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| 1 | 断裂-层序双控机制下的热液活动及成储效应——以塔里木盆地塔河、玉北地区下奥陶统为例显示文摘塔里木盆地下古生界碳酸盐岩广泛发育,是油气勘探的重要领域。以塔里木盆地塔河、玉北地区下奥陶统为例,通过岩心观察、薄片鉴定、电子探针、C、O、Sr同位素以及REE元素分析,结合测井及地震资料,探讨了断裂系统和层序地层格架中的热液活动及成储效应。研究认为:中-细晶白云岩遭受富硅质热液流体改造强烈,表现为热褪色现象、鞍状白云石充填和充填白云石、方解石、玉髓、黄铁矿等多种矿物组合沉淀,以及较高的SiO2、FeO、MnO、BaO含量、较低的SrO含量和87Sr/86Sr值、偏负的δ18O值、较低的∑REE含量、明显的Eu正异常和Ce负异常。热液流体对白云岩储层的改造主要表现为溶蚀作用、重结晶作用和充填作用三个方面,溶蚀作用形成的次生溶蚀孔隙成为最重要的储集空间。不同尺度断裂和三级层序甚至更短周期层序界面共同构成深部热液流体运移的输导体系,对热液活动及储层发育起到强烈的控制作用,并建立了塔里木盆地塔河、玉北地区下奥陶统蓬莱坝组断裂-层序双控机制下的热液活动及成储效应的概念模型。 | 孙福宁 胡文瑄 胡忠亚 刘永立 康逊 朱峰 | 2020 | 石油与天然气地质2020，41，3： | 6 |
| 2 | 微生物异化还原水铁矿介导的Ca-Fe碳酸盐矿物形成:对铁白云石成因的启示显示文摘白云石的成因机制至今仍是地球科学领域的一个谜题(“白云石问题”).铁白云石等碳酸盐矿物具有类白云石晶体结构,因此研究这些矿物的形成机制可为解答“白云石问题”提供新线索.本研究利用一株海洋异化铁还原菌(Shewanella piezotolerans WP3),在不同钙离子浓度(0~20mmol/L)条件下,通过氧化乳酸盐诱导水铁矿还原转化为次生碳酸盐矿物,以此评估微生物在铁白云石形成过程中的作用.实验结果表明,加入Ca^(2+)可以增强S.piezotolerans WP3细胞与水铁矿颗粒之间的黏附作用,从而提高反应体系中Fe(Ⅲ)还原速率.在不同Ca^(2+)浓度条件下,菌株WP3诱导生成的次生碳酸盐矿物类别有所差异:在0mmol/L Ca^(2+)体系中生成菱铁矿,而含钙体系中则为Ca-Fe碳酸盐固溶体,且这些固溶体的钙离子含量与反应体系中初始的Ca^(2+)浓度呈正相关关系.值得注意的是,在20mmol/L Ca^(2+)体系中生成的Ca-Fe碳酸盐固溶体化学组成为Ca0.8Fe1.2(CO3)2,与铁白云石类似.此外,这些微生物成因的“类铁白云石”具有纳米晶粒的形态,晶体结构中钙和铁元素呈无序分布,并且发育较多晶体缺陷.进一步成岩模拟实验证明,“类铁白云石”可以在水热条件下转化为有序铁白云石.基于成分类比性和转化规律,微生物成因的“类铁白云石”可能是沉积物(岩)中铁白云石的重要前驱体,可以被定义为“原铁白云石”.以上新发现对理解微生物在铁白云石乃至白云石形成中的贡献具有重要的启示意义. | 刘邓 曹锦鹏 杨珊珊 殷雅婷 王鹏聪 Dominic PAPINEAU 王红梅 邱轩 罗根明 朱宗敏 王风平 | 2024 | 中国科学:地球科学2024，54，1： | 0 |
| 3 | Microbially-mediated formation of Ca-Fe carbonates during dissimilatory ferrihydrite reduction:Implications for the origin of sedimentary ankerite显示文摘The origin of sedimentary dolomite has become a long-standing problem in the Earth Sciences.Some carbonate minerals like ankerite have the same crystal structure as dolomite,hence their genesis may provide clues to help solving the dolomite problem.The purpose of this study was to probe whether microbial activity can be involved in the formation of ankerite.Bio-carbonation experiments associated with microbial iron reduction were performed in batch systems with various concentrations of Ca^(2+)(0–20 mmol/L),with a marine iron-reducing bacterium Shewanella piezotolerans WP3 as the reaction mediator,and with lactate and ferrihydrite as the respective electron donor and acceptor.Our biomineralization data showed that Ca-amendments expedited microbially-mediated ferrihydrite reduction by enhancing the adhesion between WP3 cells and ferrihydrite particles.After bioreduction,siderite occurred as the principal secondary mineral in the Ca-free systems.Instead,Ca-Fe carbonates were formed when Ca^(2+)ions were present.The CaCO_(3) content of microbially-induced Ca-Fe carbonates was positively correlated with the initial Ca2+concentration.The Ca-Fe carbonate phase produced in the 20 mmol/L Ca-amended biosystems had a chemical formula of Ca_(0.8)Fe_(1.2)(CO_(3))_(2),which is close to the theoretical composition of ankerite.This ankeritelike phase was nanometric in size and spherical,Ca-Fe disordered,and structurally defective.Our simulated diagenesis experiments further demonstrated that the resulting ankerite-like phase could be converted into ordered ankerite under hydrothermal conditions.We introduced the term“proto-ankerite”to define the Ca-Fe phases that possess near-ankerite stoichiometry but disordered cation arrangement.On the basis of the present study,we proposed herein that microbial activity is an important contributor to the genesis of sedimentary ankerite by providing the metastable Ca-Fe carbonate precursors. | Deng LIU Jinpeng CAO Shanshan YANG Yating YIN Pengcong WANG Dominic PAPINEAU Hongmei WANG Xuan QIU Genming LUO Zongmin ZHU Fengping WANG | 2024 | Science China Earth Sciences2024，67，1： | 0 |
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