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| 1 | 松辽盆地嫩江组脱羟基维生素E的分布及其地球化学意义显示文摘脱羟基维生素E是沉积物(岩)中一类具有水体盐度指示意义的生物标志化合物,在现代和古代沉积物及原油中均有检出。在松辽盆地松科1井晚白垩系嫩江组岩芯样品中检测发现的脱羟基维生素E系列化合物显示脱羟基维生素E的组成分布在剖面上的变化主要反应了沉积埋葬时的环境盐度、氧化还原状态的变化,而与母源组成、有机质成熟度等无明显相关性;其中,δ-MTTC在咸水还原性环境最为丰富,而在低盐的半咸水-淡水氧化性环境中基本缺失;α-MTTC在所有盐度环境中都很丰富,γ-MTTC的丰度则在盐水-咸水环境中明显高于低盐半咸水环境,而且在盐水环境中γ-MTTC>β-MTTC,咸水环境显示γ-MTTC<β-MTTC。研究发现,α-MTTC/γ-MTTC(α/γ)可作为α-MTTC/δ-MTTC(α/δ)比值的替代指标,当α-MTTC/γ-MTTC比值小于2时为盐水环境,比值大于15时为半咸水-淡水环境,介于之间为咸水环境。相关参数及综合分析显示嫩江组一、二段沉积时期水体盐度及氧化还原条件显著不同,嫩一段主力烃源岩沉积时期以与海水盐度相当的咸水、存在水体分层的还原性湖泊环境为主,顶部出现短期咸化的盐水环境;而嫩二段主要为半咸水-淡水氧化性湖泊环境,盐度比较稳定。 | 王丽 宋之光 | 2010 | 地球化学2010，39，5： | 10 |
| 2 | Stable carbon isotope compositions of isoprenoid chromans in Cenozoic saline lacustrine source rocks from the Western Qaidam Basin,NW China:Source implications显示文摘Although the distribution of mono-,di-and trimethylated 2-methyl-2-(4,8,12-Trimethyltrideeyl) chromans(MTTCs) is well understood as an indicator of water salinity,their origin and formation mechanism are still ambiguous and under debate.In this paper,abnormally high levels of MTTCs were detected in Cenozoic saline lacustrine source rocks from the Western Qaidam Basin.Using a two-step column chromatography method,the MTTCs and naphthalenes were separated from other aromatic compounds and concentrated in one fraction,so that the stable carbon isotope compositions of these compounds could be accurately measured.Similar carbon isotope ratios for the mono-,di-and trimethylated 2-methyl-2-(4,8,12-Trimethyltrideeyl) chromans in a given sample suggest the MTTCs may share the same biological source(s).The MTTCs from the Western Qaidam Basin have similar carbon isotope compositions to primary producer-derived pristane and phytane.However,the ? 13C values for the MTTCs showed significant differences with other primary producers-derived biomarkers(e.g.C27 and C29 steranes),probably indicating a distinct microalgae source from specific niches for the MTTC compounds.We speculate that the MTTCs distribution patterns may be controlled by the water chemistry dynamics in niches,which,in turn,is affected by hypersaline bottom water. | ZHANG YongDong JIANG AiZhu SUN YongGe XIE LiuJuan CHAI PingXia | 2012 | Chinese Science Bulletin2012，57，9： | 3 |
| 3 | 柴达木盆地西部新生代盐湖相烃源岩中脱羟基维生素E类化合物碳同位素组成及其指示意义显示文摘脱羟基维生素E类(MTTC)化合物的分布模式已被广泛地应用于水体盐度的判识,然而,对于该类化合物的来源及其成因机制在国际上仍存在着较大的争议.本文以富含MTTC化合物的柴达木西部盐湖相烃源岩为研究对象,采用二步柱色谱层析技术,分离富集MTTC化合物,使其能够进行准确的分子碳同位素测定.实验结果表明,在同一个样品中,不同碳数的MTTC化合物具有相近的稳定碳同位素组成特征,反映了MTTC化合物在生源上可能具有一致性.与指示初级生产者的其他生物标志物的稳定碳同位素组成比较发现,虽然MTTC化合物的碳同位素组成与姥鲛烷和植烷的碳同位素组成相一致,但与C27和C29甾烷的碳同位素组成仍具有明显的差异性.综合水体的生物地球化学过程,提出MTTC化合物可能与特殊生境的微藻输入有关,并且沉积有机质中MTTC化合物的分布模式主要受控于微藻的生态位,特别是下层高盐卤水对微藻发育的影响. | 张永东 蒋爱珠 孙永革 谢柳娟 柴平霞 | 2012 | 科学通报2012，57，7： | 2 |
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