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| 1 | Source apportionment of polycyclic aromatic hydrocarbons(PAHs) in a sediment core from Lake Dagze Co, Tibetan Plateau, China: Comparison of three receptor models显示文摘Receptor models are a useful tool for identifying sources of polycyclic aromatic hydrocarbons(PAHs) in multiple environmental media. In this study, three different receptor models(including the principal component analysis-multiple linear regression(PCA-MLR), positive matrix factorization(PMF), and Unmix models) were used to apportion the sources of 16 priority PAHs in a sediment core of Lake Dagze Co. The ΣPAHs(sum of all 16 measured PAHs) concentrations ranged from 51.89 to 132.82 ng/g with an average of 80.39 ng/g. TheΣ PAHs were dominated by 2-3 ring PAHs, accounting for 80.12% on average, thereby indicating that they mainly originated from biomass and coal combustion and/or from long-range atmospheric transportation. The three models produced consistent source apportionment results. The greatest contributor to ΣPAHs was biomass combustion, followed by coal combustion, vehicle emissions, and petrogenic sources. Moreover, the temporal variation of the common sources was well-correlated among models. The multi-method comparison and evaluation results showed that all three models were useful tools for source apportionment of PAHs, with the PMF model providing better results than the PCA-MLR and Unmix models. The temporal trends of factor contributions were verified by PAHs with different ring numbers. Significant correlations were found between the simulated concentrations of each source factor and the PAHs with different ring numbers(P<0.01), except for the petrogenic source identified by the Unmix model(P>0.05). This study can provide useful information for further investigation of source apportionment of PAHs in the sediment cores. | Yixin Bai Kunlin Shi Heyu Yu Nana Shang Weiyue Hao Chuan Wang Tao Huang Hao Yang Changchun Huang | 2022 | Journal of Environmental Sciences2022，34，11： | 2 |
| 2 | 人类世的地球化学标志——沉积物中的持久性有机污染物显示文摘确定人类世地层标志物是选取全球层型剖面和点(GSSP)的重要前提。目前水系沉积记录作为人类世GSSP的候选表现出显著优越性。水系沉积物中的持久性有机污染物(POPs)可以连续、高分辨率地反映人类活动影响和强度变化,通过横向对比全球POPs历史变化可以获取潜在标志物的高速增长起点。本次研究收集了3类POPs的69套数据,通过分析数据的时间趋势重建其沉积记录,以求获得全球范围内各类POPs的增长特征。全球沉积记录显示20世纪40~60年代间不同类型的POPs开始展现出不同程度的快速增长,其中多环芳烃(PAHs)和多氯联苯(PCBs)可以作为潜在的标志物指示沉积物中化学地层的界限,有机氯农药(OCPs)中只有滴滴涕(DDTs)具备这种特性。同时,这3类POPs的沉积记录可以反映人类能源消耗、农业生产和工业品商品制造等方面活动,作为标志物体现人类多种活动营力在地球系统中留下的证据。 | 王棋 李俊 袁国礼 | 2021 | 第四纪研究2021，41，6： | 1 |
| 3 | 多环芳烃和多氯联苯全球芯样沉积记录研究及现状综述显示文摘存储地质年代信息的芯样如岩芯、冰芯等是重建有机污染物沉积历史的重要工具之一,已被广泛用于研究全球有机污染物的污染历史趋势以及污染来源。与浓度相比,沉积通量能更好地反映有机污染物的沉积历史和排放情况。因此收集了全球基于芯样研究有机污染物沉积通量的相关数据,总结和分析了有机污染物在世界各地的沉积情况,全面阐述了全球有机污染物的沉积记录、空间分布以及使用芯样时应注意的问题。结果表明,多环芳烃(PAHs)在全球的沉积通量总体符合其在研究区域内的生产、排放历史;多氯联苯(PCBs)的沉积通量出现“双峰”现象;在全球气候变暖的趋势下,冰川融化可能会导致所存储的有机污染物重新释放到环境中。同时,在进行不同国家或地区沉积记录的横向比较时,应注意不同研究所测定的污染物种类、数量以及芯样覆盖年份可能会有所不同。通过总结世界各芯样的沉积记录,以期为有机污染物控制和管理提供一定的科学依据。 | 谭新来 武英欣 黄跟平 邹红艳 | 2023 | 化学试剂2023，45，6： | 0 |
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