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| 1 | Effects of SO2 and H2O on low-temperature NO conversion over F-V2O5-WO3/TiO2 catalysts显示文摘F-V2 O5-WO3/Ti02 catalysts were prepared by the impregnation method.As the content of F ions increased from 0.00 to 0.35 wt.%,the NO conversion of F-V2 O5-WO3/TiO2 catalysts initially increased and then decreased.The 0.2 F-V2 O5-WO3/TiO2 catalyst(0.2 wt.%F ion)exhibited the best denitration(De-NOx)performance,with more than 95%NO conversion in the temperature range 160-360℃,and 99.0%N2 selectivity between 110 and 280℃.The addition of an appropriate amount of F ions eroded the surface morphology of the catalyst and reduced its grain size,thus enhancing the NO conversion at low temperature as well as the sulfur and water resistance of the V2 O5-WO3/Ti02 catalyst.After selective catalytic reduction(SCR)reaction in a gas flow containing SO2 and H2 O,the number of NH3 adsorption sites,active component content,specific surface area and pore volume decreased to different degrees.Ammonium sulfate species deposited on the catalyst surface,which blocked part of the active sites and reduced the NO conversion performance of the catalyst.On-line thermal regeneration could not completely recover the catalyst activity,although it prolonged the cumulative life of the catalyst.In addition,a mechanism for the effects of S02 and H2 O on catalyst NO conversion was proposed. | Quanming Liang Jian Li Hong He Tao Yue Li Tong | 2020 | Journal of Environmental Sciences2020，32，4： | 3 |
| 2 | 添加Cl离子对V_2O_5-WO_3/TiO_2催化剂低温NO转化率的影响显示文摘考察添加不同含量Cl离子对浸渍法制备的Cl-V_2O_5-WO_3/TiO_2催化剂低温NO转化率的影响。随着Cl离子质量添加量从0增加到2.5%,Cl-V_2O_5-WO_3/TiO_2催化剂NO转化率先升高后降低,结合在含有SO_2和H2O的SCR实验结果,确定1.5%Cl-V_2O_5-WO_3/TiO_2为性能最优催化剂。在反应温度为149-362℃,NO转化率大于95%;在145-385℃,NO转化率大于90%。采用XRF、BET、XRD、TG、FT-IR和H2-TPR等方法表征了催化剂的物理化学性能和结构。结果表明,在反应气氛中加入SO_2和H2O后,催化剂比表面积和孔容均减小,副反应产物含有NH+4和SO_2-4。适量Cl离子可以抑制硫物种沉积,减少副反应产物生成,增强催化剂抗中毒能力。 | 梁全明 梁文俊 张铁军 樊星 宋丽云 李坚 何洪 岳涛 | 2018 | 燃料化学学报2018，46，11： | 1 |
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