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1生物油电催化加氢提质技术研究进展显示文摘生物油是一种可再生的碳中和有机资源,在液体燃料和高值化学品生产中显示出较大的潜力,对其大规模利用有助于实现碳中和目标。生物油因其固有的腐蚀性和化学不稳定性而需要提质以提高其应用价值。电催化加氢能够在常温常压下实现生物油加氢提质,该方法反应条件温和、操作简单、能源效率高,具有碳中和属性,为生物油提质提供了新的选择。综述了近年来生物油电催化加氢的研究进展,分析了不同生物油模型化合物在电催化加氢过程中的作用机理。讨论了真实生物油样品的电催化加氢实例,以证明电催化应用于生物油提质的可行性。最后,针对生物油电催化加氢提质技术面临的困难和挑战,提出了该领域未来的研究方向和重点,并展望了生物油电催化加氢提质工业化应用的前景。邓伟 林镇浩 熊哲 汪雪棚 徐俊 江龙 苏胜 汪一 胡松 向军 2021化工学报2021,72,10:2
2A review on catalytic & non-catalytic bio-oil upgrading in supercritical fluids显示文摘This review article summarizes the key published research on the topic of bio-oil upgrading using catalytic and non-catalytic supercritical fluid(SCF)conditions.The precious metal catalysts Pd,Ru and Pt on various supports are frequently chosen for catalytic bio-oil upgrading in SCFs.This is reportedly due to their favourable catalytic activity during the process including hydrotreating,hydrocracking,and esterification,which leads to improvements in liquid yield,heating value,and pH of the upgraded bio-oil.Due to the costs associated with precious metal catalysts,some researchers have opted for non-precious metal catalysts such as acidic HZSM-5 which can promote esterification in supercritical ethanol.On the other hand,SCFs have been effectively used to upgrade crude bio-oil without a catalyst.Supercritical methanol,ethanol,and water are most commonly used and demonstrate catalyst like activities such as facilitating esterification reactions and reducing solid yield by alcoholysis and hydrolysis,respectively.Sainab Omar Yang Yang Jiawei Wang 2021Frontiers of Chemical Science and Engineering2021,15,1:0
3Preface to the CSCST-25 Special lssue显示文摘The Chinese Society of Chemical Science and Technology in the United Kingdom(CSCST)was established in 1994 in London by an elite group of Chinese chemists and chemical engineers in the UK with the main aim to promote interaction,network and collaboration among the Chinese academics,postdoctoral researchers and PhDs,but not limited to,in the United Kingdom(UK)higher education institutions and relevant industries.Since then,the CSCST community has continuously grown and further contributed to the various fields of Chemical Science,Engineering and Technology in the UK,as well as worldwide.Xiaolei Fan Jiawei Wang 2019Frontiers of Chemical Science and Engineering2019,13,4:0
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