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| 1 | MoSe_(2)/ReS_(2) vdW异质结的第一性原理计算研究显示文摘我们基于第一性原理计算方法,构建了MoSe_(2)/ReS_(2) vdW异质结计算模型,并对异质结构的稳定性、电子和光学特性进行了研究,并探讨了其在光催化水分解中的应用。MoSe_(2)/ReS_(2) vdW异质结具有1.321 eV的间接带隙,且是一种II型异质结构。光吸收谱显示异质结构具有可见光到紫外光区域的广泛的光学吸收范围。带边位置显示导带底和价带顶都跨越了水的氧化还原电位,这意味着它们能够进行水的氧化和还原反应。综上所述,MoSe_(2)/ReS_(2) vdW异质结在可见光范围下可能具有提高光催化效率的潜力。 | 赵红生 王佳斌 李双进 邵凯凯 | 2023 | 广州化工2023，51，7： | 0 |
| 2 | Design and fabrication of self-suspending aluminum-plastic/semiconductor photocatalyst devices for solar energy conversion显示文摘The design and synthesis of self-suspending photocatalyst device with easy recyclability is important for practical application.Here,this work utilizes aluminum-plastic package waste as raw material to prepare an aluminum-plastic supported TiO_(2)(AP-TiO_(2))photocatalyst device through 3D printing design and surface deposition method.A series of characterizations were carried out to explore the structure,morphology and performance of the AP-TiO_(2)device.Under UV light illumination,the AP-TiO_(2)-50 efficiently degrade 93.6%tetracycline hydrochloride(THC)after 4 hr,which increases by 8.3%compared with that of TiO_(2)powder suspension system with the same catalyst amount.Based on it,AP-ZnO,AP-CdS,AP-g-C_3N_4and AP-Pt-TiO_(2)are also fabricated,and applied in photocatalytic degradation and hydrogen evolution,which all exhibit higher photoactivities than powder suspension systems.This work provides a new avenue for the fabrication of advanced recyclable photocatalyst device.Moreover,the work offers a novel sight for the high-value utilization of aluminum-plastic package waste,which has positive implications for environmental protection. | Zhi-Ang Zhao Jingyun Mao Chengjing Lu Shuangqiao Yang Qingrong Qian Qinghua Chen Hun Xue Xiaoli Sun Min-Quan Yang | 2024 | Journal of Environmental Sciences2024，，2： | 0 |
| 3 | g-C_(3)N_(4)基异质结光催化剂研究进展显示文摘石墨相氮化碳(g-C_(3)N_(4))是一种典型的非金属n型聚合物半导体光催化剂.因其具有合适的带隙(2.7 eV),高的热稳定性和化学稳定性,较强的可见光响应等优良特性而被广泛关注.基于g-C_(3)N_(4)构建出2种或2种以上的半导体异质结,具有提高可见光利用率,增强氧化还原能力,促进光生载流子转移和分离等作用,因而成为一种提高光催化活性的可行和高效策略.综述了近年来g-C_(3)N_(4)基异质结的构建及其光催化机理的研究进展,并进一步展望了研究前景. | 秦建宇 贾密英 张艳峰 | 2023 | 河北师范大学学报(自然科学版)2023，47，3： | 0 |
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