(EMW)absorption performance.When the matching thickness is 2.5 mm,the minimum reflection loss(RLmin)of the composite is-51.68 dB,and the effective absorption bandwidth(RL<-10 dB)is 7.76 GHz.These results show that the prepared CeO_(2)/Co@CNT composite has excellent EMW absorption properties.It is expected to be a candidate material for EMW absorption. | Jixi Zhou Xinmeng Huang Di Lan Yuhang Cheng Fengyi Xue Chenyu Jia Guanglei Wu Zirui Jia | 2024 | Nano Research2024，17，3： | 0 |
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