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| 1 | 高温热稳定性Au/β-Mo2C催化剂的制备及在逆水煤气变换反应中的应用显示文摘以程序升温碳化法合成β-Mo2C载体,采用原位沉淀法制备负载量不同的Au/β-M o2C催化剂,利用XRD、STEM和氮气吸附-脱附等手段对Au在载体表面的分散性、微观形貌及孔结构等进行表征,并在逆水煤气变换(RWGS)反应中对其高温热稳定性进行了研究。XRD表征结果表明,在34.44°、38.02°、39.44°、52.12°、61.53°、69.62°和74.65°处出现了β-Mo2C对应的(100)、(002)、(101)、(102)、(110)、(103)和(200)晶面的X射线特征衍射峰;同时,未出现Au物种的特征吸收峰,说明Au负载量较低的0.1%和0.5%的催化剂上Au纳米粒子的分散性较好。STEM表征结果也显示,当负载量较低(0.5%、1.0%和2.0%)时,金纳米粒子以2 nm左右的原子簇形式均匀分散并锚定在β-M o2C载体上。氮气吸附-脱附表征结果表明,催化剂具有良好的介孔结构。反应评价结果表明,0.2%Au/β-Mo2C催化剂在RWGS反应中具有较好的催化活性和较高的CO选择性,且反应后孔结构良好,Au纳米粒子仍然均匀分散,说明Au/β-Mo2C催化剂在此反应中具有较高的催化性能和高温热稳定性。 | 刘孟杰 丁巍 戴咏川 赵玉柱 赵越 郝元川 | 2020 | 燃料化学学报2020，48，3： | 1 |
| 2 | A New Paradigm for Simulating and Forecasting China's Economic Growth in the Medium and Long Term显示文摘Taking the system philosophy of human-earth relationship as the theoretical axis,and under the three-dimensional goals of economic growth,social development,and protection of the ecological environment,this paper constructs the supporting system of China’s economic development.On this basis,guided by the basic principles of system theory and system dynamics,and combined with the theories of other related disciplines,we constructed an economic geography-system dynamics(EG-SD)integrated forecasting model to simulate and quantitatively forecast China’s economic growth in the medium and long term.China’s economic growth will be affected by quantifiable and unquantifiable factors.If the main unquantifiable factors are not taken into account in the simulation and prediction of China’s economic growth in the medium and long term,the accuracy and objectivity of the prediction results will be diminished.Therefore,based on situation analysis(Strengths,Weaknesses,Opportunities,and Threats,SWOT),we combined scenario analysis with the Delphi method,and established a qualitative prediction simulation model(referred to as the S-D compound prediction model)to make up for the shortcomings associated with quantitative simulation predictions.EG-SD and S-D are organically combined to construct a simulation and prediction paradigm of China’s economic growth in the medium and long term.This paradigm not only realizes the integration of various forecasting methods and the combination of qualitative and quantitative measures,but also realizes the organic combination of unquantifiable and quantifiable elements by innovatively introducing fuzzy simulation of system dynamics,which renders the simulation and prediction results more objective and accurate. | SUN Dongqi LU Jiayi | 2022 | Chinese Geographical Science2022，32，1： | 0 |
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