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| 1 | Investigation of Li-ion transport in Li7P3S11 and solid-state lithium batteries显示文摘The high Li-ion conductivity of the Li7P3S11 sulfide-based solid electrolyte makes it a promising candidate for all-solid-state lithium batteries. The Li-ion transport over electrode-electrolyte and electrolyteelectrolyte interfaces, vital for the performance of solid-state batteries, is investigated by impedance spectroscopy and solid-state NMR experiments. An all-solid-state Li-ion battery is assembled with the Li7P3S11 electrolyte, nano-Li2S cathode and Li-In foil anode, showing a relatively large initial discharge capacity of 1139.5 m Ah/g at a current density of 0.064 m A/cm^ 2 retaining 850.0 m Ah/g after 30 cycles. Electrochemical impedance spectroscopy suggests that the decrease in capacity over cycling is due to the increased interfacial resistance between the electrode and the electrolyte. 1D exchange ^7Li NMR quantifies the interfacial Li-ion transport between the uncycled electrode and the electrolyte, resulting in a diffusion coefficient of 1.70(3) ×10^-14cm^2/s at 333 K and an energy barrier of 0.132 e V for the Li-ion transport between Li2S cathode and Li7P3S11 electrolyte. This indicates that the barrier for Li-ion transport over the electrode-electrolyte interface is small. However, the small diffusion coefficient for Li-ion diffusion between the Li2S and the Li7P3S11 suggests that these contact interfaces between electrode and electrolyte are relatively scarce, challenging the performance of these solid-state batteries. | Chuang Yu Swapna Ganapathy Ernst R.H.van Eck Lambert van Eijck Niek de Klerk Erik M.Kelder Marnix Wagemaker | 2019 | Journal of Energy Chemistry2019，28，11： | 2 |
| 2 | Continuous circuit coprecipitation of arsenic(V) with ferric iron by lime neutralization: Process parameter effects on arsenic removal and precipitate quality显示文摘 | Richard Jack De Klerk Yongfeng Jia Renaud Daenzer Mario A. Gomez George P. Demopoulos | 2011 | Hydrometallurgy2011，，： | 2 |
| 3 | A randomised, multicentre study of ceftriaxone versus standard therapy in the treatment of lower respiratory tract infections 显示文摘 | de Klerk G J van Steijn J H Lobatto S | 1999 | Int J Antimicrob Agents1999，12，2： | 2 |
| 4 | The spectrum of antecedent infections in Guillain-Barré syndrome: A case-control study显示文摘 | B. C. Jacobs P. H. Rothbarth F. G.A. van der Meché P. Herbrink P. I.M. Schmitz M. A. de Klerk P. A. van Doorn | 1998 | Neurology1998，，4： | 2 |
| 5 | MTHFR 677C→T polymorphism and risk of coronary heart disease: a meta-analysis显示文摘 | Klerk M -Verhoef P Clarke R | 2002 | JAMA2002，288，： | 1 |
| 6 | Early-life respiratory vi-ral infections,atopic sensitization,and risk of subsequent develop-ment of persistent asthma 显示文摘 | Kusel MM de Klerk NH Kebadze T | 2007 | J Allergy Clin Immunol2007，119，5： | 1 |
| 7 | Relative val- ue of erythrocyte sedimentation rate and C-reactive proteili in as-sessment of disease activity in ankylosing spondylitis显示文摘 | Spoorenberg A van der Heijde D de Klerk E | 1999 | J Rheu matol1999，26，： | 1 |
| 8 | Maternal health in pregnancy and intellectual disability in the offspring:a populationbased study显示文摘 | Leonard H de Klerk N Bourke J | 2006 | Ann Epidemiol2006，16，： | 1 |
| 9 | Isomerization of 1-butene to isobutene at low temperature显示文摘 | Klerk A | 2004 | Industrial and Engineering Chemistry Research2004，43，： | 1 |
| 10 | Bone seeking radiopharma- ceuticals for palliation of pain in cancer patients with osseous me- tastases显示文摘 | Lam MG de Klerk JM van Rijk PP | 2007 | Anticancer Agents Med Chem2007，714，： | 1 |
| 11 | Cardiac sarcoidosis evaluated with gadolinium-enhanced magnetic resonance and contrast-enhanced 64-slice computed tomography 显示文摘 | SMEDEMA J TRUTER R de KLERK P | 2006 | Int J Cardiol2006，112，2： | 1 |
| 12 | A mild treatment strategy for in-vitro fertilisation:a randomised non-inferiority trial显示文摘 | Heijnen EM Eijkemans MJ De Klerk C | 2007 | Lancet2007，369，9563： | 1 |
| 13 | Real-time NASBA for detection of Strawberry vein banding virus 显示文摘 | Vasková D Spak J Klerks MM | 2004 | European Journal of Plant Pathology2004，110，： | 1 |
| 14 | 显示文摘 | Klerk J D Weinert R W Mcavoy B R | 1979 | IEEE Transations on Sonics and Ultrasonics1979，26，： | 1 |
| 15 | Association betweenantenatal cytokine production and the development of atopy andasthma at age 6 years 显示文摘 | Macaubas C de Klerk NH Holt BJ | 2003 | Lancet2003，362，9391： | 1 |
| 16 | Linear α-olefins from linear internal olefins by a boron-based continuous double-bond isomerization process显示文摘 | Klerk A D Hadebe S W Govender J R | 2007 | Industrial and Engineering Chemistry Research2007，46，： | 1 |
| 17 | Mechanisms of heparin induced anticancer activity in experimental cancer models显示文摘 | Niers TM Klerk CP DiNisio M | 2007 | Crit Rev Oncol Hematol2007，61，： | 1 |
| 18 | The mortality of women exposed environmentallyand domestically to blue asbestos at Wittenoom, Western Australia显示文摘 | REID A HEYWORTH J DE KLERK N | 2008 | Occup Environ Med2008，65，11： | 1 |
| 19 | A rapid method of predictingwidth and extent of hydraulically induced fractures显示文摘 | Gcertsma J De Klerk F | 1969 | Journal of Petroleum Technology1969，21，12： | 1 |
| 20 | Comparison of methods of extracting salmonella enterica serovar enteritidis DNA from environmental substrates and quantification of organisms by using a general internal procedural control 显示文摘 | KLERKS M M VAN BRUGGEN A H C ZIJLSTRA C DONNIKOV M | 2006 | Appl Environ Microbiol2006，72，： | 1 |
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