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| 1 | Advanced Electrode Materials in Lithium Batteries:Retrospect and Prospect显示文摘Lithium-(Li-)ion batteries have revolutionized our daily life towards wireless and clean style,and the demand for batteries with higher energy density and better safety is highly required.The next-generation batteries with innovatory chemistry,material,and engineering breakthroughs are in strong pursuit currently.Herein,the key historical developments of practical electrode materials in Li-ion batteries are summarized as the cornerstone for the innovation of next-generation batteries.In addition,the emerging electrode materials for next-generation batteries are discussed as the revolving challenges and potential strategies.Finally,the future scenario of high-energy-density rechargeable batteries is presented.The combination of theory and experiment under multiscale is highlighted to promote the development of emerging electrode materials. | Xin Shen Xue-Qiang Zhang Fei Ding Jia-Qi Huang Rui Xu Xiang Chen Chong Yan Fang-Yuan Su Cheng-Meng Chen Xingjiang Liu Qiang Zhang | 2021 | Energy Material Advances2021，，1： | 4 |
| 2 | Recent Advances and Opportunities of Lead-Free Perovskite Nanocrystal for Optoelectronic Application显示文摘Metal halide perovskite nanocrystals(NCs),as a new class of light-emitting and light-harvesting materials,have recently attracted intensive attention for an impressive variety of optoelectronic applications.However,the lead toxicity and poor stability of such materials severely restrict their practical applications and future commercialization.Lead-free perovskite NCs and their derivatives,designed by the reasonable chemical substitution of Pb with other nontoxic elements,are recently booming as an attractive alternative to lead-based counterparts.In this review,we firstly present a comprehensive overview of currently explored lead-free perovskite NCs with an emphasis on their design routes,morphologies,optoelectronic properties,and environmental stability issues.Then,we discuss the preliminary achievements of lead-free perovskite NCs in versatile optoelectronic applications,such as light-emitting devices,solar cells,photodetectors,and photocatalysis.We finish this review with a critical outlook into the currently existing challenges and possible development opportunities of this rapidly evolving field. | Fei Zhang Zhuangzhuang Ma Zhifeng Shi Xu Chen Di Wu Xinjian Li Chongxin Shan | 2021 | Energy Material Advances2021，，1： | 3 |
| 3 | Formation of Stable Interphase of Polymer-in-Salt Electrolyte in All-Solid-State Lithium Batteries显示文摘The integration of solid-polymer electrolytes into all-solid-state lithium batteries is highly desirable to overcome the limitations of current battery configurations that have a low energy density and severe safety concerns.Polyacrylonitrile is an appealing matrix for solid-polymer electrolytes;however,the practical utilization of such polymer electrolytes in all-solid-state cells is impeded by inferior ionic conductivity and instability against a lithium-metal anode.In this work,we show that a polymer-in-salt electrolyte based on polyacrylonitrile with a lithium salt as the major component exhibits a wide electrochemically stable window,a high ionic conductivity,and an increased lithium-ion transference number.The growth of dendrites from the lithium-metal anode was suppressed effectively by the polymer-in-salt electrolyte to increase the safety features of the batteries.In addition,we found that a stable interphase was formed between the lithium-metal anode and the polymer-in-salt electrolyte to restrain the uncontrolled parasitic reactions,and we demonstrated an all-solid-state battery configuration with a LiFePO4 cathode and the polymer-in-salt electrolyte,which exhibited a superior cycling stability and rate capability. | Hongcai Gao Nicholas S.Grundish Yongjie Zhao Aijun Zhou John B.Goodenough | 2021 | Energy Material Advances2021，，1： | 2 |
| 4 | Large Scale One-Pot Synthesis of Monodispersed Na_(3)(VOPO_(4))_(2)F Cathode for Na-Ion Batteries显示文摘Na-ion batteries(NIBs)have received significant interest as potential candidates for large-scale energy storage owing to the widespread distribution of sodium and superior low-temperature performance.However,their commercial application is usually hindered by the high production cost and inadequate performance for electrode materials,particularly for cathodes.Na_(3)(VOPO_(4))_(2)F(NVOPF)has been recognized as one of the most promising cathodes for high-energy NIBs owing to the high working voltage and energy density.Here,we report a facile highly efficient room-temperature solution protocol for large-scale synthesis of NVOPF cathode for NIBs.By simply regulating pH,NVOPF can be obtained,which delivered a discharge capacity of 120.2 mAh g^(-1) at 0.1 C and 72%capacity retention over 8000 cycles at 25 C.Besides,the kilogram-level NVOPF products have been synthesized,and 26650 cylindrical cells were fabricated,which exhibit excellent cycling stabilities,remarkable lowtemperature performance with comparable safety features.We hope our findings could provide insights on the industrial application of NVOPF in NIBs. | Qiangqiang Zhang Xing Shen Quan Zhou Kaixuan Li Feixiang Ding Yaxiang Lu Junmei Zhao Liquan Chen Yong-Sheng Hu | 2022 | Energy Material Advances2022，，1： | 2 |
| 5 | Insight into the electrode mechanism in lithium-sulfur batteries with ordered microporous carbon confined sulfur as the cathode显示文摘 | LI Z YUAN L X YI Z Q | 2014 | Advanced Energy Materials2014，4，13： | 1 |
| 6 | Hollow carbon nanospheres with superior rate capability for sodium-based batteries显示文摘 | Tang K Fu L White R J | 2012 | Advanced Energy Materials2012，2，7： | 1 |
| 7 | The current move of lithium ion batteries towards the next phase显示文摘 | TAE-HEE K JEONG-SEOK P SUNG K | 2012 | Advanced Energy Materials2012，2，7： | 1 |
| 8 | Metal-air batteries with high energy density: Li-air versus Zn-air显示文摘 | LEE J S KIM S T CAO R G | 2011 | Advanced Energy Materials2011，1，1： | 1 |
| 9 | Carbon Nanotube - Enhanced Growth of Silicon Nanowires as an Anode for High - Performance Lithi- um - Ion Batteries显示文摘 | Xianglong Li Jeong - Hyun Cho | 2012 | Advanced Energy Materials2012，2，1： | 1 |
| 10 | Morphology-performance relationships in high-efficiency all-polymer solar cells 显示文摘 | Zhou N J Lin H Lou S J | 2014 | Advanced Energy Materials2014，4，3： | 1 |
| 11 | Autonomic shutdown of lithium-ion batteries using thermoresponsive microspheres显示文摘 | Baginska M Blaiszik B J Merriman R J | 2012 | Advanced Energy Materials2012，2，5： | 1 |
| 12 | Carbonized Chicken Eggshell Membranes with 3D Architectures as High-Performance Electrode Materials for Super- capacitors显示文摘 | LI Z ZHANG L AMIRKHIZ B S et at | 2012 | Advanced Energy Materials2012，2，4： | 1 |
| 13 | Hydrothermal and solvothermal process towards development of LiMPO4 (M=Fe,Mn) nanomaterials for lithium-ion batteries 显示文摘 | KEMPAIAH M HONMA I | 2012 | Advanced Energy Materials2012，，2： | 1 |
| 14 | Quantum-dot sensitized solar cells employing hierarchical CuzS microspheres wrapped by reduced graphene oxide nanosheets as effec- tive counter electrodes显示文摘 | Ye M D Chen C Zhang N | 2014 | Advanced Energy Materials2014，，20： | 1 |
| 15 | Towards high power high energy aqueous sodium-ion batteries: the NaTi2(PO4)J NaMnO2 system显示文摘 | Li Z Young D Xiang K | 2013 | Advanced Energy Materials2013，3，3： | 1 |
| 16 | Novel K3V2(PO4)3/C bundled nanowires as superior sodium-ion battery elec- trode with ultrahigh cycling stability显示文摘 | Wang X P Niu C J Meng J S | 2015 | Advanced Energy Materials2015，5，15： | 1 |
| 17 | Carbon nanomaterials for dye-sensitized solar cell applications: a bright future 显示文摘 | Brennan L J Byrne M T Bari M | 2011 | Advanced Energy Materials2011，1，4： | 1 |
| 18 | Tailoring electrode/ electrolyte interracial properties in flexible supercapaci- tors by applying pressure显示文摘 | Masarapu C Wang L P Li X | 2012 | Advanced Energy Materials2012，2，5： | 1 |
| 19 | High-performance fiber-shaped all-solid-state asymmetric supercapacitors based on ultrathin Mn O2nanosheet/carbon fiber cathodes for wearable electronics显示文摘 | YU N YIN H ZHANG W | 2016 | Advanced Energy Materials2016，6，15： | 1 |
| 20 | Ion migra- tion and the role of preconditioning cycles in the stabi- lization of the J-V characteristics of inverted hybrid per- ovskite solar cells 显示文摘 | De Bastiani M DelrErba G Gandini M | 2016 | Advanced Energy Materials2016，6，15： | 1 |
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