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| 1 | 我国霾和光化学污染观测研究进展显示文摘霾和光化学污染已成为我国最严重的环境气象灾害,受到政府和公众广泛关注。针对我国的环境气象问题,国内外科研人员开展了大量研究工作,发表了一系列的研究成果。该文对近年来我国霾和光化学污染的观测、分析和影响研究方面的文献进行综述,为将来相关研究提供基础。在霾污染方面,主要回顾了霾的现象与判别、组成与来源、影响霾的气象因素、霾的长期趋势等方面的研究进展。在光化学污染方面,主要回顾了污染的特征与水平、污染的区域化、臭氧垂直分布、地面臭氧影响因素、臭氧污染发展趋势等方面的研究进展。此外,还概括了霾和光化学污染危害研究主要成果,在文献综述的基础上,提出了未来研究中值得关注的几方面问题,包括进一步加强霾和雾的科学判识方法、污染物相互作用、污染-气象-化学-生态间耦合效应研究,特别关注光化学污染发展态势,加强长期观测资料的积累、分析与应用等。 | 徐晓斌 | 2016 | 应用气象学报2016，27，5： | 34 |
| 2 | Surface Ozone in Jiuzhaigou National Park, Eastern Rim of the Qinghai-Tibet Plateau, China显示文摘Located in southwestern China, Jiuzhaigou National Park is one of the most popular tourism destinations in China, famous for its unique aquatic ecosystems and beautiful forests. However, plants in the park may be at high ozone risk as a result of the intensive use of diesel tour buses in the park. In addition, Jiuzhaigou is close to a region with relatively high regional anthropogenic NO x emissions. During the growing season, also the peak season of tourism, we measured ozone concentration at two sites within the Park and these were: Jiuzhaigou Bureau (JB) and Long Lake (LL). The results indicate that ozone concentrations were not high enough to cause foliar injury during the monitoring period, although the risk of ozone to plants was higher in spring than in summer and autumn. Diurnal ozone cycles at JB and LL displayed significantly higher ozone concentrations in the daytime than in the nighttime, suggesting photochemical production of ozone during the day and ozone deposition during the night as a result of the nocturnal boundary layer. In parallel with the seasonal change of background surface ozone in the Northern Hemisphere, maximum daily 8-h average ozone concentration (MDA8) and daily ozone concentration decreased from spring to autumn at the two sites. This temporal variation in Jiuzhaigou was most likely associated with the downward mixing of ozone-rich air from the free troposphere, because all the high-ozone events (MDA8 > 70.0 ppb) were observed in spring and ozone-rich air from the free troposphere was the dominant cause. In summary, our data suggest that ozone concentrations in Jiuzhaigou were more affected by the regional-scale of background pattern in air quality and meteorological conditions than by local tourist activities. | QIAO Xue TANG Ya Daniel JAFFE CHEN Pan XIAO Weiyang DENG Guiping | 2012 | Journal of Mountain Science2012，9，5： | 2 |
| 3 | Two-year measurements of surface ozone at Dangxiong,a remote highland site in the Tibetan Plateau显示文摘Measurements of surface O3 and carbon monoxide(CO) were made from September 2009 to August 2011 at Dangxiong(30.48°N, 91.10°E, 4187 m a.s.l.), a remote highland site in a southern valley of the Nyainqêntanglha Mountains in the Tibetan Plateau, China. The monthly mean O3 mixing ratio ranged from 29.1 to 51.4 ppb, with an average of 38.5 ppb, and the maximum value was observed in May. The average diurnal cycle of O3 concentration showed a minimum in early morning and a maximum in the afternoon, with a broader 'high platform' from the late morning to the late afternoon, and resembled that of surface wind speed. The concentration of surface O3 was highly significantly correlated with tropospheric column O3 over the regions surrounding Dangxiong and with that of surface O3 observed at a site north of the Nyainqêntanglha Mountains, suggesting a good regional representativeness of surface O3 at Dangxiong. In the afternoon when stronger winds blew, surface air showed distinct features of free-atmospheric air, with higher O3, lower CO, and lower relative humidity(RH). The negative O3–CO and O3–RH correlations in most months indicate a significant influence of air masses from the free troposphere. Trajectory analysis suggests that air masses originating from the south of the site make a negative net contribution to surface O3 and a positive contribution to CO and humidity, and those from the northwest sector contribute conversely to the respective quantities. | Weili Lin Xiaobin Xu Xiangdong Zheng Jaxi Dawa Ciren Baima Jin Ma | 2015 | Journal of Environmental Sciences2015，27，5： | 1 |
| 4 | 中国区域大气本底站近地面臭氧来源贡献及区域代表性显示文摘回顾了关于长距离输送对中国区域本底大气臭氧的影响,以及中国区域大气本底站臭氧变化及其区域代表性两方面的研究进展。来自不同污染源区O_(3)的长距离输送对中国区域O_(3)影响的研究结果分歧较大,贡献最显著的源区和受体地区也存在争议;同时,鲜有研究考虑到平流层对对流层的O_(3)贡献,而这部分贡献在前体物排放很少的本底地区非常重要。中国区域各大气本底观测站分别与其周围一定范围内的区域具有相同的对流层O_(3)柱浓度最大值月份分布,而对与人体健康密切相关的近地面O_(3)区域特征的分析尚未深入开展;鉴于研究方法的局限性,也尚未深入揭示形成O_(3)变化区域特征的复杂成因。基于现有研究进展和不足之处,如何利用全球大气化学-环流模式的示踪模拟结果,定量评估来自全球不同地区的O_(3)对中国本底大气O_(3)的影响,并进一步评估中国区域6个大气本底站近地面O_(3)季节变化的区域代表性,是亟待解决的科学问题。 | 刘宁微 马建中 安兴琴 林伟立 徐婉筠 徐晓斌 李得勤 李荣平 | 2022 | 大气科学学报2022，45，5： | 1 |
| 5 | 宇宙成因核素7Be和10Be示踪大气垂直传输交换研究进展显示文摘示踪大气垂直传输交换过程对了解大气中化学物质传输路径、气候变化过程及预测大气环境变化趋势具有重要的科学意义。大气7Be和10Be生成后就迅速被氧化,随干/湿沉降过程到达地表,通过分析其中7Be和10Be浓度以及10Be/7Be值可示踪平流层—对流层交换过程。为全面了解7Be和10Be示踪大气垂直传输交换过程及研究现状,从7Be和10Be的浓度及其比值的分布规律及影响机制方面剖析其对平流层—对流层交换的示踪,对相关示踪研究取得的成果进行了总结和评述。10Be/7Be值作为平流层—对流层交换灵敏示踪剂,相比7Be可避免对流层干/湿沉降及不同气团稀释作用影响,明显地避免纬度变化和太阳周期变化带来自身产率变化的影响。最后指出7Be和10Be示踪平流层—对流层交换时需要注意由南北半球区别、地区纬度变化及研究地点的地理位置特征等带来的影响;各地区长周期高精度的7Be和10Be数据对沉降通量研究、平流层—对流层交换示踪、全球气候模型的建立及验证具有重要作用;重悬浮粉尘对10Be浓度和10Be/7Be值的影响不可忽视,Al元素校正法是去除扬尘影响较为有效的校正方式。 | 刘许柯 付云翀 周卫健 张丽 赵国庆 | 2020 | 地球科学进展2020，35，10： | 1 |
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